DE69213002T2 - Zusammensetzungen für reifenlauffläche - Google Patents
Zusammensetzungen für reifenlaufflächeInfo
- Publication number
- DE69213002T2 DE69213002T2 DE69213002T DE69213002T DE69213002T2 DE 69213002 T2 DE69213002 T2 DE 69213002T2 DE 69213002 T DE69213002 T DE 69213002T DE 69213002 T DE69213002 T DE 69213002T DE 69213002 T2 DE69213002 T2 DE 69213002T2
- Authority
- DE
- Germany
- Prior art keywords
- rubber
- phr
- composition
- tire
- sulfur
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Expired - Fee Related
Links
- 239000000203 mixture Substances 0.000 title claims abstract description 38
- 229920001971 elastomer Polymers 0.000 claims abstract description 40
- 239000005060 rubber Substances 0.000 claims abstract description 39
- 229920000459 Nitrile rubber Polymers 0.000 claims abstract description 19
- 229920003048 styrene butadiene rubber Polymers 0.000 claims abstract description 17
- NINIDFKCEFEMDL-UHFFFAOYSA-N Sulfur Chemical compound [S] NINIDFKCEFEMDL-UHFFFAOYSA-N 0.000 claims abstract description 15
- 229910052717 sulfur Inorganic materials 0.000 claims abstract description 15
- 239000011593 sulfur Substances 0.000 claims abstract description 15
- 150000001875 compounds Chemical class 0.000 claims abstract description 14
- XLOMVQKBTHCTTD-UHFFFAOYSA-N Zinc monoxide Chemical compound [Zn]=O XLOMVQKBTHCTTD-UHFFFAOYSA-N 0.000 claims abstract description 12
- 239000011787 zinc oxide Substances 0.000 claims abstract description 6
- 239000005063 High cis polybutadiene Substances 0.000 claims abstract description 5
- 238000010059 sulfur vulcanization Methods 0.000 claims description 7
- AUZONCFQVSMFAP-UHFFFAOYSA-N disulfiram Chemical compound CCN(CC)C(=S)SSC(=S)N(CC)CC AUZONCFQVSMFAP-UHFFFAOYSA-N 0.000 claims description 6
- -1 thiuram sulfides Chemical class 0.000 claims description 6
- 229920002857 polybutadiene Polymers 0.000 claims description 5
- 229960002447 thiram Drugs 0.000 claims description 4
- OFHMODDLBXETIK-UHFFFAOYSA-N methyl 2,3-dichloropropanoate Chemical compound COC(=O)C(Cl)CCl OFHMODDLBXETIK-UHFFFAOYSA-N 0.000 claims description 3
- 239000003921 oil Substances 0.000 claims description 3
- LGBYJXBCVZKJBL-UHFFFAOYSA-N 1-[(2-oxoazepan-1-yl)disulfanyl]azepan-2-one Chemical compound O=C1CCCCCN1SSN1C(=O)CCCCC1 LGBYJXBCVZKJBL-UHFFFAOYSA-N 0.000 claims description 2
- QRYFCNPYGUORTK-UHFFFAOYSA-N 4-(1,3-benzothiazol-2-yldisulfanyl)morpholine Chemical compound C1COCCN1SSC1=NC2=CC=CC=C2S1 QRYFCNPYGUORTK-UHFFFAOYSA-N 0.000 claims description 2
- 239000004606 Fillers/Extenders Substances 0.000 claims description 2
- 230000015556 catabolic process Effects 0.000 claims description 2
- 238000006731 degradation reaction Methods 0.000 claims description 2
- 239000012990 dithiocarbamate Substances 0.000 claims description 2
- 150000004659 dithiocarbamates Chemical class 0.000 claims description 2
- 239000000945 filler Substances 0.000 claims description 2
- 150000002357 guanidines Chemical class 0.000 claims description 2
- 229940083094 guanine derivative acting on arteriolar smooth muscle Drugs 0.000 claims description 2
- 150000002391 heterocyclic compounds Chemical class 0.000 claims description 2
- 239000003112 inhibitor Substances 0.000 claims description 2
- 239000004014 plasticizer Substances 0.000 claims description 2
- 239000012744 reinforcing agent Substances 0.000 claims description 2
- 150000003585 thioureas Chemical class 0.000 claims description 2
- KUAZQDVKQLNFPE-UHFFFAOYSA-N thiram Chemical compound CN(C)C(=S)SSC(=S)N(C)C KUAZQDVKQLNFPE-UHFFFAOYSA-N 0.000 claims description 2
- 239000012991 xanthate Substances 0.000 claims description 2
- 239000006057 Non-nutritive feed additive Substances 0.000 claims 1
- 239000000654 additive Substances 0.000 claims 1
- 239000002174 Styrene-butadiene Substances 0.000 abstract description 10
- 239000005062 Polybutadiene Substances 0.000 abstract description 6
- 239000006229 carbon black Substances 0.000 abstract description 4
- 239000004615 ingredient Substances 0.000 abstract description 4
- 235000021355 Stearic acid Nutrition 0.000 abstract description 2
- 239000010692 aromatic oil Substances 0.000 abstract description 2
- QIQXTHQIDYTFRH-UHFFFAOYSA-N octadecanoic acid Chemical compound CCCCCCCCCCCCCCCCCC(O)=O QIQXTHQIDYTFRH-UHFFFAOYSA-N 0.000 abstract description 2
- OQCDKBAXFALNLD-UHFFFAOYSA-N octadecanoic acid Natural products CCCCCCCC(C)CCCCCCCCC(O)=O OQCDKBAXFALNLD-UHFFFAOYSA-N 0.000 abstract description 2
- 239000008117 stearic acid Substances 0.000 abstract description 2
- 239000001993 wax Substances 0.000 abstract description 2
- PPBRXRYQALVLMV-UHFFFAOYSA-N Styrene Chemical compound C=CC1=CC=CC=C1 PPBRXRYQALVLMV-UHFFFAOYSA-N 0.000 description 18
- 238000005096 rolling process Methods 0.000 description 10
- NLHHRLWOUZZQLW-UHFFFAOYSA-N Acrylonitrile Chemical compound C=CC#N NLHHRLWOUZZQLW-UHFFFAOYSA-N 0.000 description 5
- 229920013649 Paracril Polymers 0.000 description 5
- 238000005299 abrasion Methods 0.000 description 5
- 239000000243 solution Substances 0.000 description 5
- 239000003795 chemical substances by application Substances 0.000 description 4
- 239000000463 material Substances 0.000 description 4
- 230000000704 physical effect Effects 0.000 description 4
- 229920001577 copolymer Polymers 0.000 description 3
- YXIWHUQXZSMYRE-UHFFFAOYSA-N 1,3-benzothiazole-2-thiol Chemical compound C1=CC=C2SC(S)=NC2=C1 YXIWHUQXZSMYRE-UHFFFAOYSA-N 0.000 description 2
- HLBZWYXLQJQBKU-UHFFFAOYSA-N 4-(morpholin-4-yldisulfanyl)morpholine Chemical compound C1COCCN1SSN1CCOCC1 HLBZWYXLQJQBKU-UHFFFAOYSA-N 0.000 description 2
- KAKZBPTYRLMSJV-UHFFFAOYSA-N Butadiene Chemical compound C=CC=C KAKZBPTYRLMSJV-UHFFFAOYSA-N 0.000 description 2
- 239000005065 High vinyl polybutadiene Substances 0.000 description 2
- 238000013329 compounding Methods 0.000 description 2
- 238000005336 cracking Methods 0.000 description 2
- 239000000839 emulsion Substances 0.000 description 2
- 230000009477 glass transition Effects 0.000 description 2
- 238000000034 method Methods 0.000 description 2
- 150000002825 nitriles Chemical class 0.000 description 2
- 239000000126 substance Substances 0.000 description 2
- MFHNAXHSHOCFEC-UHFFFAOYSA-N 1,1-diphenylguanidine Chemical compound C=1C=CC=CC=1N(C(=N)N)C1=CC=CC=C1 MFHNAXHSHOCFEC-UHFFFAOYSA-N 0.000 description 1
- YHMYGUUIMTVXNW-UHFFFAOYSA-N 1,3-dihydrobenzimidazole-2-thione Chemical compound C1=CC=C2NC(S)=NC2=C1 YHMYGUUIMTVXNW-UHFFFAOYSA-N 0.000 description 1
- BUZICZZQJDLXJN-UHFFFAOYSA-N 3-azaniumyl-4-hydroxybutanoate Chemical compound OCC(N)CC(O)=O BUZICZZQJDLXJN-UHFFFAOYSA-N 0.000 description 1
- GIUBHMDTOCBOPA-UHFFFAOYSA-N 3h-1,3-benzothiazole-2-thione;zinc Chemical compound [Zn].C1=CC=C2SC(S)=NC2=C1 GIUBHMDTOCBOPA-UHFFFAOYSA-N 0.000 description 1
- MHKLKWCYGIBEQF-UHFFFAOYSA-N 4-(1,3-benzothiazol-2-ylsulfanyl)morpholine Chemical compound C1COCCN1SC1=NC2=CC=CC=C2S1 MHKLKWCYGIBEQF-UHFFFAOYSA-N 0.000 description 1
- ZZMVLMVFYMGSMY-UHFFFAOYSA-N 4-n-(4-methylpentan-2-yl)-1-n-phenylbenzene-1,4-diamine Chemical compound C1=CC(NC(C)CC(C)C)=CC=C1NC1=CC=CC=C1 ZZMVLMVFYMGSMY-UHFFFAOYSA-N 0.000 description 1
- 239000004215 Carbon black (E152) Substances 0.000 description 1
- BWGNESOTFCXPMA-UHFFFAOYSA-N Dihydrogen disulfide Chemical compound SS BWGNESOTFCXPMA-UHFFFAOYSA-N 0.000 description 1
- 229920010800 Duradene Polymers 0.000 description 1
- 229920002943 EPDM rubber Polymers 0.000 description 1
- PDQAZBWRQCGBEV-UHFFFAOYSA-N Ethylenethiourea Chemical compound S=C1NCCN1 PDQAZBWRQCGBEV-UHFFFAOYSA-N 0.000 description 1
- 244000043261 Hevea brasiliensis Species 0.000 description 1
- KFFQABQEJATQAT-UHFFFAOYSA-N N,N'-dibutylthiourea Chemical compound CCCCNC(=S)NCCCC KFFQABQEJATQAT-UHFFFAOYSA-N 0.000 description 1
- 239000004614 Process Aid Substances 0.000 description 1
- MNOILHPDHOHILI-UHFFFAOYSA-N Tetramethylthiourea Chemical compound CN(C)C(=S)N(C)C MNOILHPDHOHILI-UHFFFAOYSA-N 0.000 description 1
- OCKWAZCWKSMKNC-UHFFFAOYSA-N [3-octadecanoyloxy-2,2-bis(octadecanoyloxymethyl)propyl] octadecanoate Chemical compound CCCCCCCCCCCCCCCCCC(=O)OCC(COC(=O)CCCCCCCCCCCCCCCCC)(COC(=O)CCCCCCCCCCCCCCCCC)COC(=O)CCCCCCCCCCCCCCCCC OCKWAZCWKSMKNC-UHFFFAOYSA-N 0.000 description 1
- 239000012190 activator Substances 0.000 description 1
- 229920005549 butyl rubber Polymers 0.000 description 1
- 229920003211 cis-1,4-polyisoprene Polymers 0.000 description 1
- 230000000052 comparative effect Effects 0.000 description 1
- 239000002131 composite material Substances 0.000 description 1
- 230000008094 contradictory effect Effects 0.000 description 1
- 239000013068 control sample Substances 0.000 description 1
- 230000007423 decrease Effects 0.000 description 1
- LEOJDCQCOZOLTQ-UHFFFAOYSA-N dibutylcarbamothioyl n,n-dibutylcarbamodithioate Chemical compound CCCCN(CCCC)C(=S)SC(=S)N(CCCC)CCCC LEOJDCQCOZOLTQ-UHFFFAOYSA-N 0.000 description 1
- 229920003244 diene elastomer Polymers 0.000 description 1
- LMBWSYZSUOEYSN-UHFFFAOYSA-N diethyldithiocarbamic acid Chemical compound CCN(CC)C(S)=S LMBWSYZSUOEYSN-UHFFFAOYSA-N 0.000 description 1
- 229940096818 dipentamethylenethiuram disulfide Drugs 0.000 description 1
- 229950004394 ditiocarb Drugs 0.000 description 1
- 150000002148 esters Chemical class 0.000 description 1
- 239000000446 fuel Substances 0.000 description 1
- 229930195733 hydrocarbon Natural products 0.000 description 1
- 150000002430 hydrocarbons Chemical class 0.000 description 1
- IUJLOAKJZQBENM-UHFFFAOYSA-N n-(1,3-benzothiazol-2-ylsulfanyl)-2-methylpropan-2-amine Chemical compound C1=CC=C2SC(SNC(C)(C)C)=NC2=C1 IUJLOAKJZQBENM-UHFFFAOYSA-N 0.000 description 1
- DEQZTKGFXNUBJL-UHFFFAOYSA-N n-(1,3-benzothiazol-2-ylsulfanyl)cyclohexanamine Chemical compound C1CCCCC1NSC1=NC2=CC=CC=C2S1 DEQZTKGFXNUBJL-UHFFFAOYSA-N 0.000 description 1
- 229940032017 n-oxydiethylene-2-benzothiazole sulfenamide Drugs 0.000 description 1
- 229920003052 natural elastomer Polymers 0.000 description 1
- 229920001194 natural rubber Polymers 0.000 description 1
- 239000012188 paraffin wax Substances 0.000 description 1
- KNBRWWCHBRQLNY-UHFFFAOYSA-N piperidine-1-carbothioylsulfanyl piperidine-1-carbodithioate Chemical compound C1CCCCN1C(=S)SSC(=S)N1CCCCC1 KNBRWWCHBRQLNY-UHFFFAOYSA-N 0.000 description 1
- 229920001195 polyisoprene Polymers 0.000 description 1
- 229920000642 polymer Polymers 0.000 description 1
- 239000003755 preservative agent Substances 0.000 description 1
- 238000010058 rubber compounding Methods 0.000 description 1
- 229920003051 synthetic elastomer Polymers 0.000 description 1
- 150000003557 thiazoles Chemical class 0.000 description 1
- BOXSVZNGTQTENJ-UHFFFAOYSA-L zinc dibutyldithiocarbamate Chemical compound [Zn+2].CCCCN(C([S-])=S)CCCC.CCCCN(C([S-])=S)CCCC BOXSVZNGTQTENJ-UHFFFAOYSA-L 0.000 description 1
- NEYNBSGIXOOZGZ-UHFFFAOYSA-L zinc;butoxymethanedithioate Chemical compound [Zn+2].CCCCOC([S-])=S.CCCCOC([S-])=S NEYNBSGIXOOZGZ-UHFFFAOYSA-L 0.000 description 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L9/00—Compositions of homopolymers or copolymers of conjugated diene hydrocarbons
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B60—VEHICLES IN GENERAL
- B60C—VEHICLE TYRES; TYRE INFLATION; TYRE CHANGING; CONNECTING VALVES TO INFLATABLE ELASTIC BODIES IN GENERAL; DEVICES OR ARRANGEMENTS RELATED TO TYRES
- B60C1/00—Tyres characterised by the chemical composition or the physical arrangement or mixture of the composition
- B60C1/0016—Compositions of the tread
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L9/00—Compositions of homopolymers or copolymers of conjugated diene hydrocarbons
- C08L9/06—Copolymers with styrene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L9/00—Compositions of homopolymers or copolymers of conjugated diene hydrocarbons
- C08L9/02—Copolymers with acrylonitrile
Landscapes
- Chemical & Material Sciences (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Organic Chemistry (AREA)
- Engineering & Computer Science (AREA)
- Mechanical Engineering (AREA)
- Compositions Of Macromolecular Compounds (AREA)
- Tires In General (AREA)
Applications Claiming Priority (2)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| US69842491A | 1991-05-10 | 1991-05-10 | |
| PCT/US1992/003016 WO1992020737A2 (en) | 1991-05-10 | 1992-04-15 | Tire tread compositions |
Publications (2)
| Publication Number | Publication Date |
|---|---|
| DE69213002D1 DE69213002D1 (de) | 1996-09-26 |
| DE69213002T2 true DE69213002T2 (de) | 1997-01-30 |
Family
ID=24805185
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| DE69213002T Expired - Fee Related DE69213002T2 (de) | 1991-05-10 | 1992-04-15 | Zusammensetzungen für reifenlauffläche |
Country Status (11)
| Country | Link |
|---|---|
| EP (1) | EP0583369B1 (https=) |
| JP (1) | JP2682740B2 (https=) |
| KR (1) | KR100188355B1 (https=) |
| CN (1) | CN1048510C (https=) |
| AT (1) | ATE141631T1 (https=) |
| BR (1) | BR9205985A (https=) |
| CA (1) | CA2109202A1 (https=) |
| DE (1) | DE69213002T2 (https=) |
| MX (1) | MX9202157A (https=) |
| TW (1) | TW197462B (https=) |
| WO (1) | WO1992020737A2 (https=) |
Cited By (1)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| DE102015214731A1 (de) | 2015-08-03 | 2017-02-09 | Continental Reifen Deutschland Gmbh | Kautschukmischung und Fahrzeugreifen |
Families Citing this family (16)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US5569697A (en) * | 1995-05-08 | 1996-10-29 | Uniroyal Chemical Company, Inc. | Tire tread composition |
| KR20010097999A (ko) * | 2000-04-27 | 2001-11-08 | 신형인 | 천연고무의 소련방법 |
| RU2209362C1 (ru) * | 2002-04-03 | 2003-07-27 | Открытое акционерное общество "Научно-исследовательский институт резиновых покрытий и изделий" | Способ изготовления комбинированного газового баллона |
| KR100475948B1 (ko) * | 2002-06-29 | 2005-03-10 | 현대자동차주식회사 | 동특성 및 내열내구력이 우수한 방진고무 조성물 |
| JP4088261B2 (ja) * | 2004-03-04 | 2008-05-21 | 住友ゴム工業株式会社 | トレッド用ゴム組成物 |
| JP5291858B2 (ja) * | 2004-03-16 | 2013-09-18 | 株式会社ブリヂストン | ゴム組成物及びこれを用いた空気入りタイヤ |
| MY140477A (en) * | 2006-01-16 | 2009-12-31 | Ube Industries | Rubber composition for tire and tire |
| DE102008037837A1 (de) * | 2007-08-27 | 2009-04-09 | Toyo Tire & Rubber Co., Ltd., Osaka-shi | Gummimischung für einen Reifen und Herstellungsverfahren dafür |
| CN101434716B (zh) * | 2007-11-16 | 2012-03-21 | 四川轮胎橡胶（集团）股份有限公司 | 半钢丝子午线轮胎带束层压延胶料 |
| US7956146B2 (en) * | 2009-02-24 | 2011-06-07 | The Goodyear Tire & Rubber Company | Tire with tread of polybutadiene rubber |
| JP5342684B1 (ja) * | 2012-09-11 | 2013-11-13 | 住友ゴム工業株式会社 | インナーライナーを備えた空気入りタイヤ |
| CN104530512A (zh) * | 2014-12-18 | 2015-04-22 | 三角轮胎股份有限公司 | 含1,2-聚丁二烯树脂的轿车轮胎胎面橡胶组合物 |
| CN104610617A (zh) * | 2015-01-30 | 2015-05-13 | 柳州市中配橡塑配件制造有限公司 | 耐磨橡胶 |
| US11453763B2 (en) | 2018-03-16 | 2022-09-27 | The North Face Apparel Corp. | Rubber terpene footwear |
| CN109337141B (zh) * | 2018-09-10 | 2021-03-23 | 肇庆骏鸿实业有限公司 | 低阻轮胎胎面胶及其制备方法和应用 |
| JP7505178B2 (ja) * | 2019-11-25 | 2024-06-25 | 住友ゴム工業株式会社 | 自動二輪車用タイヤ |
Family Cites Families (5)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US2397050A (en) * | 1944-03-01 | 1946-03-19 | Goodrich Co B F | Synthetic rubber composition |
| US3305516A (en) * | 1964-12-02 | 1967-02-21 | Goodyear Tire & Rubber | Synthetic rubber compositions and pneumatic tire treads prepared therefrom |
| JPS59199735A (ja) * | 1983-04-28 | 1984-11-12 | Nippon Zeon Co Ltd | タイヤ・トレツド用ゴム組成物 |
| US4585826A (en) * | 1985-01-28 | 1986-04-29 | The Firestone Tire & Rubber Company | Natural rubber containing compositions with increased tear strength |
| US4894420A (en) * | 1988-09-14 | 1990-01-16 | The Goodyear Tire & Rubber Company | Tire with tread of selective rubber blend |
-
1992
- 1992-04-15 CA CA002109202A patent/CA2109202A1/en not_active Abandoned
- 1992-04-15 DE DE69213002T patent/DE69213002T2/de not_active Expired - Fee Related
- 1992-04-15 AT AT92911793T patent/ATE141631T1/de not_active IP Right Cessation
- 1992-04-15 BR BR9205985A patent/BR9205985A/pt not_active IP Right Cessation
- 1992-04-15 EP EP92911793A patent/EP0583369B1/en not_active Expired - Lifetime
- 1992-04-15 WO PCT/US1992/003016 patent/WO1992020737A2/en not_active Ceased
- 1992-04-15 KR KR1019930703373A patent/KR100188355B1/ko not_active Expired - Fee Related
- 1992-04-15 JP JP4510883A patent/JP2682740B2/ja not_active Expired - Fee Related
- 1992-04-21 TW TW081103125A patent/TW197462B/zh active
- 1992-05-08 MX MX9202157A patent/MX9202157A/es not_active IP Right Cessation
- 1992-05-09 CN CN92103440A patent/CN1048510C/zh not_active Expired - Fee Related
Cited By (2)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| DE102015214731A1 (de) | 2015-08-03 | 2017-02-09 | Continental Reifen Deutschland Gmbh | Kautschukmischung und Fahrzeugreifen |
| DE102015214731B4 (de) | 2015-08-03 | 2024-10-17 | Continental Reifen Deutschland Gmbh | Fahrzeugreifen |
Also Published As
| Publication number | Publication date |
|---|---|
| TW197462B (https=) | 1993-01-01 |
| WO1992020737A3 (en) | 1993-01-07 |
| MX9202157A (es) | 1992-11-01 |
| JP2682740B2 (ja) | 1997-11-26 |
| DE69213002D1 (de) | 1996-09-26 |
| KR100188355B1 (ko) | 1999-06-01 |
| EP0583369A1 (en) | 1994-02-23 |
| CN1048510C (zh) | 2000-01-19 |
| CA2109202A1 (en) | 1992-11-11 |
| EP0583369B1 (en) | 1996-08-21 |
| JPH06507662A (ja) | 1994-09-01 |
| WO1992020737A2 (en) | 1992-11-26 |
| CN1066665A (zh) | 1992-12-02 |
| ATE141631T1 (de) | 1996-09-15 |
| BR9205985A (pt) | 1994-09-27 |
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