WO2013116241A1 - Système de détection de gamma-neutron composite - Google Patents

Système de détection de gamma-neutron composite Download PDF

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Publication number
WO2013116241A1
WO2013116241A1 PCT/US2013/023684 US2013023684W WO2013116241A1 WO 2013116241 A1 WO2013116241 A1 WO 2013116241A1 US 2013023684 W US2013023684 W US 2013023684W WO 2013116241 A1 WO2013116241 A1 WO 2013116241A1
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WO
WIPO (PCT)
Prior art keywords
neutron
detector
gamma
layer
scintillator
Prior art date
Application number
PCT/US2013/023684
Other languages
English (en)
Inventor
Tsahi Gozani
Michael Joseph King
Donald Bennett Hilliard
Joseph Bendahan
Original Assignee
Rapiscan Systems, Inc.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Rapiscan Systems, Inc. filed Critical Rapiscan Systems, Inc.
Priority to EP13744250.5A priority Critical patent/EP2810096A4/fr
Priority to JP2014555627A priority patent/JP2015510589A/ja
Priority to CA2863633A priority patent/CA2863633C/fr
Priority to IN6515DEN2014 priority patent/IN2014DN06515A/en
Priority to GB1413624.6A priority patent/GB2513765A/en
Priority to KR1020147021796A priority patent/KR20140119092A/ko
Priority to BR112014019120A priority patent/BR112014019120A8/pt
Priority to CN201380014938.2A priority patent/CN104169741A/zh
Priority to AU2013215286A priority patent/AU2013215286B2/en
Priority to MX2014009411A priority patent/MX350345B/es
Publication of WO2013116241A1 publication Critical patent/WO2013116241A1/fr

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Classifications

    • G—PHYSICS
    • G01—MEASURING; TESTING
    • G01T—MEASUREMENT OF NUCLEAR OR X-RADIATION
    • G01T3/00—Measuring neutron radiation
    • G01T3/06—Measuring neutron radiation with scintillation detectors
    • G—PHYSICS
    • G01—MEASURING; TESTING
    • G01T—MEASUREMENT OF NUCLEAR OR X-RADIATION
    • G01T1/00—Measuring X-radiation, gamma radiation, corpuscular radiation, or cosmic radiation
    • G01T1/16—Measuring radiation intensity
    • G01T1/20—Measuring radiation intensity with scintillation detectors
    • G01T1/2008—Measuring radiation intensity with scintillation detectors using a combination of different types of scintillation detectors, e.g. phoswich
    • G—PHYSICS
    • G01—MEASURING; TESTING
    • G01T—MEASUREMENT OF NUCLEAR OR X-RADIATION
    • G01T3/00—Measuring neutron radiation
    • G01T3/008—Measuring neutron radiation using an ionisation chamber filled with a gas, liquid or solid, e.g. frozen liquid, dielectric

Definitions

  • the present specification generally relates to the field of detection of radioactive materials, specifically to systems and techniques for detecting neutrons and gamma rays and more specifically to a neutron and gamma-ray based detection system and method that is cost- effective, compact, and fabricated from readily available materials.
  • Physical shipment of materials is an integral part of any economy.
  • the materials are shipped in a type of shipping containment or cargo box.
  • Such containments or boxes include semi-trailers, large trucks, and rail cars as well as inter-modal containers that can be carried on container ships or cargo planes.
  • shipping or cargo containers can be used for illegal transportation of contraband such as nuclear and radioactive materials. Detection of these threats require a rapid, safe and accurate inspection system for determining the presence of hidden nuclear materials, especially at state and national borders, along with transit points such as airports and shipping ports.
  • passive and active detection techniques are employed for the detection of concealed nuclear materials.
  • Passive detection techniques are based on the principle that nuclear and radiological threats emit gamma, and in some cases neutron, radiation that can be detected.
  • passive detection systems can be easily deployed, they suffer from a number of drawbacks, including high rates of false positives and misdetections caused by unavoidable factors such as depression of the natural background by the vehicle being scanned and its contents, variation in natural background spectrum due to benign cargo such as clay tiles, fertilizers, etc., and the presence of radio therapeutic isotopes in the cargo with gamma lines at or near threat lines.
  • gamma sources are self-shielded and/or can readily be externally shielded, which makes them difficult to detect, since the radiation is absorbed in the shielding.
  • gamma detectors make poor neutron detectors and good neutron detectors tend to be poor gamma detectors.
  • DDA Differential Dieaway Analysis
  • Detection of delayed neutrons is an unequivocal method to detect fissile materials even in the presence of shielding mechanism(s) to hide the nuclear materials and notwithstanding the low background compared to delayed gamma rays. Because the number of delayed neutrons is two orders of magnitude lower than the number of delayed gamma rays, efficient and large area detectors are required for best sensitivity in neutron detection.
  • Each of the detector systems described above is not without drawbacks.
  • these devices generally utilize accelerators that produce high energy neutrons with a broad spectrum of energies.
  • the absorption/scattering of neutrons traveling at specific energies is difficult to detect given the large number of neutrons that pass through the object without interaction.
  • the "fingerprint" generated from the device is extremely small, difficult to analyze, and often leads to significant numbers of false positive or false negative test results.
  • the most commonly used neutron detector is a He-3 gas proportional chamber.
  • He- 3 interacts with a neutron to produce a He-4 ion.
  • This ion is accelerated in the electric field of the detector to the point that it becomes sufficiently energetic to cause ionisation of other gas atoms.
  • an avalanche breakdown of the gas can be generated, which results in a measurable current pulse at the output of the detector.
  • pressurizing the gas the probability of a passing thermal neutron interacting in the gas can be increased to a reasonable level.
  • He-3 is a relative scarce material and it does not occur naturally. This makes the availability and future supply of such detectors somewhat uncertain. Further, a special permit is required to transport pressurized He-3 tubes, which can be cumbersome and potentially problematic.
  • the most common globally deployed passive radioactive material detectors employ a neutron moderator 105 in an upper portion, having a plurality of He-3 detector tubes 116 embedded therein covered by a lead shield 108 and a lower portion comprising a plastic scintillator and moderator 110 with a PMT (Photo Multiplier Tube) 115 embedded therein, as shown in FIG. 1A.
  • This detector configuration however, still employs the scarce He-3.
  • FIG. IB another commonly deployed detector where the gamma-ray and neutron detectors are separate is shown in FIG. IB. As shown in FIG.
  • neutron moderator 105 comprising a plurality of He-3 detector tubes 116 is positioned adjacent to plastic scintillator 110, comprising a PMT 115 and a lead shield 108.
  • This detector configuration still employs the scarce He-3 and takes up a larger footprint.
  • the present specification describes, in one embodiment, a thinly-coated 10 B flat-panel ionization chamber neutron detector, which can be deployed as a direct drop-in replacement for current Radiation Portal Monitor (RPM) He detectors.
  • RPM Radiation Portal Monitor
  • the detector of the present specification comprises an argon gas cell sandwiched between boron-coated anode and cathode electrode plates.
  • multiple cells are stacked together to increase the intrinsic efficiency of the detector.
  • the detector is multi-layered and includes greater than 20 layers.
  • multiple detector unit cells are "tiled" to achieve areas of us to 1 square meter. In one embodiment, large detector units are folded for ease of transportation.
  • parallel plate geometry is employed, which allows for integration of neutron moderating sheets, such as polyethylene, on the back of the electrode plates to thermalize the neutrons and then detect them with high efficiency.
  • the moderator can be replaced with plastic scintillator sheets that can be viewed with a large area photomultiplier tube to detect gamma-rays in addition to neutrons, as is the case with existing RPMs.
  • the present specification further describes a large-area detector that is simple in its construction and manufacture, easily scalable with respect to the unit cell detector, easily adaptable to a variety of applications, and low cost.
  • the present specification is directed towards a neutron unit cell detector, comprising: a first and a second layer, comprising a polyethylene, for moderating a fast neutron; a third and a fourth layer comprising B-10, for capturing a moderated fast neutron, wherein the third and fourth layers are positioned between the first and second layers; and a gas cell layer positioned between the third and fourth layers, which, when a neutron is captured, emit charged particles that ionize the gas in the gas cell layer creating free electron and ion pairs.
  • the neutron detector comprises a plurality of unit cell detectors, which are stacked, thereby increasing detector efficiency.
  • the present specification is directed towards a gamma-neutron unit cell detector, comprising: a first and a second layer comprising gamma sensitive plastic scintillators for moderating a fast neutron and detecting gamma rays; a third and a fourth layer comprising B-10 for capturing a moderated fast neutron, wherein the third and fourth layers are positioned between the first and second layers; and a gas cell layer positioned between the third and fourth layers, which, when a neutron is captured, emit charged particles that ionize the gas in the gas cell layer creating free electron and ion pairs.
  • the gamma-neutron detector comprises a plurality of unit cell detectors, which are stacked, thereby increasing detector efficiency.
  • the plastic scintillator comprises at least one of an organic solid scintillator, an inorganic solid scintillator, or a liquid scintillator positioned between glass layers.
  • the present specification is directed towards a method for manufacturing a scalable, low-cost, large-area boron substrate for use in a detector comprising: employing a thin copper foil sheet as a metallic base; attaching the copper foil to a rigid layer to form a composite base for providing large areal structural strength; etching a tile pattern and individual electrical lines into the composite base by immersing the composite base in a ferric - chloride solution; mounting the composite base onto a drum for vacuum deposition; and depositing boron onto a surface of the copper foil to form the said boron substrate, wherein a mask is used to block the deposition of boron onto the electrical lines.
  • the thickness of the copper foil ranges from 50 to 100 ⁇ .
  • the rigid layer comprises Kapton.
  • the method of manufacturing the large area boron substrate optionally comprises the step of fabricating a fast neutron detector by laminating the boron substrate onto a sheet of polyethylene.
  • FIG. 1A illustrates a prior art radioactive material detector comprising a neutron moderator and a plastic scintillator, in which He-3 is employed;
  • FIG. IB illustrates a prior art radioactive material detector comprising a neutron moderator and a plastic scintillator, in which He-3 is employed;
  • FIG. 1C is a schematic layout of the composite gamma-neutron detector according to one embodiment of the present invention.
  • FIG. 2 illustrates an exemplary neutron detector based on mixtures of silver activated zinc sulfide
  • FIG. 3 illustrates an exemplary neutron detector based on mixtures of silver activated zinc sulfide that also uses a plastic scintillator for gamma ray detection
  • FIG. 4 illustrates experimental results with the silver activated zinc sulfide based neutron detector
  • FIG. 5 illustrates pulse signals as a function of time for gamma interactions and neutron interactions, respectively
  • FIG. 6 illustrates discrimination between gamma ray and neutron measurement signals
  • FIG. 7A illustrates one embodiment of the detector of present invention with multiple layers of gamma and neutron detector materials to increase neutron sensitivity
  • FIG. 7B illustrates another embodiment of the detector of present invention with angled detector slabs to increase neutron detection efficiency
  • FIG. 8 illustrates an exemplary readout circuit used with the detection system of the present invention
  • FIG. 9 illustrates an exemplary application of the gamma-neutron detector of the present invention in a drive-by vehicle
  • FIG. 10 illustrates another exemplary application of gamma-neutron detectors in a drive- thru scanning configuration
  • FIG. 11 illustrates yet another exemplary application of the gamma-neutron detector combined with a mobile X-ray scanner for generating composite gamma-neutron X-ray images
  • FIG. 12 illustrates another embodiment of the combined gamma-neutron detector and based X-ray imaging system in a portal or gantry configuration
  • FIG. 13 illustrates the gamma-neutron detector in a portable configuration, according to one embodiment of the present invention
  • FIG. 14 illustrates a parallel plate based Boron- 10 (B-10) detector, according to one embodiment of the present invention
  • FIGS. 15A illustrates a fast neutron detector geometry, in a first embodiment
  • FIGS. 15B illustrates a fast neutron detector geometry, in a second embodiment
  • FIG. 16A illustrates an exemplary manner in which scalability can be achieved for manufacturing the B-10 detector of the present specification
  • FIG. 16B illustrates an exemplary manner in which scalability can be achieved for manufacturing the B-10 detector of the present specification
  • FIG. 16C illustrates an exemplary manner in which scalability can be achieved for manufacturing the B-10 detector of the present specification
  • FIG. 17 is a graph illustrating detection efficiency of the B-10 detector of the present specification.
  • FIG. 18 is a graph showing the fast neutron detection efficiency of the 10 B neutron detector of the present specification compared with a He-based Differential Die -Away Analysis (DDAA) detector;
  • DDAA He-based Differential Die -Away Analysis
  • FIG. 19A illustrates a first manufacturing step for fabricating the large area boron substrate of the present specification
  • FIG. 19B illustrates a second manufacturing step for fabricating the large area boron substrate of the present specification
  • FIG. 19C illustrates a third manufacturing step for fabricating the large area boron substrate of the present specification
  • FIG. 19D illustrates a fourth manufacturing step for fabricating the large area boron substrate of the present specification
  • FIG. 19E illustrates a fifth manufacturing step for fabricating the large area boron substrate of the present specification.
  • FIG. 19F illustrates a sixth manufacturing step for fabricating the large area boron substrate of the present specification.
  • the present specification discloses systems and methods for detecting radiological threats using a composite gamma-neutron detector which can be configured to have a high sensitivity for both gamma and neutron detection, with a sufficient separation of the gamma and neutron signatures.
  • the system of the present invention allows for maximum threat detection with minimum false alarms, and thus increased throughput.
  • the present specification is directed towards a composite gamma-neutron detection system and method that is cost-effective, compact, and wherein the neutron detector is fabricated from readily available materials.
  • nuclei have a high cross-section for detection of thermal neutrons. These nuclei include He, Gd, Cd and two particularly high cross-section nuclei: Li-6 and B-10. In each case, after the interaction of a high cross-section nucleus with a thermal neutron, the result is an energetic ion and a secondary energetic charged particle.
  • the interaction of a neutron with a B-10 nucleus can be characterized by the following equation:
  • materials such as Cd, Gd and other materials having a high thermal capture cross section with no emission of heavy particles produce low energy internal conversion electrons, Auger electrons, X-rays, and gamma rays ranging in energy from a few keV to several MeV emitted at substantially the same time. Therefore, a layer of these materials, either when mixed in a scintillator base or when manufactured in a scintillator, such as Gadolinium Oxysulfide (GOS) or Cadmium Tungstate (CWO) will produce light (probably less than heavier particles).
  • GOS typically comes with two activators, resulting in slow (on the order of 1 ms) and fast (on the order of 5 ⁇ ) decays.
  • CWO has a relatively fast decay constant. Depending on the overall energy, a significant portion of the energy will be deposited in the layer, while some of the electrons will deposit the energy in the surrounding scintillator. In addition, the copious X-rays and gamma rays produced following thermal capture will interact in the surrounding scintillator. Thus, neutron interactions will result in events with both slow and fast decay constants. In many cases, neutron signals will consist of a signal with both slow and fast components (referred to as "coincidence") due to electron interlacing in the layer and gamma rays interacting in the surrounding scintillator.
  • the scintillation response of the material that surrounds the Li-6 or B-10 nuclei can be tuned such that this light can be transported through a second scintillator, such as a plastic scintillator in one embodiment, with a characteristic which is selected to respond to gamma radiation only.
  • a second scintillator such as a plastic scintillator in one embodiment, with a characteristic which is selected to respond to gamma radiation only.
  • the material that surrounds the Li-6 or B-10 is not a scintillator, but a transparent non-scintillating plastic resulting in a detector that is only sensitive to neutrons.
  • the plastic scintillator is both neutron and gamma sensitive.
  • a neutron is thermalized and subsequently captured by the H in the detector, a 2.22 MeV gamma ray is also emitted and often detected.
  • the present invention achieves a composite gamma- neutron detector capable of detecting neutrons as well as gamma radiation with high sensitivity.
  • the composite detector of the present invention also provides an excellent separation of the gamma and neutron signatures. It should be noted herein that in addition to charged particles, B-10 produces gamma rays. Therefore, in using materials that produce gamma rays following neutron capture, the result may be a detection that looks like gamma rays. Most applications, however, want to detect neutrons; thus, the detector of the present invention is advantageous in that it also detects the neutrons.
  • FIG. 1C illustrates a schematic layout of the composite gamma-neutron detector 100 according to one embodiment of the present invention.
  • the detector design employs two gamma-sensitive scintillation panels (gamma-detectors) 101 and 102 that surround a single neutron detector 103.
  • the neutron detector 103 further comprises a single slab of neutron sensitive composite scintillator, in which nuclei of a neutron sensitive material such as Li-6 or B-10 are mixed with a scintillation material such as ZnS.
  • a density of 20 - 30% by volume can be achieved for the neutron sensitive material (such as Li-6) while maintaining an efficient scintillation response from ZnS.
  • gamma detector panels can be fabricated from solid scintillation materials (without a substrate) such as, but not limited to organic scintillators, including solid plastic scintillators (e.g. NE102) and anthracene; inorganic scintillators including Nal(Tl), CsI(Tl), CsI(Na), and BaF 2 .
  • organic scintillators including solid plastic scintillators (e.g. NE102) and anthracene; inorganic scintillators including Nal(Tl), CsI(Tl), CsI(Na), and BaF 2 .
  • the neutron detector may be comprised of binder molecules such as, but not limited to styrenes dissolved in suitable solvents as the base substrate.
  • binder molecules such as, but not limited to styrenes dissolved in suitable solvents as the base substrate.
  • a plastic film forms which, once dry, is quite stable and self-supporting.
  • the scintillation material for example ZnS
  • the neutron specific element i.e. Gd, Li, B, etc.
  • a Gd, Li or B loaded liquid scintillator (generally based on the anthracene molecule with suitable organometallic compounds to increase scintillation efficiency) can be sealed in the gap between the gamma scintillation panels.
  • a thin glass barrier will be placed between the neutron scintillator and the gamma-detector to prevent chemical interaction between the two scintillator materials.
  • a typical panel size ranges from 0.1 m x 0.1 m for handheld applications up to 2 m x 1 m for large fixed site installations. Above this maximum size, light collection starts to become an issue as does physical handling and packaging. Below the minimum size, detection efficiency will start to drop below useful levels, resulting in increasingly long measurement times.
  • the gamma detector is thicker than the neutron detector.
  • the gamma detector thickness will advantageously be no less than 0.01 m (for hand held applications) up to 0.2 m for large fixed site systems.
  • the front gamma detector may be optimized to a different thickness compared to the back gamma detector in order to maximize overall gamma and neutron detection efficiency. For example, a front gamma detector thickness of 0.05 m and a rear gamma detector thickness of 0.1 m would be applicable to a large fixed site system.
  • the neutron detector will generally be thin to minimize gamma interaction probability and to maximize the chance of light escape from the scintillator.
  • a typical neutron detector based on a solid screen scintillator would be in the range of 0.5-1 mm thick while a liquid neutron scintillator may be in the range of 0.01 to 0.05 m thick.
  • Optical signals from both the gamma detectors 101, 102 and the neutron detector 103 are readout by one or more photodetectors, which in one embodiment are photomultiplier tubes (PMTs) 104.
  • the optical signals are thus converted to electronic signals which are then processed by a pulse processor 105 which assigns interactions separately due to gamma and neutron interactions 106 and 107, respectively.
  • the gamma-sensitive 101 and 102 panels are advantageously fabricated from a plastic scintillator with a fast decay time, such as less than 0.1 ⁇ .
  • the Li-6 or B-10 nuclei of the neutron detector 103 are advantageously mixed with a scintillation material having a slower decay time, such as ZnS.
  • the decay time for the scintillation material is greater than 1 ⁇ .
  • the difference in decay times for scintillators in gamma detectors and in neutron detector contributes to provide a significant separation between the gamma and neutron signatures 106 and 107.
  • it is desirable to select a scintillation material with low atomic number so as to minimise the probability of direct excitation by a passing gamma ray which causes enhanced gamma-neutron rejection.
  • the Li-6 or B-10 is mixed with a material with very fast response
  • the detector can measure neutrons at a very high counting rate, in particular when no scintillator is used to surround it.
  • scintillation materials such as ZnS can absorb their own light and therefore there is a limit to the thickness of a scintillation based detector in ZnS. It may be noted that this thickness is typically only a few millimetres. Further, since light is emitted isotropically during each scintillation event, it is efficient to form the scintillator into a wide area screen where light emission can be captured from both sides of the screen simultaneously. Therefore, in one embodiment the scintillator based neutron detector 103 is designed as a screen with a wide area, such that light may be collected with a high efficiency from both sides of the screen.
  • the detection efficiency of a 1mm thick Li-6/ZnS screen is of the same order as that of a pressurised He-3 gas proportional tube several cm in diameter. That is, the Li-6/ZnS based neutron detector of the present invention offers equivalent or greater detection efficiency as compared to the pressurised He-3 gas tube detector, at a much reduced size.
  • a neutron detector is based on mixtures of silver activated zinc sulfide, ZnS(Ag), with the mixtures containing materials with high thermal neutron-capture cross section with emission of heavy particles, such as 6 Li or 10 B. That is, the mixtures consist of thermal neutron absorbers that produce heavy-particle emission following thermal capture.
  • FIG. 2 illustrates one such exemplary neutron detector 200.
  • the detector 200 consists of one or more thin screens 201, comprising the ZnS(Ag) based mixtures, as described above.
  • the screens 201 in one embodiment, have a thickness of about 0.5 mm and are embedded in a transparent hydrogenous light guide 202.
  • Light guide 202 also serves as a neutron moderator.
  • the light produced by neutron interaction in the ZnS(Ag) phosphorus screen is collected by the light guide 202 into a photodetector, such as a photomultiplier tube (PMT) 203, which produces a signal from which the neutrons are counted, using the counter 204.
  • a photodetector such as a photomultiplier tube (PMT) 203
  • the detector 200 further comprises a plastic scintillator 205, which serves as a gamma-ray detector and moderator.
  • the plastic scintillator may be made up polyvinyl toluene or PVT, or any other suitable plastic scintillator material known in the art.
  • Light produced by gamma-ray interactions in the scintillator 205 is detected by another PMT 206, which produces a signal from which the gamma-ray events are counted, using the counter 207.
  • counter 207 is a Multi-Channel Analyzer (MCA) that is used to measure the spectra of the gamma rays.
  • MCA Multi-Channel Analyzer
  • a reflector foil 208 is placed between the plastic scintillator 205 and the screen(s) 201 to prevent cross-contamination between optical signals from the neutron and gamma detection materials.
  • the reflector is used to prevent light produced from the gamma rays to be collected with the same PMT as light produced by the neutrons. This prevents appearance of false neutron counts from gamma rays. Due to the reflector 208, some of the light produced by neutron interactions in the screen will be reflected back into the light guide.
  • FIG. 2 provides a compact gamma-ray/neutron detector with the advantages of standard electronics and significantly high gamma-ray rejection. A small fraction of gamma rays will interact with the Li-6 sheet and will produce a low-intensity signal. This signal can be removed by thresholding, at the expense of some neutron detection.
  • a pulse shape discriminator can be employed within neutron channel 204 to enhance gamma-ray rejection.
  • FIG. 3 Another exemplary detector 300 for simultaneous neutron and gamma-ray detection is shown in FIG. 3.
  • the light guide material is replaced by a plastic scintillator 301, which serves as the gamma-ray detector, moderator and light guide.
  • the detector 300 also includes screens 302, which are preferably thin and fabricated from ZnS(Ag) based mixtures for neutron detection.
  • the neutrons and gamma-ray events are separated employing a Pulse-Shape Discrimination (PSD) circuit 303 between the pulses 304 generated from the ZnS(Ag) and plastic scintillator (PVT).
  • PSD Pulse-Shape Discrimination
  • gamma-ray rejection is obtained as the light produced by electron interaction in the screen have similar decay time as the PVT's and will be eliminated with PSD.
  • the light produced is transported via the transparent and neutron moderating medium 301 to a Photomultiplier Tube (PMT) 305 where the light is converted to a measurable signal to measure gamma as well as neutron events.
  • PMT Photomultiplier Tube
  • FIG. 4 illustrates the performance of an exemplary detector with a 6 LiF:ZnS(Ag) screen embedded in a light-guide with two 6 LiF concentrations and thickness.
  • the results in FIG. 4 show the signal for the 1 :2 weight ratio and screen thickness of 0.45 mm. Similar results were obtained with simulations employing 1, 2 and 3 6 LiF:ZnS(Ag) screens embedded in polyethylene, and detection efficiencies ranging from around 12% to 22% were obtained. One of ordinary skill in the art would appreciate that this efficiency is comparable to the highest efficiency achievable with closely-packed three rows He detectors, which is around 25%.
  • the signal distribution in FIG. 4 shows that not all the particle energy absorption is converted to light and that some of the light may be absorbed by the screen. This demonstrates the need for a comprehensive optimization where the right concentration of 6 Li is obtained to produce high neutron absorption, while still having sufficient interactions in the scintillator to produce a sizeable light output.
  • the screen thickness, the number of screens and moderator thickness are also important optimization parameters.
  • a major advantage of ZnS(Ag) phosphorus is the large light output for heavy particles compared with electrons produced by gamma-ray interactions. Also, due to the small thickness of the screen, the gamma-ray detection efficiency is low. Further, since the time-decay of the PVT light is ⁇ 3 ns, similar to that of the light produced by electrons in the ZnS(Ag) screen, PSD will also reject gamma rays interacting in the PVT.
  • neutrons generated by radioactive materials of interest have a range of energies, and that the efficiency of neutron interaction in the detector will generally increase markedly as the energy of the interacting neutron decreases.
  • most He-3 detectors are located within a hydrogen rich moderating material, such as polythene, whose function is to promote neutron scattering of high energy neutrons such that they lose substantial amounts of energy in order to increase the probability of detection in the He-3 gas proportional counter.
  • the gamma detector is advantageously designed to provide a dual function of gamma detection and neutron moderation to further improve the detection efficiency for neutrons.
  • a plastic scintillator material is quite an efficient moderator as this feature is incorporated in the overall detector design.
  • FIG. 5 illustrates pulse signals, as a function of time corresponding to gamma interactions and neutron interactions in the composite detector of the present invention.
  • the scintillation characteristics curve 502 of the neutron sensitive scintillator is very different from the characteristics 501 of the surrounding gamma sensitive detector.
  • These two characteristic signals 501 and 502 can be further tuned to exhibit a significant difference. This can be done by using appropriate pulse shape discrimination methods.
  • both the total energy deposited in the detector and the types of interaction are determined. While the total energy can be determined by analysing the peak magnitude of the pulse signal, the type of interaction is determined by analysing the rate of decay of the scintillation pulse.
  • FIG. 6 illustrates the discrimination between gamma rays and neutrons for 252Cf and 60Co source, when analog Pulse-Shape Discrimination is applied to separate gamma rays from neutron events. While curve 601 reflects measurement of gamma rays emitted from 60Co source, curve 602 reflects measurement of neutrons emitted from 252Cf source. It would be apparent to those of ordinary skill in the art that the two curves are separate and distinctly identifiable.
  • the gamma-ray rejection is improved by subtracting a calibrated fraction of gamma-ray counts from the measured neutron counts.
  • the digital pulse processing is advantageously performed directly at the output of the detector. Since data rates can be quite high, processing at the detector helps filter the data down to a low bandwidth for transmission on to other processing systems. This data can be used to monitor the amount of radioactivity that is detected and to raise suitable alarms and/or display data by a number of means.
  • the neutron reaction may also create an associated gamma-ray emission.
  • the excited Gd-158 nucleus decays with the emission of a gamma-ray.
  • This gamma-ray is produced within a finite time of the neutron interaction and, therefore, it is possible to include the gamma-ray response that is measured in the surrounding gamma-detector in combination with the neutron scintillator response to produce a combined signal using the principle of pulse shape discrimination and time domain correlation.
  • FIG. 1C illustrates an exemplary configuration for a composite detector
  • alternative detector configurations may be established in order to further enhance neutron and gamma detection efficiency.
  • FIGS. 7A and 7B Two exemplary alternative configurations are illustrated in FIGS. 7A and 7B.
  • a first configuration combines multiple layers of gamma sensitive scintillator slabs 701 and neutron sensitive scintillator slabs 702 placed alternately with each other, in a direction substantially perpendicular to the direction of arrival of incident radiation 705.
  • the efficiency of the gamma-neutron detector scales in proportion to the number of slabs of detector material; although this is a diminishing effect due to preferential absorption of radiation in the first layers of the detector compared to the later layers of the detector.
  • Neutron sensitivity is significantly enhanced when the detector slabs are arranged in this configuration.
  • FIG. 7B In another configuration shown in FIG. 7B, multiple layers of gamma detector materials 710 and neutron detector materials 720 are placed alternately with each other and are oriented at an angle to the direction of the incoming radiation 715. That is, layers 710 and 720 are not parallel to the direction of the incoming radiation 715.
  • Such a detector configuration with angled detector slabs significantly increases neutron detection efficiency. This is because a neutron or photon in this case has a longer path length through each detector slab, which contributes to detection efficiency, as compared to the arrangement of slabs shown in FIG. 7A.
  • this arrangement of detectors is also more expensive to fabricate and requires more extensive readout circuits.
  • the composite gamma-neutron detector of the present invention described with reference to FIGS. 1, 7 A and 7B is not limited to plastic scintillator gamma detector with Li-6/ZnS neutron detector.
  • the composite detector may be configured using Nal(Tl) as the gamma detector, along with a lithium, boron or gadolinium based liquid scintillator with a very fast decay time.
  • the Nal(Tl) gamma detector will provide significant pulse height information about the gamma ray interaction while the neutron detector will continue to provide information about the incident neutron flux.
  • a neutron scintillator can be used which provides different pulse shapes due to fast and thermal neutron interactions, where each pulse shape is different to that selected for the gamma detector.
  • FIG. 8 illustrates an exemplary detector readout circuit architecture.
  • the circuit 800 comprises a photomultiplier tube (PMT) 801, which is operated with its cathode 802 held at negative high voltage with a grounded anode 803.
  • the anode 803 is AC coupled using a transformer 804 to a high speed sampling analogue-to-digital converter (ADC) 805.
  • the ADC 805 forms a time domain sample of the incoming signal from the PMT 801.
  • the ADC operates at a clock speed of 100 MHz or more to provide at most 10 ns sampling periods for accurate measurement of peak height and of the rise and fall decay times.
  • a filtering circuit is advantageously included between the PMT 801 and the input to the ADC 805 to act as a Nyquist filter to prevent unwanted aliasing in the sampled data.
  • an LCR multi-pole filter is implemented using the AC coupling transformer 804 as the inductive component.
  • the PMT 801 may be d.c. coupled to the input of the ADC 805 using a high bandwidth analogue amplifier. A variety of other circuit configurations will be apparent to one skilled in the art.
  • the digital data produced by the ADC is advantageously passed directly to a digital processing circuit, such as a field programmable gate array (FPGA) 806.
  • the FPGA provides high speed digital pulse shape processing and is configured to (1) record the time of arrival of a pulse, (2) determine the magnitude of the pulse and (3) determine the fall time of the pulse in order to discriminate between neutron and gamma interactions.
  • This pulse-by-pulse data is histogrammed to a random access memory 807 and can subsequently be analysed by a software program running on a computer 808 to resolve detected count rates relative to a dynamically adjusted baseline.
  • the result may be indicated to an operator through a visual display screen 809, a visual indicator, an audible sounder or any other suitable device in order to signal when a radioactive substance has been detected.
  • FIG. 9 shows an application of a composite gamma-neutron detector in a mobile system, in a drive -by scanning configuration.
  • the gamma-neutron detector 901 is positioned in a vehicle 902. This configuration allows rapid re-location of the detector 901 from one site to another, and is also useful for covert scanning of vehicles as they pass along a road.
  • the vehicle 902 is driven to a location, such as a roadside, and the detection system 901 is activated.
  • one or more sensors that are located on the vehicle 902 determine the presence of a passing object to be scanned, such as a passing vehicle, and the detection system 901 is turned on automatically.
  • the gamma-neutron detector 901 is turned off automatically. Once scanning at a given location is completed, the vehicle 902 can simply be driven to a new location and scanning can recommence as required. This feature provides the capability for random location scanning in a reasonably covert manner.
  • the gamma-neutron detector in its off state is used to record the natural background radiation and this natural background rate is used to set an appropriate alarm threshold for when additional activity is detected in a passing vehicle during the on state of the scanner.
  • the composite gamma-neutron detector 901 is installed in a vehicle 902 that can be driven past stationary targets at a known velocity. As the vehicle 902 drives by, radiation emission data is collected in order to determine the presence of radioactive materials in the stationary object.
  • FIG. 10 shows another application of one or more composite gamma-neutron detectors in a drive-through scanning configuration.
  • a plurality of composite gamma neutron detectors 1001, 1002 and 1003 are arranged as a fixed drive through system, in a portal configuration having a right, left, and top side, through which cargo vehicles such as 1004 can be driven.
  • the signals from the detectors 1001, 1002 and 1003 are processed and the result can be seen on a display 1005.
  • the display is also coupled to audible 1006 and visual 1007 alarms which are automatically generated, when radioactive material is suspected on the vehicle 1004 being scanned.
  • the result on display 1005 and the alarms 1006 and 1007 may be used to determine if the vehicle 1004 needs further search, and the vehicle may be diverted to a holding area, for example, for a manual search.
  • the drive through scanning system of FIG. 10 also employs a traffic control system 1008, which operates a barrier 1009 for stopping the vehicles for inspection. The barrier is lifted automatically once the scan results appear on the display 1005.
  • one or more gamma-neutron detectors of the present invention are installed with a baggage handling system employed at airports. In this manner, the system of present invention may also be used for detection of radioactive materials in baggage passing through an airport terminal. In another alternative configuration, one or more gamma detectors of the present invention can be installed in air cargo facilities and at the entrance of scrap metal facilities.
  • a gamma-neutron detector is combined with a mobile X-ray scanner for generating composite gamma-neutron X-ray images.
  • a gamma-neutron detector 1101 is installed on a mobile X-ray scanner 1100.
  • the mobile X-ray scanner 1100 further comprises an X-ray scanning system 1102 mounted on a vehicle 1103.
  • the radioactive signal from the gamma- neutron detector 1101 is acquired simultaneously with a transmission X-ray image from the X- ray scanning system 1102.
  • the gamma-neutron detector of the present invention is combined with an X-ray imaging system, in a portal or gantry configuration.
  • a plurality of gamma-neutron detectors 1201 are co-located with a transmission X-ray system 1202 arranged in a portal configuration.
  • Objects or vehicles under inspection can be passed through this portal or gantry.
  • This mode of operation again allows the radioactive signals to be correlated with an X-ray image of the object under inspection thereby increasing detection efficiency. For example, the occurrence of a high-attenuation area observed in the X-ray image and a small increase in gamma-ray and/or neutron signal below the threshold could indicate the presence of a shielded radioactive source.
  • FIG. 13 shows another embodiment of a gamma-neutron detector in a portable, hand-held configuration.
  • a gamma-neutron detection instrument 1300 is shown.
  • the instrument comprises a main unit 1301 and a handle 1302.
  • the scintillation panels of the composite gamma-neutron detector (not shown) are located in the main unit 1301, while the electronics and battery are advantageously located in the handle 1302 of the instrument.
  • An embedded indicator 1303 provides feedback to the operator on the amount of radiation present in the vicinity of the instrument 1300. This configuration is very useful for random searching, especially small objects and in searching nooks and corners within a vehicle.
  • the novel approach of the present invention combines a neutron scintillation detector with a gamma detector to form a hybrid gamma-neutron detector.
  • This approach provides the advantage of detecting dual signatures, thereby increasing detection efficiency.
  • the system of present invention also provides an excellent separation of the neutron signal from the gamma signal.
  • the system of present invention may be used in various configurations, depending upon the application, including but not limited to, fixed, drive -through portal, gantry, portable and hand-held.
  • the combined detector can be used for sea cargo inspection, and vehicle inspection in land crossings and scrap- metal facilities, in baggage and air cargo scanning, and other applications.
  • the combined neutron-gamma detector of the present invention and/or the neutron detector portion and/or the gamma detector portion is further designed to meet ANSI standards for radiation detection.
  • the present invention does not limit the use of the system with a particular nucleus.
  • any suitable material with high neutron thermal capture cross-section with emission of particles such as Lithium (Li-6), Boron (B-10), Cadmium (Cd), Gadolinium (Gd), and Helium (3 -He) may be used for radioactive material detection with the system of present invention. This feature helps to keep cost and supply under control.
  • the combined gamma-neutron detector of the present invention is more compact and lighter as compared to He- 3 based systems, as the detector of present invention only uses, in one embodiment, one set of electronics whereas He-3 based systems multiple sets of electronics are employed. It should be noted herein that in other embodiments, the present invention may be used with a plurality of electronic sets.
  • RPM Radiation Portal Monitors
  • plastic scintillators to detect gamma rays and moderated He detectors to measure neutrons. It is important to note that in typical RPMs, only one or two He tubes are used per module with a suboptimal moderating configuration to reduce cost. This results in a neutron detection efficiency of few percent.
  • the proposed neutron detector can replace He detectors in Radiation Portal Monitors
  • the detectors of present invention do not contain hazardous materials, are commercially available, do not require special transport permits, are very rugged - mechanically as well as environmentally, and are easy to manufacture at a reasonable cost.
  • the detectors are also suitable for handheld and backpack detectors, where efficiencies exceed that of He.
  • the present approach is suitable for integrated neutron and gamma-ray detectors, as it employs a single PMT with relatively simple and compact electronics.
  • B like He, has a high thermal neutron capture cross-section and emits two detectable high energy charged particles, but unlike He, is naturally abundant.
  • the supply of ⁇ is rapidly dwindling and as a result, He gas has become extremely expensive and difficult to obtain.
  • boron coated detectors have been available in the past and for example, utilized as reactor neutron flux monitors, they were inefficient, limiting their usage.
  • the present specification describes in one embodiment, a thinly-coated B flat-panel ionization chamber neutron detector, which can be deployed as a direct drop-in replacement for current Radiation Portal Monitor (RPM) He detectors.
  • the 10 B coating has a thickness range of 0.1 to 2.0 micron.
  • the 10 B coating is 1.0 micron thick.
  • a thicker coating means the energy losses are greater from the charge particle traversing through the coating into the gas chamber. This results in a detriment to the signal.
  • a thicker coating can increase detection efficiency lowering the number of layers required to reach a certain efficiency.
  • the detector of the present specification comprises an argon gas cell sandwiched between boron-coated anode and cathode electrode plates.
  • parallel plate geometry is employed, which allows for integration of neutron moderating sheets, such as polyethylene, on the back of the electrode plates to thermalize the neutrons and then detect them with high efficiency.
  • the moderator can be replaced with plastic scintillator sheets that can be viewed with a large area photomultiplier tube to detect gamma-rays in addition to neutrons, as is the case with existing RPMs.
  • the present specification further describes a large-area detector that is simple in its construction and manufacture, easily scalable with respect to the unit cell detector, easily adaptable to a variety of applications, and low cost.
  • the approach in developing a large-area 10 B- based He replacement detector focuses on utilizing a parallel plate ionization chamber concept, which is illustrated in FIG. 14.
  • the basic geometry of one unit cell detector consists of a first boron layer 1401 and a second boron layer 1402, which are high- voltage biased, sandwiching a gas cell 1403.
  • the two layers of boron capture thermal neutrons. When a neutron is captured, two charged particles, 7 Li and alpha are emitted and ionize the gas, thereby creating free ions and electrons.
  • the voltage applied 1405 sweeps the charges creating a signal.
  • a 7 Li and alpha particle are emitted in opposite directions.
  • One particle ionizes the gas in the gas cell 1403 creating free electron and ion pairs.
  • the high- voltage bias sweeps the ions creating a signal pulse proportional to the number of electron/ion pairs created. Because the chamber does not rely on multiplication of electrons, which proportional counters utilize to increase signal, lower voltages can be applied.
  • an alpha particle receives 1.47 MeV, while it receives 1.78 MeV in about 6% of the reactions.
  • 1 0 B has the second highest thermal neutron capture cross-section for a low-Z material.
  • the cross-section is 3837 barns, while 3 He has a cross-section of 5333 barns. Because 10 B has such a high thermal neutron capture cross-section, 10 B-based detectors can achieve 3 He equivalent efficiencies.
  • the large-area parallel plate ionization chamber can not only be designed to be a pure thermal neutron detector, it can be designed and optimized to detect fast neutrons as well.
  • Fast neutron detection is in many cases more relevant to the inspection arena than pure thermal neutron detection efficiencies, as all neutrons, when produced, are "fast" (with energies above 0.1 MeV). Indeed fast fission neutrons are one of the most important signatures of a fission event.
  • multiple unit cell detectors of FIG. 14 are stacked together to increase the intrinsic efficiency of the detector.
  • the detector is multi-layered and includes greater than 20 layers.
  • FIGS. 15 A and 15B illustrate a first and second embodiment of fast neutron detector geometries, respectively, that can replace large-area Radiation Portal Monitors.
  • a unit cell detector comprises a first polyethylene layer 1501, a first boron-coated metallic layer 1503, a gas cell layer 1505, a second boron-coated layer 1507, and a second polyethylene layer 1509.
  • gas cell layer 1505 is comprised of argon.
  • a fast neutron gets moderated by the polyethylene layer, thermalizes, and gets captured by the boron.
  • the polyethylene layers thus serve to moderate fast neutrons.
  • a photon detector is integrated with the neutron detector.
  • a plastic scintillator is integrated into the detector in the form of two layers 1510 and 1520.
  • the plastic scintillator serves a dual purpose; it can moderate fast neutrons and can detect gamma rays as well, since it is a gamma ray scintillation detector.
  • FIG. 15A can replace the He module in the current RPMs; the design of FIG. 15B in a single module, can replace the entire gamma ray and neutron detection modules of current RPMs.
  • FIG. 16A through 16C illustrate three exemplary steps via which scalability can be achieved.
  • FIG. 16A shows two stacked unit cell detectors 1601 described in detail with respect to FIGS. 15A and 15B.
  • the stacked detector has dimensions in the range of 10cm x 10 cm x 1 cm.
  • the stacked detector which comprises two unit cell detectors 1601 comprise a total of four boron layers 1605, two argon gas cells 1607 and three kapton layers 1609.
  • the kapton layers 1609 are used to provide rigidity to the thin boron coatings.
  • suitable materials may also be used for the purpose.
  • the detector By adding more boron, or stated differently, by adding more layers of boron, by stacking more than one unit cell detector, the amount of neutron absorbing material within the detector stack is increased. With more boron, there is a greater likelihood of detecting a neutron because as the neutron passes through the detector there is a greater chance that it will interact with at least one layer of boron. Thus, in one embodiment, multiple unit cell detectors are stacked together to increase the intrinsic efficiency of the detector. In one embodiment, the detector is multi-layered and includes greater than 20 layers.
  • FIG. 16B illustrates another embodiment of scaling the detector of the present invention.
  • unit cells are "tiled" to achieve areas of up to 1 m .
  • Each square 1605 in the detector matrix 1606 represents one unit cell detector and by having a 10 tile x 10 tile detector, large areas can be achieved.
  • Each tile has a separate electrical line 1607 feeding into a data acquisition system. Tiles are separated by grooves 1608 for electrical insulation.
  • FIG. 16C shows the detector 1610 in a foldable geometry, which allows reaching much larger areas by attaching lm x lm detectors, such as those shown in FIG. 16B, folded together into a package. Folding allows for greater transportability of the detectors, which, when unfolded, achieves much larger detection areas, thereby increasing detection efficiencies.
  • FIG. 17 illustrates the detection efficiency of the B-10 detector of the present invention by plotting the number of 10 B layers 1701 required to achieve the same thermal neutron detection efficiency 1702, as that of a 2-inch diameter He tube having 4 atm pressure.
  • the number of capture events for each layer of l- ⁇ thick 10 B is calculated. This thickness was chosen because the 1.47 MeV alpha particle range in boron metal is around 3.5 ⁇ . If the layer of boron is too thick, the charged particles lose all their energy inside the layer and get lost without contributing to the signal. Referring to FIG. 17, it can be seen that 40 l- ⁇ thick
  • the large-area 10 B thermal neutron detector can also be a good fast neutron detector. In many active interrogation techniques, it is the detection of fast neutrons that indicate hidden special nuclear materials.
  • FIG. 18 compares the fast neutron detection efficiency of the 10 B neutron detector of the present invention to a He-based Differential Die-Away Analysis (DDAA) detector.
  • the DDAA technique can detect the thermal neutron induced fission neutrons after the thermalized interrogating source neutrons die-away within the detector.
  • the figure plots the die-away time 1801 of the 10 B neutron detector and the detection efficiency 1802 of the detector as a function of polyethylene thickness, since polyethylene is layered inside 10 B detector.
  • the DDAA detector achieves a die-away time of 40 with a detection efficiency of around 25%. That means, for the same die-away time as the DDAA detector, each polyethylene layer in the 10 B neutron detector must be a thickness of 6 mm, as shown by the curve 1801. Subsequently, the intrinsic detection efficiency of the 10 B neutron detector at this point is around 20%), as shown by curve 1802, which is very similar to the DDAA detector.
  • FIGS. 19A through 19F illustrate, in a step-wise manner, one embodiment of a fabrication procedure for a large-area boron substrate layer as used in the manufacture of the unit cell detector of the present invention, having an area of about 1 m , in one embodiment.
  • the methods proposed follow established semiconductor techniques, which are economical and scalable.
  • a very thin sheet of copper foil 1911 is utilized as the metallic base for good electrical conductivity.
  • the thickness of copper foil 1911 is in the range of 50 - 100 ⁇ .
  • the copper foil sheet 1901 has an area that is 100 cm .
  • the copper foil 1911 is attached to a more rigid layer 1912, such as a Kapton layer, which provides the large areal structural strength.
  • a more rigid layer 1912 such as a Kapton layer, which provides the large areal structural strength.
  • the copper/Kapton layer is then immersed in a ferric-chloride solution for etching of the 10 cm x 10 cm tile pattern and individual electrical lines.
  • step 1930 shows the deposition of boron 1931 onto the copper surface 1911.
  • the substrates attached to the drum 1933 are rotated around in a sputtering chamber (not shown).
  • the sputtering chamber comprises a magnetron 1934 for Bi 0 C/B 4 C sputtering. With the use of a linear sputtering source 1934, the target-to-substrate distance can be decreased and also the losses of boron in one-dimension can be constrained.
  • the rate of deposition can be increased through maximizing magnetron power densities and through scaling methods.
  • an extra electron emitter embedded within the boron target during sputtering.
  • the use of extra electrons increases the stability and temperature of the depositions which leads to faster and more stable boron films.
  • the method of using an extra electron emitter is described in United States Patent Number 7,931,787, to Hilliard, entitled “Electron- Assisted Deposition Process and Apparatus", which is herein incorporated by reference in its entirety.
  • a mask 1935 is used to block the deposition of boron onto the etched electrical lines, thus keeping the lines from shorting.
  • the large-area boron layer 1941 is taken out of the vacuum and is ready for installation onto the detector.
  • a fast neutron detector is fabricated onto the detector, wherein the boron/copper/kapton layer 1951 is laminated onto a sheet of polyethylene 1952.
  • each individual substrate layer as described with respect to FIGS. 15a and 15b, are then stacked/layered into the detector, thereby increasing the amount of boron and maximizing the neutron detection efficiency.
  • the unit cell detector of the present invention comprises at least two boron coated metal layer sandwiching a gas cell.
  • the detector comprises a plurality of unit cell detectors, which may include a total of more than 20 layers.

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Abstract

La présente invention concerne un détecteur de gamma-neutron basé sur des mélanges d'absorbeurs de neutrons thermiques qui produisent une émission de particules lourdes suivant une capture thermique. Dans une configuration, un détecteur à base B-10 est utilisé dans une géométrie de plaques d'électrode parallèles qui intègre des feuilles de modérateur de neutrons, telles que le polyéthylène, au dos des plaques d'électrode pour amener les neutrons à l'état thermique et ensuite les détecter avec une grande efficacité. Le modérateur peut également être remplacé par des feuilles de scintillateur de matière plastique vues à l'aide d'un tube photomultiplicateur à grande surface pour détecter également des rayons gamma. Le détecteur peut être utilisé dans plusieurs configurations de balayage comprenant une configuration de portique, une configuration de conduite à travers, une configuration de conduite le long, une configuration à main et une configuration à sac à dos, etc.
PCT/US2013/023684 2012-02-04 2013-01-29 Système de détection de gamma-neutron composite WO2013116241A1 (fr)

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EP13744250.5A EP2810096A4 (fr) 2012-02-04 2013-01-29 Système de détection de gamma-neutron composite
JP2014555627A JP2015510589A (ja) 2012-02-04 2013-01-29 ガンマ線‐中性子複合検出システム
CA2863633A CA2863633C (fr) 2012-02-04 2013-01-29 Systeme de detection de gamma-neutron composite
IN6515DEN2014 IN2014DN06515A (fr) 2012-02-04 2013-01-29
GB1413624.6A GB2513765A (en) 2012-02-04 2013-01-29 Composite gamma-neutron detection system
KR1020147021796A KR20140119092A (ko) 2012-02-04 2013-01-29 복합형 감마선-중성자 검출시스템
BR112014019120A BR112014019120A8 (pt) 2012-02-04 2013-01-29 Sistema de detecção composto de radiação gama e nêutrons
CN201380014938.2A CN104169741A (zh) 2012-02-04 2013-01-29 复合伽马中子检测系统
AU2013215286A AU2013215286B2 (en) 2012-02-04 2013-01-29 Composite gamma-neutron detection system
MX2014009411A MX350345B (es) 2012-02-04 2013-01-29 Sistema de detección de composición de neutrones y rayos gamma.

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EP2810096A1 (fr) 2014-12-10
JP2015510589A (ja) 2015-04-09
EP2810096A4 (fr) 2016-02-17
GB2513765A (en) 2014-11-05
MX2014009411A (es) 2016-08-26
IN2014DN06515A (fr) 2015-06-12
AU2013215286B2 (en) 2015-08-27
AU2013215286A1 (en) 2014-08-28
CA2863633C (fr) 2017-02-21
GB201413624D0 (en) 2014-09-17
KR20140119092A (ko) 2014-10-08
MX350345B (es) 2017-09-05
BR112014019120A8 (pt) 2017-07-11
BR112014019120A2 (fr) 2017-06-20
CA2863633A1 (fr) 2013-08-08
CN104169741A (zh) 2014-11-26

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