WO2009025291A1 - 直接液体型燃料電池用隔膜、及びその製造方法 - Google Patents

直接液体型燃料電池用隔膜、及びその製造方法 Download PDF

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Publication number
WO2009025291A1
WO2009025291A1 PCT/JP2008/064814 JP2008064814W WO2009025291A1 WO 2009025291 A1 WO2009025291 A1 WO 2009025291A1 JP 2008064814 W JP2008064814 W JP 2008064814W WO 2009025291 A1 WO2009025291 A1 WO 2009025291A1
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WO
WIPO (PCT)
Prior art keywords
group
producing
liquid fuel
separation membrane
direct liquid
Prior art date
Application number
PCT/JP2008/064814
Other languages
English (en)
French (fr)
Inventor
Takenori Isomura
Kenji Fukuta
Original Assignee
Tokuyama Corporation
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Priority to US12/674,562 priority Critical patent/US20110250525A1/en
Application filed by Tokuyama Corporation filed Critical Tokuyama Corporation
Priority to EP08827759A priority patent/EP2192645B1/en
Priority to AT08827759T priority patent/ATE535954T1/de
Priority to JP2009529043A priority patent/JP5349313B2/ja
Priority to KR1020107003832A priority patent/KR101461699B1/ko
Publication of WO2009025291A1 publication Critical patent/WO2009025291A1/ja

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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2275—Heterogeneous membranes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F8/00—Chemical modification by after-treatment
    • C08F8/44—Preparation of metal salts or ammonium salts
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1009—Fuel cells with solid electrolytes with one of the reactants being liquid, solid or liquid-charged
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1023—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having only carbon, e.g. polyarylenes, polystyrenes or polybutadiene-styrenes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1072—Polymeric electrolyte materials characterised by the manufacturing processes by chemical reactions, e.g. insitu polymerisation or insitu crosslinking
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F2800/00—Copolymer characterised by the proportions of the comonomers expressed
    • C08F2800/20—Copolymer characterised by the proportions of the comonomers expressed as weight or mass percentages
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F2810/00—Chemical modification of a polymer
    • C08F2810/20—Chemical modification of a polymer leading to a crosslinking, either explicitly or inherently
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2325/00—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring; Derivatives of such polymers
    • C08J2325/02—Homopolymers or copolymers of hydrocarbons
    • C08J2325/04—Homopolymers or copolymers of styrene
    • C08J2325/08—Copolymers of styrene
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Sustainable Energy (AREA)
  • Sustainable Development (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Medicinal Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Materials Engineering (AREA)
  • Fuel Cell (AREA)
  • Manufacture Of Macromolecular Shaped Articles (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
  • Conductive Materials (AREA)
  • Macromonomer-Based Addition Polymer (AREA)

Abstract

　　本発明によりａ）１個の重合性基と、少なくとも１個のハロゲノアルキル基と、少なくとも１個の該ハロゲノアルキル基の第４級アンモニウム基に誘導する反応に対する不活性基とが、結合する芳香環を有してなる芳香族系重合性単量体、ｂ）架橋性重合性単量体、ｃ）重合開始剤、を含む重合性組成物と多孔質膜とを接触させて、前記重合性組成物を多孔質膜の有する空隙部に充填させた後、前記重合性組成物を重合硬化させ、次いで樹脂膜中の前記ハロゲノアルキル基を第４級アンモニウム基に誘導する直接液体型燃料電池用隔膜の製造方法が開示される。
PCT/JP2008/064814 2007-08-23 2008-08-20 直接液体型燃料電池用隔膜、及びその製造方法 WO2009025291A1 (ja)

Priority Applications (5)

Application Number Priority Date Filing Date Title
US12/674,562 US20110250525A1 (en) 2007-08-23 2008-02-26 Separation membrane for direct liquid fuel cell and method for producing the same
EP08827759A EP2192645B1 (en) 2007-08-23 2008-08-20 Separation membrane for direct liquid fuel cell and method for producing the same
AT08827759T ATE535954T1 (de) 2007-08-23 2008-08-20 Trennmembran für eine direkt- flüssigbrennstoffzelle und herstellungsverfahren dafür
JP2009529043A JP5349313B2 (ja) 2007-08-23 2008-08-20 直接液体型燃料電池用隔膜、及びその製造方法
KR1020107003832A KR101461699B1 (ko) 2007-08-23 2008-08-20 직접 액체형 연료 전지용 격막 및 그의 제조방법

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2007217448 2007-08-23
JP2007-217448 2007-08-23

Publications (1)

Publication Number Publication Date
WO2009025291A1 true WO2009025291A1 (ja) 2009-02-26

Family

ID=40378190

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/JP2008/064814 WO2009025291A1 (ja) 2007-08-23 2008-08-20 直接液体型燃料電池用隔膜、及びその製造方法

Country Status (6)

Country Link
US (1) US20110250525A1 (ja)
EP (1) EP2192645B1 (ja)
JP (1) JP5349313B2 (ja)
KR (1) KR101461699B1 (ja)
AT (1) ATE535954T1 (ja)
WO (1) WO2009025291A1 (ja)

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2010021158A1 (ja) * 2008-08-22 2010-02-25 国立大学法人東京工業大学 Ｏｈ－伝導体およびその製造方法
WO2011115175A1 (ja) * 2010-03-16 2011-09-22 株式会社トクヤマ 水難溶性陰イオン伝導性樹脂
JP2013513705A (ja) * 2009-12-11 2013-04-22 プロメラス， エルエルシー 第四アンモニウム官能基を有するノルボルネン型ポリマー

Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPH09216964A (ja) 1996-02-09 1997-08-19 Nitto Denko Corp 多孔質フィルムおよびそれを用いた電池用セパレータ並びに電池
JPH11135137A (ja) 1997-10-31 1999-05-21 Asahi Glass Co Ltd 固体高分子電解質型メタノール燃料電池
JPH11273695A (ja) 1998-03-19 1999-10-08 Asahi Glass Co Ltd 固体高分子電解質型メタノール燃料電池
JPH11335473A (ja) * 1998-05-26 1999-12-07 Tokuyama Corp イオン交換膜およびその用途
JP2000331693A (ja) 1999-05-19 2000-11-30 Asahi Glass Co Ltd 固体高分子型燃料電池
JP2002338721A (ja) 2001-05-16 2002-11-27 Asahi Kasei Corp ポリオレフィン樹脂多孔質フィルム
JP2003157862A (ja) * 2001-11-20 2003-05-30 Tokuyama Corp イオン交換樹脂膜及びその製造方法
JP2004055165A (ja) * 2002-07-16 2004-02-19 Akihiko Tanioka スチレン系高分子電解質及びその製造方法
JP2007188788A (ja) * 2006-01-13 2007-07-26 Tokuyama Corp 陰イオン交換樹脂膜形成用４級化剤、ガス拡散電極膜、固体電解質膜及びそれを具備する固体高分子型燃料電池

Family Cites Families (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPH0714489B2 (ja) * 1988-06-13 1995-02-22 東京有機化学工業株式会社 陰イオン交換樹脂
JPH07289924A (ja) * 1994-03-01 1995-11-07 Tohoku Electric Power Co Inc シリカ除去用樹脂
JPH09150066A (ja) * 1995-11-28 1997-06-10 Mitsubishi Chem Corp 陰イオン交換樹脂の製造法
JP3543476B2 (ja) * 1996-03-26 2004-07-14 三菱化学株式会社 架橋共重合体の製造方法
US7868051B2 (en) * 2004-09-10 2011-01-11 Tokuyama Corporation Separation membrane for fuel battery and process for producing the same
JP2007042573A (ja) * 2005-06-29 2007-02-15 Kuraray Co Ltd 固体高分子型燃料電池用高分子電解質膜、膜−電極接合体及び燃料電池
EP2506357B1 (en) * 2006-02-28 2015-06-17 Tokuyama Corporation Separation membrane for direct liquid fuel cell and method for producing same
US20090053578A1 (en) * 2006-03-14 2009-02-26 Takenori Isomura Separation Membrane for Direct Liquid Fuel Cell
JP5059341B2 (ja) * 2006-05-09 2012-10-24 株式会社トクヤマ 直接液体型燃料電池用隔膜

Patent Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPH09216964A (ja) 1996-02-09 1997-08-19 Nitto Denko Corp 多孔質フィルムおよびそれを用いた電池用セパレータ並びに電池
JPH11135137A (ja) 1997-10-31 1999-05-21 Asahi Glass Co Ltd 固体高分子電解質型メタノール燃料電池
JPH11273695A (ja) 1998-03-19 1999-10-08 Asahi Glass Co Ltd 固体高分子電解質型メタノール燃料電池
JPH11335473A (ja) * 1998-05-26 1999-12-07 Tokuyama Corp イオン交換膜およびその用途
JP2000331693A (ja) 1999-05-19 2000-11-30 Asahi Glass Co Ltd 固体高分子型燃料電池
JP2002338721A (ja) 2001-05-16 2002-11-27 Asahi Kasei Corp ポリオレフィン樹脂多孔質フィルム
JP2003157862A (ja) * 2001-11-20 2003-05-30 Tokuyama Corp イオン交換樹脂膜及びその製造方法
JP2004055165A (ja) * 2002-07-16 2004-02-19 Akihiko Tanioka スチレン系高分子電解質及びその製造方法
JP2007188788A (ja) * 2006-01-13 2007-07-26 Tokuyama Corp 陰イオン交換樹脂膜形成用４級化剤、ガス拡散電極膜、固体電解質膜及びそれを具備する固体高分子型燃料電池

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2010021158A1 (ja) * 2008-08-22 2010-02-25 国立大学法人東京工業大学 Ｏｈ－伝導体およびその製造方法
JP2013513705A (ja) * 2009-12-11 2013-04-22 プロメラス， エルエルシー 第四アンモニウム官能基を有するノルボルネン型ポリマー
WO2011115175A1 (ja) * 2010-03-16 2011-09-22 株式会社トクヤマ 水難溶性陰イオン伝導性樹脂

Also Published As

Publication number Publication date
JPWO2009025291A1 (ja) 2010-11-25
US20110250525A1 (en) 2011-10-13
JP5349313B2 (ja) 2013-11-20
EP2192645B1 (en) 2011-11-30
ATE535954T1 (de) 2011-12-15
EP2192645A4 (en) 2010-12-29
EP2192645A1 (en) 2010-06-02
KR101461699B1 (ko) 2014-11-13
KR20100057819A (ko) 2010-06-01

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