WO2006001419A1 - 燃料電池 - Google Patents
燃料電池 Download PDFInfo
- Publication number
- WO2006001419A1 WO2006001419A1 PCT/JP2005/011733 JP2005011733W WO2006001419A1 WO 2006001419 A1 WO2006001419 A1 WO 2006001419A1 JP 2005011733 W JP2005011733 W JP 2005011733W WO 2006001419 A1 WO2006001419 A1 WO 2006001419A1
- Authority
- WO
- WIPO (PCT)
- Prior art keywords
- fuel
- liquid fuel
- fuel cell
- liquid
- storage tank
- Prior art date
Links
Classifications
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
- H01M8/04082—Arrangements for control of reactant parameters, e.g. pressure or concentration
- H01M8/04201—Reactant storage and supply, e.g. means for feeding, pipes
- H01M8/04208—Cartridges, cryogenic media or cryogenic reservoirs
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/1009—Fuel cells with solid electrolytes with one of the reactants being liquid, solid or liquid-charged
- H01M8/1011—Direct alcohol fuel cells [DAFC], e.g. direct methanol fuel cells [DMFC]
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
- H01M8/04082—Arrangements for control of reactant parameters, e.g. pressure or concentration
- H01M8/04186—Arrangements for control of reactant parameters, e.g. pressure or concentration of liquid-charged or electrolyte-charged reactants
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
Definitions
- the present invention relates to a fuel cell, and more particularly to a small fuel cell suitable for use as a power source for portable electronic devices such as a mobile phone, a notebook personal computer, and a PDA.
- portable electronic devices such as a mobile phone, a notebook personal computer, and a PDA.
- a fuel cell includes a fuel cell in which an air electrode layer, an electrolyte layer, and a fuel electrode layer are stacked, a fuel supply unit for supplying fuel as a reducing agent to the fuel electrode layer, and an air electrode A battery that has an air supply part for supplying air as an oxidant to the layer, and causes an electrochemical reaction in the fuel cell by the fuel and oxygen in the air to obtain electric power outside.
- liquid fuel cells described in each of these patent documents supply the liquid fuel from the fuel tank to the fuel electrode by capillary force, and therefore do not require a pump for pumping the liquid fuel. There is.
- liquid fuel is injected into the cell by capillary force.
- the fuel cell system is known to be used after vaporizing the liquid fuel in the fuel vaporization layer (see, for example, Patent Document 8).
- Patent Document 8 There is a problem that it has not been improved, and the fuel cell of this structure has a problem that it is difficult to downsize because it is a system used as fuel after vaporizing the liquid
- Patent Document 1 JP-A-5-258760 (Claims, Examples, etc.)
- Patent Document 2 JP-A-5-307970 (Claims, Examples, etc.)
- Patent Document 6 Japanese Patent Laid-Open No. 2003-299946 (Claims, Examples, etc.)
- Patent Document 7 Japanese Patent Laid-Open No. 2003-340273 (Claims, Examples, etc.)
- gas-impermeable thin film member is at least one selected from a metal foil, a metal oxide deposit, and a diamond-like carbon coating.
- the storage box is formed by joining at least two parts, and at least one of the joining forces between the parts is smaller than the joining force of the liquid fuel supply valve.
- the fuel cell according to any one of (1) to (13), which is set.
- FIG. 1 is a schematic cross-sectional view showing a fuel cell according to a first embodiment of the present invention in a vertical cross-sectional manner.
- FIG. 2 is a schematic cross-sectional view showing a fuel storage tank used in the fuel cell according to the first embodiment of the present invention in a vertical cross-sectional form.
- FIG. 3 (a) to (e) show the valve body structure of the fuel outflow valve provided in the fuel outflow portion of the first embodiment of the present invention
- (a) is a perspective view of the valve body
- (b) ) Is a plan view of the valve body
- (c) is a longitudinal section view of the valve body
- (d) is a plan view of the adapter
- (e) is a longitudinal section view of the adapter
- (f) is a state in which the valve body is loaded on the adapter.
- G is a longitudinal sectional view of a state in which a valve body is loaded on an adapter.
- [FIG. 4] (a) is a perspective view of a fuel unit cell of the fuel cell according to the first embodiment of the present invention, and (b) is a longitudinal sectional view of the fuel unit cell.
- Examples of the material of the follower 14 include petroleum oils such as mineral oil, polydaricol, polyester, polybutene, and silicone oil, aliphatic metal sarcophagus, modified clay, silica gel, carbon black, natural or synthetic rubber, and various synthetics. Examples thereof include those obtained by increasing the viscosity by adding a solvent to a polymer.
- liquid fuel F is added into a sealed space 15 provided between the liquid fuel storage body 11 and the storage box body 16. Pressurizing gas to be pressed is enclosed.
- This pressurized gas pressurizes the liquid fuel F including the follower 14 accommodated in the accommodating container 12 whose rear end is opened.
- the inert gas such as nitrogen gas, argon gas, helium gas, etc.
- the pressurized state is that the liquid fuel F flows out from the fuel outflow portion 13 well, and the fuel is pressurized in the space portion 15 when left in a high temperature environment, and the liquid fuel boils.
- the pressurized state is 1200 to 3000 hPa from the viewpoint of preventing evaporation and ensuring the durability of the cartridge itself.
- a force is described for the case where no external pressurizing device is provided as the pressurizing unit, and the pressurizing unit may be provided outside the fuel storage tank as the pressurizing unit. If permitted, a device for pressurization may be provided outside the fuel storage tank.
- the space 15 and the device for pressurization can communicate with each other anywhere in the storage box 16 of the fuel storage tank and the members 16a to 16d constituting the storage box. It is desirable to provide a common member.
- the communicating member include a valve body and a vent pipe, but it is preferable to provide a vent pipe that is responsive to the pressure adjustment in consideration of adjusting the pressure.
- a cock or the like for blocking pressurized gas may be provided at any part of the communication member.
- the space 15 is formed. Further, if at least a part of the storage box 16 forms a collapsing part that allows the pressurized gas enclosed in the space to escape to the outside air when the fuel storage tank is exposed to high temperatures, the space 15 is formed. Further, when an unexpected pressure is reached, such as under a high temperature, the first fitting or collapse (break) of the joint is placed at the joint part of the joint member 16c, and the fuel supply body from the valve body of the fuel outflow part 13 is placed. It is possible to prevent a sudden fuel blowout from 30.
- This valve body 60 has a valve receiving portion 6 la in a main body portion 61, and a valve member 63 having a reverse T-shaped cross section is constantly biased to the valve receiving portion 61 by an elastic body 62 such as a spring member or a spring member.
- the liquid fuel supply member 30 is closed and is opened to supply liquid fuel.
- the liquid fuel can boil and evaporate even when left in a high temperature environment without providing an external device for pressurization. Stable supply of liquid fuel directly to the fuel electrode of the fuel cell body, loss of liquid fuel during storage, and easy use of fuel, and miniaturization of the fuel cell can be achieved. A fuel cell will be obtained.
- the fuel storage tank 10 uses three liquid fuel storage bodies 11 having the same structure, and the liquid fuel storage body 11 and the storage box body 16 are connected to each other. Fuel is supplied through a fuel supply pipe 31 inserted into the valve body 13a of the fuel outflow portion 13 and a structure in which a pressurized gas G for pressurizing the liquid fuel F is sealed in a large space portion 15a provided therebetween.
- a point connected to the supply body 30, a point provided with a follow-up auxiliary member 14 a made of PP resin body in the follower 14, and a pressurized gas G in the large space 15 a of the fuel storage tank 10 is pressurized
- a pressurizing device 70 for pressurization is provided outside the fuel storage tank 10 as a pressurizing means, and a member 16d and a large space portion 15a constituting the housing box 16 of the fuel storage tank 10 are provided in the pressurizing apparatus 70. Communicating with This is different from the first embodiment in that a vent pipe 71, which is a common member, is attached and a cock 72 that cuts off the supply of pressurized gas is provided in the vent pipe 71.
- the fuel cell of the present invention can be variously modified within the scope of the technical idea of the present invention that is not limited to the above embodiments.
- the fuel cell 20 may have a cylindrical shape, a prismatic shape, or a plate-like shape, and the fuel supply cell 30 may be connected not only in series but also in parallel. It may be.
- the direct methanol type fuel cell has been described.
- the present invention can be directly
- the present invention can be suitably applied to a polymer-modified membrane type fuel cell including a reformed type that is not limited to a methanol type fuel cell, and has a large capacity (for example, 100 ml or more).
- Tube-type fuel storage when installing liquid fuel When the diameter of the container is increased, the amount of the follower is increased accordingly, or
- a fuel storage tank having a configuration conforming to the following and FIG. 2 was prepared.
- Liquid fuel F Filled with 2g of 70wt% methanol liquid (specific gravity 0.8872).
- a gel-like follower (specific gravity 0.90) having the following composition was used.
- Mineral oil Diana process oil MC-W90 (manufactured by Idemitsu Kosan Co., Ltd.) 93 parts by weight
- Hydrophobic silica Aerosil R-974D 6 parts by weight
- Storage box 16 length 120 mm, outer diameter 14 mm, inner diameter of 12 mm, polypropylene extruded tubing [light transmittance of 95%, an oxygen gas permeability of 2500cc '25 ⁇ m / m 2 - 24hr- atm (25 ° C, 65% RH)] and sealed at both ends with a polypropylene lid.
- Fuel outlet (valve, according to Fig. 3): Length 5mm, outer diameter 6mm, inner diameter lmm, butyl rubber, stripe length 1.5mm
- Example 1 is the same as Example 1 except that the fuel storage container 12 and the storage box 16 of the fuel storage tank 10 are changed to the following configurations.
- Fuel-storing vessel 11 outer surface portion to poly Bulle alcohol [oxygen gas permeability 0. Ice ⁇ 2 5 ⁇ m / m 2 - 24hr - atm (25 ° C, 65% RH) ] was applied, length 100 mm, outer diameter 8 mm, an inner diameter of 6 mm, polypropylene tubes [light transmittance of 95%, an oxygen gas permeability of 2500cc '25 ⁇ m / m 2 - 24hr - atm (25 ° C, 65% RH) ].
- the film thickness of polybulal alcohol was 20 ⁇ m.
- Storage box 16 Poly Bulle alcohol to the outer surface portion [oxygen gas permeability 0. Ice ⁇ 25 ⁇ m / m 2 - 24hr - atm (25 ° C, 65% RH) ] was applied, length 120 mm, outer diameter 14 mm, inner diameter 12 mm, polypropylene tubes [light transmittance of 95%, an oxygen gas permeability of 2500cc '25 ⁇ m / m 2 - 24hr - atm (25 ° C, 65% RH) ] across the polypropylene lid Sealed container using.
- the film thickness of polybulu alcohol was 20 m.
- a fuel storage tank having a configuration conforming to the following and FIG. 2 was prepared.
- Fuel-storing vessel 12 length 100 mm, outer diameter 8 mm, an inner diameter of 6 mm, an inner layer of ethylene vinyl alcohol copolymer ⁇ [EVOH: oxygen gas permeability 0. 5cc - 25 ⁇ m / m 2 - 24hr- atm (25 ° C, 65% 13 ⁇ 41)], an outer layer of polypropylene [oxygen gas permeability 2500 ( ⁇ '25 1117111 2' 24hr. atm (25 ° C, 65% RH) ] coextruded tubes with [light transmittance of 95%].
- the EVOH film thickness was 100 m.
- Liquid fuel F Filled with 2g of 70wt% methanol liquid (specific gravity 0.872).
- Storage box 16 Length 120mm, outer diameter 14mm, inner diameter 12mm, inner layer is ethylene vinyl alcohol copolymer resin (EVOH: Oxygen gas permeability 0.5cc-25 ⁇ m / m 2 -24hr-atm (25 ° C, 65% 13 ⁇ 41)), outer layer co-extruded tube with polypropylene (oxygen gas permeability 2500 ( ⁇ '25 1117111 2 '24 hr ⁇ atm (25 ° C, 65% RH))) (light transmittance 95%
- the container was sealed with polypropylene covers at both ends, and the EVOH film thickness was 100 / zm.
- Example 1 is the same as Example 1 except that the fuel storage container 12 and the storage box 16 of the fuel storage tank 10 are changed to the following configurations.
- Fuel container 12 Tube with a silica vapor deposition film (GL-N, manufactured by Toppan Printing Co., Ltd.) on a polypropylene tube with a length of 100 mm, an outer diameter of 8 mm, and an inner diameter of 6 mm (light transmittance of 95%, oxygen gas permeability of 100 '25 1117111 2 '24111:'&1; 111 (25 ° ⁇ , 65% RH)].
- GL-N silica vapor deposition film
- Storage box 16 Polypropylene extruded tube with length 120mm, outer diameter 14mm, inner diameter 12mm (light transmittance 95%, oxygen gas permeability 2500cc'25 ⁇ m / m 2 -24hr-atm (25 ° C, 65% RH)) with a silica vapor deposited film (GL-N, manufactured by Toppan Printing Co., Ltd.) [light transmittance 95%, oxygen gas permeability 100 '25 1117111 2 '24111:'&1; 111 (25 ° ⁇ , 65% RH)] and sealed both ends with polypropylene lids.
- GL-N silica vapor deposited film
- the fuel storage container 12 of the fuel storage tank 10 does not include the storage box body 16 filled with the liquid fuel and follower of the first embodiment. Was used.
- the fuel emission rate is 95% to 100%.
- Fuel emission rate is 70% to less than 95%.
- Fuel emission rate is less than 70%.
- Each fuel tank was left in a constant temperature bath at 60 ° C for 30 minutes, and then the state of the fuel container was visually evaluated according to the following evaluation criteria.
- Examples 1 to 4 that fall within the scope of the present invention are superior to Reference Example 1 in terms of fuel outflow and fuel when left in a high temperature environment. It was also found to have excellent boiling prevention properties.
- liquid fuel is stably supplied and stored, and there is no loss of liquid fuel, and even when left in a high-temperature environment, boiling and evaporation of liquid fuel are unlikely to occur! understood.
- the liquid fuel reservoir of the present invention can be used for fuel storage in a small fuel cell suitable for use as a power source for portable electronic devices such as mobile phones, notebook computers, and PDAs. .
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- Life Sciences & Earth Sciences (AREA)
- Engineering & Computer Science (AREA)
- Manufacturing & Machinery (AREA)
- Sustainable Development (AREA)
- Sustainable Energy (AREA)
- Chemical & Material Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Electrochemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Fuel Cell (AREA)
Abstract
Description
Claims
Priority Applications (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
JP2006528667A JP4956187B2 (ja) | 2004-06-25 | 2005-06-27 | 燃料電池 |
US11/629,410 US7883815B2 (en) | 2004-06-25 | 2005-06-27 | Fuel-storing tank for fuel cell |
EP05765151A EP1770809B1 (en) | 2004-06-25 | 2005-06-27 | Fuel cell |
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
JP2004188177 | 2004-06-25 | ||
JP2004-188177 | 2004-06-25 |
Publications (1)
Publication Number | Publication Date |
---|---|
WO2006001419A1 true WO2006001419A1 (ja) | 2006-01-05 |
Family
ID=35781856
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
PCT/JP2005/011733 WO2006001419A1 (ja) | 2004-06-25 | 2005-06-27 | 燃料電池 |
Country Status (6)
Country | Link |
---|---|
US (1) | US7883815B2 (ja) |
EP (1) | EP1770809B1 (ja) |
JP (1) | JP4956187B2 (ja) |
KR (1) | KR100821779B1 (ja) |
CN (1) | CN100444451C (ja) |
WO (1) | WO2006001419A1 (ja) |
Families Citing this family (4)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JP5063935B2 (ja) * | 2006-06-02 | 2012-10-31 | 東洋製罐株式会社 | 燃料電池カートリッジ用ポリエステル製容器 |
DE102006030236A1 (de) * | 2006-06-30 | 2008-01-03 | Fraunhofer-Gesellschaft zur Förderung der angewandten Forschung e.V. | Direktoxidationsbrennstoffzelle für den konvektionsfreien Transport des Brennstoffs und Verfahren zum Betreiben der Brennstoffzelle |
JP4280784B2 (ja) * | 2007-07-06 | 2009-06-17 | 三菱鉛筆株式会社 | ガス発生装置 |
WO2009026441A1 (en) | 2007-08-22 | 2009-02-26 | Societe Bic | Non-interchangeable connecting valves for fuel cartridges |
Citations (14)
Publication number | Priority date | Publication date | Assignee | Title |
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JPS5966066A (ja) | 1982-10-06 | 1984-04-14 | Hitachi Ltd | 液体燃料電池 |
JPH06188008A (ja) | 1992-04-01 | 1994-07-08 | Toshiba Corp | 燃料電池 |
JP2001093551A (ja) * | 1999-09-21 | 2001-04-06 | Toshiba Corp | 燃料電池用液体燃料収容容器および燃料電池 |
JP2001102069A (ja) | 1999-09-29 | 2001-04-13 | Toshiba Corp | 燃料電池 |
JP2002121431A (ja) | 2000-10-12 | 2002-04-23 | Hiroshi Takimoto | 記録液 |
EP1313160A1 (de) | 2001-11-13 | 2003-05-21 | SFC Smart Fuel Cell AG | Vorrichtung zur Brennstoffversorgung von Brennstoffzellen |
JP2003229158A (ja) | 2001-11-28 | 2003-08-15 | Casio Comput Co Ltd | 電源システム及びその電源システムを備える電子機器 |
JP2003299946A (ja) | 2002-04-05 | 2003-10-21 | Casio Comput Co Ltd | 化学反応装置及び電源システム |
JP2003340273A (ja) | 2002-05-30 | 2003-12-02 | Casio Comput Co Ltd | 化学反応装置及び燃料電池システム並びにその製造方法 |
JP2004063200A (ja) * | 2002-07-26 | 2004-02-26 | Mitsubishi Pencil Co Ltd | 直接メタノール型燃料電池 |
JP2004247136A (ja) * | 2003-02-13 | 2004-09-02 | Nec Corp | 燃料供給カートリッジ、燃料電池装置、および燃料供給方法 |
JP2005032598A (ja) * | 2003-07-07 | 2005-02-03 | Sony Corp | 燃料タンク及びこれを用いた燃料電池システム |
JP2005038803A (ja) * | 2003-07-03 | 2005-02-10 | Tokai Corp | 燃料電池用燃料容器 |
JP2005228663A (ja) * | 2004-02-16 | 2005-08-25 | Tokai Corp | 燃料電池用燃料容器 |
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JPH05307970A (ja) | 1992-04-30 | 1993-11-19 | Aqueous Res:Kk | 液体燃料電池 |
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US6824905B2 (en) | 2001-01-15 | 2004-11-30 | Casio Computer Co., Ltd. | Power supply system and device driven by power supply system |
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2005
- 2005-06-27 CN CNB2005800211938A patent/CN100444451C/zh not_active Expired - Fee Related
- 2005-06-27 KR KR1020077000348A patent/KR100821779B1/ko not_active IP Right Cessation
- 2005-06-27 WO PCT/JP2005/011733 patent/WO2006001419A1/ja active Application Filing
- 2005-06-27 JP JP2006528667A patent/JP4956187B2/ja not_active Expired - Fee Related
- 2005-06-27 EP EP05765151A patent/EP1770809B1/en not_active Expired - Fee Related
- 2005-06-27 US US11/629,410 patent/US7883815B2/en not_active Expired - Fee Related
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JPS5966066A (ja) | 1982-10-06 | 1984-04-14 | Hitachi Ltd | 液体燃料電池 |
JPH06188008A (ja) | 1992-04-01 | 1994-07-08 | Toshiba Corp | 燃料電池 |
JP2001093551A (ja) * | 1999-09-21 | 2001-04-06 | Toshiba Corp | 燃料電池用液体燃料収容容器および燃料電池 |
JP2001102069A (ja) | 1999-09-29 | 2001-04-13 | Toshiba Corp | 燃料電池 |
JP2002121431A (ja) | 2000-10-12 | 2002-04-23 | Hiroshi Takimoto | 記録液 |
EP1313160A1 (de) | 2001-11-13 | 2003-05-21 | SFC Smart Fuel Cell AG | Vorrichtung zur Brennstoffversorgung von Brennstoffzellen |
JP2003229158A (ja) | 2001-11-28 | 2003-08-15 | Casio Comput Co Ltd | 電源システム及びその電源システムを備える電子機器 |
JP2003299946A (ja) | 2002-04-05 | 2003-10-21 | Casio Comput Co Ltd | 化学反応装置及び電源システム |
JP2003340273A (ja) | 2002-05-30 | 2003-12-02 | Casio Comput Co Ltd | 化学反応装置及び燃料電池システム並びにその製造方法 |
JP2004063200A (ja) * | 2002-07-26 | 2004-02-26 | Mitsubishi Pencil Co Ltd | 直接メタノール型燃料電池 |
JP2004247136A (ja) * | 2003-02-13 | 2004-09-02 | Nec Corp | 燃料供給カートリッジ、燃料電池装置、および燃料供給方法 |
JP2005038803A (ja) * | 2003-07-03 | 2005-02-10 | Tokai Corp | 燃料電池用燃料容器 |
JP2005032598A (ja) * | 2003-07-07 | 2005-02-03 | Sony Corp | 燃料タンク及びこれを用いた燃料電池システム |
JP2005228663A (ja) * | 2004-02-16 | 2005-08-25 | Tokai Corp | 燃料電池用燃料容器 |
Non-Patent Citations (1)
Title |
---|
See also references of EP1770809A4 * |
Also Published As
Publication number | Publication date |
---|---|
KR100821779B1 (ko) | 2008-04-14 |
EP1770809A1 (en) | 2007-04-04 |
JP4956187B2 (ja) | 2012-06-20 |
US7883815B2 (en) | 2011-02-08 |
CN100444451C (zh) | 2008-12-17 |
CN1973395A (zh) | 2007-05-30 |
EP1770809A4 (en) | 2008-07-23 |
KR20070041501A (ko) | 2007-04-18 |
JPWO2006001419A1 (ja) | 2008-04-17 |
EP1770809B1 (en) | 2012-05-30 |
US20070254198A1 (en) | 2007-11-01 |
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