JP4562775B2 - 均一加熱のための微細流路加熱器 - Google Patents
均一加熱のための微細流路加熱器 Download PDFInfo
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- JP4562775B2 JP4562775B2 JP2007536608A JP2007536608A JP4562775B2 JP 4562775 B2 JP4562775 B2 JP 4562775B2 JP 2007536608 A JP2007536608 A JP 2007536608A JP 2007536608 A JP2007536608 A JP 2007536608A JP 4562775 B2 JP4562775 B2 JP 4562775B2
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- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J19/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J19/0093—Microreactors, e.g. miniaturised or microfabricated reactors
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- C—CHEMISTRY; METALLURGY
- C01—INORGANIC CHEMISTRY
- C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
- C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
- C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
- C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
- C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
- C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
- C01B3/384—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts the catalyst being continuously externally heated
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- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F28—HEAT EXCHANGE IN GENERAL
- F28D—HEAT-EXCHANGE APPARATUS, NOT PROVIDED FOR IN ANOTHER SUBCLASS, IN WHICH THE HEAT-EXCHANGE MEDIA DO NOT COME INTO DIRECT CONTACT
- F28D9/00—Heat-exchange apparatus having stationary plate-like or laminated conduit assemblies for both heat-exchange media, the media being in contact with different sides of a conduit wall
- F28D9/0031—Heat-exchange apparatus having stationary plate-like or laminated conduit assemblies for both heat-exchange media, the media being in contact with different sides of a conduit wall the conduits for one heat-exchange medium being formed by paired plates touching each other
- F28D9/0043—Heat-exchange apparatus having stationary plate-like or laminated conduit assemblies for both heat-exchange media, the media being in contact with different sides of a conduit wall the conduits for one heat-exchange medium being formed by paired plates touching each other the plates having openings therein for circulation of at least one heat-exchange medium from one conduit to another
- F28D9/005—Heat-exchange apparatus having stationary plate-like or laminated conduit assemblies for both heat-exchange media, the media being in contact with different sides of a conduit wall the conduits for one heat-exchange medium being formed by paired plates touching each other the plates having openings therein for circulation of at least one heat-exchange medium from one conduit to another the plates having openings therein for both heat-exchange media
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- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F28—HEAT EXCHANGE IN GENERAL
- F28D—HEAT-EXCHANGE APPARATUS, NOT PROVIDED FOR IN ANOTHER SUBCLASS, IN WHICH THE HEAT-EXCHANGE MEDIA DO NOT COME INTO DIRECT CONTACT
- F28D9/00—Heat-exchange apparatus having stationary plate-like or laminated conduit assemblies for both heat-exchange media, the media being in contact with different sides of a conduit wall
- F28D9/0093—Multi-circuit heat-exchangers, e.g. integrating different heat exchange sections in the same unit or heat-exchangers for more than two fluids
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- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/06—Combination of fuel cells with means for production of reactants or for treatment of residues
- H01M8/0606—Combination of fuel cells with means for production of reactants or for treatment of residues with means for production of gaseous reactants
- H01M8/0612—Combination of fuel cells with means for production of reactants or for treatment of residues with means for production of gaseous reactants from carbon-containing material
- H01M8/0625—Combination of fuel cells with means for production of reactants or for treatment of residues with means for production of gaseous reactants from carbon-containing material in a modular combined reactor/fuel cell structure
- H01M8/0631—Reactor construction specially adapted for combination reactor/fuel cell
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/00781—Aspects relating to microreactors
- B01J2219/00783—Laminate assemblies, i.e. the reactor comprising a stack of plates
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/00781—Aspects relating to microreactors
- B01J2219/00819—Materials of construction
- B01J2219/00822—Metal
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/00781—Aspects relating to microreactors
- B01J2219/00819—Materials of construction
- B01J2219/00835—Comprising catalytically active material
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/00781—Aspects relating to microreactors
- B01J2219/00873—Heat exchange
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/00781—Aspects relating to microreactors
- B01J2219/00889—Mixing
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- C—CHEMISTRY; METALLURGY
- C01—INORGANIC CHEMISTRY
- C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
- C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
- C01B2203/02—Processes for making hydrogen or synthesis gas
- C01B2203/0205—Processes for making hydrogen or synthesis gas containing a reforming step
- C01B2203/0227—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step
-
- C—CHEMISTRY; METALLURGY
- C01—INORGANIC CHEMISTRY
- C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
- C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
- C01B2203/06—Integration with other chemical processes
- C01B2203/066—Integration with other chemical processes with fuel cells
-
- C—CHEMISTRY; METALLURGY
- C01—INORGANIC CHEMISTRY
- C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
- C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
- C01B2203/08—Methods of heating or cooling
- C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
- C01B2203/0811—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel
-
- C—CHEMISTRY; METALLURGY
- C01—INORGANIC CHEMISTRY
- C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
- C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
- C01B2203/08—Methods of heating or cooling
- C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
- C01B2203/0811—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel
- C01B2203/0822—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel the fuel containing hydrogen
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- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F28—HEAT EXCHANGE IN GENERAL
- F28F—DETAILS OF HEAT-EXCHANGE AND HEAT-TRANSFER APPARATUS, OF GENERAL APPLICATION
- F28F2260/00—Heat exchangers or heat exchange elements having special size, e.g. microstructures
- F28F2260/02—Heat exchangers or heat exchange elements having special size, e.g. microstructures having microchannels
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- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
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- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
- Y02P20/00—Technologies relating to chemical industry
- Y02P20/10—Process efficiency
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Description
炭化水素を利用する水素の生成反応は、下記の化学式1乃至化学式3のように多様な反応を利用して進行させることが可能である。
そして、前記下部プレート400には、被加熱体排出管460と排出ガス排出管450が形成される。
前記燃料供給孔275は、次で説明する燃料誘導溝381と連接される。
従って、被加熱体流入孔211と被加熱体排出孔262は隔離状態になる。
又、酸化剤孔331と排出ガス孔352は隔離された状態である。
さらに、被加熱体の移動流路には水素発生を容易にするべく、改質触媒のコーティングを必要とする。
前記燃焼用薄板200と熱伝達用薄板300の厚さに対する制限条件はないが、熱伝達用薄板300の場合、同一の体積内に大きい比表面積を確保するために、微細流路の幅と深さを考慮して薄板の厚さを決める必要がある。
また、この時、進行させようとする反応の形態を考慮して薄板の厚さを決定する必要がある。
また、炭化水素の燃焼が進行される薄板の場合は、0.1〜1mmの薄板を使用し、この表面に酸化触媒をコーティングして加熱システムを構成することが好ましい。
110 被加熱体流入管
111 被加熱体流入口
120 燃料流入管
121 燃料流入口
130 酸化剤流入管
131 酸化剤流入口
200 燃焼用薄板
211311 被加熱体流入孔
221,321 燃料孔
231,331 酸化剤孔
252,352 排出ガス孔
262,362 被加熱体排出孔
271 混合溝
275 燃料供給孔
381 燃料誘導溝
291,391 微細流路溝
300 熱伝達用薄板
400 下部プレート
450 排出ガス排出管
452 排出ガス排出口
460 被加熱体排出管
462 被加熱体排出口
Claims (3)
- 被加熱体流入口、燃料流入口、および酸化剤流入口を包含する上部プレートと;
被加熱体排出口および排出ガス排出口を包含する下部プレートと;
前記上部プレートと前記下部プレートとの間に交互に積層された複数の燃焼用薄板および複数の熱伝達用薄板とを包含する均一加熱のための微細流路加熱器であって;
前記燃焼用薄板と前記熱伝達用薄板の各薄板に、被加熱体流入孔、被加熱体排出孔、酸化剤孔、排出ガス孔、燃料孔、および微細流路溝が一致する位置にそれぞれ形成され;
前記燃焼用薄板の前記排出ガス孔と前記酸化剤孔とが前記微細流路溝によって連通され;
前記熱伝達用薄板の前記被加熱体流入孔と前記被加熱体排出孔とが前記微細流路溝によって連通され;
前記燃焼用薄板は、さらに前記微細流路溝と前記酸化剤孔を連通する混合溝に形成される燃料供給孔を有し、該燃料供給孔は前記熱伝達用薄板の前記燃料孔に連通された燃料誘導溝と連通して前記混合溝に燃料を供給し;
前記上部プレートおよび該上部プレートの下部面に接する前記燃焼用薄板は、前記上部プレートにおける前記被加熱体流入口、燃料流入口、および酸化剤流入口が、前記燃焼用薄板における前記被加熱体流入孔、前記燃料孔、および前記酸化剤孔とそれぞれ一致するように位置決めされ;
前記下部プレートおよび該下部プレートの上部面に接する前記熱伝達用薄板は、前記下部プレートにおける前記被加熱体排出口および前記排出ガス排出口が、前記熱伝達用薄板における前記被加熱体排出孔および前記排出ガス孔とそれぞれ一致するように位置決めされる均一加熱のための微細流路加熱器。 - 前記燃焼用薄板の微細流路溝に酸化触媒が塗布されている請求項1に記載の均一加熱のための微細流路加熱器。
- 前記熱伝達用薄板の微細流路溝に炭化水素の改質触媒が塗布されている請求項1に記載の均一加熱のための微細流路加熱器。
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
KR1020040080918A KR100599382B1 (ko) | 2004-10-11 | 2004-10-11 | 균일가열을 위한 미세유로 가열기 |
PCT/KR2005/003384 WO2006085715A1 (en) | 2004-10-11 | 2005-10-11 | Micro channel heater for even heating |
Publications (2)
Publication Number | Publication Date |
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JP2008518184A JP2008518184A (ja) | 2008-05-29 |
JP4562775B2 true JP4562775B2 (ja) | 2010-10-13 |
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JP2007536608A Active JP4562775B2 (ja) | 2004-10-11 | 2005-10-11 | 均一加熱のための微細流路加熱器 |
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US (1) | US7927750B2 (ja) |
JP (1) | JP4562775B2 (ja) |
KR (1) | KR100599382B1 (ja) |
CN (1) | CN100486017C (ja) |
WO (1) | WO2006085715A1 (ja) |
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KR20110074970A (ko) * | 2008-07-31 | 2011-07-05 | 조지아 테크 리서치 코포레이션 | 마이크로스케일 열 또는 열 및 물질 전달 시스템 |
KR101136859B1 (ko) * | 2010-02-09 | 2012-04-20 | 한국에너지기술연구원 | 미세유로 가열기를 이용한 탄화수소 개질장치 |
KR101200930B1 (ko) | 2010-05-04 | 2012-11-13 | 한국과학기술연구원 | 마이크로-매크로 채널 반응기 |
CN103687803B (zh) * | 2011-04-15 | 2016-04-27 | 韩国能源技术研究院 | 使用微通道加热器的烃重整装置 |
KR101271398B1 (ko) * | 2011-05-09 | 2013-06-11 | 한국에너지기술연구원 | 미세유로 가열기를 이용한 적층형 탄화수소 개질장치 |
JP5961941B2 (ja) * | 2011-07-27 | 2016-08-03 | 株式会社Ihi | 密閉式ガスヒータおよび密閉式ガスヒータを用いた連続加熱炉 |
KR101256816B1 (ko) * | 2011-08-11 | 2013-04-22 | 한국에너지기술연구원 | 관통형 금속촉매가 내장된 마이크로채널 wgs 반응장치 |
CN104555919B (zh) * | 2014-12-24 | 2016-08-24 | 浙江大学 | 反应载体表面多孔化的自热型醇类制氢微重整器 |
SG11201709564VA (en) * | 2015-06-08 | 2017-12-28 | Ihi Corp | Reactor |
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DE19746251C2 (de) * | 1997-10-20 | 1999-09-09 | Dbb Fuel Cell Engines Gmbh | Anlage zur Wasserdampfreformierung eines Kohlenwasserstoffs und Betriebsverfahren hierfür |
ATE261436T1 (de) | 2000-09-06 | 2004-03-15 | Roche Vitamins Ag | Verfahren zu herstellung von substituierten pyranen |
JP2002164066A (ja) * | 2000-11-22 | 2002-06-07 | Mitsubishi Heavy Ind Ltd | 積層型熱交換器 |
JP2002195777A (ja) | 2000-12-28 | 2002-07-10 | Calsonic Kansei Corp | 熱交換器 |
JP4964368B2 (ja) * | 2001-01-17 | 2012-06-27 | 本田技研工業株式会社 | 燃料電池用燃料ガス生成装置 |
JP2002352841A (ja) * | 2001-05-30 | 2002-12-06 | Nissan Motor Co Ltd | 水蒸気改質反応器 |
JP4363002B2 (ja) * | 2002-04-18 | 2009-11-11 | 日産自動車株式会社 | 燃料改質システムとその暖機装置 |
JP4423847B2 (ja) * | 2002-10-25 | 2010-03-03 | カシオ計算機株式会社 | 小型化学反応装置 |
JP2004261911A (ja) | 2003-02-28 | 2004-09-24 | Mitsubishi Heavy Ind Ltd | チャンネル構造体及びその製造方法 |
KR100437135B1 (ko) | 2004-02-24 | 2004-07-03 | 주식회사 스펙 | 마이크로 열교환기 및 제작방법 |
KR100473504B1 (ko) * | 2004-09-13 | 2005-03-09 | 주식회사 스펙 | 마이크로 믹서 |
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- 2004-10-11 KR KR1020040080918A patent/KR100599382B1/ko active IP Right Grant
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2005
- 2005-10-11 US US11/576,156 patent/US7927750B2/en active Active
- 2005-10-11 CN CNB2005800347088A patent/CN100486017C/zh active Active
- 2005-10-11 JP JP2007536608A patent/JP4562775B2/ja active Active
- 2005-10-11 WO PCT/KR2005/003384 patent/WO2006085715A1/en active Application Filing
Also Published As
Publication number | Publication date |
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KR100599382B1 (ko) | 2006-07-12 |
JP2008518184A (ja) | 2008-05-29 |
US7927750B2 (en) | 2011-04-19 |
CN100486017C (zh) | 2009-05-06 |
WO2006085715A1 (en) | 2006-08-17 |
KR20060031935A (ko) | 2006-04-14 |
CN101040400A (zh) | 2007-09-19 |
US20080050634A1 (en) | 2008-02-28 |
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