JP2015532929A - リグニンを有用化合物に変換する改善された方法 - Google Patents

リグニンを有用化合物に変換する改善された方法 Download PDF

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Publication number
JP2015532929A
JP2015532929A JP2015538336A JP2015538336A JP2015532929A JP 2015532929 A JP2015532929 A JP 2015532929A JP 2015538336 A JP2015538336 A JP 2015538336A JP 2015538336 A JP2015538336 A JP 2015538336A JP 2015532929 A JP2015532929 A JP 2015532929A
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Prior art keywords
lignin
reactor
catalyst
slurry
conversion
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Pending
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JP2015538336A
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English (en)
Japanese (ja)
Inventor
シャルマ、クリシュナ
マーレー、アロン
リバ、スティーヴン
ガスタルド、ダン
エリオット、グリッツ・アーフ
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Biochemtex SpA
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Biochemtex SpA
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Priority claimed from PCT/EP2013/053626 external-priority patent/WO2013124457A2/fr
Priority claimed from US13/775,229 external-priority patent/US20130225853A1/en
Priority claimed from US13/775,242 external-priority patent/US9340476B2/en
Application filed by Biochemtex SpA filed Critical Biochemtex SpA
Publication of JP2015532929A publication Critical patent/JP2015532929A/ja
Pending legal-status Critical Current

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    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C27/00—Processes involving the simultaneous production of more than one class of oxygen-containing compounds
    • C07C27/04—Processes involving the simultaneous production of more than one class of oxygen-containing compounds by reduction of oxygen-containing compounds
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G3/00—Production of liquid hydrocarbon mixtures from oxygen-containing organic materials, e.g. fatty oils, fatty acids
    • C10G3/50—Production of liquid hydrocarbon mixtures from oxygen-containing organic materials, e.g. fatty oils, fatty acids in the presence of hydrogen, hydrogen donors or hydrogen generating compounds
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G3/00—Production of liquid hydrocarbon mixtures from oxygen-containing organic materials, e.g. fatty oils, fatty acids
    • C10G3/50—Production of liquid hydrocarbon mixtures from oxygen-containing organic materials, e.g. fatty oils, fatty acids in the presence of hydrogen, hydrogen donors or hydrogen generating compounds
    • C10G3/52—Hydrogen in a special composition or from a special source
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G45/00—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
    • C10G45/02—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G45/00—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
    • C10G45/02—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing
    • C10G45/04—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G45/00—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
    • C10G45/02—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing
    • C10G45/04—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used
    • C10G45/06—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used containing nickel or cobalt metal, or compounds thereof
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G45/00—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
    • C10G45/02—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing
    • C10G45/04—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used
    • C10G45/06—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used containing nickel or cobalt metal, or compounds thereof
    • C10G45/08—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used containing nickel or cobalt metal, or compounds thereof in combination with chromium, molybdenum, or tungsten metals, or compounds thereof
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/10—Feedstock materials
    • C10G2300/1011—Biomass
    • C10G2300/1014—Biomass of vegetal origin
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2400/00—Products obtained by processes covered by groups C10G9/00 - C10G69/14
    • C10G2400/02—Gasoline
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2400/00—Products obtained by processes covered by groups C10G9/00 - C10G69/14
    • C10G2400/04—Diesel oil
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2400/00—Products obtained by processes covered by groups C10G9/00 - C10G69/14
    • C10G2400/06—Gasoil
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2400/00—Products obtained by processes covered by groups C10G9/00 - C10G69/14
    • C10G2400/08—Jet fuel
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G45/00—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P30/00—Technologies relating to oil refining and petrochemical industry
    • Y02P30/20—Technologies relating to oil refining and petrochemical industry using bio-feedstock

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  • Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Processing Of Solid Wastes (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Catalysts (AREA)
  • Low-Molecular Organic Synthesis Reactions Using Catalysts (AREA)
JP2015538336A 2012-10-28 2013-07-09 リグニンを有用化合物に変換する改善された方法 Pending JP2015532929A (ja)

Applications Claiming Priority (39)

Application Number Priority Date Filing Date Title
US201261719486P 2012-10-28 2012-10-28
US61/719,486 2012-10-28
US201361751919P 2013-01-13 2013-01-13
US61/751,919 2013-01-13
US201361764611P 2013-02-14 2013-02-14
US61/764,611 2013-02-14
US201361765402P 2013-02-15 2013-02-15
US61/765,402 2013-02-15
EPPCT/EP2013/053629 2013-02-22
EPPCT/EP2013/053628 2013-02-22
EPPCT/EP2013/053630 2013-02-22
USPCT/US2013/027393 2013-02-22
EPPCT/EP2013/053625 2013-02-22
PCT/EP2013/053626 WO2013124457A2 (fr) 2012-02-24 2013-02-22 Procédé continu de conversion de lignine en composés utiles
PCT/EP2013/053629 WO2013124459A2 (fr) 2012-02-24 2013-02-22 Procédé continu de conversion de lignine en composés utiles
PCT/US2013/027393 WO2013142006A2 (fr) 2012-02-24 2013-02-22 Procédé en continu de conversion de la lignine en composés utiles
EPPCT/EP2013/053631 2013-02-22
PCT/EP2013/053630 WO2013124460A2 (fr) 2012-02-24 2013-02-22 Procédé continu de conversion de lignine en composés utiles
PCT/EP2013/053628 WO2013124458A2 (fr) 2012-02-24 2013-02-22 Procédé continu de conversion de lignine en composés utiles
PCT/EP2013/053625 WO2013124456A2 (fr) 2012-02-24 2013-02-22 Procédé continu destiné à la conversion de lignine en composés utiles
EPPCT/EP2013/053626 2013-02-22
PCT/EP2013/053631 WO2013124461A2 (fr) 2012-02-24 2013-02-22 Procédé continu destiné à la conversion de lignine en composés utiles
US13/775,229 US20130225853A1 (en) 2012-02-24 2013-02-24 Continuous process for conversion of lignin to useful compounds
US13/775,238 US9035117B2 (en) 2012-02-24 2013-02-24 Continuous process for conversion of lignin to useful compounds
US13/775,239 US9732021B2 (en) 2012-02-24 2013-02-24 Continuous process for conversion of lignin to useful compounds
US13/775,239 2013-02-24
US13/775,242 US9340476B2 (en) 2012-02-24 2013-02-24 Continuous process for conversion of lignin to useful compounds
US13/775,242 2013-02-24
US13/775,238 2013-02-24
US13/775,241 2013-02-24
US13/775,230 US9139501B2 (en) 2012-02-24 2013-02-24 Continuous process for conversion of lignin to useful compounds
US13/775,230 2013-02-24
US13/775,229 2013-02-24
US13/775,241 US20130225856A1 (en) 2012-02-24 2013-02-24 Continuous process for conversion of lignin to useful compounds
US13/775,240 US9162951B2 (en) 2012-02-24 2013-02-24 Continuous process for conversion of lignin to useful compounds
US13/775,240 2013-02-24
US201361837262P 2013-06-20 2013-06-20
US61/837,262 2013-06-20
PCT/EP2013/064456 WO2014063842A1 (fr) 2012-10-28 2013-07-09 Procédé de conversion de lignine en composés utiles

Publications (1)

Publication Number Publication Date
JP2015532929A true JP2015532929A (ja) 2015-11-16

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JP2015538336A Pending JP2015532929A (ja) 2012-10-28 2013-07-09 リグニンを有用化合物に変換する改善された方法

Country Status (6)

Country Link
JP (1) JP2015532929A (fr)
CN (1) CN104854219A (fr)
CA (1) CA2889701A1 (fr)
RU (1) RU2015119801A (fr)
WO (1) WO2014063842A1 (fr)
ZA (1) ZA201503790B (fr)

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2015536926A (ja) * 2012-10-28 2015-12-24 バイオケムテック・ソチエタ・ペル・アチオニＢｉｏｃｈｅｍｔｅｘ Ｓ．Ｐ．Ａ． リグニンを有用化合物に変換する連続法
JP2018062492A (ja) * 2016-10-14 2018-04-19 株式会社Kri リグニン含有バイオマスからフェノール類の製造方法
KR20190111264A (ko) * 2018-03-22 2019-10-02 한국과학기술연구원 바이오매스를 이용한 고리형 및/또는 방향족 화합물의 제조방법

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WO2016058621A1 (fr) * 2014-10-16 2016-04-21 Biochemtex S.P.A. Composition d'origine biologique
CN109289903B (zh) * 2018-09-19 2020-09-22 华南理工大学 一种用于木质素加氢解聚的HZSM-5负载型Fe-Pd双金属催化剂及其制备方法
CN111217679B (zh) * 2018-11-27 2022-07-22 中国科学院大连化学物理研究所 一种双功能催化剂一步法解聚木质素到苯酚的方法
US12065618B2 (en) * 2020-05-06 2024-08-20 Gti Energy Hydrodeoxygenation of oxygenated polymers to liquid hydrocarbons

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JP2010505034A (ja) * 2006-09-26 2010-02-18 ユーオーピー エルエルシー 一工程水素化分解による、リグニン及びセルロース廃棄物からの、ガソリン、ディーゼル、ナフテン類及び芳香族化合物の製造
WO2011117705A2 (fr) * 2010-03-24 2011-09-29 Eni S.P.A. Procédé pour la conversion de lignine en hydrocarbures liquides

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CN102476980B (zh) * 2010-11-30 2014-06-04 中国科学院大连化学物理研究所 钨基催化剂在木质素催化加氢制芳香族化合物中的应用
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JP2003260359A (ja) * 2002-01-22 2003-09-16 Kataleuna Gmbh Catalysts 球状の金属含有触媒、その製造方法及び芳香族化合物の水素化方法
JP2010505034A (ja) * 2006-09-26 2010-02-18 ユーオーピー エルエルシー 一工程水素化分解による、リグニン及びセルロース廃棄物からの、ガソリン、ディーゼル、ナフテン類及び芳香族化合物の製造
WO2011117705A2 (fr) * 2010-03-24 2011-09-29 Eni S.P.A. Procédé pour la conversion de lignine en hydrocarbures liquides

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2015536926A (ja) * 2012-10-28 2015-12-24 バイオケムテック・ソチエタ・ペル・アチオニＢｉｏｃｈｅｍｔｅｘ Ｓ．Ｐ．Ａ． リグニンを有用化合物に変換する連続法
JP2018062492A (ja) * 2016-10-14 2018-04-19 株式会社Kri リグニン含有バイオマスからフェノール類の製造方法
KR20190111264A (ko) * 2018-03-22 2019-10-02 한국과학기술연구원 바이오매스를 이용한 고리형 및/또는 방향족 화합물의 제조방법
KR102110466B1 (ko) 2018-03-22 2020-05-13 한국과학기술연구원 바이오매스를 이용한 고리형 및/또는 방향족 화합물의 제조방법

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CN104854219A (zh) 2015-08-19
RU2015119801A (ru) 2016-12-20
CA2889701A1 (fr) 2014-05-01
ZA201503790B (en) 2016-08-31
WO2014063842A1 (fr) 2014-05-01

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