EP1989157A1 - Mélanges de matériaux de construction contenant des additifs sous forme de microparticules gonflant dans le mélange de matériaux - Google Patents
Mélanges de matériaux de construction contenant des additifs sous forme de microparticules gonflant dans le mélange de matériauxInfo
- Publication number
- EP1989157A1 EP1989157A1 EP07704234A EP07704234A EP1989157A1 EP 1989157 A1 EP1989157 A1 EP 1989157A1 EP 07704234 A EP07704234 A EP 07704234A EP 07704234 A EP07704234 A EP 07704234A EP 1989157 A1 EP1989157 A1 EP 1989157A1
- Authority
- EP
- European Patent Office
- Prior art keywords
- shell
- microparticles
- building material
- core
- polymeric core
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Withdrawn
Links
Classifications
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B24/00—Use of organic materials as active ingredients for mortars, concrete or artificial stone, e.g. plasticisers
- C04B24/24—Macromolecular compounds
- C04B24/26—Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B24/00—Use of organic materials as active ingredients for mortars, concrete or artificial stone, e.g. plasticisers
- C04B24/24—Macromolecular compounds
- C04B24/26—Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds
- C04B24/2641—Polyacrylates; Polymethacrylates
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B16/00—Use of organic materials as fillers, e.g. pigments, for mortars, concrete or artificial stone; Treatment of organic materials specially adapted to enhance their filling properties in mortars, concrete or artificial stone
- C04B16/04—Macromolecular compounds
- C04B16/08—Macromolecular compounds porous, e.g. expanded polystyrene beads or microballoons
- C04B16/085—Macromolecular compounds porous, e.g. expanded polystyrene beads or microballoons expanded in situ, i.e. during or after mixing the mortar, concrete or artificial stone ingredients
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B24/00—Use of organic materials as active ingredients for mortars, concrete or artificial stone, e.g. plasticisers
- C04B24/04—Carboxylic acids; Salts, anhydrides or esters thereof
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B24/00—Use of organic materials as active ingredients for mortars, concrete or artificial stone, e.g. plasticisers
- C04B24/24—Macromolecular compounds
- C04B24/26—Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds
- C04B24/2664—Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds of ethylenically unsaturated dicarboxylic acid polymers, e.g. maleic anhydride copolymers
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B28/00—Compositions of mortars, concrete or artificial stone, containing inorganic binders or the reaction product of an inorganic and an organic binder, e.g. polycarboxylate cements
- C04B28/02—Compositions of mortars, concrete or artificial stone, containing inorganic binders or the reaction product of an inorganic and an organic binder, e.g. polycarboxylate cements containing hydraulic cements other than calcium sulfates
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B2103/00—Function or property of ingredients for mortars, concrete or artificial stone
- C04B2103/0045—Polymers chosen for their physico-chemical characteristics
- C04B2103/0049—Water-swellable polymers
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B2103/00—Function or property of ingredients for mortars, concrete or artificial stone
- C04B2103/0045—Polymers chosen for their physico-chemical characteristics
- C04B2103/0057—Polymers chosen for their physico-chemical characteristics added as redispersable powders
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B2103/00—Function or property of ingredients for mortars, concrete or artificial stone
- C04B2103/0045—Polymers chosen for their physico-chemical characteristics
- C04B2103/0065—Polymers characterised by their glass transition temperature (Tg)
-
- C—CHEMISTRY; METALLURGY
- C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
- C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
- C04B2111/00—Mortars, concrete or artificial stone or mixtures to prepare them, characterised by specific function, property or use
- C04B2111/20—Resistance against chemical, physical or biological attack
- C04B2111/29—Frost-thaw resistance
Definitions
- the structure of a cement-bound concrete is traversed by capillary pores (radius: 2 ⁇ m - 2 mm) or gel pores (radius: 2 - 50 nm). Pore water contained therein differs in its state form depending on the pore diameter.
- These hydrophobic salts reduce the surface tension of the water and accumulate at the interface between cement grain, air and water. They stabilize the microbubbles and are therefore found in the hardening concrete on the surfaces of these air pores again.
- the notation (meth) acrylate as used herein means both methacrylate, e.g. Methyl methacrylate, ethyl methacrylate, etc., as well as acrylate, e.g. Methyl acrylate, ethyl acrylate, etc., as well as mixtures of both.
- the shell (B) consists predominantly of nonionic, ethylenically unsaturated monomers.
- Preferred such monomers are styrene, butadiene, vinyltoluene, ethylene, vinyl acetate, vinyl chloride, vinylidene chloride, acrylonitrile, acrylamide, methacrylamide, C1-C12-alkyl esters of (meth) acrylic acid or mixtures thereof.
- Tg (P) denotes the glass transition temperature of the copolymer to be calculated in degrees Kelvin.
- Tg (A), Tg (B), Tg (C), etc. designate the respective glass transition temperatures (in degrees Kelvin) of the high molecular weight homopolymers of monomers A, B, C, etc. measured by dynamic heat flow differential calorimetry (Dynamic Scanning Calorimetry, DSC).
- the polymer content of the microparticles used can be from 2 to 98% by weight (weight of polymer based on the total weight of the water-filled particle).
Landscapes
- Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Ceramic Engineering (AREA)
- Materials Engineering (AREA)
- Structural Engineering (AREA)
- Organic Chemistry (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Inorganic Chemistry (AREA)
- Curing Cements, Concrete, And Artificial Stone (AREA)
- Graft Or Block Polymers (AREA)
Abstract
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
DE102006009842A DE102006009842A1 (de) | 2006-03-01 | 2006-03-01 | Additive Baustoffmischungen mit Mikropartikeln die in der Mischung quellen |
PCT/EP2007/050882 WO2007099005A1 (fr) | 2006-03-01 | 2007-01-30 | Mélanges de matériaux de construction contenant des additifs sous forme de microparticules gonflant dans le mélange de matériaux |
Publications (1)
Publication Number | Publication Date |
---|---|
EP1989157A1 true EP1989157A1 (fr) | 2008-11-12 |
Family
ID=37964600
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
EP07704234A Withdrawn EP1989157A1 (fr) | 2006-03-01 | 2007-01-30 | Mélanges de matériaux de construction contenant des additifs sous forme de microparticules gonflant dans le mélange de matériaux |
Country Status (11)
Country | Link |
---|---|
US (1) | US20070208107A1 (fr) |
EP (1) | EP1989157A1 (fr) |
JP (1) | JP5473337B2 (fr) |
KR (1) | KR20080102140A (fr) |
CN (1) | CN101028970B (fr) |
BR (1) | BRPI0708410A2 (fr) |
CA (1) | CA2644507A1 (fr) |
DE (1) | DE102006009842A1 (fr) |
MX (1) | MX2008011030A (fr) |
RU (1) | RU2432337C2 (fr) |
WO (1) | WO2007099005A1 (fr) |
Families Citing this family (24)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US7498373B2 (en) * | 2001-02-07 | 2009-03-03 | Roehm Gmbh & Co. Kg | Hot sealing compound for aluminum foils applied to polypropylene and polystyrene |
DE10350786A1 (de) * | 2003-10-29 | 2005-06-02 | Röhm GmbH & Co. KG | Mischungen zur Herstellung von Reaktivschmelzklebstoffen sowie daraus erhältliche Reaktivschmelzklebstoffe |
DE102004035937A1 (de) * | 2004-07-23 | 2006-02-16 | Röhm GmbH & Co. KG | Plastisole mit verringerter Wasseraufnahme |
DE102005042389A1 (de) * | 2005-06-17 | 2006-12-28 | Röhm Gmbh | Heißversiegelungsmasse für Aluminium- und Polyethylenterephthalatfolien gegen Polypropylen-Polyvinylchlorid- und Polystyrolbehälter |
DE102005045458A1 (de) * | 2005-09-22 | 2007-03-29 | Röhm Gmbh | Verfahren zur Herstellung von ABA-Triblockcopolymeren auf (Meth)acrylatbasis |
DE102005052130A1 (de) * | 2005-10-28 | 2007-05-03 | Röhm Gmbh | Spritzbare Akustikmassen |
DE102006007563A1 (de) * | 2006-02-16 | 2007-08-30 | Röhm Gmbh | Verfahren zum Verkleben von Werkstoffen mit nanoskaligen superparamagnetischen Poly(meth)acrylatpolymeren |
DE102006009511A1 (de) * | 2006-02-28 | 2007-08-30 | Röhm Gmbh | Synthese von Polyester-pfropf-Poly(meth)acrylat |
DE102006009586A1 (de) * | 2006-02-28 | 2007-09-06 | Röhm Gmbh | Heißversiegelungsmasse für Aluminium- und Polyethylenterephthalatfolien gegen Polypropylen-Polyvinylchlorid- und Polystyrolbehälter |
DE102006015846A1 (de) * | 2006-04-03 | 2007-10-04 | Röhm Gmbh | Kupferentfernung aus ATRP-Produkten mittels Zugabe von Schwefelverbindungen |
DE102006035726A1 (de) | 2006-07-28 | 2008-01-31 | Evonik Röhm Gmbh | Verfahren zur Herstellung von ABA-Triblockcopolymeren auf (Meth)acrylatbasis |
DE102006037352A1 (de) * | 2006-08-09 | 2008-02-14 | Evonik Röhm Gmbh | Verfahren zur Herstellung von säureterminierten ATRP-Produkten |
DE102006037351A1 (de) * | 2006-08-09 | 2008-02-14 | Evonik Röhm Gmbh | Verfahren zur Herstellung von hydroxytelecheler ATRP-Produkten |
DE102006048154A1 (de) * | 2006-10-10 | 2008-04-17 | Evonik Röhm Gmbh | Verfahren zur Herstellung von silyltelechelen Polymeren |
DE102006057145A1 (de) * | 2006-11-22 | 2008-05-29 | Evonik Röhm Gmbh | Verfahren zur Herstellung verbesserter Bindemittel für Plastisole |
CN102050637B (zh) * | 2010-11-23 | 2012-11-14 | 哈尔滨工业大学深圳研究生院 | 一种泡沫混凝土材料、泡沫混凝土及制备方法 |
JP5353916B2 (ja) * | 2011-02-01 | 2013-11-27 | トヨタ自動車株式会社 | 絶縁樹脂材料の製造方法 |
KR101308094B1 (ko) * | 2011-04-18 | 2013-09-12 | 계명대학교 산학협력단 | 코어-쉘 구조를 갖는 시멘트 페이스트의 마이크로캡슐 흡수제 및 그 제조방법 |
US9333685B2 (en) | 2012-04-19 | 2016-05-10 | AkzoNobel Chemicals International B.V. | Apparatus and system for expanding expandable polymeric microspheres |
US9365453B2 (en) * | 2012-04-19 | 2016-06-14 | Construction Research & Technology Gmbh | Admixture and method for freeze-thaw damage resistance and scaling damage resistance of cementitious compositions |
DE102012213978A1 (de) * | 2012-08-07 | 2014-02-13 | Evonik Degussa Gmbh | Unterkritisch formulierte Beschichtungen |
US10640422B2 (en) | 2013-12-06 | 2020-05-05 | Construction Research & Technology Gmbh | Method of manufacturing cementitious compositions |
RU2562313C1 (ru) * | 2014-08-01 | 2015-09-10 | федеральное государственное автономное образовательное учреждение высшего образования "Нижегородский государственный университет им. Н.И. Лобачевского" | Цементная композиция |
WO2020045515A1 (fr) * | 2018-08-31 | 2020-03-05 | 株式会社日本触媒 | Additif pour matériau hydraulique |
Citations (2)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE19833061A1 (de) * | 1998-07-22 | 2000-02-03 | Elotex Ag Sempach Station | Verfahren zur Herstellung wäßriger Dispersionen von Latexteilchen mit heterogener Morphologie, die mit dem Verfahren erhältlichen Latexteilchen, die Dispersionen und redispergierbaren Pulver sowie deren Verwendung |
US20050284340A1 (en) * | 2004-06-15 | 2005-12-29 | Vickers Thomas M Jr | Providing freezing and thawing resistance to cementitious compositions |
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NL7505525A (nl) * | 1975-05-12 | 1976-11-16 | Akzo Nv | Werkwijze voor de bereiding van een vorstbesten- dig beton. |
US4594363A (en) * | 1985-01-11 | 1986-06-10 | Rohm And Haas Company | Production of core-sheath polymer particles containing voids, resulting product and use |
US5328952A (en) * | 1992-02-14 | 1994-07-12 | Rohm And Haas Company | Multi-stage polymer latex cement modifier and process of making |
EP0654454A1 (fr) * | 1993-11-22 | 1995-05-24 | Rohm And Haas Company | Poudre de polymère coeur/enveloppe |
EP0725092A3 (fr) * | 1995-02-06 | 1997-08-27 | Chemie Linz Gmbh | Poudre redispersible de polymère coeur-enveloppe, sa préparation et son usage |
JPH08217513A (ja) * | 1995-02-09 | 1996-08-27 | Mitsubishi Chem Basf Co Ltd | ポリマーセメント組成物 |
US6288174B1 (en) * | 1995-07-07 | 2001-09-11 | Mitsubishi Rayon Co., Ltd. | Powdery material and modifier for cementitious material |
JPH09110495A (ja) * | 1995-10-12 | 1997-04-28 | Lion Corp | 半たわみ性舗装用ポリマーエマルジョン |
ID18920A (id) * | 1996-11-15 | 1998-05-20 | Rohm & Haas | Komposisi lapisan dengan gloss rendah |
JPH10152357A (ja) * | 1996-11-18 | 1998-06-09 | Mitsui Chem Inc | 押出成形用水硬性モルタル組成物、セメント成形体の製造方法、セメント成形体、及び、セメント硬化体形成方法 |
US6498209B1 (en) * | 1998-03-31 | 2002-12-24 | Roehm Gmbh & Co. Kg | Poly(meth)acrylate plastisols |
DE19826412C2 (de) * | 1998-06-16 | 2002-10-10 | Roehm Gmbh | Geruchsvermindertes, kalthärtendes (Meth)acrylat-Reaktionsharz für Bodenbeschichtungen, dieses Reaktionsharz aufweisende Bodenbeschichtungen sowie Verfahren zur Herstellung solcher Bodenbeschichtungen |
DE19833062A1 (de) * | 1998-07-22 | 2000-02-03 | Elotex Ag Sempach Station | Redispergierbares Pulver und dessen wäßrige Dispersion, Verfahren zur Herstellung sowie Verwendung |
DE19928352A1 (de) * | 1999-06-21 | 2000-12-28 | Roehm Gmbh | Verbesserte Poly(meth)acrylatptastisole und Verfahren zu ihrer Herstellung |
JP2001253742A (ja) * | 2000-03-10 | 2001-09-18 | Lion Corp | 水硬性無機質硬化体の凍結融解抵抗性向上剤 |
KR100867391B1 (ko) * | 2000-09-21 | 2008-11-06 | 롬 앤드 하스 캄파니 | 가볍게 개질된 점토 및 이를 포함하는 조성물의 에멀젼중합 방법 |
US7498373B2 (en) * | 2001-02-07 | 2009-03-03 | Roehm Gmbh & Co. Kg | Hot sealing compound for aluminum foils applied to polypropylene and polystyrene |
JP4282982B2 (ja) * | 2001-12-26 | 2009-06-24 | 旭化成ケミカルズ株式会社 | 樹脂モルタル用ラテックス及び樹脂モルタル組成物 |
DE10227898A1 (de) * | 2002-06-21 | 2004-01-15 | Röhm GmbH & Co. KG | Verfahren zur Herstellung sprühgetrockneter Poly(meth)acrylatpolymere, ihre Verwendung als Polymerkomponente für Plastisole und damit hergestellte Plastisole |
JP2004238245A (ja) * | 2003-02-05 | 2004-08-26 | Sekisui Chem Co Ltd | 金属スラグ含有セメント組成物 |
DE10350786A1 (de) * | 2003-10-29 | 2005-06-02 | Röhm GmbH & Co. KG | Mischungen zur Herstellung von Reaktivschmelzklebstoffen sowie daraus erhältliche Reaktivschmelzklebstoffe |
DE102004035937A1 (de) * | 2004-07-23 | 2006-02-16 | Röhm GmbH & Co. KG | Plastisole mit verringerter Wasseraufnahme |
DE102005042389A1 (de) * | 2005-06-17 | 2006-12-28 | Röhm Gmbh | Heißversiegelungsmasse für Aluminium- und Polyethylenterephthalatfolien gegen Polypropylen-Polyvinylchlorid- und Polystyrolbehälter |
DE102005046681A1 (de) * | 2005-09-29 | 2007-04-05 | Construction Research & Technology Gmbh | Verwendung von polymeren Mikropartikeln in Baustoffmischungen |
DE102006008969A1 (de) * | 2006-02-23 | 2007-08-30 | Röhm Gmbh | Additive Baustoffmischungen mit Mikropartikeln mit sehr dünnen Schalen |
DE102006008965A1 (de) * | 2006-02-23 | 2007-08-30 | Röhm Gmbh | Additive Baustoffmischungen mit Mikropartikeln verschiedener Größe |
-
2006
- 2006-03-01 DE DE102006009842A patent/DE102006009842A1/de not_active Withdrawn
- 2006-03-24 US US11/387,977 patent/US20070208107A1/en not_active Abandoned
- 2006-05-10 CN CN2006100817395A patent/CN101028970B/zh not_active Expired - Fee Related
-
2007
- 2007-01-30 WO PCT/EP2007/050882 patent/WO2007099005A1/fr active Application Filing
- 2007-01-30 KR KR1020087021278A patent/KR20080102140A/ko not_active Application Discontinuation
- 2007-01-30 MX MX2008011030A patent/MX2008011030A/es unknown
- 2007-01-30 EP EP07704234A patent/EP1989157A1/fr not_active Withdrawn
- 2007-01-30 BR BRPI0708410-2A patent/BRPI0708410A2/pt not_active Application Discontinuation
- 2007-01-30 CA CA002644507A patent/CA2644507A1/fr not_active Abandoned
- 2007-01-30 JP JP2008556735A patent/JP5473337B2/ja not_active Expired - Fee Related
- 2007-01-30 RU RU2008138648/03A patent/RU2432337C2/ru not_active IP Right Cessation
Patent Citations (2)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE19833061A1 (de) * | 1998-07-22 | 2000-02-03 | Elotex Ag Sempach Station | Verfahren zur Herstellung wäßriger Dispersionen von Latexteilchen mit heterogener Morphologie, die mit dem Verfahren erhältlichen Latexteilchen, die Dispersionen und redispergierbaren Pulver sowie deren Verwendung |
US20050284340A1 (en) * | 2004-06-15 | 2005-12-29 | Vickers Thomas M Jr | Providing freezing and thawing resistance to cementitious compositions |
Non-Patent Citations (1)
Title |
---|
See also references of WO2007099005A1 * |
Also Published As
Publication number | Publication date |
---|---|
MX2008011030A (es) | 2008-09-08 |
JP2009528242A (ja) | 2009-08-06 |
JP5473337B2 (ja) | 2014-04-16 |
KR20080102140A (ko) | 2008-11-24 |
CN101028970A (zh) | 2007-09-05 |
WO2007099005A1 (fr) | 2007-09-07 |
RU2008138648A (ru) | 2010-04-10 |
CN101028970B (zh) | 2013-06-12 |
DE102006009842A1 (de) | 2007-09-06 |
BRPI0708410A2 (pt) | 2011-05-31 |
US20070208107A1 (en) | 2007-09-06 |
RU2432337C2 (ru) | 2011-10-27 |
CA2644507A1 (fr) | 2007-09-07 |
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