EE03962B1 - Bensofenooni ühendid, meetodid nende valmistamiseks, kompositsioon ja meetodid seene või taime seenhaiguse tõrjeks - Google Patents

Bensofenooni ühendid, meetodid nende valmistamiseks, kompositsioon ja meetodid seene või taime seenhaiguse tõrjeks

Info

Publication number
EE03962B1
EE03962B1 EE9800301A EEP9800301A EE03962B1 EE 03962 B1 EE03962 B1 EE 03962B1 EE 9800301 A EE9800301 A EE 9800301A EE P9800301 A EEP9800301 A EE P9800301A EE 03962 B1 EE03962 B1 EE 03962B1
Authority
EE
Estonia
Prior art keywords
methods
fungal
preparation
composition
benzophenone compounds
Prior art date
Application number
EE9800301A
Other languages
English (en)
Estonian (et)
Inventor
Edith Elise Rehnig Annerose
Curtze Juergen
Morschhaeuser Gerd
Stumm Karl-Otto
Albert Guido
Reichert Gunther
Simon Werner
Waldeck Andreas
Van Tuyl Cotter Henry
Original Assignee
American Cyanamid Company
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Family has litigation
First worldwide family litigation filed litigation Critical https://patents.darts-ip.com/?family=25435014&utm_source=google_patent&utm_medium=platform_link&utm_campaign=public_patent_search&patent=EE03962(B1) "Global patent litigation dataset” by Darts-ip is licensed under a Creative Commons Attribution 4.0 International License.
Application filed by American Cyanamid Company filed Critical American Cyanamid Company
Publication of EE9800301A publication Critical patent/EE9800301A/xx
Publication of EE03962B1 publication Critical patent/EE03962B1/xx

Links

Classifications

    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C205/00—Compounds containing nitro groups bound to a carbon skeleton
    • C07C205/45—Compounds containing nitro groups bound to a carbon skeleton the carbon skeleton being further substituted by at least one doubly—bound oxygen atom, not being part of a —CHO group
    • A—HUMAN NECESSITIES
    • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
    • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
    • A01N35/00—Biocides, pest repellants or attractants, or plant growth regulators containing organic compounds containing a carbon atom having two bonds to hetero atoms with at the most one bond to halogen, e.g. aldehyde radical
    • A01N35/04—Biocides, pest repellants or attractants, or plant growth regulators containing organic compounds containing a carbon atom having two bonds to hetero atoms with at the most one bond to halogen, e.g. aldehyde radical containing aldehyde or keto groups, or thio analogues thereof, directly attached to an aromatic ring system, e.g. acetophenone; Derivatives thereof, e.g. acetals
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C45/00—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds
    • C07C45/45—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by condensation
    • C07C45/46—Friedel-Crafts reactions
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C45/00—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds
    • C07C45/61—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups
    • C07C45/67—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton
    • C07C45/673—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by change of size of the carbon skeleton
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C45/00—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds
    • C07C45/61—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups
    • C07C45/67—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton
    • C07C45/673—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by change of size of the carbon skeleton
    • C07C45/676—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by change of size of the carbon skeleton by elimination of carboxyl groups
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C45/00—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds
    • C07C45/61—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups
    • C07C45/67—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton
    • C07C45/68—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C45/00—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds
    • C07C45/61—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups
    • C07C45/67—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton
    • C07C45/68—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms
    • C07C45/70—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms by reaction with functional groups containing oxygen only in singly bound form
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C45/00—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds
    • C07C45/61—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups
    • C07C45/67—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton
    • C07C45/68—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms
    • C07C45/70—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms by reaction with functional groups containing oxygen only in singly bound form
    • C07C45/71—Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms by reaction with functional groups containing oxygen only in singly bound form being hydroxy groups
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C49/00—Ketones; Ketenes; Dimeric ketenes; Ketonic chelates
    • C07C49/76—Ketones containing a keto group bound to a six-membered aromatic ring
    • C07C49/84—Ketones containing a keto group bound to a six-membered aromatic ring containing ether groups, groups, groups, or groups
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C65/00—Compounds having carboxyl groups bound to carbon atoms of six—membered aromatic rings and containing any of the groups OH, O—metal, —CHO, keto, ether, groups, groups, or groups
    • C07C65/21—Compounds having carboxyl groups bound to carbon atoms of six—membered aromatic rings and containing any of the groups OH, O—metal, —CHO, keto, ether, groups, groups, or groups containing ether groups, groups, groups, or groups
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C65/00—Compounds having carboxyl groups bound to carbon atoms of six—membered aromatic rings and containing any of the groups OH, O—metal, —CHO, keto, ether, groups, groups, or groups
    • C07C65/21—Compounds having carboxyl groups bound to carbon atoms of six—membered aromatic rings and containing any of the groups OH, O—metal, —CHO, keto, ether, groups, groups, or groups containing ether groups, groups, groups, or groups
    • C07C65/24—Compounds having carboxyl groups bound to carbon atoms of six—membered aromatic rings and containing any of the groups OH, O—metal, —CHO, keto, ether, groups, groups, or groups containing ether groups, groups, groups, or groups polycyclic

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Plant Pathology (AREA)
  • Agronomy & Crop Science (AREA)
  • Engineering & Computer Science (AREA)
  • Dentistry (AREA)
  • General Health & Medical Sciences (AREA)
  • Wood Science & Technology (AREA)
  • Zoology (AREA)
  • Environmental Sciences (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Agricultural Chemicals And Associated Chemicals (AREA)
EE9800301A 1997-08-20 1998-08-19 Bensofenooni ühendid, meetodid nende valmistamiseks, kompositsioon ja meetodid seene või taime seenhaiguse tõrjeks EE03962B1 (et)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US08/914,966 US5945567A (en) 1997-08-20 1997-08-20 Fungicidal 2-methoxybenzophenones

Publications (2)

Publication Number Publication Date
EE9800301A EE9800301A (et) 1999-04-15
EE03962B1 true EE03962B1 (et) 2003-02-17

Family

ID=25435014

Family Applications (1)

Application Number Title Priority Date Filing Date
EE9800301A EE03962B1 (et) 1997-08-20 1998-08-19 Bensofenooni ühendid, meetodid nende valmistamiseks, kompositsioon ja meetodid seene või taime seenhaiguse tõrjeks

Country Status (25)

Country Link
US (2) US5945567A (es)
JP (1) JP4416851B2 (es)
KR (2) KR100659806B1 (es)
CN (2) CN1147456C (es)
AR (1) AR016392A1 (es)
BG (1) BG64048B1 (es)
BR (1) BR9803198B1 (es)
CA (1) CA2245124C (es)
CO (1) CO5050332A1 (es)
CZ (1) CZ294488B6 (es)
EA (1) EA002606B1 (es)
EE (1) EE03962B1 (es)
GE (1) GEP20032878B (es)
HR (1) HRP980439B1 (es)
HU (1) HU225229B1 (es)
ID (1) ID20744A (es)
IL (2) IL125788A (es)
MY (1) MY126559A (es)
PL (1) PL193675B1 (es)
RO (1) RO120905B1 (es)
SK (1) SK283231B6 (es)
TR (1) TR199801629A2 (es)
TW (1) TW382013B (es)
UA (1) UA46826C2 (es)
ZA (1) ZA987489B (es)

Families Citing this family (55)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US6242498B1 (en) * 1997-08-20 2001-06-05 Juergen Curtze Fungicidal 2,6,6′-trimethylbenzophenones
US6277856B1 (en) * 1998-09-25 2001-08-21 American Cynamid Co. Fungicidal mixtures
US6383984B1 (en) 1999-01-29 2002-05-07 Basf Aktiengesellschaft Aqueous suspension concentrate
US6613806B1 (en) 1999-01-29 2003-09-02 Basf Corporation Enhancement of the efficacy of benzoylbenzenes
US6444618B1 (en) 1999-01-29 2002-09-03 Basf Aktiengesellschaft Crop protection emulsifiable concentrate containing defoaming agents
US6346535B1 (en) 1999-01-29 2002-02-12 American Cyanamid Company Fungicidal mixtures
US6521628B1 (en) 1999-01-29 2003-02-18 Basf Aktiengesellschaft Fungicidal mixtures
GB9912220D0 (en) 1999-05-26 1999-07-28 Novartis Ag Organic compounds
GB9912219D0 (en) 1999-05-26 1999-07-28 Novartis Ag Organic compounds
DK1185173T3 (da) * 1999-06-14 2003-09-22 Syngenta Participations Ag Fungicide kombinationer
KR100651090B1 (ko) 1999-07-15 2006-11-29 바스프 악티엔게젤샤프트 5- 및(또는) 6-치환-2-히드록시벤조산 에스테르의 제조 방법
US6559336B2 (en) 1999-07-15 2003-05-06 Basf Aktiengesellschaft Process for the preparation of 5- and/or 6-substituted-2-hydroxybenzoic acid esters
US6699874B2 (en) 1999-09-24 2004-03-02 Basf Aktiengesellschaft Fungicidal mixtures
GB0010198D0 (en) * 2000-04-26 2000-06-14 Novartis Ag Organic compounds
GB0028702D0 (en) * 2000-11-24 2001-01-10 Novartis Ag Organic compounds
EP1365654A1 (de) * 2001-01-18 2003-12-03 Basf Aktiengesellschaft Fungizide mischungen aus benzophenonen und imidazolderivaten
EP1373181A1 (de) * 2001-03-13 2004-01-02 Basf Aktiengesellschaft Benzophenone, deren herstellung und verwendung zur bekämpfung von pflanzenpathogenen pilzen
NZ535307A (en) * 2002-03-21 2007-09-28 Basf Ag Fungicidal mixtures comprising prothioconazole and boscalid
PT1523238E (pt) * 2002-07-11 2009-03-05 Basf Se Uso de fungicidas
WO2004045288A2 (de) * 2002-11-15 2004-06-03 Basf Aktiengesellschaft Fungizide mischungen zur bekämpfung von reispathogenen
UA79182C2 (en) * 2002-12-13 2007-05-25 Basf Ag Method for the production of benzophenones
DE10349501A1 (de) 2003-10-23 2005-05-25 Bayer Cropscience Ag Synergistische fungizide Wirkstoffkombinationen
EP2255627A3 (de) 2004-04-30 2012-09-26 Basf Se Fungizide Mischungen
DE102004049761A1 (de) * 2004-10-12 2006-04-13 Bayer Cropscience Ag Fungizide Wirkstoffkombinationen
DE102005015677A1 (de) 2005-04-06 2006-10-12 Bayer Cropscience Ag Synergistische fungizide Wirkstoffkombinationen
PL1912503T3 (pl) 2005-08-05 2014-12-31 Basf Se Mieszaniny grzybobójcze zawierające podstawione anilidy kwasu 1-metylopirazol-4-ilokarboksylowego
DE102006023263A1 (de) 2006-05-18 2007-11-22 Bayer Cropscience Ag Synergistische Wirkstoffkombinationen
US20100041682A1 (en) 2006-09-18 2010-02-18 Langewald Juergen Ternary Pesticidal Mixtures
EP2258177A3 (en) 2006-12-15 2011-11-09 Rohm and Haas Company Mixtures comprising 1-methylcyclopropene
AR065197A1 (es) 2007-02-06 2009-05-20 Basf Se Insecticidas como safeners para fungicidas con accion fitotoxica
BRPI0810144A2 (pt) 2007-04-23 2014-10-14 Basf Se Método para aumentar saúde das plantas e/ou controlar pestes em plantas
EP2324710A1 (en) 2007-09-20 2011-05-25 Basf Se Combinations comprising a fungicidal strain and at least one additional fungicide
ES2381320T3 (es) 2007-09-26 2012-05-25 Basf Se Composiciones fungicidas ternarias que comprenden boscalida y clorotalonil
CN107266306A (zh) * 2009-07-07 2017-10-20 拜耳知识产权有限责任公司 制备（2,4‑二甲基联苯‑3‑基）乙酸、其酯及中间体化合物的方法
WO2011026796A1 (en) 2009-09-01 2011-03-10 Basf Se Synergistic fungicidal mixtures comprising lactylates and method for combating phytopathogenic fungi
MX2013006737A (es) 2010-12-20 2013-07-15 Basf Se Mezclas de activos pesticida que comprende compuestos de pirazol.
EP2481284A3 (en) 2011-01-27 2012-10-17 Basf Se Pesticidal mixtures
EP3378313A1 (en) 2011-03-23 2018-09-26 Basf Se Compositions containing polymeric, ionic compounds comprising imidazolium groups
EP2750507A2 (en) 2011-09-02 2014-07-09 Basf Se Agricultural mixtures comprising arylquinazolinone compounds
BR122019015118B1 (pt) 2012-06-20 2020-04-07 Basf Se mistura pesticida, composição, composição agrícola, métodos para o combate ou controle das pragas de invertebrados, para a proteção dos vegetais em crescimento ou dos materias de propagação vegetal, para a proteção de material de propagação vegetal, uso de umamistura pesticida e métodos para o combate dos fungos fitopatogênicos nocivos e para proteger vegetais de fungos fitopatogênicos nocivos
CN102823597A (zh) * 2012-09-13 2012-12-19 陕西上格之路生物科学有限公司 一种含苯菌酮和苯氧喹啉的杀菌组合物
WO2014056780A1 (en) 2012-10-12 2014-04-17 Basf Se A method for combating phytopathogenic harmful microbes on cultivated plants or plant propagation material
US10759767B2 (en) 2012-12-20 2020-09-01 BASF Agro B.V. Compositions comprising a triazole compound
EP2783569A1 (en) 2013-03-28 2014-10-01 Basf Se Compositions comprising a triazole compound
EP2835052A1 (en) 2013-08-07 2015-02-11 Basf Se Fungicidal mixtures comprising pyrimidine fungicides
WO2015036059A1 (en) 2013-09-16 2015-03-19 Basf Se Fungicidal pyrimidine compounds
US20160221964A1 (en) 2013-09-16 2016-08-04 Basf Se Fungicidal pyrimidine compounds
CN103858872B (zh) * 2014-03-15 2017-06-30 海南正业中农高科股份有限公司 含苯菌酮的农药组合物
EP2979549A1 (en) 2014-07-31 2016-02-03 Basf Se Method for improving the health of a plant
CA2963446A1 (en) 2014-10-24 2016-04-28 Basf Se Nonampholytic, quaternizable and water-soluble polymers for modifying the surface charge of solid particles
CN107033006B (zh) * 2016-02-04 2018-12-18 长沙理工大学 一种二芳基酮的制备方法
RU2735252C2 (ru) * 2016-04-15 2020-10-29 Исихара Сангио Кайся, Лтд. Способ усиления эффектов борьбы с болезнями растений фунгицида арилфенилкетона и способ борьбы с болезнями растений
IL257535B (en) 2018-02-14 2020-01-30 N3 Coat Ltd Benzophenone compounds as light catalysts for polyolefins
GB2592668A (en) * 2020-03-06 2021-09-08 Rotam Agrochem Int Co Ltd A novel form of metrafenone, a process for its preparation and use of the same
CN113060808A (zh) * 2021-03-19 2021-07-02 衡阳市建衡实业有限公司 一种含聚氯化铝的水处理剂及其制备方法

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US5248817A (en) * 1991-07-15 1993-09-28 Merck & Co., Inc. Process for aromatic bromination
CZ294096B6 (cs) * 1995-01-20 2004-10-13 Americanácyanamidácompany Benzofenonové sloučeninyŹ způsob jejich výrobyŹ fungicidní prostředky s jejich obsahem a způsob ochrany rostlin

Also Published As

Publication number Publication date
IL125788A (en) 2005-11-20
BR9803198A (pt) 2000-03-28
PL193675B1 (pl) 2007-03-30
SK113198A3 (en) 2000-02-14
KR19990023639A (ko) 1999-03-25
HUP9801900A2 (hu) 1999-06-28
PL328112A1 (en) 1999-03-01
GEP20032878B (en) 2003-02-25
CN1147456C (zh) 2004-04-28
KR100659806B1 (ko) 2007-05-17
HU225229B1 (en) 2006-08-28
KR100693645B1 (ko) 2007-03-14
JP4416851B2 (ja) 2010-02-17
EA002606B1 (ru) 2002-06-27
HU9801900D0 (en) 1998-10-28
CO5050332A1 (es) 2001-06-27
TR199801629A3 (tr) 1999-10-21
SK283231B6 (sk) 2003-04-01
CA2245124C (en) 2008-08-05
ZA987489B (en) 2000-02-21
IL169544A (en) 2009-08-03
HRP980439A2 (en) 1999-06-30
JPH11171818A (ja) 1999-06-29
MY126559A (en) 2006-10-31
BR9803198B1 (pt) 2008-11-18
TR199801629A2 (xx) 1999-10-21
CA2245124A1 (en) 1999-02-20
KR20060014458A (ko) 2006-02-15
HUP9801900A3 (en) 2001-02-28
BG102704A (en) 1999-10-29
EE9800301A (et) 1999-04-15
ID20744A (id) 1999-02-25
EA199800645A1 (ru) 1999-02-25
CZ256898A3 (cs) 1999-03-17
CZ294488B6 (cs) 2005-01-12
RO120905B1 (ro) 2006-09-29
CN1217317A (zh) 1999-05-26
AR016392A1 (es) 2001-07-04
CN1300084C (zh) 2007-02-14
BG64048B1 (bg) 2003-11-28
TW382013B (en) 2000-02-11
UA46826C2 (uk) 2002-06-17
US5922905A (en) 1999-07-13
US5945567A (en) 1999-08-31
HRP980439B1 (en) 2003-08-31
IL125788A0 (en) 1999-04-11
CN1495153A (zh) 2004-05-12

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