DE102013008472A1 - Mehrlagige Schichtanordnung für einen Festkörperelektrolyt - Google Patents

Mehrlagige Schichtanordnung für einen Festkörperelektrolyt Download PDF

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Publication number
DE102013008472A1
DE102013008472A1 DE102013008472.5A DE102013008472A DE102013008472A1 DE 102013008472 A1 DE102013008472 A1 DE 102013008472A1 DE 102013008472 A DE102013008472 A DE 102013008472A DE 102013008472 A1 DE102013008472 A1 DE 102013008472A1
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DE
Germany
Prior art keywords
layer
electrolyte
cathode
oxygen content
layers
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
DE102013008472.5A
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German (de)
English (en)
Inventor
Markus Haydn
Matthias Rüttinger
Thomas Jung
Thomas Franco
Kai ORTNER
Sven Uhlenbruck
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Forschungszentrum Juelich GmbH
Plansee Composite Materials GmbH
Fraunhofer Gesellschaft zur Foerderung der Angewandten Forschung eV
Original Assignee
Plansee Composite Materials GmbH
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Plansee Composite Materials GmbH filed Critical Plansee Composite Materials GmbH
Priority to DE102013008472.5A priority Critical patent/DE102013008472A1/de
Priority to US14/892,891 priority patent/US10312540B2/en
Priority to KR1020157033280A priority patent/KR20160010465A/ko
Priority to TW103117554A priority patent/TWI634696B/zh
Priority to EP14728826.0A priority patent/EP3000149B1/de
Priority to CN201480029350.9A priority patent/CN105493327B/zh
Priority to JP2016514298A priority patent/JP6600300B2/ja
Priority to CA2911454A priority patent/CA2911454A1/en
Priority to DK14728826.0T priority patent/DK3000149T3/en
Priority to PCT/EP2014/001352 priority patent/WO2014187559A1/de
Publication of DE102013008472A1 publication Critical patent/DE102013008472A1/de
Ceased legal-status Critical Current

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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1004—Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/1213—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the electrode/electrolyte combination or the supporting material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H01M8/1246—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0068—Solid electrolytes inorganic
    • H01M2300/0071—Oxides
    • H01M2300/0074—Ion conductive at high temperature
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0068—Solid electrolytes inorganic
    • H01M2300/0071—Oxides
    • H01M2300/0074—Ion conductive at high temperature
    • H01M2300/0077—Ion conductive at high temperature based on zirconium oxide
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0088—Composites
    • H01M2300/0094—Composites in the form of layered products, e.g. coatings
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H01M8/1246—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides
    • H01M8/1253—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides the electrolyte containing zirconium oxide
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

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  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Fuel Cell (AREA)
  • Inert Electrodes (AREA)
  • Conductive Materials (AREA)
DE102013008472.5A 2013-05-21 2013-05-21 Mehrlagige Schichtanordnung für einen Festkörperelektrolyt Ceased DE102013008472A1 (de)

Priority Applications (10)

Application Number Priority Date Filing Date Title
DE102013008472.5A DE102013008472A1 (de) 2013-05-21 2013-05-21 Mehrlagige Schichtanordnung für einen Festkörperelektrolyt
US14/892,891 US10312540B2 (en) 2013-05-21 2014-05-20 Multi-layered layer arrangement for a solid electrolyte
KR1020157033280A KR20160010465A (ko) 2013-05-21 2014-05-20 고체 전해질을 위한 다층 샌드위치 구조
TW103117554A TWI634696B (zh) 2013-05-21 2014-05-20 用於固體電解質的多層層排列
EP14728826.0A EP3000149B1 (de) 2013-05-21 2014-05-20 Mehrlagige schichtanordnung für einen festkörperelektrolyt
CN201480029350.9A CN105493327B (zh) 2013-05-21 2014-05-20 固体电解质的多层层装置
JP2016514298A JP6600300B2 (ja) 2013-05-21 2014-05-20 固体電解質用多重層配置構成
CA2911454A CA2911454A1 (en) 2013-05-21 2014-05-20 Multi-layered layer arrangement for a solid electrolyte
DK14728826.0T DK3000149T3 (en) 2013-05-21 2014-05-20 Multilayer laminate device for a solid-body electrolyte
PCT/EP2014/001352 WO2014187559A1 (de) 2013-05-21 2014-05-20 Mehrlagige schichtanordnung für einen festkörperelektrolyt

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DE102013008472.5A DE102013008472A1 (de) 2013-05-21 2013-05-21 Mehrlagige Schichtanordnung für einen Festkörperelektrolyt

Publications (1)

Publication Number Publication Date
DE102013008472A1 true DE102013008472A1 (de) 2014-11-27

Family

ID=50897525

Family Applications (1)

Application Number Title Priority Date Filing Date
DE102013008472.5A Ceased DE102013008472A1 (de) 2013-05-21 2013-05-21 Mehrlagige Schichtanordnung für einen Festkörperelektrolyt

Country Status (10)

Country Link
US (1) US10312540B2 (https=)
EP (1) EP3000149B1 (https=)
JP (1) JP6600300B2 (https=)
KR (1) KR20160010465A (https=)
CN (1) CN105493327B (https=)
CA (1) CA2911454A1 (https=)
DE (1) DE102013008472A1 (https=)
DK (1) DK3000149T3 (https=)
TW (1) TWI634696B (https=)
WO (1) WO2014187559A1 (https=)

Families Citing this family (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP6014807B2 (ja) * 2014-11-20 2016-10-26 株式会社プラズマイオンアシスト 燃料電池用セパレータ又は燃料電池用集電部材、及びその製造方法
CN105762391B (zh) * 2016-04-15 2019-01-08 暨南大学 组件组成一体化的质子导体低温固体氧化物电池及其制备
CN112771702A (zh) * 2018-09-12 2021-05-07 格利恩技术私人有限公司 具有卤素螯合剂的电池
US10930844B2 (en) 2018-10-11 2021-02-23 International Business Machines Corporation Three-terminal oxygen intercalation neuromorphic devices
KR102932418B1 (ko) 2019-12-16 2026-02-26 삼성전자주식회사 복합 고체전해질, 이를 포함하는 전기화학 셀, 및 상기 복합 고체전해질의 제조방법

Citations (8)

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Publication number Priority date Publication date Assignee Title
WO2002017420A2 (en) 2000-08-18 2002-02-28 Honeywell International Inc. Integrated sofc
WO2005057685A2 (en) 2003-12-02 2005-06-23 Nanodynamics, Inc. Anode-supported sofc with cermet electrolyte
AT8975U1 (de) 2006-02-27 2007-03-15 Plansee Se Poröser körper
WO2007045111A1 (de) 2005-10-19 2007-04-26 Eidgenössische Technische Hochschule Zürich Dünnfilm und damit hergestelltes verbundelement
DE102007015358A1 (de) 2007-03-30 2008-10-02 Forschungszentrum Jülich GmbH Schichtsystem für einen Elektrolyten einer Hochtemperatur-Brennstoffzelle sowie Verfahren zur Herstellung desselben
EP2083466A1 (en) 2008-01-24 2009-07-29 Institute of Nuclear Energy Research Process for the fabrication of a sputter deposited fully dense electrolyte layer embedded in a high performance membrane electrolyte assembly of solid oxide fuel cell
EP1520290B1 (de) 2002-06-17 2010-08-25 Fraunhofer-Gesellschaft zur Förderung der angewandten Forschung e.V. Vorrichtung zur beschichtung von substraten mittels physikalischer dampfabscheidung über den hohlkathodeneffekt
EP1513623B1 (en) 2002-05-29 2012-09-12 Honda Giken Kogyo Kabushiki Kaisha Sub-micron electrolyte thin film on nano-porous substrate by oxidation of metal film

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US5171645A (en) * 1991-01-08 1992-12-15 Gas Research Institute, Inc. Zirconia-bismuth oxide graded electrolyte
AU5634896A (en) * 1996-05-01 1997-11-19 Gas Research Institute, Inc. Stable high conductivity functionally gradient compositionally layered solid state electrolytes and membranes
JP3843766B2 (ja) 2000-07-04 2006-11-08 日産自動車株式会社 固体電解質型燃料電池
JP4840718B2 (ja) * 2001-08-14 2011-12-21 日産自動車株式会社 固体酸化物形燃料電池
JP2003142123A (ja) * 2001-11-05 2003-05-16 Nissan Motor Co Ltd 固体電解質型燃料電池
JP4054867B2 (ja) * 2001-12-04 2008-03-05 独立行政法人産業技術総合研究所 導電性酸化ジルコニウム
JP4135891B2 (ja) * 2002-11-07 2008-08-20 独立行政法人産業技術総合研究所 固体電解質型燃料電池用電解質材料の製造方法、及び固体電解質型燃料電池セルの製造方法
JP5260052B2 (ja) * 2004-06-10 2013-08-14 テクニカル ユニバーシティ オブ デンマーク 固体酸化物型燃料電池
JP2006164801A (ja) * 2004-12-08 2006-06-22 Toyota Motor Corp 固体電解質、それを備えた燃料電池およびそれらの製造方法
US7767358B2 (en) * 2005-05-31 2010-08-03 Nextech Materials, Ltd. Supported ceramic membranes and electrochemical cells and cell stacks including the same
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KR20120080375A (ko) * 2011-01-07 2012-07-17 삼성전자주식회사 연료전지용 양극 소재, 이를 포함하는 연료전지용 양극과 그 양극의 제조방법, 및 고체산화물 연료전지
KR101215338B1 (ko) * 2011-06-20 2012-12-26 주식회사 엑스에프씨 고체 산화물 연료전지용 전해질막, 그 제조방법 및 이를 채용한 연료전지
CN102593480B (zh) * 2012-02-23 2014-12-10 上海交通大学 固体氧化物燃料电池掺杂钛酸盐支撑固体电解质多层膜及其制备方法

Patent Citations (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2002017420A2 (en) 2000-08-18 2002-02-28 Honeywell International Inc. Integrated sofc
EP1513623B1 (en) 2002-05-29 2012-09-12 Honda Giken Kogyo Kabushiki Kaisha Sub-micron electrolyte thin film on nano-porous substrate by oxidation of metal film
EP1520290B1 (de) 2002-06-17 2010-08-25 Fraunhofer-Gesellschaft zur Förderung der angewandten Forschung e.V. Vorrichtung zur beschichtung von substraten mittels physikalischer dampfabscheidung über den hohlkathodeneffekt
WO2005057685A2 (en) 2003-12-02 2005-06-23 Nanodynamics, Inc. Anode-supported sofc with cermet electrolyte
WO2007045111A1 (de) 2005-10-19 2007-04-26 Eidgenössische Technische Hochschule Zürich Dünnfilm und damit hergestelltes verbundelement
AT8975U1 (de) 2006-02-27 2007-03-15 Plansee Se Poröser körper
DE102007015358A1 (de) 2007-03-30 2008-10-02 Forschungszentrum Jülich GmbH Schichtsystem für einen Elektrolyten einer Hochtemperatur-Brennstoffzelle sowie Verfahren zur Herstellung desselben
EP2083466A1 (en) 2008-01-24 2009-07-29 Institute of Nuclear Energy Research Process for the fabrication of a sputter deposited fully dense electrolyte layer embedded in a high performance membrane electrolyte assembly of solid oxide fuel cell

Also Published As

Publication number Publication date
DK3000149T3 (en) 2017-08-28
JP2016524282A (ja) 2016-08-12
TWI634696B (zh) 2018-09-01
US10312540B2 (en) 2019-06-04
KR20160010465A (ko) 2016-01-27
WO2014187559A1 (de) 2014-11-27
JP6600300B2 (ja) 2019-10-30
CN105493327A (zh) 2016-04-13
CA2911454A1 (en) 2014-11-27
EP3000149A1 (de) 2016-03-30
EP3000149B1 (de) 2017-05-10
CN105493327B (zh) 2018-01-30
TW201505246A (zh) 2015-02-01
WO2014187559A8 (de) 2016-02-18
US20160118680A1 (en) 2016-04-28

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