DE102009003610A1 - Trockene dreiwege-katalytische Reduktion von Gasturbinen-NOx - Google Patents
Trockene dreiwege-katalytische Reduktion von Gasturbinen-NOx Download PDFInfo
- Publication number
- DE102009003610A1 DE102009003610A1 DE102009003610A DE102009003610A DE102009003610A1 DE 102009003610 A1 DE102009003610 A1 DE 102009003610A1 DE 102009003610 A DE102009003610 A DE 102009003610A DE 102009003610 A DE102009003610 A DE 102009003610A DE 102009003610 A1 DE102009003610 A1 DE 102009003610A1
- Authority
- DE
- Germany
- Prior art keywords
- gas
- combustion chamber
- exhaust gas
- egr
- compressor
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Withdrawn
Links
- 238000010531 catalytic reduction reaction Methods 0.000 title description 4
- 239000003054 catalyst Substances 0.000 claims abstract description 59
- 238000002485 combustion reaction Methods 0.000 claims abstract description 58
- 239000000446 fuel Substances 0.000 claims abstract description 24
- 239000003570 air Substances 0.000 claims abstract description 15
- 238000010248 power generation Methods 0.000 claims abstract description 15
- 239000012080 ambient air Substances 0.000 claims abstract description 13
- 238000011084 recovery Methods 0.000 claims abstract description 9
- 239000000203 mixture Substances 0.000 claims abstract description 7
- 239000007789 gas Substances 0.000 claims description 133
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 claims description 39
- 239000001301 oxygen Substances 0.000 claims description 39
- 229910052760 oxygen Inorganic materials 0.000 claims description 39
- 238000000034 method Methods 0.000 claims description 36
- 230000005611 electricity Effects 0.000 claims description 7
- 238000007254 oxidation reaction Methods 0.000 claims description 6
- 230000003647 oxidation Effects 0.000 claims description 5
- 238000001816 cooling Methods 0.000 claims description 4
- 229910052751 metal Inorganic materials 0.000 claims description 4
- 239000002184 metal Substances 0.000 claims description 4
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 claims description 3
- 238000002156 mixing Methods 0.000 claims description 2
- -1 platinum group metals Chemical class 0.000 claims description 2
- 238000004064 recycling Methods 0.000 claims 1
- 230000001590 oxidative effect Effects 0.000 abstract description 2
- UGFAIRIUMAVXCW-UHFFFAOYSA-N Carbon monoxide Chemical compound [O+]#[C-] UGFAIRIUMAVXCW-UHFFFAOYSA-N 0.000 description 52
- 229910002091 carbon monoxide Inorganic materials 0.000 description 50
- 230000008569 process Effects 0.000 description 29
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 description 22
- 229930195733 hydrocarbon Natural products 0.000 description 14
- 150000002430 hydrocarbons Chemical class 0.000 description 14
- MWUXSHHQAYIFBG-UHFFFAOYSA-N Nitric oxide Chemical class O=[N] MWUXSHHQAYIFBG-UHFFFAOYSA-N 0.000 description 13
- CURLTUGMZLYLDI-UHFFFAOYSA-N Carbon dioxide Chemical compound O=C=O CURLTUGMZLYLDI-UHFFFAOYSA-N 0.000 description 12
- 239000004215 Carbon black (E152) Substances 0.000 description 11
- 239000012530 fluid Substances 0.000 description 11
- 229910052757 nitrogen Inorganic materials 0.000 description 11
- 238000006722 reduction reaction Methods 0.000 description 11
- 230000009467 reduction Effects 0.000 description 10
- 230000002829 reductive effect Effects 0.000 description 9
- 238000010586 diagram Methods 0.000 description 8
- 229910002092 carbon dioxide Inorganic materials 0.000 description 6
- 239000001569 carbon dioxide Substances 0.000 description 6
- 239000000567 combustion gas Substances 0.000 description 6
- 238000006243 chemical reaction Methods 0.000 description 5
- 239000003344 environmental pollutant Substances 0.000 description 5
- QGZKDVFQNNGYKY-UHFFFAOYSA-N Ammonia Chemical compound N QGZKDVFQNNGYKY-UHFFFAOYSA-N 0.000 description 4
- 230000002411 adverse Effects 0.000 description 4
- VNWKTOKETHGBQD-UHFFFAOYSA-N methane Chemical compound C VNWKTOKETHGBQD-UHFFFAOYSA-N 0.000 description 4
- 231100000719 pollutant Toxicity 0.000 description 4
- HZAXFHJVJLSVMW-UHFFFAOYSA-N 2-Aminoethan-1-ol Chemical compound NCCO HZAXFHJVJLSVMW-UHFFFAOYSA-N 0.000 description 3
- 238000010521 absorption reaction Methods 0.000 description 3
- 239000000470 constituent Substances 0.000 description 3
- 230000008030 elimination Effects 0.000 description 3
- 238000003379 elimination reaction Methods 0.000 description 3
- 238000005516 engineering process Methods 0.000 description 3
- 238000012986 modification Methods 0.000 description 3
- 230000004048 modification Effects 0.000 description 3
- BASFCYQUMIYNBI-UHFFFAOYSA-N platinum Chemical group [Pt] BASFCYQUMIYNBI-UHFFFAOYSA-N 0.000 description 3
- 238000000926 separation method Methods 0.000 description 3
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 2
- XEEYBQQBJWHFJM-UHFFFAOYSA-N Iron Chemical compound [Fe] XEEYBQQBJWHFJM-UHFFFAOYSA-N 0.000 description 2
- 229910021529 ammonia Inorganic materials 0.000 description 2
- 238000003421 catalytic decomposition reaction Methods 0.000 description 2
- 230000003197 catalytic effect Effects 0.000 description 2
- 150000001875 compounds Chemical class 0.000 description 2
- 230000007812 deficiency Effects 0.000 description 2
- 230000007613 environmental effect Effects 0.000 description 2
- 239000003546 flue gas Substances 0.000 description 2
- 239000007788 liquid Substances 0.000 description 2
- 238000004519 manufacturing process Methods 0.000 description 2
- 239000003345 natural gas Substances 0.000 description 2
- 230000036961 partial effect Effects 0.000 description 2
- BUHVIAUBTBOHAG-FOYDDCNASA-N (2r,3r,4s,5r)-2-[6-[[2-(3,5-dimethoxyphenyl)-2-(2-methylphenyl)ethyl]amino]purin-9-yl]-5-(hydroxymethyl)oxolane-3,4-diol Chemical compound COC1=CC(OC)=CC(C(CNC=2C=3N=CN(C=3N=CN=2)[C@H]2[C@@H]([C@H](O)[C@@H](CO)O2)O)C=2C(=CC=CC=2)C)=C1 BUHVIAUBTBOHAG-FOYDDCNASA-N 0.000 description 1
- 229910018072 Al 2 O 3 Inorganic materials 0.000 description 1
- 229910052684 Cerium Inorganic materials 0.000 description 1
- VVNCNSJFMMFHPL-VKHMYHEASA-N D-penicillamine Chemical compound CC(C)(S)[C@@H](N)C(O)=O VVNCNSJFMMFHPL-VKHMYHEASA-N 0.000 description 1
- 229910002060 Fe-Cr-Al alloy Inorganic materials 0.000 description 1
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 description 1
- 239000002250 absorbent Substances 0.000 description 1
- 230000002745 absorbent Effects 0.000 description 1
- 238000009825 accumulation Methods 0.000 description 1
- 230000002378 acidificating effect Effects 0.000 description 1
- 230000009471 action Effects 0.000 description 1
- 238000004378 air conditioning Methods 0.000 description 1
- BFNBIHQBYMNNAN-UHFFFAOYSA-N ammonium sulfate Chemical compound N.N.OS(O)(=O)=O BFNBIHQBYMNNAN-UHFFFAOYSA-N 0.000 description 1
- 229910052921 ammonium sulfate Inorganic materials 0.000 description 1
- 235000011130 ammonium sulphate Nutrition 0.000 description 1
- 239000000919 ceramic Substances 0.000 description 1
- 239000004035 construction material Substances 0.000 description 1
- 239000000356 contaminant Substances 0.000 description 1
- 238000005260 corrosion Methods 0.000 description 1
- 230000007797 corrosion Effects 0.000 description 1
- 238000000354 decomposition reaction Methods 0.000 description 1
- 230000007423 decrease Effects 0.000 description 1
- 230000003247 decreasing effect Effects 0.000 description 1
- 238000010494 dissociation reaction Methods 0.000 description 1
- 230000005593 dissociations Effects 0.000 description 1
- 230000000694 effects Effects 0.000 description 1
- 238000010304 firing Methods 0.000 description 1
- 239000011888 foil Substances 0.000 description 1
- 238000010438 heat treatment Methods 0.000 description 1
- 239000001257 hydrogen Substances 0.000 description 1
- 229910052739 hydrogen Inorganic materials 0.000 description 1
- 229910052742 iron Inorganic materials 0.000 description 1
- 238000002955 isolation Methods 0.000 description 1
- 239000000463 material Substances 0.000 description 1
- 150000002739 metals Chemical class 0.000 description 1
- 229910017464 nitrogen compound Inorganic materials 0.000 description 1
- 150000002830 nitrogen compounds Chemical class 0.000 description 1
- 229910052697 platinum Inorganic materials 0.000 description 1
- 150000003222 pyridines Chemical class 0.000 description 1
- 230000001105 regulatory effect Effects 0.000 description 1
- 230000002441 reversible effect Effects 0.000 description 1
- 238000004904 shortening Methods 0.000 description 1
- 239000000779 smoke Substances 0.000 description 1
- 239000007787 solid Substances 0.000 description 1
- 230000003068 static effect Effects 0.000 description 1
- 229910052717 sulfur Inorganic materials 0.000 description 1
- 239000002341 toxic gas Substances 0.000 description 1
- 229910052726 zirconium Inorganic materials 0.000 description 1
Classifications
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F02—COMBUSTION ENGINES; HOT-GAS OR COMBUSTION-PRODUCT ENGINE PLANTS
- F02C—GAS-TURBINE PLANTS; AIR INTAKES FOR JET-PROPULSION PLANTS; CONTROLLING FUEL SUPPLY IN AIR-BREATHING JET-PROPULSION PLANTS
- F02C3/00—Gas-turbine plants characterised by the use of combustion products as the working fluid
- F02C3/34—Gas-turbine plants characterised by the use of combustion products as the working fluid with recycling of part of the working fluid, i.e. semi-closed cycles with combustion products in the closed part of the cycle
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
- B01D53/34—Chemical or biological purification of waste gases
- B01D53/74—General processes for purification of waste gases; Apparatus or devices specially adapted therefor
- B01D53/86—Catalytic processes
- B01D53/8621—Removing nitrogen compounds
- B01D53/8625—Nitrogen oxides
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
- B01D53/34—Chemical or biological purification of waste gases
- B01D53/74—General processes for purification of waste gases; Apparatus or devices specially adapted therefor
- B01D53/86—Catalytic processes
- B01D53/8643—Removing mixtures of carbon monoxide or hydrocarbons and nitrogen oxides
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F02—COMBUSTION ENGINES; HOT-GAS OR COMBUSTION-PRODUCT ENGINE PLANTS
- F02C—GAS-TURBINE PLANTS; AIR INTAKES FOR JET-PROPULSION PLANTS; CONTROLLING FUEL SUPPLY IN AIR-BREATHING JET-PROPULSION PLANTS
- F02C6/00—Plural gas-turbine plants; Combinations of gas-turbine plants with other apparatus; Adaptations of gas-turbine plants for special use
- F02C6/18—Plural gas-turbine plants; Combinations of gas-turbine plants with other apparatus; Adaptations of gas-turbine plants for special use using the waste heat of gas-turbine plants outside the plants themselves, e.g. gas-turbine power heat plants
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D2255/00—Catalysts
- B01D2255/10—Noble metals or compounds thereof
- B01D2255/102—Platinum group metals
- B01D2255/1021—Platinum
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D2255/00—Catalysts
- B01D2255/20—Metals or compounds thereof
- B01D2255/204—Alkaline earth metals
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D2255/00—Catalysts
- B01D2255/20—Metals or compounds thereof
- B01D2255/206—Rare earth metals
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D2255/00—Catalysts
- B01D2255/20—Metals or compounds thereof
- B01D2255/207—Transition metals
- B01D2255/20715—Zirconium
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D2255/00—Catalysts
- B01D2255/20—Metals or compounds thereof
- B01D2255/209—Other metals
- B01D2255/2092—Aluminium
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E20/00—Combustion technologies with mitigation potential
- Y02E20/16—Combined cycle power plant [CCPP], or combined cycle gas turbine [CCGT]
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02T—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO TRANSPORTATION
- Y02T10/00—Road transport of goods or passengers
- Y02T10/10—Internal combustion engine [ICE] based vehicles
- Y02T10/12—Improving ICE efficiencies
Landscapes
- Engineering & Computer Science (AREA)
- Chemical & Material Sciences (AREA)
- Environmental & Geological Engineering (AREA)
- Health & Medical Sciences (AREA)
- Combustion & Propulsion (AREA)
- Mechanical Engineering (AREA)
- General Engineering & Computer Science (AREA)
- Biomedical Technology (AREA)
- Analytical Chemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Oil, Petroleum & Natural Gas (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Sustainable Development (AREA)
- Life Sciences & Earth Sciences (AREA)
- Exhaust Gas After Treatment (AREA)
- Exhaust Gas Treatment By Means Of Catalyst (AREA)
Applications Claiming Priority (2)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| US12/153,231 | 2008-05-15 | ||
| US12/153,231 US8397482B2 (en) | 2008-05-15 | 2008-05-15 | Dry 3-way catalytic reduction of gas turbine NOx |
Publications (1)
| Publication Number | Publication Date |
|---|---|
| DE102009003610A1 true DE102009003610A1 (de) | 2009-11-19 |
Family
ID=41180580
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| DE102009003610A Withdrawn DE102009003610A1 (de) | 2008-05-15 | 2009-03-12 | Trockene dreiwege-katalytische Reduktion von Gasturbinen-NOx |
Country Status (5)
| Country | Link |
|---|---|
| US (2) | US8397482B2 (https=) |
| JP (1) | JP5674281B2 (https=) |
| DE (1) | DE102009003610A1 (https=) |
| FR (1) | FR2931204B1 (https=) |
| RU (1) | RU2502883C2 (https=) |
Cited By (7)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| EP2392796A1 (en) * | 2010-06-07 | 2011-12-07 | EADS Deutschland GmbH | Device for the emission reduction of a turboshaft engine and corresponding method |
| CN102953817A (zh) * | 2011-08-25 | 2013-03-06 | 通用电气公司 | 动力设备及操作方法 |
| EP2689122A4 (en) * | 2011-03-22 | 2015-05-06 | Exxonmobil Upstream Res Co | SYSTEMS AND METHODS FOR CONTROLLING COMBUSTION IN ST-CHIOMETRIC PROPORTIONS IN LOW-EMISSION TURBINE SYSTEMS |
| US9120049B2 (en) | 2011-03-01 | 2015-09-01 | Exxonmobil Upstream Research Company | Apparatus and systems having a rotary valve assembly and swing adsorption processes related thereto |
| US9751041B2 (en) | 2015-05-15 | 2017-09-05 | Exxonmobil Upstream Research Company | Apparatus and system for swing adsorption processes related thereto |
| US9861929B2 (en) | 2015-05-15 | 2018-01-09 | Exxonmobil Upstream Research Company | Apparatus and system for swing adsorption processes related thereto |
| AT527170A1 (de) * | 2023-05-02 | 2024-11-15 | Polytechnik Luft Und Feuerungstechnik Gmbh | Verfahren und Vorrichtung zum Erzeugen eines Rauchgases |
Families Citing this family (155)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US7942008B2 (en) * | 2006-10-09 | 2011-05-17 | General Electric Company | Method and system for reducing power plant emissions |
| WO2009041617A1 (ja) * | 2007-09-28 | 2009-04-02 | Central Research Institute Of Electric Power Industry | タービン設備及び発電設備 |
| US7861511B2 (en) * | 2007-10-30 | 2011-01-04 | General Electric Company | System for recirculating the exhaust of a turbomachine |
| US8056318B2 (en) * | 2007-11-08 | 2011-11-15 | General Electric Company | System for reducing the sulfur oxides emissions generated by a turbomachine |
| US7874141B2 (en) * | 2007-11-16 | 2011-01-25 | General Electric Company | Auxiliary fluid source for an EGR purge system |
| WO2009120779A2 (en) | 2008-03-28 | 2009-10-01 | Exxonmobil Upstream Research Company | Low emission power generation and hydrocarbon recovery systems and methods |
| CN104098070B (zh) | 2008-03-28 | 2016-04-13 | 埃克森美孚上游研究公司 | 低排放发电和烃采收系统及方法 |
| SG195533A1 (en) | 2008-10-14 | 2013-12-30 | Exxonmobil Upstream Res Co | Methods and systems for controlling the products of combustion |
| US7926256B2 (en) | 2008-10-27 | 2011-04-19 | General Electric Company | Inlet system for an EGR system |
| AU2010256517B2 (en) | 2009-06-05 | 2016-03-10 | Exxonmobil Upstream Research Company | Combustor systems and methods for using same |
| CH701803A1 (de) * | 2009-09-03 | 2011-03-15 | Alstom Technology Ltd | Gasturbogruppe und Verfahren zum Betrieb einer solchen Gasturbogruppe. |
| BR112012010294A2 (pt) | 2009-11-12 | 2017-11-07 | Exxonmobil Upstream Res Co | sistema integrado, e, método para a recuperação de hidrocarboneto de baixa emissão com produção de energia |
| US20110146282A1 (en) * | 2009-12-18 | 2011-06-23 | General Electric Company | System and method for reducing sulfur compounds within fuel stream for turbomachine |
| US9003761B2 (en) * | 2010-05-28 | 2015-04-14 | General Electric Company | System and method for exhaust gas use in gas turbine engines |
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| MY167118A (en) * | 2010-07-02 | 2018-08-10 | Exxonmobil Upstream Res Co | Low emission triple-cycle power generation systems and methods |
| TWI593878B (zh) * | 2010-07-02 | 2017-08-01 | 艾克頌美孚上游研究公司 | 用於控制燃料燃燒之系統及方法 |
| AU2011271634B2 (en) * | 2010-07-02 | 2016-01-28 | Exxonmobil Upstream Research Company | Stoichiometric combustion with exhaust gas recirculation and direct contact cooler |
| TWI564475B (zh) * | 2010-07-02 | 2017-01-01 | 艾克頌美孚上游研究公司 | 低排放之三循環動力產生系統和方法 |
| WO2012018458A1 (en) | 2010-08-06 | 2012-02-09 | Exxonmobil Upstream Research Company | System and method for exhaust gas extraction |
| CN103069130B (zh) | 2010-08-06 | 2016-02-24 | 埃克森美孚上游研究公司 | 优化化学计量燃烧的系统和方法 |
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Also Published As
| Publication number | Publication date |
|---|---|
| RU2009109266A (ru) | 2010-09-20 |
| JP2009276053A (ja) | 2009-11-26 |
| US8397482B2 (en) | 2013-03-19 |
| US8991149B2 (en) | 2015-03-31 |
| FR2931204A1 (fr) | 2009-11-20 |
| RU2502883C2 (ru) | 2013-12-27 |
| US20120098276A1 (en) | 2012-04-26 |
| FR2931204B1 (fr) | 2018-03-30 |
| JP5674281B2 (ja) | 2015-02-25 |
| US20090284013A1 (en) | 2009-11-19 |
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