CN106418666B

CN106418666B - Additive for composite plant extract cigarette

Info

Publication number: CN106418666B
Application number: CN201610873664.8A
Authority: CN
Inventors: 裴永隆
Original assignee: China Tobacco Jiangxi Industrial Co Ltd
Current assignee: China Tobacco Jiangxi Industrial Co Ltd
Priority date: 2016-09-30
Filing date: 2016-09-30
Publication date: 2021-08-17
Anticipated expiration: 2036-09-30
Also published as: CN106418666A

Abstract

The invention provides a composite plant extract additive for cigarettes, which can reduce the content of harmful ingredients such as nicotine, tar, hydrocyanic acid and crotonaldehyde in smoke after the laurel leaf, the tsaoko amomum fruit, the pepper, the pine needle, the paniculate swallowwort root, the cactus, the reed rhizome, the eucalyptus leaf, the mulberry and the like in a formula are reasonably proportioned, but the irritation of the smoke is enhanced due to the adoption of a large amount of pepper in the formula, so that the smoking taste of the cigarettes is influenced. After the preparation process disclosed by the invention is adopted, the irritation of the pepper can be eliminated, the smoking taste of the cigarette is improved, the contents of hydrocyanic acid and crotonaldehyde in mainstream smoke can be further reduced, and the influence of harmful substances in the smoke on the health of a human body is reduced.

Description

Additive for composite plant extract cigarette

Technical Field

The invention relates to the field of tobacco additives, in particular to a composite plant extract tobacco additive.

Background

In recent years, with the increasing importance of governments, health organizations and the public on the problem of 'smoking and health', harmful components in cigarette mainstream smoke become one of the focuses of people, and therefore, China also puts forward a target of providing healthy cigarettes for consumers.

The harmful components in the mainstream smoke of the cigarette mainly comprise carbon monoxide, hydrocyanic acid, ammonia, benzo [ a ] pyrene, phenol, crotonaldehyde and the like. At present, industry standards and detection methods for the content of main harmful components in main stream smoke are established, so that the production process related to cigarettes is further improved or the cigarette additive capable of reducing the harmful components in the main stream smoke is developed.

Disclosure of Invention

The invention aims to provide a composite plant extract additive for cigarettes.

The invention also aims to provide a preparation method of the composite plant extract cigarette additive.

In order to achieve the above purpose, the technical scheme adopted by the invention is as follows:

a composite plant extract cigarette additive is prepared from the following raw materials in parts by weight: 10-20 parts of laurel leaf, 20-30 parts of tsaoko amomum fruit, 30-40 parts of pepper, 1-5 parts of pine needle, 1-5 parts of paniculate swallowwort root, 40-50 parts of cactus, 20-30 parts of reed rhizome, 1-3 parts of eucalyptus leaf, 20-30 parts of mulberry, 5-10 parts of glutinous rice, 3-8 parts of sodium dehydroacetate and 1-3 parts of magnesium stearate;

preferably, the composite plant extract cigarette additive is prepared from the following raw materials in parts by weight: 16 parts of laurel leaf, 24 parts of tsaoko amomum fruit, 35 parts of pepper, 2 parts of pine needle, 3 parts of paniculate swallowwort root, 45 parts of cactus, 28 parts of reed rhizome, 2 parts of eucalyptus leaf, 24 parts of mulberry, 7 parts of glutinous rice, 5 parts of sodium dehydroacetate and 2 parts of magnesium stearate;

the preparation method of the composite plant extract cigarette additive comprises the following steps:

(1) soaking laurel leaf, fructus Tsaoko, pricklyash peel, pine needle and glutinous rice in 400 parts by weight of potassium permanganate solution with the concentration of 0.2-0.5g/L for 10-15min, washing with clear water for 3-4 times, drying in the air, crushing into coarse powder, mixing the coarse powder with magnesium stearate, adding ethanol solution with the mass fraction of 60-80% which is 5-8 times of the weight of the coarse powder, performing reflux extraction at the constant temperature of 82 ℃ for 2-3h, and filtering to obtain filtrate a;

(2) soaking the cynanchum paniculatum, the cactus and the reed rhizome in 300 parts by weight of 10-18% ethanol solution at 40-45 ℃ for 6-8h, filtering to obtain filter residue and filtrate b, adding eucalyptus leaves, mulberry, sodium dehydroacetate and 600 parts by weight of 500-fold water into the filter residue, performing reflux extraction at 60 ℃ under reduced pressure for 40-60min, and filtering to obtain filtrate c;

(3) mixing the filtrate a, the filtrate b and the filtrate c, evaporating and concentrating to obtain a paste.

The laurel leaf is dried leaf of sweet laurel of evergreen tree of Lauraceae, is popular spice, and can be used for pickling or soaking food, stewing, filling and fish etc. Fragrant but slightly bitter. Simultaneously has the effects of invigorating stomach and regulating qi-flowing, and can be used for treating abdominal distention and pain; it is indicated for traumatic injury, scabies and tinea by external application.

The fructus Tsaoko is dry mature fruit of Tsaoko of Zingiberaceae. The tsaoko amomum fruit has special and thick spicy flavor, can remove fishy smell and promote appetite, is a good product in cooking condiments, and is praised as one of five flavors in food seasoning by people. Cao Guo can dry dampness and dispel cold. It is better than Cao Dou kou in warm and dry property. Can be used for treating spleen and stomach cold deficiency, abdominal pain, emesis or diarrhea.

The fructus Zanthoxyli is dried mature pericarp of Rutaceae plant fructus Zanthoxyli. Can remove fishy smell of meat; promoting salivary secretion, and stimulating appetite; the blood vessel is expanded, thereby having the function of lowering blood pressure.

The folium Pini is needle leaf of Pinus sibirica, Pinus thunbergii, Pinus tabulaeformis, Pinus koraiensis, Pinus sylvestris, Pinus massoniana, etc. of Pinus of Pinaceae. Dispelling pathogenic wind, promoting blood circulation, improving eyesight, tranquilizing mind, removing toxic substance, relieving itching, removing halitosis, removing dry mouth and tongue, and treating constipation. Can be used for treating influenza, rheumatic arthralgia, traumatic injury, nyctalopia, hypertension, and neurasthenia; it is used externally to treat chilblain.

The radix Cynanchi Paniculati is dried root and rhizome of radix Cynanchi Paniculati of Asclepiadaceae. The distribution is distributed in most areas of the country. Produced in Jiangsu, Hebei, Hunan, Anhui, Guizhou, Guangxi, northeast, etc.

The radix et caulis Opuntiae Dillenii is whole succulent strain of Opuntia ficus-indica of Opuntia of Cactaceae. Southern coastal areas are commonly cultivated, and are wild in the southern Guangdong, southern Guangxi and southern Hainan coastal areas. Has the effects of promoting qi and blood circulation, removing toxic substances, relieving swelling, cooling blood and stopping bleeding. It is commonly used for stomachache, tumor mass, dysentery, laryngalgia, cough due to lung heat, tuberculosis, hemoptysis, hematemesis, hemorrhoidal bleeding, pyocutaneous disease, furunculosis, mastalgia, mumps, tinea, snake and insect bite, scald, and cold injury.

The rhizoma Phragmitis is the rhizome of Phragmites communis of the monocotyledonous family Gramineae. Clearing heat and purging fire, promoting fluid production to quench thirst, relieving restlessness, arresting vomiting and promoting urination.

The folium Eucalypti Globueli is leaf of Eucalyptus globulus Labill of Myrtaceae. Distributed in Guangxi, Yunnan, Sichuan and other places. Is cold in nature, bitter and pungent in flavor, and has the effects of dispelling wind, relieving exterior syndrome, clearing away heat and toxic materials, killing parasites and relieving itching. It is commonly used for common cold, hyperpyrexia, headache, cough and asthma due to lung heat, pertussis, abdominal distending pain, diarrhea and dysentery, hookworm filariasis, malaria, rheumatalgia, carbuncle, sore, toxic swelling, eczema, scabies, burn and scald, and traumatic hemorrhage.

The mulberry is a mature fruit of mulberry, has a sweet taste and a lot of juice, and is one of fruits which are frequently eaten by people. Mulberry is sweet and cold in nature, and has the effects of tonifying liver and kidney, promoting fluid production and moistening dryness, blackening hair and improving eyesight and the like. Mulberry is a fresh fruit which is usually adopted by common people for diuresis, health care and summer heat relieving, and the special efficacy of the mulberry is recorded in compendium of materia Medica.

The glutinous rice is hulled glutinous rice. The glutinous rice contains protein, fat, sugar, calcium, phosphorus, iron, vitamin B1, vitamin B2, nicotinic acid, starch and the like, is rich in nutrition, is a warm-tonifying and body-strengthening food, has the effects of tonifying middle-jiao and Qi, strengthening spleen and stomach and stopping sweating due to debility, and has a certain relieving effect on poor appetite, abdominal distension and diarrhea.

According to the formula, the contents of harmful ingredients such as nicotine, tar, hydrocyanic acid and crotonaldehyde in the smoke can be reduced after the laurel leaf, the tsaoko amomum fruit, the pepper, the pine needle, the paniculate swallowwort root, the cactus, the reed rhizome, the eucalyptus leaf, the mulberry and the like are reasonably proportioned, but the irritation of the smoke is enhanced due to the adoption of a large amount of the pepper in the formula, so that the smoking taste of the cigarette is influenced. After the preparation process disclosed by the invention is adopted, the irritation of the pepper can be eliminated, the smoking taste of the cigarette is improved, the contents of hydrocyanic acid and crotonaldehyde in mainstream smoke can be further reduced, and the influence of harmful substances in the smoke on the health of a human body is reduced.

After the composite plant extract cigarette additive prepared in the embodiments 1-3 of the invention is used in cigarettes, compared with blank control samples, the cigarette smoking style is unchanged, the smoke fineness and softness degree is improved, the miscellaneous gas is reduced, the stimulation degree is reduced, and the oral comfort degree is obviously improved. Example 4 without the preparation process of the present invention, the prepared cigarette additive is used in cigarettes, and the irritation and offensive odor are large, which may affect the smoking quality of the cigarettes.

The composite plant extract cigarette additive can obviously reduce the content of harmful substances such as nicotine, crotonaldehyde and the like in smoke, and the smoke is fine and soft, has small irritation and good cigarette smoking taste.

DETAILED DESCRIPTION OF EMBODIMENT (S) OF INVENTION

The invention discloses a composite plant extract additive for cigarettes, which can be realized by appropriately improving process parameters by referring to the content in the text by the technical personnel in the field. It is expressly intended that all such similar substitutes and modifications which would be obvious to one skilled in the art are deemed to be included in the invention. While the products and methods of this invention have been described in terms of preferred embodiments, it will be apparent to those of ordinary skill in the art that variations and modifications in the methods described herein, as well as other suitable variations and combinations, may be made to implement and use the invention without departing from the spirit and scope of the invention.

Example 1: a composite plant extract cigarette additive is prepared from the following raw materials in parts by weight: 10 parts of laurel leaf, 20 parts of tsaoko amomum fruit, 30 parts of pepper, 1 part of pine needle, 1 part of paniculate swallowwort root, 40 parts of cactus, 20 parts of reed rhizome, 1 part of eucalyptus leaf, 20 parts of mulberry, 5 parts of glutinous rice, 3 parts of sodium dehydroacetate and 1 part of magnesium stearate;

(1) soaking laurel leaf, fructus Tsaoko, pricklyash peel, pine needle and glutinous rice in 300 parts by weight of 0.2g/L potassium permanganate solution for 10min, washing with clear water for 4 times, drying in the air, crushing into coarse powder, mixing the coarse powder with magnesium stearate, adding ethanol solution with the mass fraction of 60% which is 5 times of the weight of the coarse powder, carrying out reflux extraction at the constant temperature of 82 ℃ for 3h, and filtering to obtain filtrate a;

(2) soaking the cynanchum paniculatum, the cactus and the reed rhizome in 200 parts by weight of 10% ethanol solution at 40 ℃ for 6 hours, filtering to obtain filter residue and a filtrate b, adding eucalyptus leaves, mulberry, sodium dehydroacetate and 500 parts by weight of water into the filter residue, performing reduced pressure reflux extraction at 60 ℃ for 40min, and filtering to obtain a filtrate c;

Example 2: a composite plant extract cigarette additive is prepared from the following raw materials in parts by weight: 20 parts of laurel leaf, 30 parts of tsaoko amomum fruit, 40 parts of pepper, 5 parts of pine needle, 5 parts of paniculate swallowwort root, 50 parts of cactus, 30 parts of reed rhizome, 3 parts of eucalyptus leaf, 30 parts of mulberry, 10 parts of glutinous rice, 8 parts of sodium dehydroacetate and 3 parts of magnesium stearate;

(1) the laurel leaf, the tsaoko amomum fruit, the pepper, the pine needle and the sticky rice are soaked for 15min by 400 parts by weight of potassium permanganate solution with the concentration of 0.5g/L, then washed by clear water for 3 times, aired and crushed into coarse powder, the coarse powder is mixed with magnesium stearate, ethanol solution with the mass fraction of 80 percent and the weight 8 times that of the coarse powder is added, reflux extraction is carried out for 3h at the constant temperature of 82 ℃, and then filtration is carried out to obtain filtrate a;

(2) soaking the paniculate swallowwort root, the cactus and the reed rhizome in 300 parts by weight of 18% ethanol solution at 45 ℃ for 8 hours, filtering to obtain filter residue and filtrate b, adding eucalyptus leaves, mulberry, sodium dehydroacetate and 600 parts by weight of water into the filter residue, performing reduced pressure reflux extraction at 60 ℃ for 60 minutes, and filtering to obtain filtrate c;

Example 3: a composite plant extract cigarette additive is prepared from the following raw materials in parts by weight: 16 parts of laurel leaf, 24 parts of tsaoko amomum fruit, 35 parts of pepper, 2 parts of pine needle, 3 parts of paniculate swallowwort root, 45 parts of cactus, 28 parts of reed rhizome, 2 parts of eucalyptus leaf, 24 parts of mulberry, 7 parts of glutinous rice, 5 parts of sodium dehydroacetate and 2 parts of magnesium stearate;

(1) the laurel leaf, the tsaoko amomum fruit, the pepper, the pine needle and the sticky rice are soaked for 15min by 400 parts by weight of potassium permanganate solution with the concentration of 0.3g/L, then washed by clear water for 3 times, aired and crushed into coarse powder, the coarse powder is mixed with magnesium stearate, ethanol solution with the mass fraction of 75 percent and the weight 6 times that of the coarse powder is added, reflux extraction is carried out for 2h at the constant temperature of 82 ℃, and then filtration is carried out to obtain filtrate a;

(2) soaking the paniculate swallowwort root, the cactus and the reed rhizome in 280 parts by weight of ethanol solution with the mass fraction of 15% at 40 ℃ for 6 hours, filtering to obtain filter residue and filtrate b, adding eucalyptus leaves, mulberry, sodium dehydroacetate and 600 parts by weight of water into the filter residue, performing reduced pressure reflux extraction at 60 ℃ for 60 minutes, and filtering to obtain filtrate c;

Example 4: a composite plant extract cigarette additive is prepared by the following steps: crushing laurel leaf, tsaoko amomum fruit, pepper, pine needle, paniculate swallowwort root, cactus, reed rhizome, eucalyptus leaf, mulberry and glutinous rice into coarse powder, mixing the coarse powder with sodium dehydroacetate and magnesium stearate, adding an ethanol solution which is 8 times of the weight of the coarse powder and has a mass fraction of 80%, carrying out reflux extraction at a constant temperature of 82 ℃ for 3 hours, filtering an extracting solution, carrying out reflux extraction at a temperature of 82 ℃ for 2 times and 2 hours each time, combining the extracting solutions obtained in the three times, filtering, evaporating and concentrating the filtrate into paste, thus obtaining the Chinese medicinal composition.

The rest is the same as example 3.

The tobacco additive prepared in the embodiment 1-4 is added into tobacco shreds according to 0.1% of the weight of the tobacco shreds, when in use, the tobacco additive is dissolved into 90% ethanol solution by mass fraction to ensure that the mass fraction of the tobacco additive is 10-20%, and then the tobacco additive is rolled into a cigarette sample. The same cut tobacco without the tobacco additive of the invention described in the embodiments 1-4 is used as a comparison sample, the same cigarette material is adopted to be rolled into a cigarette sample, and the cigarette is subjected to smoke analysis. The content of tar in the smoke is determined according to GB/T19609-. The results are shown in tables 1-4.

TABLE 1 comparison of analysis results of nicotine content in flue gas

Group of	Nicotine (mg/count)	Extent of decrease (%)
			Blank comparative sample	1.30	/
Example 1	1.14	12.3
			Example 2	1.17	10.0
Example 3	1.11	14.6
			Example 4	1.18	9.2

TABLE 2 comparison of analysis results of tar content in flue gas

Group of	Tar (mg/count)	Extent of decrease (%)
			Blank comparative sample	13.6	/
Example 1	11.2	17.6
			Example 2	11.4	16.2
Example 3	10.7	21.3
			Example 4	11.3	16.9

TABLE 3 comparison of analysis results of hydrocyanic acid content in flue gas

Group of	Hydrocyanic acid (μ g/count)	Extent of decrease (%)
			Blank comparative sample	54.9	/
Example 1	44.0	19.9
			Example 2	42.3	23.0
Example 3	40.9	25.5
			Example 4	50.4	8.2

TABLE 4 comparison of analysis results of crotonaldehyde content in flue gas

Group of	Crotonaldehyde (μ g/count)	Extent of decrease (%)
			Blank comparative sample	45.8	/
Example 1	39.1	14.6
			Example 2	38.8	15.3
Example 3	36.4	20.5
			Example 4	42.9	6.3

Claims

1. The additive for the composite plant extract cigarette is characterized in that: the feed is prepared from the following raw materials in parts by weight: 10-20 parts of laurel leaf, 20-30 parts of tsaoko amomum fruit, 30-40 parts of pepper, 1-5 parts of pine needle, 1-5 parts of paniculate swallowwort root, 40-50 parts of cactus, 20-30 parts of reed rhizome, 1-3 parts of eucalyptus leaf, 20-30 parts of mulberry, 5-10 parts of glutinous rice, 3-8 parts of sodium dehydroacetate and 1-3 parts of magnesium stearate;

2. The additive for composite plant extract cigarette as claimed in claim 1, wherein: the feed is prepared from the following raw materials in parts by weight: 16 parts of laurel leaf, 24 parts of tsaoko amomum fruit, 35 parts of pepper, 2 parts of pine needle, 3 parts of paniculate swallowwort root, 45 parts of cactus, 28 parts of reed rhizome, 2 parts of eucalyptus leaf, 24 parts of mulberry, 7 parts of glutinous rice, 5 parts of sodium dehydroacetate and 2 parts of magnesium stearate.

3. The additive for composite plant extract cigarette as claimed in claim 1, wherein: the preparation method of the composite plant extract cigarette additive comprises the following steps: