CN101223253B - 聚合物分散体和电催化剂油墨 - Google Patents

聚合物分散体和电催化剂油墨 Download PDF

Info

Publication number
CN101223253B
CN101223253B CN200680025965XA CN200680025965A CN101223253B CN 101223253 B CN101223253 B CN 101223253B CN 200680025965X A CN200680025965X A CN 200680025965XA CN 200680025965 A CN200680025965 A CN 200680025965A CN 101223253 B CN101223253 B CN 101223253B
Authority
CN
China
Prior art keywords
electrocatalyst
ink
materials
liquid medium
prepare
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
CN200680025965XA
Other languages
English (en)
Chinese (zh)
Other versions
CN101223253A (zh
Inventor
D·C·丰加兰
P·卡皮拉
C·N·马尔德
M·I·佩奇
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Johnson Matthey Hydrogen Technologies Ltd
Original Assignee
Johnson Matthey PLC
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Johnson Matthey PLC filed Critical Johnson Matthey PLC
Publication of CN101223253A publication Critical patent/CN101223253A/zh
Application granted granted Critical
Publication of CN101223253B publication Critical patent/CN101223253B/zh
Expired - Fee Related legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Images

Classifications

    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09DCOATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
    • C09D11/00Inks
    • C09D11/52Electrically conductive inks
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B01PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01JCHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/02Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides
    • B01J31/06Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides containing polymers
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00Use of inorganic substances as compounding ingredients
    • C08K3/28Nitrogen-containing compounds
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8647Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites
    • H01M4/8652Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites as mixture
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8663Selection of inactive substances as ingredients for catalytic active masses, e.g. binders, fillers
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8803Supports for the deposition of the catalytic active composition
    • H01M4/881Electrolytic membranes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8825Methods for deposition of the catalytic active composition
    • H01M4/8828Coating with slurry or ink
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1004Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/102Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1023Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having only carbon, e.g. polyarylenes, polystyrenes or polybutadiene-styrenes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/1039Polymeric electrolyte materials halogenated, e.g. sulfonated polyvinylidene fluorides
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/1069Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1081Polymeric electrolyte materials characterised by the manufacturing processes starting from solutions, dispersions or slurries exclusively of polymers
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02PCLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50Manufacturing or production processes characterised by the final manufactured product

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Electrochemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Organic Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Materials Engineering (AREA)
  • Wood Science & Technology (AREA)
  • Sustainable Energy (AREA)
  • Composite Materials (AREA)
  • Sustainable Development (AREA)
  • Polymers & Plastics (AREA)
  • Medicinal Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Inert Electrodes (AREA)
  • Catalysts (AREA)
  • Compositions Of Macromolecular Compounds (AREA)
CN200680025965XA 2005-05-18 2006-05-16 聚合物分散体和电催化剂油墨 Expired - Fee Related CN101223253B (zh)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
GB0510119.1 2005-05-18
GBGB0510119.1A GB0510119D0 (en) 2005-05-18 2005-05-18 Polymer dispersion and electrocatalyst ink
PCT/GB2006/050112 WO2006123187A1 (en) 2005-05-18 2006-05-16 Polymer dispersion and electrocatalyst ink

Publications (2)

Publication Number Publication Date
CN101223253A CN101223253A (zh) 2008-07-16
CN101223253B true CN101223253B (zh) 2011-03-09

Family

ID=34708361

Family Applications (1)

Application Number Title Priority Date Filing Date
CN200680025965XA Expired - Fee Related CN101223253B (zh) 2005-05-18 2006-05-16 聚合物分散体和电催化剂油墨

Country Status (8)

Country Link
US (1) US9127182B2 (enExample)
EP (1) EP1882020B1 (enExample)
JP (1) JP4987857B2 (enExample)
KR (1) KR101270857B1 (enExample)
CN (1) CN101223253B (enExample)
CA (1) CA2608299A1 (enExample)
GB (1) GB0510119D0 (enExample)
WO (1) WO2006123187A1 (enExample)

Families Citing this family (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB0614909D0 (en) * 2006-07-27 2006-09-06 Johnson Matthey Plc Catalyst
KR20120044384A (ko) * 2009-08-21 2012-05-07 바스프 에스이 무기 및/또는 유기 산-함유 촉매 잉크 및 전극, 촉매-코팅된 멤브레인, 가스 확산 전극 및 멤브레인-전극 유닛의 제조에서의 그 촉매 잉크의 용도
WO2013125182A1 (ja) * 2012-02-23 2013-08-29 凸版印刷株式会社 固体高分子形燃料電池用膜電極接合体及びその製造方法と固体高分子形燃料電池
US9865883B2 (en) * 2014-02-14 2018-01-09 Nissan North America, Inc. Fuel cell electrodes using high density support material
JP6206371B2 (ja) * 2014-10-14 2017-10-04 トヨタ自動車株式会社 燃料電池用電極触媒層の製造方法
KR102291918B1 (ko) 2016-04-04 2021-08-23 디옥시드 머티리얼즈, 인크. 촉매 층 및 전해장치
CN112744972B (zh) * 2020-12-31 2022-02-22 中国科学院生态环境研究中心 电芬顿-膜蒸馏协同水处理的装置及方法
GB2607883A (en) 2021-06-11 2022-12-21 Johnson Matthey Hydrogen Technologies Ltd Electrocatalyst ink

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP0731520A1 (en) * 1995-03-09 1996-09-11 Johnson Matthey Public Limited Company Materials for use in catalytic electrode manufacture
US5861222A (en) * 1996-03-23 1999-01-19 Degussa Aktiengesellschaft Gas diffusion electrode for membrane fuel cells and method of its production
US20040028806A1 (en) * 2002-04-24 2004-02-12 Makoto Higami Process for producing electrolyte membrane-bonded electrode and varnish composition used therein
CN1581546A (zh) * 2004-05-14 2005-02-16 武汉理工大学 一种高温质子交换膜燃料电池膜电极及制备方法

Family Cites Families (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4043933A (en) * 1976-06-15 1977-08-23 United Technologies Corporation Method of fabricating a fuel cell electrode
JPS58165266A (ja) * 1982-03-26 1983-09-30 Hitachi Ltd 燃料電池
US4849253A (en) * 1987-05-29 1989-07-18 International Fuel Cell Corporation Method of making an electrochemical cell electrode
US5672439A (en) * 1995-12-18 1997-09-30 Ballard Power Systems, Inc. Method and apparatus for reducing reactant crossover in an electrochemical fuel cell
JP3873387B2 (ja) 1997-07-25 2007-01-24 株式会社ジーエス・ユアサコーポレーション 高分子電解質膜−反応部接合体の製造方法
US6277512B1 (en) * 1999-06-18 2001-08-21 3M Innovative Properties Company Polymer electrolyte membranes from mixed dispersions
JP2002280003A (ja) * 2001-03-21 2002-09-27 Matsushita Electric Ind Co Ltd 高分子電解質型燃料電池用電極と電解質膜電極接合体の製造方法
GB0200253D0 (en) * 2002-01-08 2002-02-20 Johnson Matthey Plc Improved material for electrode manufacture
JP3941515B2 (ja) * 2002-01-15 2007-07-04 トヨタ自動車株式会社 燃料電池電極用触媒層の製造方法及び燃料電池電極用触媒層製造用インクの製造方法
AU2003244123A1 (en) * 2002-06-17 2004-03-11 Daikin Industries, Ltd. Fluoropolymer dispersion and process for producing fluoropolymer dispersion
JP2005123106A (ja) * 2003-10-20 2005-05-12 Toyota Motor Corp 燃料電池用膜・電極接合体の製造方法
KR100601984B1 (ko) * 2005-01-20 2006-07-18 삼성에스디아이 주식회사 담지 촉매 및 그 제조방법

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP0731520A1 (en) * 1995-03-09 1996-09-11 Johnson Matthey Public Limited Company Materials for use in catalytic electrode manufacture
US5861222A (en) * 1996-03-23 1999-01-19 Degussa Aktiengesellschaft Gas diffusion electrode for membrane fuel cells and method of its production
US20040028806A1 (en) * 2002-04-24 2004-02-12 Makoto Higami Process for producing electrolyte membrane-bonded electrode and varnish composition used therein
CN1581546A (zh) * 2004-05-14 2005-02-16 武汉理工大学 一种高温质子交换膜燃料电池膜电极及制备方法

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
JP特开2005-123106A 2005.05.12

Also Published As

Publication number Publication date
KR101270857B1 (ko) 2013-06-07
JP4987857B2 (ja) 2012-07-25
WO2006123187A1 (en) 2006-11-23
JP2008540793A (ja) 2008-11-20
EP1882020B1 (en) 2013-07-10
CN101223253A (zh) 2008-07-16
EP1882020A1 (en) 2008-01-30
KR20080023300A (ko) 2008-03-13
CA2608299A1 (en) 2006-11-23
GB0510119D0 (en) 2005-06-22
US9127182B2 (en) 2015-09-08
US20080292943A1 (en) 2008-11-27

Similar Documents

Publication Publication Date Title
US5716437A (en) Materials for use in electrode manufacture
EP2990109B1 (en) Catalyst and electrode catalyst layer for fuel cell having the catalyst
EP2991142B1 (en) Catalyst, electrode catalyst layer using said catalyst, membrane electrode assembly, and fuel cell
EP2990105B1 (en) Catalyst, and electrode catalyst layer, film electrode assembly, and fuel cell each including said catalyst
US6911411B2 (en) Catalyst agglomerates for membrane electrode assemblies
CN101425585A (zh) 包含析氧反应催化剂的电极
Lee et al. Preparation of low Pt loading electrodes on Nafion (Na+)-bonded carbon layer with galvanostatic pulses for PEMFC application
Cieluch et al. Manufacturing and investigation of MEAs for PEMWE based on glass fibre reinforced PFSA/ssPS composite membranes and catalyst-coated substrates prepared via catalyst electrodeposition
WO2017159820A1 (ja) 電極触媒層形成用ペースト及びその製造方法、並びに膜-電極触媒層接合体、ガス拡散電極、固体高分子型燃料電池及び固体高分子型水電解セルの製造方法
Berber et al. A potential polymer formulation of a durable carbon-black catalyst with a significant fuel cell performance over a wide operating temperature range
CN101223253B (zh) 聚合物分散体和电催化剂油墨
Titheridge et al. Investigating Cathode Ionomer Content and Assembly Techniques for Anion Exchange Membrane Water Electrolyzers
CN102403517B (zh) 用于制造减小龟裂的电极的工艺和材料
KR101769681B1 (ko) 촉매 전극층, 막전극 접합체 및 연료 전지
JP2011113739A (ja) 燃料電池のカソード電極触媒
CN103733403B (zh) 燃料电池用电极、燃料电池用电极的制造方法、聚合物电解质燃料电池以及催化剂墨水
Zhiani et al. Optimization of Nafion content in Nafion–polyaniline nano-composite modified cathodes for PEMFC application
KR101658839B1 (ko) 연료전지용 막-전극 접합체의 제조방법
Darab et al. Pt nanoparticles dispersion influence on fuel cell performance
JP7247693B2 (ja) 燃料電池触媒層及びその製造方法
US20230223557A1 (en) Catalyst preparation
CN112310420A (zh) 燃料电池用电极、膜电极组件、芯片、催化剂层、催化剂分散液及其制备方法

Legal Events

Date Code Title Description
C06 Publication
PB01 Publication
C10 Entry into substantive examination
SE01 Entry into force of request for substantive examination
C14 Grant of patent or utility model
GR01 Patent grant
ASS Succession or assignment of patent right

Owner name: JOHNSON MATTHEY FUEL CELLS LTD.

Free format text: FORMER OWNER: JOHNSON MATTY PUBLIC LIMITED CO.

Effective date: 20121206

C41 Transfer of patent application or patent right or utility model
TR01 Transfer of patent right

Effective date of registration: 20121206

Address after: London, England

Patentee after: JOHNSON MATTHEY PLC

Address before: London, England

Patentee before: Johnson Matthey PLC

CP01 Change in the name or title of a patent holder

Address after: London

Patentee after: Johnson Matthey Hydrogen Technology Co.,Ltd.

Address before: London

Patentee before: JOHNSON MATTHEY PLC

CP01 Change in the name or title of a patent holder
CF01 Termination of patent right due to non-payment of annual fee

Granted publication date: 20110309

CF01 Termination of patent right due to non-payment of annual fee