WO2008108221A1 - 環状グアニジンイオン液体 - Google Patents

環状グアニジンイオン液体 Download PDF

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Publication number
WO2008108221A1
WO2008108221A1 PCT/JP2008/053295 JP2008053295W WO2008108221A1 WO 2008108221 A1 WO2008108221 A1 WO 2008108221A1 JP 2008053295 W JP2008053295 W JP 2008053295W WO 2008108221 A1 WO2008108221 A1 WO 2008108221A1
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WIPO (PCT)
Prior art keywords
ionic liquid
group
cyclic guanidine
alkyl group
electrolytes
Prior art date
Application number
PCT/JP2008/053295
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English (en)
French (fr)
Inventor
Atsushi Kawada
Aya Tashiro
Toshihiro Kumagai
Original Assignee
Nippon Steel Chemical Co., Ltd.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Nippon Steel Chemical Co., Ltd. filed Critical Nippon Steel Chemical Co., Ltd.
Priority to KR1020097018938A priority Critical patent/KR101451355B1/ko
Priority to US12/529,590 priority patent/US8129543B2/en
Priority to EP08720881.5A priority patent/EP2135862A4/en
Priority to JP2009502523A priority patent/JP5243404B2/ja
Priority to CN2008800056705A priority patent/CN101616898B/zh
Publication of WO2008108221A1 publication Critical patent/WO2008108221A1/ja
Priority to US13/358,491 priority patent/US8450478B2/en

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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/056—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes
    • H01M10/0564—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes the electrolyte being constituted of organic materials only
    • H01M10/0566—Liquid materials
    • H01M10/0568—Liquid materials characterised by the solutes
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D233/00—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings
    • C07D233/04—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member
    • C07D233/28—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member with hetero atoms or with carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, e.g. ester or nitrile radicals, directly attached to ring carbon atoms
    • C07D233/44—Nitrogen atoms not forming part of a nitro radical
    • C07D233/48—Nitrogen atoms not forming part of a nitro radical with acyclic hydrocarbon or substituted acyclic hydrocarbon radicals, attached to said nitrogen atoms
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D233/00—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings
    • C07D233/04—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member
    • C07D233/28—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member with hetero atoms or with carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, e.g. ester or nitrile radicals, directly attached to ring carbon atoms
    • C07D233/44—Nitrogen atoms not forming part of a nitro radical
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D239/00—Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings
    • C07D239/02—Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings
    • C07D239/06—Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member
    • C07D239/08—Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member with hetero atoms directly attached in position 2
    • C07D239/12—Nitrogen atoms not forming part of a nitro radical
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D239/00—Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings
    • C07D239/02—Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings
    • C07D239/06—Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member
    • C07D239/08—Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member with hetero atoms directly attached in position 2
    • C07D239/12—Nitrogen atoms not forming part of a nitro radical
    • C07D239/14—Nitrogen atoms not forming part of a nitro radical with only hydrogen atoms, hydrocarbon or substituted hydrocarbon radicals, attached to said nitrogen atoms
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    • C07—ORGANIC CHEMISTRY
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    • C07D401/00—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom
    • C07D401/02—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings
    • C07D401/04—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings directly linked by a ring-member-to-ring-member bond
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    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D403/00—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00
    • C07D403/02—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00 containing two hetero rings
    • C07D403/04—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00 containing two hetero rings directly linked by a ring-member-to-ring-member bond
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D417/00—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00
    • C07D417/02—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00 containing two hetero rings
    • C07D417/04—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00 containing two hetero rings directly linked by a ring-member-to-ring-member bond
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    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
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    • H01G11/58—Liquid electrolytes
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    • H01G11/58—Liquid electrolytes
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    • H01G9/00—Electrolytic capacitors, rectifiers, detectors, switching devices, light-sensitive or temperature-sensitive devices; Processes of their manufacture
    • H01G9/20—Light-sensitive devices
    • H01G9/2004—Light-sensitive devices characterised by the electrolyte, e.g. comprising an organic electrolyte
    • H01G9/2013—Light-sensitive devices characterised by the electrolyte, e.g. comprising an organic electrolyte the electrolyte comprising ionic liquids, e.g. alkyl imidazolium iodide
    • H—ELECTRICITY
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    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/36—Accumulators not provided for in groups H01M10/05-H01M10/34
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    • H01G9/20—Light-sensitive devices
    • H01G9/2027—Light-sensitive devices comprising an oxide semiconductor electrode
    • H01G9/2031—Light-sensitive devices comprising an oxide semiconductor electrode comprising titanium oxide, e.g. TiO2
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    • H01G9/00—Electrolytic capacitors, rectifiers, detectors, switching devices, light-sensitive or temperature-sensitive devices; Processes of their manufacture
    • H01G9/20—Light-sensitive devices
    • H01G9/2059—Light-sensitive devices comprising an organic dye as the active light absorbing material, e.g. adsorbed on an electrode or dissolved in solution
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
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    • Y02E10/00—Energy generation through renewable energy sources
    • Y02E10/50—Photovoltaic [PV] energy
    • Y02E10/542—Dye sensitized solar cells
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    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
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    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
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  • Chemical & Material Sciences (AREA)
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  • Inorganic Chemistry (AREA)
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  • Secondary Cells (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Primary Cells (AREA)
  • Plural Heterocyclic Compounds (AREA)
  • Electric Double-Layer Capacitors Or The Like (AREA)
  • Separation Using Semi-Permeable Membranes (AREA)

Abstract

　より広い電位範囲で安定であり、高いイオン伝導性を有するイオン液体を提供する。 　このイオン液体は、下記式（１）で表される環状グアニジン塩からなる。式中、R1及びR2は独立にアルキル基またはアルコキシアルキル基を示し、Xはメチレン基、酸素原子、硫黄原子またはＲ3Ｎを示す。Ｒ3はアルキル基、アルコキシアルキル基またはアシル基を示す。ｌ、ｍ、ｎは１以上、６以下の整数を示す。Ｙ-は(R4SO2)2N-、R4SO3 -、R4COO-、BF4-、PF6 -、NO3 -、(CN)2N-、(CHO)2N-、NCS-、R4OSO3 -、R4SO2S-、およびハロゲンイオン等の一価のアニオンを示す。このイオン液体は、各種電解質として有用であり、特に電気化学セルの電解質として有用である。
PCT/JP2008/053295 2007-03-06 2008-02-26 環状グアニジンイオン液体 WO2008108221A1 (ja)

Priority Applications (6)

Application Number Priority Date Filing Date Title
KR1020097018938A KR101451355B1 (ko) 2007-03-06 2008-02-26 환상 구아니딘 이온 액체
US12/529,590 US8129543B2 (en) 2007-03-06 2008-02-26 Cyclic guanidine ionic liquid
EP08720881.5A EP2135862A4 (en) 2007-03-06 2008-02-26 IONIC LIQUID OF CYCLIC GUANIDINE
JP2009502523A JP5243404B2 (ja) 2007-03-06 2008-02-26 環状グアニジンイオン液体
CN2008800056705A CN101616898B (zh) 2007-03-06 2008-02-26 环状胍离子液体
US13/358,491 US8450478B2 (en) 2007-03-06 2012-01-25 Cyclic guanidine ionic liquid

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2007-055629 2007-03-06
JP2007055629 2007-03-06

Related Child Applications (2)

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US12/529,590 A-371-Of-International US8129543B2 (en) 2007-03-06 2008-02-26 Cyclic guanidine ionic liquid
US13/358,491 Division US8450478B2 (en) 2007-03-06 2012-01-25 Cyclic guanidine ionic liquid

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WO2008108221A1 true WO2008108221A1 (ja) 2008-09-12

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PCT/JP2008/053295 WO2008108221A1 (ja) 2007-03-06 2008-02-26 環状グアニジンイオン液体

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US (2) US8129543B2 (ja)
EP (1) EP2135862A4 (ja)
JP (1) JP5243404B2 (ja)
KR (1) KR101451355B1 (ja)
CN (1) CN101616898B (ja)
WO (1) WO2008108221A1 (ja)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN106111086A (zh) * 2016-06-22 2016-11-16 江南大学 一种吸附Pd2+金属离子的离子型高分子吸附剂及其制备方法
CN113522357A (zh) * 2021-08-20 2021-10-22 山东瑞博龙化工科技股份有限公司 一种离子液体催化剂及其制备方法与应用

Families Citing this family (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN101616898B (zh) * 2007-03-06 2012-01-04 新日铁化学株式会社 环状胍离子液体
CN101875635A (zh) * 2010-06-30 2010-11-03 彩虹集团公司 一种环状胍盐离子液体及其制备方法
US8865094B2 (en) 2012-09-13 2014-10-21 Ut-Battelle, Llc Methods for separating medical isotopes using ionic liquids
US9300009B2 (en) 2012-10-22 2016-03-29 Ut-Battelle, Llc Electrolyte compositions for lithium ion batteries
US9455439B2 (en) 2012-11-21 2016-09-27 Ut-Battelle, Llc Nitrogen—sulfur—carbon nanocomposites and their application as cathode materials in lithium—sulfur batteries
DE102013202252A1 (de) * 2013-02-12 2014-08-28 Siemens Aktiengesellschaft Dünnschichtkondensatoren mit hoher Integrationsdichte
US11005127B2 (en) 2015-05-05 2021-05-11 Ut-Battelle, Llc Stable fluorinated alkylated lithium malonatoborate salts for lithium-ion battery applications
US11795583B2 (en) 2021-01-21 2023-10-24 Ut-Battelle, Llc Plasticized melt spinning process using ionic liquids for production of polyacrylonitrile fibers

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JP2003062467A (ja) 2001-08-24 2003-03-04 Central Glass Co Ltd イオン液体組成物
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JP2004067543A (ja) 2002-08-02 2004-03-04 Koei Chem Co Ltd Ｎ−アルコキシエチル脂環式アンモニウム塩及びその製造法
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See also references of EP2135862A4
SYNTHETIC COMMUNICATION, vol. 34, 2004, pages 3083 - 3089

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN106111086A (zh) * 2016-06-22 2016-11-16 江南大学 一种吸附Pd2+金属离子的离子型高分子吸附剂及其制备方法
CN113522357A (zh) * 2021-08-20 2021-10-22 山东瑞博龙化工科技股份有限公司 一种离子液体催化剂及其制备方法与应用

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JP5243404B2 (ja) 2013-07-24
CN101616898B (zh) 2012-01-04
EP2135862A4 (en) 2014-10-01
US8450478B2 (en) 2013-05-28
US20120123115A1 (en) 2012-05-17
US8129543B2 (en) 2012-03-06
JPWO2008108221A1 (ja) 2010-06-10
CN101616898A (zh) 2009-12-30
EP2135862A1 (en) 2009-12-23
KR20090118969A (ko) 2009-11-18
US20100121074A1 (en) 2010-05-13
KR101451355B1 (ko) 2014-10-15

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