US20100012237A1 - Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions - Google Patents

Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions Download PDF

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Publication number
US20100012237A1
US20100012237A1 US12/499,598 US49959809A US2010012237A1 US 20100012237 A1 US20100012237 A1 US 20100012237A1 US 49959809 A US49959809 A US 49959809A US 2010012237 A1 US2010012237 A1 US 2010012237A1
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US
United States
Prior art keywords
ammonium
oxidative
ammonium nitrate
nitrate
oxidizing compound
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Abandoned
Application number
US12/499,598
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English (en)
Inventor
Alan B. Levy
James A. Kweeder
Jose Carrazza
Kenneth D. Kunz
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Honeywell International Inc
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Honeywell International Inc
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Honeywell International Inc filed Critical Honeywell International Inc
Priority to US12/499,598 priority Critical patent/US20100012237A1/en
Priority to RU2011103258/13A priority patent/RU2515379C2/ru
Priority to TR2019/09929T priority patent/TR201909929T4/tr
Priority to CN200980135789.9A priority patent/CN102149656B/zh
Priority to EP09825152.3A priority patent/EP2315736B1/en
Priority to PCT/US2009/049993 priority patent/WO2010053604A2/en
Priority to DE9825152T priority patent/DE09825152T1/de
Priority to ES09825152T priority patent/ES2734511T3/es
Priority to JP2011518798A priority patent/JP5596682B2/ja
Priority to AU2009311605A priority patent/AU2009311605B2/en
Priority to CA2731093A priority patent/CA2731093C/en
Assigned to HONEYWELL INTERNATIONAL INC. reassignment HONEYWELL INTERNATIONAL INC. ASSIGNMENT OF ASSIGNORS INTEREST (SEE DOCUMENT FOR DETAILS). Assignors: CARRAZZA, JOSE, KURZ, KENNETH D., KWEEDER, JAMES A., LEVY, ALAN B.
Publication of US20100012237A1 publication Critical patent/US20100012237A1/en
Priority to EG2011010101A priority patent/EG26334A/en
Priority to US13/026,834 priority patent/US8652277B2/en
Abandoned legal-status Critical Current

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    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01CAMMONIA; CYANOGEN; COMPOUNDS THEREOF
    • C01C1/00Ammonia; Compounds thereof
    • C01C1/18Nitrates of ammonium
    • CCHEMISTRY; METALLURGY
    • C05FERTILISERS; MANUFACTURE THEREOF
    • C05CNITROGENOUS FERTILISERS
    • C05C1/00Ammonium nitrate fertilisers
    • CCHEMISTRY; METALLURGY
    • C05FERTILISERS; MANUFACTURE THEREOF
    • C05CNITROGENOUS FERTILISERS
    • C05C1/00Ammonium nitrate fertilisers
    • C05C1/02Granulation; Pelletisation; Stabilisation; Colouring
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01PINDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2002/00Crystal-structural characteristics
    • C01P2002/80Crystal-structural characteristics defined by measured data other than those specified in group C01P2002/70
    • C01P2002/88Crystal-structural characteristics defined by measured data other than those specified in group C01P2002/70 by thermal analysis data, e.g. TGA, DTA, DSC
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01PINDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2006/00Physical properties of inorganic compounds
    • C01P2006/32Thermal properties
    • C01P2006/37Stability against thermal decomposition

Definitions

  • ammonium nitrate (including double salts comprising ammonium nitrate) has important uses in the field of agriculture in general and fertilization in particular.
  • ammonium nitrate in many of the forms in which it has heretofore been commonly used, is relatively difficult and potentially hazardous to handle commercially in large amounts, and/or to store in great masses (such as occur in commercial warehouses and storage bins), especially for relatively long periods of time.
  • many of the forms of ammonium nitrate heretofore commonly used have had a tendency to detonate under relatively mild conditions and have, therefore, sometimes been abused and misused as an explosive material.
  • non-explosive composition including a substantially homogeneous blend of solid state ammonium nitrate having an average particle diameter of about 1 to about 1000 ⁇ m and non-oxidizing particulate matter having an average particle diameter of about 1 to about 1000 ⁇ m.
  • a method of forming stable ammonium nitrate composite material including (a) reducing the average size of ammonium nitrate having an average particle diameter greater than about 1 mm; and (b) blending said ammonium nitrate with a substantially non-oxidizing compound having an average particle diameter of about 1,000 ⁇ m or less to produce a substantially homogeneous blend of ammonium nitrate and said non-oxidizing compound having an average particle diameter of about 1 to about 1,000 ⁇ m to form a substantially non-explosive powder.
  • FIG. 1 is a thermogram of DTG and DTA as a function of temperature for a typical ammonium nitrate.
  • FIG. 2 is a thermogram of DTG and DTA as a function of temperature for ammonium nitrate sulfate double salt.
  • FIG. 3 is a thermogram of DTG and DTA as a function of temperature for one of our ammonium nitrate composites.
  • FIG. 4 is a thermogram of DTG and DTA as a function of temperature for another one of our ammonium nitrate composites.
  • FIG. 5 is a thermogram of DTG and DTA as a function of temperature for yet another one of our ammonium nitrate composites.
  • FIG. 6 is a thermogram of DTG and DTA. as a function of temperature for still another one of our ammonium nitrate composites.
  • FIG. 7 is a thermogram of DTG and DTA as a function of temperature for still another one of our ammonium nitrate composites.
  • FIG. 8 is a thermogram of DTG and DTA as a function of temperature for still another one of our ammonium nitrate composites.
  • ammonium nitrate compositions comprising ammonium nitrate and at least a second compound, wherein the second compound preferably has the effect of substantially reducing the oxidative tendencies of ammonium nitrate.
  • the second compound may be a non-oxidizing salt which is preferably incorporated into the composite by intimately mixing fine particles of ammonium nitrate with fine particles of the at least one second compound.
  • fine particle refers to particles and collections of particles having an average particle size of about 1000 ⁇ m or less.
  • the fine particles are preferably fine powders.
  • the methods may comprise forming fine particles of ammonium nitrate, forming fine particles of a second compound, mixing the fine particles to a desired substantially homogeneous composition, and then granulating the homogeneous composition to produce a material comprising granules of the desired size.
  • the second compound may be selected from at least from the group consisting of: non-oxidative or low-oxidative ammonium salts such as ammonium sulfate, ammonium phosphate, ammonium molybdenate, ammonium hexaflourosilicate and the like; non-oxidative or low-oxidative calcium salts such as calcium nitrate, calcium carbonate and the like; non-oxidative or low-oxidative potassium salts such as potassium nitrate, potassium phosphate and the like; and other salts such as magnesium nitrate, neodymium hydroxynitrate and the like.
  • non-oxidative or low-oxidative ammonium salts such as ammonium sulfate, ammonium phosphate, ammonium molybdenate, ammonium hexaflourosilicate and the like
  • non-oxidative or low-oxidative calcium salts such as calcium nitrate, calcium carbonate and the like
  • ammonium nitrate composition refers broadly to compositions which comprise ammonium nitrate in any form.
  • the composites may have a wide range of relative ammonium nitrate:second compound concentrations.
  • the mole ratio of ammonium nitrate to the second compound is preferably from about 0.8:1 to about 1:1.2, with a molar ratio of about 1:1 being more preferred.
  • the ammonium nitrate used to form the composites is preferably fertilizer grade material of at least about 90 wt. % purity, more preferably, at least about 95 wt. % purity, and even more preferably at least about 97 wt. % purity. Because of the hazards of mixing organic materials with ammonium nitrate, it is highly desirable that neither the ammonium sulfate nor the second compound contains more than about 0.2 wt. % organic impurities.
  • One method for forming the composites comprises blending, with low energy input, ammonium nitrate particles of a size readily commercially available, preferably having an average particle diameter of greater than about 1 mm, with fine particles of the low-oxidizing or non-oxidizing second compound, and then granulating the blend to produce a homogeneous blend of fine particles of both ammonium nitrate and the second compound.
  • This process is preferred due to concern that handling and storage of fine particle size ammonium nitrate, in the absence of the anti-oxidizing compounds, can create conditions in which detonation, deflagration or explosion are relatively more likely.
  • the ammonium nitrate is diluted with the second compound in fine particle size as the fine particles of ammonium nitrate are formed. The blend of fine particles can then be handled, stored and further processed much more safely.
  • the granulation process may comprise providing the blend of fine particles comprising ammonium nitrate and the second compound and introducing the blend of particles to a granulator containing a non-thermoreactive acids or mixture of acids such as sulfuric acid and/or nitric acid, in an ammoniating environment, wherein ammonium sulfate at least partially covers or coats particles or groups of particles forming the blend of fine particles.
  • a granulator containing a non-thermoreactive acids or mixture of acids such as sulfuric acid and/or nitric acid
  • ammonium sulfate at least partially covers or coats particles or groups of particles forming the blend of fine particles.
  • This causes agglomeration or growth of particles that further include ammonium sulfate coatings that can further improve the safety of the composite material.
  • Those skilled in the art in view of these teachings, can adapt this granulation technique and other known granulation techniques to produce materials having the properties, including the particle size, desired for a
  • our method can include (a) reducing the average size of ammonium nitrate having an average particle diameter greater than about 1 mm; and (b) blending said ammonium nitrate with a substantially non-oxidizing compound having an average particle diameter of about 1,000 ⁇ m or less to produce a substantially homogeneous blend of ammonium nitrate and said non-oxidizing compound having an average particle diameter of about 1 to about 1,000 ⁇ m to form a substantially non-explosive powder.
  • our methods also include the step of compacting the particles.
  • FIG. 1 Fused ammonium nitrate (AN) was tested using Seiko Instruments SSC-5200 that collects Differential Thermal Analysis (DTA) data simultaneously with the Thermogravimetric Analysis (TGA) data.
  • DTA Differential Thermal Analysis
  • TGA Thermogravimetric Analysis
  • FIG. 1 illustrates typical results from testing of AN, showing its relative instability and oxidation potential.
  • Fused ammonium nitrate sulfate (ANS) 1:2 double salt was tested using the same analytical equipment described in connection with Comparative Example 1.
  • the resulting thermogram in FIG. 2 illustrates typical results from testing of 1:2 ANS double salt, showing its relative-stability.
  • thermogramic results are shown in Table 2 and FIGS. 7-8 .

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Fertilizers (AREA)
  • Inorganic Compounds Of Heavy Metals (AREA)
  • Catalysts (AREA)
  • Compounds Of Alkaline-Earth Elements, Aluminum Or Rare-Earth Metals (AREA)
  • Agricultural Chemicals And Associated Chemicals (AREA)
US12/499,598 2008-07-15 2009-07-08 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions Abandoned US20100012237A1 (en)

Priority Applications (13)

Application Number Priority Date Filing Date Title
US12/499,598 US20100012237A1 (en) 2008-07-15 2009-07-08 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions
ES09825152T ES2734511T3 (es) 2008-07-15 2009-07-09 Materiales compuestos de nitrato de amonio débilmente oxidantes y procedimientos para preparar dichas composiciones
JP2011518798A JP5596682B2 (ja) 2008-07-15 2009-07-09 弱酸化性硝酸アンモニウム複合材料および当該組成物の調製方法
CN200980135789.9A CN102149656B (zh) 2008-07-15 2009-07-09 弱氧化性硝酸铵复合材料及这种组合物的制备方法
EP09825152.3A EP2315736B1 (en) 2008-07-15 2009-07-09 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions
PCT/US2009/049993 WO2010053604A2 (en) 2008-07-15 2009-07-09 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions
DE9825152T DE09825152T1 (de) 2008-07-15 2009-07-09 Schwach oxidierende ammoniumnitrat-verbundmaterialien und verfahren zur herstellung solcher zusammensetzungen
RU2011103258/13A RU2515379C2 (ru) 2008-07-15 2009-07-09 Слабо окислительный композитный материал на основе нитрата аммония и способ его изготовления
TR2019/09929T TR201909929T4 (tr) 2009-07-08 2009-07-09 Zayıf yükseltgen amonyum nitrat kompozit materyaller ve bu bileşimlerin hazırlanmasına yönelik yöntemler.
AU2009311605A AU2009311605B2 (en) 2008-07-15 2009-07-09 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions
CA2731093A CA2731093C (en) 2008-07-15 2009-07-09 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions
EG2011010101A EG26334A (en) 2008-07-15 2011-01-16 Weak oxidation of compounds of ammonium nitrate and methods for the preparation of such formulations
US13/026,834 US8652277B2 (en) 2008-07-15 2011-02-14 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US8089808P 2008-07-15 2008-07-15
US12/499,598 US20100012237A1 (en) 2008-07-15 2009-07-08 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions

Related Child Applications (1)

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US13/026,834 Division US8652277B2 (en) 2008-07-15 2011-02-14 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions

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US20100012237A1 true US20100012237A1 (en) 2010-01-21

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US12/499,598 Abandoned US20100012237A1 (en) 2008-07-15 2009-07-08 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions
US13/026,834 Active 2030-09-21 US8652277B2 (en) 2008-07-15 2011-02-14 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions

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US13/026,834 Active 2030-09-21 US8652277B2 (en) 2008-07-15 2011-02-14 Weakly oxidizing ammonium nitrate composite materials and methods for preparing such compositions

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US (2) US20100012237A1 (enExample)
EP (1) EP2315736B1 (enExample)
JP (1) JP5596682B2 (enExample)
CN (1) CN102149656B (enExample)
AU (1) AU2009311605B2 (enExample)
CA (1) CA2731093C (enExample)
DE (1) DE09825152T1 (enExample)
EG (1) EG26334A (enExample)
ES (1) ES2734511T3 (enExample)
RU (1) RU2515379C2 (enExample)
WO (1) WO2010053604A2 (enExample)

Families Citing this family (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
TN2014000159A1 (fr) * 2014-04-15 2015-09-30 Ouadday Mohamed Engrais azoté à base de nitrate d'ammonium non explosif et ininflammable
US12338189B2 (en) 2023-05-24 2025-06-24 Defuse Technologies, LLC Desensitized fertilizer compositions and methods of making same

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US3223518A (en) * 1961-08-18 1965-12-14 Archer Daniels Midland Granular fertilizer having a plurality of coatings and the process of making
US3366468A (en) * 1965-02-10 1968-01-30 Samuel J. Porter Method of desensitizing fertilizer grade ammonium nitrate and the product obtained
US4125368A (en) * 1974-05-31 1978-11-14 Toms River Chemical Corp. Metallized monoazo dyes
US4409016A (en) * 1981-06-19 1983-10-11 Unie Van Kunstmestfabrieken, B.V. Process for preparing thermally stable ammonium nitrate-containing granules of high bulk density
US4913725A (en) * 1986-05-16 1990-04-03 Sumitomo Chemical Company, Limited Granular fertilizer compositions
US6372191B1 (en) * 1999-12-03 2002-04-16 Autoliv Asp, Inc. Phase stabilized ammonium nitrate and method of making the same
US6641662B2 (en) * 1998-02-17 2003-11-04 The Trustees Of Columbia University In The City Of New York Method for fabricating ultra thin single-crystal metal oxide wave retarder plates and waveguide polarization mode converter using the same
US6641622B2 (en) * 2001-01-23 2003-11-04 Trw Inc. Process for preparing phase-stabilized ammonium nitrate
US7014828B2 (en) * 2000-01-04 2006-03-21 Kemira Growhow Oyj Process for stabilizing ammonium nitrate
US20070199357A1 (en) * 2006-01-13 2007-08-30 Honeywell International Inc. Compositions comprising ammonium nitrate double salts

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US3223518A (en) * 1961-08-18 1965-12-14 Archer Daniels Midland Granular fertilizer having a plurality of coatings and the process of making
US3366468A (en) * 1965-02-10 1968-01-30 Samuel J. Porter Method of desensitizing fertilizer grade ammonium nitrate and the product obtained
US4125368A (en) * 1974-05-31 1978-11-14 Toms River Chemical Corp. Metallized monoazo dyes
US4409016A (en) * 1981-06-19 1983-10-11 Unie Van Kunstmestfabrieken, B.V. Process for preparing thermally stable ammonium nitrate-containing granules of high bulk density
US4913725A (en) * 1986-05-16 1990-04-03 Sumitomo Chemical Company, Limited Granular fertilizer compositions
US6641662B2 (en) * 1998-02-17 2003-11-04 The Trustees Of Columbia University In The City Of New York Method for fabricating ultra thin single-crystal metal oxide wave retarder plates and waveguide polarization mode converter using the same
US6372191B1 (en) * 1999-12-03 2002-04-16 Autoliv Asp, Inc. Phase stabilized ammonium nitrate and method of making the same
US7014828B2 (en) * 2000-01-04 2006-03-21 Kemira Growhow Oyj Process for stabilizing ammonium nitrate
US7147830B2 (en) * 2000-01-04 2006-12-12 Kemira Growhow Oyj Stabilized ammonium nitrate granules
US6641622B2 (en) * 2001-01-23 2003-11-04 Trw Inc. Process for preparing phase-stabilized ammonium nitrate
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Also Published As

Publication number Publication date
CA2731093A1 (en) 2010-05-14
WO2010053604A3 (en) 2010-08-26
EP2315736B1 (en) 2019-04-10
AU2009311605B2 (en) 2014-02-27
CA2731093C (en) 2016-02-09
EP2315736A4 (en) 2015-03-04
AU2009311605A1 (en) 2010-05-14
WO2010053604A2 (en) 2010-05-14
CN102149656A (zh) 2011-08-10
US8652277B2 (en) 2014-02-18
RU2011103258A (ru) 2012-08-20
EP2315736A2 (en) 2011-05-04
RU2515379C2 (ru) 2014-05-10
EG26334A (en) 2013-08-19
JP2011528314A (ja) 2011-11-17
JP5596682B2 (ja) 2014-09-24
DE09825152T1 (de) 2012-02-02
CN102149656B (zh) 2016-06-22
ES2734511T3 (es) 2019-12-10
US20110132051A1 (en) 2011-06-09

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