RU2003128600A - Способ получения синтез-газа - Google Patents

Способ получения синтез-газа Download PDF

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RU2003128600A
RU2003128600A RU2003128600/04A RU2003128600A RU2003128600A RU 2003128600 A RU2003128600 A RU 2003128600A RU 2003128600/04 A RU2003128600/04 A RU 2003128600/04A RU 2003128600 A RU2003128600 A RU 2003128600A RU 2003128600 A RU2003128600 A RU 2003128600A
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Russia
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steam
reforming
water vapor
autothermal
units
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RU2003128600/04A
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English (en)
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RU2345948C9 (ru
RU2345948C2 (ru
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Нильс ЭРИКСТРУП (DK)
Нильс ЭРИКСТРУП
Томас РОСТРУП-НИЛЬСЕН (DK)
Томас РОСТРУП-НИЛЬСЕН
Петер Сайер КРИСТЕНСЕН (DK)
Петер Сайер Кристенсен
Йенс-Хенрик Бак ХАНСЕН (DK)
Йенс-Хенрик Бак ХАНСЕН
Иб ДЮБКЬЯР (DK)
Иб ДЮБКЬЯР
Ким ААСБЕРГ-ПЕТЕРСЕН (DK)
Ким Аасберг-Петерсен
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Хальдор Топсеэ А/С (DK)
Хальдор Топсеэ А/С
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    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2/00—Production of liquid hydrocarbon mixtures of undefined composition from oxides of carbon
    • C10G2/30—Production of liquid hydrocarbon mixtures of undefined composition from oxides of carbon from carbon monoxide with hydrogen
    • C10G2/32—Production of liquid hydrocarbon mixtures of undefined composition from oxides of carbon from carbon monoxide with hydrogen with the use of catalysts
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10L—FUELS NOT OTHERWISE PROVIDED FOR; NATURAL GAS; SYNTHETIC NATURAL GAS OBTAINED BY PROCESSES NOT COVERED BY SUBCLASSES C10G, C10K; LIQUEFIED PETROLEUM GAS; ADDING MATERIALS TO FUELS OR FIRES TO REDUCE SMOKE OR UNDESIRABLE DEPOSITS OR TO FACILITATE SOOT REMOVAL; FIRELIGHTERS
    • C10L3/00—Gaseous fuels; Natural gas; Synthetic natural gas obtained by processes not covered by subclass C10G, C10K; Liquefied petroleum gas
    • C10L3/06—Natural gas; Synthetic natural gas obtained by processes not covered by C10G, C10K3/02 or C10K3/04
    • C10L3/08—Production of synthetic natural gas
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
    • C01B3/382—Multi-step processes
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0205—Processes for making hydrogen or synthesis gas containing a reforming step
    • C01B2203/0227—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step
    • C01B2203/0233—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step the reforming step being a steam reforming step
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0205—Processes for making hydrogen or synthesis gas containing a reforming step
    • C01B2203/0227—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step
    • C01B2203/0244—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step the reforming step being an autothermal reforming step, e.g. secondary reforming processes
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/06—Integration with other chemical processes
    • C01B2203/062—Hydrocarbon production, e.g. Fischer-Tropsch process
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08—Methods of heating or cooling
    • C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0838—Methods of heating the process for making hydrogen or synthesis gas by heat exchange with exothermic reactions, other than by combustion of fuel
    • C01B2203/0844—Methods of heating the process for making hydrogen or synthesis gas by heat exchange with exothermic reactions, other than by combustion of fuel the non-combustive exothermic reaction being another reforming reaction as defined in groups C01B2203/02 - C01B2203/0294
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/10—Catalysts for performing the hydrogen forming reactions
    • C01B2203/1005—Arrangement or shape of catalyst
    • C01B2203/1011—Packed bed of catalytic structures, e.g. particles, packing elements
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/10—Catalysts for performing the hydrogen forming reactions
    • C01B2203/1005—Arrangement or shape of catalyst
    • C01B2203/1023—Catalysts in the form of a monolith or honeycomb
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/14—Details of the flowsheet
    • C01B2203/141—At least two reforming, decomposition or partial oxidation steps in parallel
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/14—Details of the flowsheet
    • C01B2203/142—At least two reforming, decomposition or partial oxidation steps in series
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/14—Details of the flowsheet
    • C01B2203/148—Details of the flowsheet involving a recycle stream to the feed of the process for making hydrogen or synthesis gas
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/80—Aspect of integrated processes for the production of hydrogen or synthesis gas not covered by groups C01B2203/02 - C01B2203/1695
    • C01B2203/82—Several process steps of C01B2203/02 - C01B2203/08 integrated into a single apparatus
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00—Technologies relating to chemical industry
    • Y02P20/50—Improvements relating to the production of bulk chemicals
    • Y02P20/52—Improvements relating to the production of bulk chemicals using catalysts, e.g. selective catalysts

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Organic Chemistry (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Engineering & Computer Science (AREA)
  • General Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Combustion & Propulsion (AREA)
  • Inorganic Chemistry (AREA)
  • Hydrogen, Water And Hydrids (AREA)
  • Catalysts (AREA)

Claims (10)

1. Способ получения синтез-газа каталитическим реформингом с водяным паром углеводородсодержащего сырья параллельно в автотермической реформинг-установке с водяным паром и в одной или нескольких последовательных реформинг-установках с водяным паром, причем тепло для реакций реформинга с водяным паром в одной или нескольких реформинг-установках с водяным паром обеспечивают непрямым теплообменом с объединенными потоками газа, отходящего от одной или нескольких реформинг-установок с водяным паром с автотермической реформинг-установкой в водяным паром, и где газ, содержащий оксид углерода, добавляют к сырью перед реформингом с водяным паром в автотермической реформинг-установке с водяным паром и/или перед реформингом с водяным паром в одной или нескольких реформинг-установках с водяным паром, а газ, содержащий оксид углерода, имеющий мольное отношение водорода к углероду менее 4,5, добавляют в количестве, приводящем к потоку продукта, имеющего мольное отношение водорода к оксиду углерода между, приблизительно, 1,8 и 2,3.
2. Способ по п.1, где одна или несколько реформинг-установок с водяным паром представляют собой адиабатические реформинг-установки с водяным паром и/или теплообменные реформинг-установки с водяным паром.
3. Способ по п.2, где сырье для одной или нескольких адиабатических реформинг-установок с водяным паром подогревают непрямым теплообменом с объединенными потоками газов, отходящих от одной или нескольких реформинг-установок с водяным паром и автотермической реформинг-установки с водяным паром.
4. Способ по п.2, где тепло для теплообменной реформинг-установки обеспечивают непрямым теплообменом с объединенными потоками газов, отходящих от одной или нескольких реформинг-установок с водяным паром и автотермической реформинг-установки с водяным паром.
5. Способ по п.1, где катализатор в, по меньшей мере, одной из реформинг-установок с водяным паром находится в форме гранул или каталитического средства.
6. Способ по п.5, где каталитическое средство размещено на структурированных металлических или керамических элементах или на монолитах.
7. Способ по п.1, где активный каталитический материал в первой из реформинг-установок с водяным паром представляет собой никель, а активный материал в последней из реформинг-установок с водяным паром представляет собой благородный металл или смесь благородных металлов.
8. Способ по п.3, где подогрев объединяют с каталитическим реформингом с водяным паром между, по меньшей мере, одной из адиабатических реформинг-установок с водяным паром.
9. Способ по п.1, где окислитель для автотермической реформинг-установки с водяным паром содержит, по меньшей мере, 90% кислорода по объему.
10. Способ по любому из предшествующих пунктов, где газ, содержащий оксид углерода, представляет собой остаточный газ из процесса Фишера-Тропша.
RU2003128600/04A 2002-09-26 2003-09-25 Способ получения синтез-газа для производства углеводородов RU2345948C9 (ru)

Applications Claiming Priority (6)

Application Number Priority Date Filing Date Title
DK200201434 2002-09-26
DKPA200201434 2002-09-26
DKPA200201434 2002-09-26
DK200201433 2002-09-26
DKPA200201433 2002-09-26
DKPA200201433 2002-09-26

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RU2003128600A true RU2003128600A (ru) 2005-03-27
RU2345948C2 RU2345948C2 (ru) 2009-02-10
RU2345948C9 RU2345948C9 (ru) 2010-03-20

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US (1) US7074347B2 (ru)
EP (1) EP1403216B1 (ru)
JP (1) JP4351010B2 (ru)
KR (1) KR101003726B1 (ru)
CN (1) CN1308224C (ru)
AT (1) ATE502894T1 (ru)
AU (1) AU2003248393B2 (ru)
CA (1) CA2442770C (ru)
DE (1) DE60336444D1 (ru)
NO (1) NO339753B1 (ru)
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CN1308224C (zh) 2007-04-04
JP2004269343A (ja) 2004-09-30
CA2442770A1 (en) 2004-03-26
AU2003248393A1 (en) 2004-04-22
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US20040063798A1 (en) 2004-04-01
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JP4351010B2 (ja) 2009-10-28
EP1403216A1 (en) 2004-03-31
DE60336444D1 (de) 2011-05-05
KR101003726B1 (ko) 2010-12-23
NO20034284L (no) 2004-03-29
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