JP6010529B2 - 白金ニッケル触媒合金 - Google Patents
白金ニッケル触媒合金 Download PDFInfo
- Publication number
- JP6010529B2 JP6010529B2 JP2013508155A JP2013508155A JP6010529B2 JP 6010529 B2 JP6010529 B2 JP 6010529B2 JP 2013508155 A JP2013508155 A JP 2013508155A JP 2013508155 A JP2013508155 A JP 2013508155A JP 6010529 B2 JP6010529 B2 JP 6010529B2
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- JP
- Japan
- Prior art keywords
- catalyst
- fuel cell
- lattice constant
- measured
- alloy
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
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- 239000003054 catalyst Substances 0.000 title claims description 98
- 229910045601 alloy Inorganic materials 0.000 title description 15
- 239000000956 alloy Substances 0.000 title description 15
- PCLURTMBFDTLSK-UHFFFAOYSA-N nickel platinum Chemical compound [Ni].[Pt] PCLURTMBFDTLSK-UHFFFAOYSA-N 0.000 title 1
- 239000000446 fuel Substances 0.000 claims description 38
- 239000002245 particle Substances 0.000 claims description 16
- 239000000463 material Substances 0.000 claims description 10
- 239000010409 thin film Substances 0.000 claims description 8
- 210000000170 cell membrane Anatomy 0.000 claims description 4
- 230000003197 catalytic effect Effects 0.000 claims description 2
- BASFCYQUMIYNBI-UHFFFAOYSA-N platinum Chemical compound [Pt] BASFCYQUMIYNBI-UHFFFAOYSA-N 0.000 description 50
- 210000004027 cell Anatomy 0.000 description 33
- 230000000694 effects Effects 0.000 description 18
- 239000000203 mixture Substances 0.000 description 18
- 229910002844 PtNi Inorganic materials 0.000 description 14
- 239000012528 membrane Substances 0.000 description 12
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 description 10
- 239000001301 oxygen Substances 0.000 description 10
- 229910052760 oxygen Inorganic materials 0.000 description 10
- 238000000034 method Methods 0.000 description 9
- 229910001260 Pt alloy Inorganic materials 0.000 description 8
- 238000002441 X-ray diffraction Methods 0.000 description 8
- 238000004453 electron probe microanalysis Methods 0.000 description 8
- 239000013078 crystal Substances 0.000 description 7
- 229910052759 nickel Inorganic materials 0.000 description 7
- 229910002845 Pt–Ni Inorganic materials 0.000 description 5
- 229910052697 platinum Inorganic materials 0.000 description 5
- 230000009467 reduction Effects 0.000 description 5
- 229910002056 binary alloy Inorganic materials 0.000 description 4
- 239000011572 manganese Substances 0.000 description 4
- 230000010757 Reduction Activity Effects 0.000 description 3
- 229910052751 metal Inorganic materials 0.000 description 3
- 239000002184 metal Substances 0.000 description 3
- 238000004846 x-ray emission Methods 0.000 description 3
- 230000008901 benefit Effects 0.000 description 2
- 238000000151 deposition Methods 0.000 description 2
- 238000000892 gravimetry Methods 0.000 description 2
- 238000005259 measurement Methods 0.000 description 2
- 238000004544 sputter deposition Methods 0.000 description 2
- 238000004876 x-ray fluorescence Methods 0.000 description 2
- PWHULOQIROXLJO-UHFFFAOYSA-N Manganese Chemical compound [Mn] PWHULOQIROXLJO-UHFFFAOYSA-N 0.000 description 1
- 238000005275 alloying Methods 0.000 description 1
- 230000004075 alteration Effects 0.000 description 1
- 230000008859 change Effects 0.000 description 1
- 239000003153 chemical reaction reagent Substances 0.000 description 1
- 230000001419 dependent effect Effects 0.000 description 1
- 230000008021 deposition Effects 0.000 description 1
- 239000006185 dispersion Substances 0.000 description 1
- 239000003792 electrolyte Substances 0.000 description 1
- 238000002474 experimental method Methods 0.000 description 1
- 239000010408 film Substances 0.000 description 1
- 239000007789 gas Substances 0.000 description 1
- 230000006872 improvement Effects 0.000 description 1
- 238000003475 lamination Methods 0.000 description 1
- 229910052748 manganese Inorganic materials 0.000 description 1
- 238000000691 measurement method Methods 0.000 description 1
- 238000012986 modification Methods 0.000 description 1
- 230000004048 modification Effects 0.000 description 1
- 239000002086 nanomaterial Substances 0.000 description 1
- 230000003647 oxidation Effects 0.000 description 1
- 238000007254 oxidation reaction Methods 0.000 description 1
- 239000005518 polymer electrolyte Substances 0.000 description 1
- 230000008569 process Effects 0.000 description 1
- 229910052723 transition metal Inorganic materials 0.000 description 1
- 150000003624 transition metals Chemical class 0.000 description 1
- 238000001771 vacuum deposition Methods 0.000 description 1
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 1
Images
Classifications
-
- C—CHEMISTRY; METALLURGY
- C22—METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
- C22C—ALLOYS
- C22C30/00—Alloys containing less than 50% by weight of each constituent
-
- C—CHEMISTRY; METALLURGY
- C22—METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
- C22C—ALLOYS
- C22C19/00—Alloys based on nickel or cobalt
- C22C19/03—Alloys based on nickel or cobalt based on nickel
-
- C—CHEMISTRY; METALLURGY
- C22—METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
- C22C—ALLOYS
- C22C5/00—Alloys based on noble metals
- C22C5/04—Alloys based on a platinum group metal
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M4/90—Selection of catalytic material
- H01M4/92—Metals of platinum group
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
Landscapes
- Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Materials Engineering (AREA)
- Mechanical Engineering (AREA)
- Metallurgy (AREA)
- Organic Chemistry (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Electrochemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Catalysts (AREA)
- Inert Electrodes (AREA)
Applications Claiming Priority (3)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| US32804910P | 2010-04-26 | 2010-04-26 | |
| US61/328,049 | 2010-04-26 | ||
| PCT/US2011/033949 WO2011139693A2 (en) | 2010-04-26 | 2011-04-26 | Platinum nickel catalyst alloy |
Related Child Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| JP2016181479A Division JP2016209882A (ja) | 2010-04-26 | 2016-09-16 | 白金ニッケル触媒合金 |
Publications (3)
| Publication Number | Publication Date |
|---|---|
| JP2013533795A JP2013533795A (ja) | 2013-08-29 |
| JP2013533795A5 JP2013533795A5 (enExample) | 2014-05-08 |
| JP6010529B2 true JP6010529B2 (ja) | 2016-10-19 |
Family
ID=44626641
Family Applications (2)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| JP2013508155A Active JP6010529B2 (ja) | 2010-04-26 | 2011-04-26 | 白金ニッケル触媒合金 |
| JP2016181479A Pending JP2016209882A (ja) | 2010-04-26 | 2016-09-16 | 白金ニッケル触媒合金 |
Family Applications After (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| JP2016181479A Pending JP2016209882A (ja) | 2010-04-26 | 2016-09-16 | 白金ニッケル触媒合金 |
Country Status (5)
| Country | Link |
|---|---|
| US (1) | US8557484B2 (enExample) |
| EP (1) | EP2564456B1 (enExample) |
| JP (2) | JP6010529B2 (enExample) |
| CN (1) | CN102947990B (enExample) |
| WO (1) | WO2011139693A2 (enExample) |
Families Citing this family (13)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| CA2847210C (en) * | 2011-09-01 | 2020-04-14 | Simon TRUDEL | Electrocatalytic materials, and methods for manufacturing same |
| JP2016522962A (ja) * | 2013-04-23 | 2016-08-04 | スリーエム イノベイティブ プロパティズ カンパニー | 触媒電極及びその製造方法 |
| JP6778472B2 (ja) * | 2015-02-12 | 2020-11-04 | 国立大学法人東京工業大学 | 白金合金粉末及びその製造方法 |
| KR101816800B1 (ko) | 2015-09-11 | 2018-01-10 | 한국과학기술연구원 | 지지체가 필요 없는 금속 나노선 및 3차원 금속 나노 촉매의 제조방법 |
| CN105449232B (zh) * | 2015-11-20 | 2018-01-30 | 吉林大学 | 过渡族金属掺杂Pt‑Al金属间化合物形成双模式孔三元合金的制备方法及应用 |
| CN105797747B (zh) * | 2016-03-01 | 2019-03-22 | 中国石化扬子石油化工有限公司 | 制备1,4-丁二醇的补充精制催化剂、其制备方法及应用 |
| EP3533096B1 (en) * | 2016-10-26 | 2021-12-01 | 3M Innovative Properties Company | Catalyst |
| JP2019534146A (ja) * | 2016-10-26 | 2019-11-28 | スリーエム イノベイティブ プロパティズ カンパニー | 触媒 |
| CN109891646B (zh) * | 2016-10-26 | 2022-06-03 | 3M创新有限公司 | 用于燃料电池的pt-ni-ir催化剂 |
| CN112243541A (zh) * | 2018-04-04 | 2021-01-19 | 3M创新有限公司 | 催化剂 |
| EP3776702B1 (en) * | 2018-04-04 | 2024-05-08 | 3M Innovative Properties Company | Catalyst comprising pt, ni, and ta |
| EP3895238B1 (en) | 2018-12-13 | 2025-08-06 | 3M Innovative Properties Company | Catalyst |
| CN111430731A (zh) * | 2020-04-01 | 2020-07-17 | 安徽师范大学 | 多孔碳载铂材料及其制备方法和应用 |
Family Cites Families (23)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US5039561A (en) | 1986-08-25 | 1991-08-13 | Minnesota Mining And Manufacturing Company | Method for preparing an article having surface layer of uniformly oriented, crystalline, organic microstructures |
| US4812352A (en) | 1986-08-25 | 1989-03-14 | Minnesota Mining And Manufacturing Company | Article having surface layer of uniformly oriented, crystalline, organic microstructures |
| US5176786A (en) | 1988-07-13 | 1993-01-05 | Minnesota Mining And Manufacturing Company | Organic thin film controlled molecular epitaxy |
| JPH04135642A (ja) | 1990-09-26 | 1992-05-11 | Tanaka Kikinzoku Kogyo Kk | 白金合金触媒とその製造方法 |
| US5336558A (en) | 1991-06-24 | 1994-08-09 | Minnesota Mining And Manufacturing Company | Composite article comprising oriented microstructures |
| US5338430A (en) | 1992-12-23 | 1994-08-16 | Minnesota Mining And Manufacturing Company | Nanostructured electrode membranes |
| US6136412A (en) | 1997-10-10 | 2000-10-24 | 3M Innovative Properties Company | Microtextured catalyst transfer substrate |
| US5879827A (en) | 1997-10-10 | 1999-03-09 | Minnesota Mining And Manufacturing Company | Catalyst for membrane electrode assembly and method of making |
| US5879828A (en) | 1997-10-10 | 1999-03-09 | Minnesota Mining And Manufacturing Company | Membrane electrode assembly |
| US6482763B2 (en) | 1999-12-29 | 2002-11-19 | 3M Innovative Properties Company | Suboxide fuel cell catalyst for enhanced reformate tolerance |
| TW200505093A (en) | 2003-07-10 | 2005-02-01 | Du Pont | Electrodes and other fuel cell components having ultra low catalyst loadings coated thereon and processes for making and using the same |
| US8211593B2 (en) | 2003-09-08 | 2012-07-03 | Intematix Corporation | Low platinum fuel cells, catalysts, and method for preparing the same |
| US7419741B2 (en) * | 2003-09-29 | 2008-09-02 | 3M Innovative Properties Company | Fuel cell cathode catalyst |
| GB0419062D0 (en) | 2004-08-27 | 2004-09-29 | Johnson Matthey Plc | Platinum alloy catalyst |
| US7622216B2 (en) | 2005-05-02 | 2009-11-24 | Gm Global Technology Operations, Inc. | Supports for fuel cell catalysts |
| US7790304B2 (en) | 2005-09-13 | 2010-09-07 | 3M Innovative Properties Company | Catalyst layers to enhance uniformity of current density in membrane electrode assemblies |
| US7622217B2 (en) * | 2005-10-12 | 2009-11-24 | 3M Innovative Properties Company | Fuel cell nanocatalyst |
| US20070160899A1 (en) * | 2006-01-10 | 2007-07-12 | Cabot Corporation | Alloy catalyst compositions and processes for making and using same |
| JP5138584B2 (ja) | 2006-03-31 | 2013-02-06 | トヨタ自動車株式会社 | 燃料電池用電極触媒の製造方法 |
| JP5294235B2 (ja) | 2006-05-25 | 2013-09-18 | 日産自動車株式会社 | 電極材料 |
| US8383293B2 (en) | 2006-11-22 | 2013-02-26 | GM Global Technology Operations LLC | Supports for fuel cell catalysts based on transition metal silicides |
| US20100035124A1 (en) | 2008-08-11 | 2010-02-11 | Gm Clobal Technology Operations, Inc. | Hybrid particle and core-shell electrode structure |
| EP2437883A2 (en) * | 2009-06-02 | 2012-04-11 | Basf Se | Catalyst for electrochemical applications |
-
2011
- 2011-04-26 EP EP11721848.7A patent/EP2564456B1/en active Active
- 2011-04-26 US US13/643,353 patent/US8557484B2/en active Active
- 2011-04-26 JP JP2013508155A patent/JP6010529B2/ja active Active
- 2011-04-26 CN CN201180030314.0A patent/CN102947990B/zh active Active
- 2011-04-26 WO PCT/US2011/033949 patent/WO2011139693A2/en not_active Ceased
-
2016
- 2016-09-16 JP JP2016181479A patent/JP2016209882A/ja active Pending
Also Published As
| Publication number | Publication date |
|---|---|
| US20130040227A1 (en) | 2013-02-14 |
| CN102947990A (zh) | 2013-02-27 |
| EP2564456B1 (en) | 2021-05-26 |
| EP2564456A2 (en) | 2013-03-06 |
| WO2011139693A3 (en) | 2012-01-12 |
| JP2016209882A (ja) | 2016-12-15 |
| WO2011139693A2 (en) | 2011-11-10 |
| US8557484B2 (en) | 2013-10-15 |
| CN102947990B (zh) | 2016-09-14 |
| JP2013533795A (ja) | 2013-08-29 |
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