JP2015518637A - 金属空気電池及び電気化学発電方法 - Google Patents
金属空気電池及び電気化学発電方法 Download PDFInfo
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- JP2015518637A JP2015518637A JP2015507335A JP2015507335A JP2015518637A JP 2015518637 A JP2015518637 A JP 2015518637A JP 2015507335 A JP2015507335 A JP 2015507335A JP 2015507335 A JP2015507335 A JP 2015507335A JP 2015518637 A JP2015518637 A JP 2015518637A
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- 238000010248 power generation Methods 0.000 title claims abstract description 10
- 238000000034 method Methods 0.000 title claims description 13
- 239000003792 electrolyte Substances 0.000 claims abstract description 18
- 239000008151 electrolyte solution Substances 0.000 claims abstract description 15
- 239000000463 material Substances 0.000 claims abstract description 8
- 229910052751 metal Inorganic materials 0.000 claims description 74
- 239000002184 metal Substances 0.000 claims description 74
- 239000000843 powder Substances 0.000 claims description 24
- RYGMFSIKBFXOCR-UHFFFAOYSA-N Copper Chemical compound [Cu] RYGMFSIKBFXOCR-UHFFFAOYSA-N 0.000 claims description 8
- 229910052802 copper Inorganic materials 0.000 claims description 8
- 239000010949 copper Substances 0.000 claims description 8
- 239000002131 composite material Substances 0.000 claims description 7
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 claims description 7
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 claims description 6
- 229910052799 carbon Inorganic materials 0.000 claims description 6
- 239000012530 fluid Substances 0.000 claims description 6
- 238000005530 etching Methods 0.000 claims description 4
- 239000011888 foil Substances 0.000 claims description 4
- PCHJSUWPFVWCPO-UHFFFAOYSA-N gold Chemical compound [Au] PCHJSUWPFVWCPO-UHFFFAOYSA-N 0.000 claims description 4
- 229910052737 gold Inorganic materials 0.000 claims description 4
- 239000010931 gold Substances 0.000 claims description 4
- 229920000642 polymer Polymers 0.000 claims description 4
- 238000009736 wetting Methods 0.000 claims description 2
- 239000004020 conductor Substances 0.000 claims 1
- 238000000151 deposition Methods 0.000 claims 1
- 239000000428 dust Substances 0.000 description 12
- 230000002209 hydrophobic effect Effects 0.000 description 4
- ZOXJGFHDIHLPTG-UHFFFAOYSA-N Boron Chemical compound [B] ZOXJGFHDIHLPTG-UHFFFAOYSA-N 0.000 description 3
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 description 3
- 229910052796 boron Inorganic materials 0.000 description 3
- 150000002736 metal compounds Chemical class 0.000 description 3
- 229910052760 oxygen Inorganic materials 0.000 description 3
- 239000001301 oxygen Substances 0.000 description 3
- 229910001111 Fine metal Inorganic materials 0.000 description 2
- WHXSMMKQMYFTQS-UHFFFAOYSA-N Lithium Chemical compound [Li] WHXSMMKQMYFTQS-UHFFFAOYSA-N 0.000 description 2
- 229920006362 Teflon® Polymers 0.000 description 2
- HCHKCACWOHOZIP-UHFFFAOYSA-N Zinc Chemical compound [Zn] HCHKCACWOHOZIP-UHFFFAOYSA-N 0.000 description 2
- 230000005540 biological transmission Effects 0.000 description 2
- AUVPWTYQZMLSKY-UHFFFAOYSA-N boron;vanadium Chemical compound [V]#B AUVPWTYQZMLSKY-UHFFFAOYSA-N 0.000 description 2
- 229910052744 lithium Inorganic materials 0.000 description 2
- 150000002739 metals Chemical class 0.000 description 2
- 230000003647 oxidation Effects 0.000 description 2
- 238000007254 oxidation reaction Methods 0.000 description 2
- 239000011701 zinc Substances 0.000 description 2
- 229910052725 zinc Inorganic materials 0.000 description 2
- QYEXBYZXHDUPRC-UHFFFAOYSA-N B#[Ti]#B Chemical compound B#[Ti]#B QYEXBYZXHDUPRC-UHFFFAOYSA-N 0.000 description 1
- 229920000271 Kevlar® Polymers 0.000 description 1
- 239000004698 Polyethylene Substances 0.000 description 1
- ZLMJMSJWJFRBEC-UHFFFAOYSA-N Potassium Chemical compound [K] ZLMJMSJWJFRBEC-UHFFFAOYSA-N 0.000 description 1
- KWYUFKZDYYNOTN-UHFFFAOYSA-M Potassium hydroxide Chemical compound [OH-].[K+] KWYUFKZDYYNOTN-UHFFFAOYSA-M 0.000 description 1
- 239000004809 Teflon Substances 0.000 description 1
- RTAQQCXQSZGOHL-UHFFFAOYSA-N Titanium Chemical compound [Ti] RTAQQCXQSZGOHL-UHFFFAOYSA-N 0.000 description 1
- 239000000853 adhesive Substances 0.000 description 1
- 230000001070 adhesive effect Effects 0.000 description 1
- 238000002485 combustion reaction Methods 0.000 description 1
- 230000008021 deposition Effects 0.000 description 1
- 230000000694 effects Effects 0.000 description 1
- 238000002848 electrochemical method Methods 0.000 description 1
- 239000007772 electrode material Substances 0.000 description 1
- 239000000446 fuel Substances 0.000 description 1
- XLYOFNOQVPJJNP-UHFFFAOYSA-M hydroxide Chemical compound [OH-] XLYOFNOQVPJJNP-UHFFFAOYSA-M 0.000 description 1
- 238000002347 injection Methods 0.000 description 1
- 239000007924 injection Substances 0.000 description 1
- 238000009434 installation Methods 0.000 description 1
- 150000002500 ions Chemical class 0.000 description 1
- 239000004761 kevlar Substances 0.000 description 1
- 239000011244 liquid electrolyte Substances 0.000 description 1
- 239000012528 membrane Substances 0.000 description 1
- 229910000510 noble metal Inorganic materials 0.000 description 1
- 230000033116 oxidation-reduction process Effects 0.000 description 1
- 239000012466 permeate Substances 0.000 description 1
- -1 polyethylene Polymers 0.000 description 1
- 229920000573 polyethylene Polymers 0.000 description 1
- 229910052700 potassium Inorganic materials 0.000 description 1
- 239000011591 potassium Substances 0.000 description 1
- 239000000243 solution Substances 0.000 description 1
- 239000010936 titanium Substances 0.000 description 1
- 229910052719 titanium Inorganic materials 0.000 description 1
- 230000007704 transition Effects 0.000 description 1
- 238000004804 winding Methods 0.000 description 1
Images
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- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M6/00—Primary cells; Manufacture thereof
- H01M6/30—Deferred-action cells
- H01M6/32—Deferred-action cells activated through external addition of electrolyte or of electrolyte components
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M12/00—Hybrid cells; Manufacture thereof
- H01M12/08—Hybrid cells; Manufacture thereof composed of a half-cell of a fuel-cell type and a half-cell of the secondary-cell type
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M12/00—Hybrid cells; Manufacture thereof
- H01M12/04—Hybrid cells; Manufacture thereof composed of a half-cell of the fuel-cell type and of a half-cell of the primary-cell type
- H01M12/06—Hybrid cells; Manufacture thereof composed of a half-cell of the fuel-cell type and of a half-cell of the primary-cell type with one metallic and one gaseous electrode
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/02—Electrodes composed of, or comprising, active material
- H01M4/64—Carriers or collectors
- H01M4/66—Selection of materials
- H01M4/661—Metal or alloys, e.g. alloy coatings
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/02—Electrodes composed of, or comprising, active material
- H01M4/64—Carriers or collectors
- H01M4/70—Carriers or collectors characterised by shape or form
- H01M4/72—Grids
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
- H01M50/40—Separators; Membranes; Diaphragms; Spacing elements inside cells
- H01M50/409—Separators, membranes or diaphragms characterised by the material
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
- H01M50/40—Separators; Membranes; Diaphragms; Spacing elements inside cells
- H01M50/46—Separators, membranes or diaphragms characterised by their combination with electrodes
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
- H01M50/40—Separators; Membranes; Diaphragms; Spacing elements inside cells
- H01M50/463—Separators, membranes or diaphragms characterised by their shape
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
- H01M8/0204—Non-porous and characterised by the material
- H01M8/0206—Metals or alloys
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
- H01M8/0247—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the form
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/02—Electrodes composed of, or comprising, active material
- H01M4/64—Carriers or collectors
- H01M4/70—Carriers or collectors characterised by shape or form
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/10—Energy storage using batteries
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
- Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
- Y02P70/50—Manufacturing or production processes characterised by the final manufactured product
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- Chemical & Material Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Electrochemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Manufacturing & Machinery (AREA)
- Life Sciences & Earth Sciences (AREA)
- Sustainable Development (AREA)
- Sustainable Energy (AREA)
- Materials Engineering (AREA)
- Hybrid Cells (AREA)
- Cell Electrode Carriers And Collectors (AREA)
- Inert Electrodes (AREA)
- Battery Electrode And Active Subsutance (AREA)
Abstract
Description
Claims (10)
- 交互に接続される複数の素子で構成され、電解液を利用して電気化学発電を行う金属空気電池であって、
a)電解液に耐えられる材料で形成される孔付きのパイプ(2)によって、第1の内部素子(1)が構成され、
b)前記パイプ(2)には、電解液(4)のためのキャビティ(3)が構成され、
c)前記パイプ(2)の外側を囲むように、金属電極(6)又は第1の電極(6)であるコレクタ(5)が配置され、
d)前記コレクタ(5)の外側には、隔膜(7)が密着するように貼り合わせられ、
e)前記隔膜(7)の外側は、第2の電極(9)である空気極(8)で被覆されている
ことを特徴とする金属空気電池。 - 前記パイプ(2)は、炭素又は重合体で製造されることを特徴とする請求項1に記載の金属空気電池。
- 第1の電極(6)として用いられるコレクタ(5)は金属格子で構成され、流体、特に、水を利用して、金属粉末が前記金属格子に塗布されていることを特徴とする請求項1又は2に記載の金属空気電池。
- 中央の孔付きのパイプ(2)の円筒面(11)には、螺旋状に巻かれた導電可能なワイヤが配置されており、前記ワイヤは、銅又は金で構成されていることを特徴とする請求項1〜3のいずれかに記載の金属空気電池。
- 中央の孔付きのパイプ(2)の円筒面(11)には、メッシュで構成され、当該メッシュは、銅又は他の導電材料の箔により製造され、特に、エッチングプロセスによって製造されることを特徴とする請求項1〜3のいずれかに記載の金属空気電池。
- 前記メッシュの厚さが0.01mm〜0.05mmであることを特徴とする請求項5に記載の金属空気電池。
- パイプ(2)、コレクタ(5)、隔膜(7)、及び空気極(8)が、同心的に交互に配置されて密着するように押し付けられることで、複合構造を形成していることを特徴とする請求項1〜6のいずれかに記載の金属空気電池。
- 請求項1〜7のいずれか1項又は複数項に記載の金属空気電池を適用し、電解液を利用して電気化学発電を行う方法であって、
中央の内部パイプに電解液を噴射し、前記電解液を、孔付きのパイプの壁上の開口を通じて内部パイプ外の乾いた金属粉末に分布させて、金属格子に付着された金属粉末を湿らせることを含む方法。 - 前記金属粉末を直接且つ完全に湿らせるように、前記開口の数及び大きさを設定することを含む請求項8に記載の方法。
- 金属電極の金属粉末を、水又は他の適する流体によって濡らさせて塗布することで、コレクタに堆積させることを含む請求項8又は9に記載の方法。
Applications Claiming Priority (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
CN201210125988.5 | 2012-04-25 | ||
CN201210125988.5A CN103378384B (zh) | 2012-04-25 | 2012-04-25 | 空气-金属-电池和电化学发电方法 |
PCT/CN2012/079489 WO2013159467A1 (zh) | 2012-04-25 | 2012-08-01 | 空气-金属-电池和电化学发电方法 |
Related Child Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
JP2016186886A Division JP2017033942A (ja) | 2012-04-25 | 2016-09-26 | 金属空気電池及び電気化学発電方法 |
Publications (1)
Publication Number | Publication Date |
---|---|
JP2015518637A true JP2015518637A (ja) | 2015-07-02 |
Family
ID=49463181
Family Applications (2)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
JP2015507335A Pending JP2015518637A (ja) | 2012-04-25 | 2012-08-01 | 金属空気電池及び電気化学発電方法 |
JP2016186886A Abandoned JP2017033942A (ja) | 2012-04-25 | 2016-09-26 | 金属空気電池及び電気化学発電方法 |
Family Applications After (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
JP2016186886A Abandoned JP2017033942A (ja) | 2012-04-25 | 2016-09-26 | 金属空気電池及び電気化学発電方法 |
Country Status (8)
Country | Link |
---|---|
US (1) | US20150222001A1 (ja) |
EP (1) | EP2843752A4 (ja) |
JP (2) | JP2015518637A (ja) |
KR (1) | KR20150021028A (ja) |
CN (1) | CN103378384B (ja) |
IN (1) | IN2014DN09715A (ja) |
RU (1) | RU2014146773A (ja) |
WO (1) | WO2013159467A1 (ja) |
Cited By (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JP2020503658A (ja) * | 2016-12-22 | 2020-01-30 | ハイドラ、ライト、インターナショナル、リミテッドHydra Light International Ltd | 金属空気燃料電池 |
Families Citing this family (2)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN104934660B (zh) * | 2015-07-14 | 2017-03-01 | 北京航空航天大学 | 一种便捷卷式超薄氧‑金属电池 |
CN108598627B (zh) * | 2018-05-16 | 2020-11-13 | 东北大学秦皇岛分校 | 一种高容量钾-氧气电池 |
Citations (4)
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GB1256419A (en) * | 1969-05-27 | 1971-12-08 | Energy Conversion Ltd | Improvements in and relating to metal/oxygen cells |
US3963519A (en) * | 1968-06-10 | 1976-06-15 | Leesona Corporation | Metal/air cell |
JPS5253933Y2 (ja) * | 1971-12-20 | 1977-12-07 | ||
US20070141440A1 (en) * | 2005-12-21 | 2007-06-21 | General Electric Company | Cylindrical structure fuel cell |
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US3671318A (en) * | 1969-06-12 | 1972-06-20 | Mc Donnell Douglas Corp | Method for producing a water activatable battery |
US4005246A (en) * | 1973-02-20 | 1977-01-25 | Yardney Electric Corporation | Reserve-type cell |
FR2345822A1 (fr) * | 1976-03-22 | 1977-10-21 | Comp Generale Electricite | Generateur electrochimique a circulation forcee |
US4341847A (en) * | 1980-10-14 | 1982-07-27 | Institute Of Gas Technology | Electrochemical zinc-oxygen cell |
US5190833A (en) * | 1990-12-31 | 1993-03-02 | Luz Electric Fuel Israel Ltd. | Electrodes for metal/air batteries and fuel cells and bipolar metal/air batteries incorporating the same |
US5716726A (en) * | 1994-12-22 | 1998-02-10 | Dreisbach Electromotive, Inc. | Electrolyte starved metal-air battery |
US6753108B1 (en) * | 1998-02-24 | 2004-06-22 | Superior Micropowders, Llc | Energy devices and methods for the fabrication of energy devices |
EP2449618A1 (en) * | 2009-06-30 | 2012-05-09 | ReVolt Technology Ltd | Metal-air flow battery |
DE102009035314B4 (de) | 2009-07-30 | 2011-07-21 | Bauer, Bernd, Dr., 71665 | Redoxbatterie mit Flüssigelektrolyt und Verfahren zum Erzeugen elektrischer Energie unter Einsatz einer solchen Batterie |
AU2011346550A1 (en) * | 2010-12-23 | 2013-07-25 | Garal Pty Ltd | Fuel cell and electrolyser structure |
CN201946716U (zh) * | 2011-03-15 | 2011-08-24 | 余建岳 | 一种金属空气电池 |
CN202871940U (zh) * | 2012-04-25 | 2013-04-10 | 新能源动力科技有限公司 | 带有空气电极和金属电极的电池 |
-
2012
- 2012-04-25 CN CN201210125988.5A patent/CN103378384B/zh active Active
- 2012-08-01 RU RU2014146773A patent/RU2014146773A/ru not_active Application Discontinuation
- 2012-08-01 US US14/396,712 patent/US20150222001A1/en not_active Abandoned
- 2012-08-01 WO PCT/CN2012/079489 patent/WO2013159467A1/zh active Application Filing
- 2012-08-01 KR KR20147032882A patent/KR20150021028A/ko active Search and Examination
- 2012-08-01 JP JP2015507335A patent/JP2015518637A/ja active Pending
- 2012-08-01 EP EP12875429.8A patent/EP2843752A4/en not_active Withdrawn
-
2014
- 2014-11-18 IN IN9715DEN2014 patent/IN2014DN09715A/en unknown
-
2016
- 2016-09-26 JP JP2016186886A patent/JP2017033942A/ja not_active Abandoned
Patent Citations (4)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US3963519A (en) * | 1968-06-10 | 1976-06-15 | Leesona Corporation | Metal/air cell |
GB1256419A (en) * | 1969-05-27 | 1971-12-08 | Energy Conversion Ltd | Improvements in and relating to metal/oxygen cells |
JPS5253933Y2 (ja) * | 1971-12-20 | 1977-12-07 | ||
US20070141440A1 (en) * | 2005-12-21 | 2007-06-21 | General Electric Company | Cylindrical structure fuel cell |
Cited By (2)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JP2020503658A (ja) * | 2016-12-22 | 2020-01-30 | ハイドラ、ライト、インターナショナル、リミテッドHydra Light International Ltd | 金属空気燃料電池 |
JP7191039B2 (ja) | 2016-12-22 | 2022-12-16 | ハイドラ、ライト、インターナショナル、リミテッド | 金属空気燃料電池 |
Also Published As
Publication number | Publication date |
---|---|
EP2843752A1 (en) | 2015-03-04 |
RU2014146773A (ru) | 2016-06-10 |
IN2014DN09715A (ja) | 2015-07-31 |
CN103378384B (zh) | 2019-06-28 |
WO2013159467A1 (zh) | 2013-10-31 |
KR20150021028A (ko) | 2015-02-27 |
EP2843752A4 (en) | 2015-12-30 |
US20150222001A1 (en) | 2015-08-06 |
JP2017033942A (ja) | 2017-02-09 |
CN103378384A (zh) | 2013-10-30 |
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