EA201171176A1 - Способ превращения природного газа в ароматические углеводороды с электрохимическим отделением водорода и электрохимическим превращением водорода в воду - Google Patents
Способ превращения природного газа в ароматические углеводороды с электрохимическим отделением водорода и электрохимическим превращением водорода в водуInfo
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- EA201171176A1 EA201171176A1 EA201171176A EA201171176A EA201171176A1 EA 201171176 A1 EA201171176 A1 EA 201171176A1 EA 201171176 A EA201171176 A EA 201171176A EA 201171176 A EA201171176 A EA 201171176A EA 201171176 A1 EA201171176 A1 EA 201171176A1
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- Eurasian Patent Office
- Prior art keywords
- hydrogen
- electrochemical
- turning
- membrane
- aromatic hydrocarbons
- Prior art date
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- 229910052739 hydrogen Inorganic materials 0.000 title abstract 5
- 239000001257 hydrogen Substances 0.000 title abstract 5
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical class [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 title abstract 3
- 150000004945 aromatic hydrocarbons Chemical class 0.000 title abstract 3
- 238000000034 method Methods 0.000 title abstract 2
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 title abstract 2
- VNWKTOKETHGBQD-UHFFFAOYSA-N methane Chemical compound C VNWKTOKETHGBQD-UHFFFAOYSA-N 0.000 title 2
- 239000003345 natural gas Substances 0.000 title 1
- 239000003054 catalyst Substances 0.000 abstract 4
- 239000012528 membrane Substances 0.000 abstract 4
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 abstract 3
- 229910052760 oxygen Inorganic materials 0.000 abstract 3
- 239000001301 oxygen Substances 0.000 abstract 3
- 150000001338 aliphatic hydrocarbons Chemical class 0.000 abstract 2
- 125000004432 carbon atom Chemical group C* 0.000 abstract 2
- 150000002431 hydrogen Chemical class 0.000 abstract 2
- 230000001590 oxidative effect Effects 0.000 abstract 2
- 239000000047 product Substances 0.000 abstract 2
- 239000012466 permeate Substances 0.000 abstract 1
- 238000000926 separation method Methods 0.000 abstract 1
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- C—CHEMISTRY; METALLURGY
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- C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
- C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
- C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
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- B01J29/00—Catalysts comprising molecular sieves
- B01J29/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites
- B01J29/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
- B01J29/60—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the type L, as exemplified by patent document US3216789
- B01J29/64—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the type L, as exemplified by patent document US3216789 containing arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
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- C01B3/501—Separation of hydrogen or hydrogen containing gases from gaseous mixtures, e.g. purification by diffusion
- C01B3/503—Separation of hydrogen or hydrogen containing gases from gaseous mixtures, e.g. purification by diffusion characterised by the membrane
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- C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
- C01B3/50—Separation of hydrogen or hydrogen containing gases from gaseous mixtures, e.g. purification
- C01B3/56—Separation of hydrogen or hydrogen containing gases from gaseous mixtures, e.g. purification by contacting with solids; Regeneration of used solids
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- C07C15/00—Cyclic hydrocarbons containing only six-membered aromatic rings as cyclic parts
- C07C15/02—Monocyclic hydrocarbons
- C07C15/04—Benzene
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- C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
- C07C2/00—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms
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- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
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- C10G50/00—Production of liquid hydrocarbon mixtures from lower carbon number hydrocarbons, e.g. by oligomerisation
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- H01L21/18—Manufacture or treatment of semiconductor devices or of parts thereof the devices having potential barriers, e.g. a PN junction, depletion layer or carrier concentration layer the devices having semiconductor bodies comprising elements of Group IV of the Periodic Table or AIIIBV compounds with or without impurities, e.g. doping materials
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- C01B2203/04—Integrated processes for the production of hydrogen or synthesis gas containing a purification step for the hydrogen or the synthesis gas
- C01B2203/042—Purification by adsorption on solids
- C01B2203/043—Regenerative adsorption process in two or more beds, one for adsorption, the other for regeneration
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- C01B2203/0465—Composition of the impurity
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- C01B2203/12—Feeding the process for making hydrogen or synthesis gas
- C01B2203/1205—Composition of the feed
- C01B2203/1211—Organic compounds or organic mixtures used in the process for making hydrogen or synthesis gas
- C01B2203/1235—Hydrocarbons
- C01B2203/1241—Natural gas or methane
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- C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
- C10G2400/00—Products obtained by processes covered by groups C10G9/00 - C10G69/14
- C10G2400/30—Aromatics
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- Chemical & Material Sciences (AREA)
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Abstract
Изобретение касается способа превращения алифатических углеводородов, имеющих от 1 до 4 атомов углерода в ароматические углеводороды, включающего следующие ступени: а) превращение потока эдукта Е, который содержит по меньшей мере один алифатический углеводород, имеющий от 1 до 4 атомов углерода, в присутствии катализатора при неокислительных условиях в поток продукта Р, содержащий ароматические углеводороды и водород, и b) электрохимическое отделение по меньшей мере части полученного при превращении водорода из потока продукта Р посредством газонепроницаемой мембраноэлектродной сборки, которая содержит по меньшей мере одну селективно проводящую протоны мембрану, а с каждой стороны мембрана содержит по меньшей мере один электродный катализатор, причем со стороны ретентата по меньшей мере часть водорода окисляется на анодном катализаторе до протонов, и протоны после пересечения мембраны со стороны пермеата превращаются на анодном катализаторе с кислородом в воду, причем кислород происходит из содержащего кислород потока О, который приводят в контакт со стороной пермеата мембраны.
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
EP09157396 | 2009-04-06 | ||
PCT/EP2010/054092 WO2010115747A1 (de) | 2009-04-06 | 2010-03-29 | Verfahren zur umsetzung von erdgas zu aromaten mit elektrochemischer abtrennung von wasserstoff und elektrochemischer umsetzung des wasserstoffs zu wasser |
Publications (2)
Publication Number | Publication Date |
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EA201171176A1 true EA201171176A1 (ru) | 2012-05-30 |
EA020178B1 EA020178B1 (ru) | 2014-09-30 |
Family
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Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
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EA201171176A EA020178B1 (ru) | 2009-04-06 | 2010-03-29 | Способ превращения природного газа в ароматические углеводороды с электрохимическим отделением водорода и электрохимическим превращением водорода в воду |
Country Status (9)
Country | Link |
---|---|
US (1) | US8575411B2 (ru) |
EP (1) | EP2417083B1 (ru) |
JP (1) | JP5623503B2 (ru) |
KR (1) | KR20120022756A (ru) |
CN (1) | CN102365252B (ru) |
EA (1) | EA020178B1 (ru) |
ES (1) | ES2530261T3 (ru) |
PL (1) | PL2417083T3 (ru) |
WO (1) | WO2010115747A1 (ru) |
Families Citing this family (12)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
EA020793B9 (ru) | 2009-04-06 | 2015-05-29 | Басф Се | Способ электрохимического отделения водорода из реакционной смеси |
EP2417084B1 (de) * | 2009-04-06 | 2014-11-26 | Basf Se | Verfahren zur umsetzung von erdgas zu aromaten mit elektrochemischer abtrennung von wasserstoff unter erzeugung von elektrischem strom und wasserstoff |
EP2417083B1 (de) | 2009-04-06 | 2014-12-03 | Basf Se | Verfahren zur umsetzung von erdgas zu aromaten mit elektrochemischer abtrennung von wasserstoff und elektrochemischer umsetzung des wasserstoffs zu wasser |
US9061961B2 (en) * | 2009-07-10 | 2015-06-23 | Basf Se | Method for direct amination of hydrocarbons to form amino hydrocarbons with the electrochemical separation of hydrocarbon |
CN102548953B (zh) | 2009-07-10 | 2014-10-08 | 巴斯夫欧洲公司 | 将烃直接胺化成氨基烃并且包括氢气的电化学分离和氢气形成水的电化学反应的方法 |
AR090777A1 (es) * | 2012-04-23 | 2014-12-03 | Shell Int Research | Un proceso para la aromatizacion de una corriente de gas que contiene metano |
AR090778A1 (es) * | 2012-04-23 | 2014-12-03 | Shell Int Research | Un proceso para la aromatizacion de una corriente de gas que contiene metano |
GB201317870D0 (en) * | 2013-10-09 | 2013-11-20 | Protia As | Process for dehydroaromatization of alkanes with in-situ hydrogen removal |
NO2876097T3 (ru) * | 2013-11-20 | 2018-07-28 | ||
WO2015132200A1 (de) * | 2014-03-05 | 2015-09-11 | Basf Se | Verfahren zur kombinierten herstellung von aromatischen kohlenwasserstoffen und aromatischen aminokohlenwasserstoffen |
CN109385643B (zh) * | 2017-08-10 | 2020-06-09 | 中国石油天然气股份有限公司 | 将甲烷转化为脂肪烃的方法、燃料电池及燃料电池的制备方法 |
CN107649114A (zh) * | 2017-09-18 | 2018-02-02 | 南昌大学 | 一种用于甲烷氧化偶联的b位为铈的烧绿石催化剂的制备方法及应用 |
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---|---|---|---|---|
GB1179033A (en) * | 1966-05-31 | 1970-01-28 | Atlantic Richfield Co | Fuel Cell and Method of Operation thereof |
NZ198555A (en) * | 1980-10-11 | 1983-11-30 | British Petroleum Co | Catalytic production of aromatic hydrocarbons |
US7019184B2 (en) * | 2002-01-28 | 2006-03-28 | Conocophillips Company | Non-oxidative conversion of gas to liquids |
JP4697921B2 (ja) * | 2002-02-22 | 2011-06-08 | 電源開発株式会社 | 電力、水素及び芳香族炭化水素の併産システム |
DE102005041140A1 (de) * | 2005-08-30 | 2007-03-01 | Basf Ag | Direktaminierung von Kohlenwasserstoffen |
DE112006003579T5 (de) * | 2005-12-28 | 2009-01-29 | Hitachi, Ltd. | Katalysator mit einer Dehydrierungsfunktion oder Hydrierungsfunktion, Brennstoffzelle unter Verwendung des Katalysators und Wasserstoff-Speicher/Zufuhr-Vorrichtung |
JP5051924B2 (ja) * | 2006-04-21 | 2012-10-17 | エクソンモービル・ケミカル・パテンツ・インク | メタン転換製造プロセス |
KR101676498B1 (ko) | 2008-04-08 | 2016-11-15 | 바스프 에스이 | 귀금속을 함유하지 않는 상응하는 촉매를 재생시키는 것에 의한 메탄 함유 혼합물의 방향족화수소이탈 방법 |
EP2276566A1 (de) | 2008-04-08 | 2011-01-26 | Basf Se | Katalysator zur dehydroaromatisierung von methan und methanhaltigen gemischen |
EA020793B9 (ru) * | 2009-04-06 | 2015-05-29 | Басф Се | Способ электрохимического отделения водорода из реакционной смеси |
EP2417084B1 (de) * | 2009-04-06 | 2014-11-26 | Basf Se | Verfahren zur umsetzung von erdgas zu aromaten mit elektrochemischer abtrennung von wasserstoff unter erzeugung von elektrischem strom und wasserstoff |
EP2417059B1 (de) * | 2009-04-06 | 2014-12-10 | Basf Se | Verfahren zur umsetzung von erdgas zu aromaten mit elektrochemischer abtrennung von wasserstoff |
EP2417083B1 (de) | 2009-04-06 | 2014-12-03 | Basf Se | Verfahren zur umsetzung von erdgas zu aromaten mit elektrochemischer abtrennung von wasserstoff und elektrochemischer umsetzung des wasserstoffs zu wasser |
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2010
- 2010-03-29 EP EP10711236.9A patent/EP2417083B1/de active Active
- 2010-03-29 CN CN201080015474.3A patent/CN102365252B/zh not_active Expired - Fee Related
- 2010-03-29 US US13/256,536 patent/US8575411B2/en active Active
- 2010-03-29 PL PL10711236T patent/PL2417083T3/pl unknown
- 2010-03-29 KR KR1020117023390A patent/KR20120022756A/ko active IP Right Grant
- 2010-03-29 ES ES10711236.9T patent/ES2530261T3/es active Active
- 2010-03-29 JP JP2012503958A patent/JP5623503B2/ja not_active Expired - Fee Related
- 2010-03-29 EA EA201171176A patent/EA020178B1/ru not_active IP Right Cessation
- 2010-03-29 WO PCT/EP2010/054092 patent/WO2010115747A1/de active Application Filing
Also Published As
Publication number | Publication date |
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CN102365252A (zh) | 2012-02-29 |
EP2417083B1 (de) | 2014-12-03 |
KR20120022756A (ko) | 2012-03-12 |
WO2010115747A1 (de) | 2010-10-14 |
US20120004482A1 (en) | 2012-01-05 |
CN102365252B (zh) | 2014-07-16 |
US8575411B2 (en) | 2013-11-05 |
EA020178B1 (ru) | 2014-09-30 |
PL2417083T3 (pl) | 2015-05-29 |
JP2012522820A (ja) | 2012-09-27 |
EP2417083A1 (de) | 2012-02-15 |
ES2530261T3 (es) | 2015-02-27 |
JP5623503B2 (ja) | 2014-11-12 |
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