DK3400098T3 - Understøttet indiumoxidkatalysator og fremgangsmåde til methanolsyntese under anvendelse heraf - Google Patents

Understøttet indiumoxidkatalysator og fremgangsmåde til methanolsyntese under anvendelse heraf Download PDF

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Publication number
DK3400098T3
DK3400098T3 DK16825384.7T DK16825384T DK3400098T3 DK 3400098 T3 DK3400098 T3 DK 3400098T3 DK 16825384 T DK16825384 T DK 16825384T DK 3400098 T3 DK3400098 T3 DK 3400098T3
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Denmark
Prior art keywords
indium oxide
oxide catalyst
procedures used
methanol synthesis
synthesis procedures
Prior art date
Application number
DK16825384.7T
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English (en)
Inventor
Daniel Curulla-Ferre
Oliver Martin
Cecilia Mondelli
Javier Perèz-Ramirez
Antonio J Martin-Fernandez
Charlotte Drouilly
Original Assignee
Total Raffinage Chimie
Eth Zuerich
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Application filed by Total Raffinage Chimie, Eth Zuerich filed Critical Total Raffinage Chimie
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Publication of DK3400098T3 publication Critical patent/DK3400098T3/da

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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/08—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of gallium, indium or thallium
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J21/00—Catalysts comprising the elements, oxides, or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium, or hafnium
    • B01J21/06—Silicon, titanium, zirconium or hafnium; Oxides or hydroxides thereof
    • B01J21/066—Zirconium or hafnium; Oxides or hydroxides thereof
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/002—Mixed oxides other than spinels, e.g. perovskite
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/60—Catalysts, in general, characterised by their form or physical properties characterised by their surface properties or porosity
    • B01J35/61—Surface area
    • B01J35/613—10-100 m2/g
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/60—Catalysts, in general, characterised by their form or physical properties characterised by their surface properties or porosity
    • B01J35/61—Surface area
    • B01J35/615—100-500 m2/g
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/60—Catalysts, in general, characterised by their form or physical properties characterised by their surface properties or porosity
    • B01J35/63—Pore volume
    • B01J35/633—Pore volume less than 0.5 ml/g
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/60—Catalysts, in general, characterised by their form or physical properties characterised by their surface properties or porosity
    • B01J35/63—Pore volume
    • B01J35/635—0.5-1.0 ml/g
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/60—Catalysts, in general, characterised by their form or physical properties characterised by their surface properties or porosity
    • B01J35/63—Pore volume
    • B01J35/638—Pore volume more than 1.0 ml/g
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0201—Impregnation
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0201—Impregnation
    • B01J37/0203—Impregnation the impregnation liquid containing organic compounds
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/03—Precipitation; Co-precipitation
    • B01J37/031—Precipitation
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/08—Heat treatment
    • B01J37/082—Decomposition and pyrolysis
    • B01J37/088—Decomposition of a metal salt
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/16—Reducing
    • B01J37/18—Reducing with gases containing free hydrogen
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C29/00—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring
    • C07C29/15—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by reduction of oxides of carbon exclusively
    • C07C29/151—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by reduction of oxides of carbon exclusively with hydrogen or hydrogen-containing gases
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C29/00—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring
    • C07C29/15—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by reduction of oxides of carbon exclusively
    • C07C29/151—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by reduction of oxides of carbon exclusively with hydrogen or hydrogen-containing gases
    • C07C29/153—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by reduction of oxides of carbon exclusively with hydrogen or hydrogen-containing gases characterised by the catalyst used
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2523/00—Constitutive chemical elements of heterogeneous catalysts
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00—Technologies relating to chemical industry
    • Y02P20/50—Improvements relating to the production of bulk chemicals
    • Y02P20/52—Improvements relating to the production of bulk chemicals using catalysts, e.g. selective catalysts

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Physics & Mathematics (AREA)
  • Thermal Sciences (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Catalysts (AREA)
DK16825384.7T 2016-01-07 2016-12-20 Understøttet indiumoxidkatalysator og fremgangsmåde til methanolsyntese under anvendelse heraf DK3400098T3 (da)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
EP16150481 2016-01-07
PCT/EP2016/081987 WO2017118572A1 (en) 2016-01-07 2016-12-20 Supported indium oxide catalyst and process for methanol synthesis using the same

Publications (1)

Publication Number Publication Date
DK3400098T3 true DK3400098T3 (da) 2020-02-24

Family

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Family Applications (1)

Application Number Title Priority Date Filing Date
DK16825384.7T DK3400098T3 (da) 2016-01-07 2016-12-20 Understøttet indiumoxidkatalysator og fremgangsmåde til methanolsyntese under anvendelse heraf

Country Status (4)

Country Link
US (1) US10668450B2 (da)
EP (1) EP3400098B1 (da)
DK (1) DK3400098T3 (da)
WO (1) WO2017118572A1 (da)

Families Citing this family (13)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2019123278A2 (en) * 2017-12-18 2019-06-27 King Abdullah University Of Science And Technology Indium-based catalysts and pre-catalysts
WO2020049082A1 (en) 2018-09-06 2020-03-12 Total S.A. Noble metal-promoted in2o3 catalyst for the hydrogenation of co2 to methanol
US11986799B2 (en) 2018-12-28 2024-05-21 Dow Global Technologies Lllc Catalysts comprising a zirconia and gallium oxide component for production of C2 to C4 olefins
WO2021239811A1 (en) 2020-05-29 2021-12-02 Total Se Gas to methanol with coproduction of hydrogen
KR20220000433A (ko) * 2020-06-25 2022-01-04 현대자동차주식회사 이산화탄소의 수소화를 통한 메탄올 합성 반응용 촉매 및 이의 제조 방법
CN116457325A (zh) 2020-11-17 2023-07-18 道达尔能源一技术 用于由富co2合成气合成甲醇的工艺
CN112827501A (zh) * 2020-12-31 2021-05-25 大连理工大学 α-MoC负载铟及其改性催化剂的可控合成及在二氧化碳加氢制甲醇反应中的应用
CN115722228A (zh) * 2021-08-31 2023-03-03 赤壁市高质量发展研究院有限公司 一种串联催化剂及低碳醇的高选择性制备方法
CN113996279B (zh) * 2021-11-10 2024-01-09 宁夏大学 In2O3-GO复合催化剂及其制备方法和应用
EP4180386A1 (en) 2021-11-16 2023-05-17 TotalEnergies OneTech Process for the continuous conversion of h2s into h2 and sulphur
CN113929560B (zh) * 2021-11-22 2023-02-24 中国华能集团清洁能源技术研究院有限公司 一种二氧化碳加氢制甲醇的方法及其应用
EP4286046A1 (de) 2022-05-30 2023-12-06 Heraeus Deutschland GmbH & Co. KG Verfahren zur herstellung eines mit edelmetall ausgestatteten indiumoxid-basierten katalysatormaterials und dessen verwendung zur katalytischen hydrierung von co2 zu methanol
CN115646478B (zh) * 2022-10-20 2024-01-26 南开大学 一种ZrO2@In2O3异质结构催化剂的制备方法及在催化CO2加氢制甲醇中的应用

Family Cites Families (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB706599A (en) 1951-03-13 1954-03-31 Basf Ag Improvements in the reaction of carbon monoxide with hydrogen to form alcohols
GB1159035A (en) 1965-08-18 1969-07-23 Ici Ltd Methanol Synthesis.
GB1496379A (en) 1976-10-13 1977-12-30 British Petroleum Co Dehydrocyclodimerising c4 hydrocarbons
US5506273A (en) * 1991-12-06 1996-04-09 Agency Of Industrial Science And Technology Catalyst for hydrogenation and method for hydrogenation therewith
EP1464384B1 (en) 2003-03-20 2005-08-17 Methanol Casale S.A. Horizontal chemical reactor, in particular for methanol synthesis
ES2368027T3 (es) 2008-02-25 2011-11-11 Haldor Topsoe A/S Método y reactor para la preparación de metanol.

Also Published As

Publication number Publication date
US20200061582A1 (en) 2020-02-27
EP3400098A1 (en) 2018-11-14
US10668450B2 (en) 2020-06-02
EP3400098B1 (en) 2019-12-04
WO2017118572A1 (en) 2017-07-13

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