DE60121243D1 - Elektrolytmembran für Polymerelektrolytbrennstoffzelle und Herstellungsverfahren dafür - Google Patents

Elektrolytmembran für Polymerelektrolytbrennstoffzelle und Herstellungsverfahren dafür

Info

Publication number
DE60121243D1
DE60121243D1 DE60121243T DE60121243T DE60121243D1 DE 60121243 D1 DE60121243 D1 DE 60121243D1 DE 60121243 T DE60121243 T DE 60121243T DE 60121243 T DE60121243 T DE 60121243T DE 60121243 D1 DE60121243 D1 DE 60121243D1
Authority
DE
Germany
Prior art keywords
manufacturing
fuel cell
polymer electrolyte
method therefor
electrolyte fuel
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Lifetime
Application number
DE60121243T
Other languages
English (en)
Inventor
Yoshiaki Higuchi
Ichiro Terada
Hiroshi Shimoda
Satoru Hommura
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
AGC Inc
Original Assignee
Asahi Glass Co Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Asahi Glass Co Ltd filed Critical Asahi Glass Co Ltd
Application granted granted Critical
Publication of DE60121243D1 publication Critical patent/DE60121243D1/de
Anticipated expiration legal-status Critical
Expired - Lifetime legal-status Critical Current

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2287—After-treatment
    • C08J5/2293—After-treatment of fluorine-containing membranes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218—Synthetic macromolecular compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2275—Heterogeneous membranes
    • C08J5/2281—Heterogeneous membranes fluorine containing heterogeneous membranes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0289—Means for holding the electrolyte
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1023—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having only carbon, e.g. polyarylenes, polystyrenes or polybutadiene-styrenes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1039—Polymeric electrolyte materials halogenated, e.g. sulfonated polyvinylidene fluorides
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1041—Polymer electrolyte composites, mixtures or blends
    • H01M8/1044—Mixtures of polymers, of which at least one is ionically conductive
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1041—Polymer electrolyte composites, mixtures or blends
    • H01M8/1053—Polymer electrolyte composites, mixtures or blends consisting of layers of polymers with at least one layer being ionically conductive
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1058—Polymeric electrolyte materials characterised by a porous support having no ion-conducting properties
    • H01M8/106—Polymeric electrolyte materials characterised by a porous support having no ion-conducting properties characterised by the chemical composition of the porous support
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1067—Polymeric electrolyte materials characterised by their physical properties, e.g. porosity, ionic conductivity or thickness
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1081—Polymeric electrolyte materials characterised by the manufacturing processes starting from solutions, dispersions or slurries exclusively of polymers
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1086—After-treatment of the membrane other than by polymerisation
    • H01M8/109—After-treatment of the membrane other than by polymerisation thermal other than drying, e.g. sintering
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1086—After-treatment of the membrane other than by polymerisation
    • H01M8/1093—After-treatment of the membrane other than by polymerisation mechanical, e.g. pressing, puncturing
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2327/00—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Derivatives of such polymers
    • C08J2327/02—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Derivatives of such polymers not modified by chemical after-treatment
    • C08J2327/12—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Derivatives of such polymers not modified by chemical after-treatment containing fluorine atoms
    • C08J2327/18—Homopolymers or copolymers of tetrafluoroethylene
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T29/00—Metal working
    • Y10T29/49—Method of mechanical manufacture
    • Y10T29/49002—Electrical device making
    • Y10T29/49108—Electric battery cell making
    • Y10T29/49112—Electric battery cell making including laminating of indefinite length material
DE60121243T 2000-03-31 2001-03-27 Elektrolytmembran für Polymerelektrolytbrennstoffzelle und Herstellungsverfahren dafür Expired - Lifetime DE60121243D1 (de)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2000096596 2000-03-31
JP2000116215 2000-04-18

Publications (1)

Publication Number Publication Date
DE60121243D1 true DE60121243D1 (de) 2006-08-17

Family

ID=26589048

Family Applications (1)

Application Number Title Priority Date Filing Date
DE60121243T Expired - Lifetime DE60121243D1 (de) 2000-03-31 2001-03-27 Elektrolytmembran für Polymerelektrolytbrennstoffzelle und Herstellungsverfahren dafür

Country Status (6)

Country Link
US (1) US6692858B2 (de)
EP (1) EP1139472B1 (de)
KR (1) KR20010095213A (de)
CN (1) CN1223036C (de)
CA (1) CA2342574A1 (de)
DE (1) DE60121243D1 (de)

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JP2001035510A (ja) * 1999-07-21 2001-02-09 Asahi Glass Co Ltd 固体高分子電解質型燃料電池
EP1263074A1 (de) * 2001-05-31 2002-12-04 Asahi Glass Co., Ltd. Ionenaustausch-Polymerdispersion und Verfahren zu seiner Herstellung
EP1263073A1 (de) * 2001-05-31 2002-12-04 Asahi Glass Co., Ltd. Membran-Elektroden-Einheit für Festelektrolyt-Brennstoffzelle und Verfahren zu ihrer Herstellung
GB0210194D0 (en) * 2002-05-03 2002-06-12 Johnson Matthey Plc Composite membrane
WO2004011535A1 (ja) * 2002-07-26 2004-02-05 Asahi Glass Company, Limited 高分子膜、その製造方法及び固体高分子型燃料電池用膜電極接合体
CN1286205C (zh) * 2002-09-30 2006-11-22 旭硝子株式会社 电解质膜的制造方法以及固体高分子型燃料电池的制造方法
US7862921B2 (en) * 2003-03-28 2011-01-04 Sumitomo Chemical Company, Limited Process for continuously producing polymer electrolyte membrane and producing apparatus therefor
WO2004093228A1 (ja) 2003-04-17 2004-10-28 Asahi Glass Company, Limited 固体高分子電解質膜、固体高分子型燃料電池用膜電極接合体及び固体高分子電解質膜の製造方法
CN100426575C (zh) * 2003-05-13 2008-10-15 旭硝子株式会社 固体高分子型燃料电池用电解质聚合物、其制造方法和膜·电极接合体
DE602005025646D1 (de) * 2004-07-12 2011-02-10 Asahi Glass Co Ltd Elektrolytmembran für eine festpolymer-brennstoffzelle, herstellungsverfahren dafür und membranelektrodenbaugruppe für eine festpolmer-brennstoffzelle
ATE431374T1 (de) * 2004-12-22 2009-05-15 Asahi Glass Co Ltd Elektrolytmembran, verfahren zu deren herstellung und membran-elektrodenanordnung für festpolymerbrennstoffzellen
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US20070087245A1 (en) * 2005-10-14 2007-04-19 Fuller Timothy J Multilayer polyelectrolyte membranes for fuel cells
JP5545609B2 (ja) * 2006-08-24 2014-07-09 独立行政法人日本原子力研究開発機構 芳香族高分子膜基材からなる高分子電解質膜、及び、その製造方法
JP2008066023A (ja) * 2006-09-05 2008-03-21 Toyota Motor Corp 電解質膜とその製造方法および該電解質膜を持つ膜電極接合体
US20080124606A1 (en) * 2006-11-10 2008-05-29 Jun Lin Stretched proton exchange membrane
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US8017257B2 (en) * 2007-01-26 2011-09-13 Asahi Glass Company, Limited Polymer, polymer electrolyte membrane for polymer electrolyte fuel cell, and membrane/electrode assembly
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JP2009064688A (ja) * 2007-09-07 2009-03-26 Toyota Auto Body Co Ltd 燃料電池用セパレータおよび同セパレータを構成するコレクタの成形方法
US8338052B2 (en) 2007-11-26 2012-12-25 Toyota Jidosha Kabushiki Kaisha Method for manufacturing a membrane-electrode assembly, with folding process
JP4600500B2 (ja) * 2007-11-26 2010-12-15 トヨタ自動車株式会社 燃料電池の製造方法
CN101320818B (zh) * 2008-07-15 2010-06-09 山东东岳神舟新材料有限公司 一种纤维增强多层含氟离子交换膜
CN101319051B (zh) * 2008-07-15 2010-12-29 山东东岳神舟新材料有限公司 一种纤维增强无机物掺杂多层含氟离子交换膜
CN101348574B (zh) * 2008-07-22 2011-06-08 山东东岳神舟新材料有限公司 一种纤维增强无机物掺杂交联含氟离子交换膜
CN101704915B (zh) * 2009-11-13 2011-05-04 山东东岳高分子材料有限公司 一种离子聚合物及含有该聚合物的离子交换膜材料
CN101773788B (zh) * 2009-12-07 2010-12-29 山东东岳高分子材料有限公司 带牺牲纤维网布增强的含氟离子交换膜
CN101728551B (zh) * 2009-12-10 2011-06-08 山东东岳神舟新材料有限公司 一种增强多层含氟离子交换膜
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CA2802948C (en) 2010-06-18 2018-08-07 Shandong Huaxia Shenzhou New Material Co., Ltd Fluorine-containing ionomer composite material with ion exchange function, preparation method and use thereof
JP5748844B2 (ja) 2010-06-18 2015-07-15 シャンドン・フアシャ・シェンゾウ・ニュー・マテリアル・カンパニー・リミテッド イオン交換機能を有するフッ素含有イオノマー複合体、その調製方法及び使用
JP5693125B2 (ja) * 2010-10-05 2015-04-01 日本ゴア株式会社 固体高分子形燃料電池
PT2735047T (pt) * 2011-09-15 2018-06-14 Siemens Ag Processo para a produção a seco de uma unidade de elétrodos de membrana, elétrodos de membrana assim como disposição de laminação
US9123932B2 (en) * 2011-11-17 2015-09-01 GM Global Technology Operations LLC Nanofiber supported catalysts as membrane additives for improved fuel cell durability
CN104134812B (zh) * 2013-05-02 2017-02-08 山东东岳高分子材料有限公司 一种纤维网增强的聚合物电解质膜及其制备方法
US20170028361A1 (en) * 2015-07-31 2017-02-02 Pall Corporation Ptfe/pfsa blended membrane
US20170028359A1 (en) * 2015-07-31 2017-02-02 Pall Corporation Coated ptfe membrane
TWI791612B (zh) * 2017-09-12 2023-02-11 美商希爾格得有限公司 用於浸漬之基底膜、經改良之浸漬產物，及其相關方法
CN108285541B (zh) * 2017-12-29 2021-06-29 山东东岳未来氢能材料股份有限公司 纳米纤维增强的含氟离子交换膜及其制备方法
CN108346813A (zh) * 2018-02-11 2018-07-31 温州市赢创新材料技术有限公司 一种纤维接枝质子交换膜及其制备方法
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CN109346751A (zh) * 2018-09-10 2019-02-15 中原工学院 一种燃料电池用复合质子交换膜的制备方法

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JPS58201823A (ja) * 1982-05-18 1983-11-24 Asahi Glass Co Ltd イオン交換膜の製造方法
JP3342726B2 (ja) * 1993-01-29 2002-11-11 旭硝子株式会社 固体高分子電解質型の燃料電池及びその製造方法
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JP2001035508A (ja) * 1999-07-19 2001-02-09 Asahi Glass Co Ltd 固体高分子電解質型燃料電池

Also Published As

Publication number Publication date
CA2342574A1 (en) 2001-09-30
KR20010095213A (ko) 2001-11-03
US6692858B2 (en) 2004-02-17
EP1139472A1 (de) 2001-10-04
EP1139472B1 (de) 2006-07-05
CN1319908A (zh) 2001-10-31
CN1223036C (zh) 2005-10-12
US20010026883A1 (en) 2001-10-04

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