CH247123A - Process for the preparation of a salt of N- (4-amino-benzenesulfone) -N'-benzyl urea. - Google Patents

Process for the preparation of a salt of N- (4-amino-benzenesulfone) -N'-benzyl urea.

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Publication number
CH247123A
CH247123A CH247123DA CH247123A CH 247123 A CH247123 A CH 247123A CH 247123D A CH247123D A CH 247123DA CH 247123 A CH247123 A CH 247123A
Authority
CH
Switzerland
Prior art keywords
amino
benzenesulfone
salt
preparation
benzyl urea
Prior art date
Application number
Other languages
German (de)
Inventor
Ag J R Geigy
Original Assignee
Ag J R Geigy
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Ag J R Geigy filed Critical Ag J R Geigy
Publication of CH247123A publication Critical patent/CH247123A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C311/00Amides of sulfonic acids, i.e. compounds having singly-bound oxygen atoms of sulfo groups replaced by nitrogen atoms, not being part of nitro or nitroso groups
    • C07C311/50Compounds containing any of the groups, X being a hetero atom, Y being any atom
    • C07C311/52Y being a hetero atom
    • C07C311/54Y being a hetero atom either X or Y, but not both, being nitrogen atoms, e.g. N-sulfonylurea

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Pharmaceuticals Containing Other Organic And Inorganic Compounds (AREA)
  • Acyclic And Carbocyclic Compounds In Medicinal Compositions (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

  

      Verfahren        zur        Herstellung        eines    Salzes des     N-(4-Ämino-benzolsulfon)-N'-benzyl-harnstoffes.            Lösungen    von Salzen der     4-Amino-benzol-          sulfonamide    werden,     sofern    sie nicht stark  alkalisch     reagieren,    vielfach für Injektionen  verwendet. Für diesen Zweck     ist    es jedoch  von Wichtigkeit, dass die     Lösungen    möglichst  neutral reagieren, da     sonst    die Gefahr der       Nekrosebildung    besteht.

   Es     wurde    nun ge  funden, dass die Salze des     N-(4-Aminobenzol-          sulfon)-N'-benzylharnstoffes    viel weniger  alkalisch reagieren als die vergleichbaren  Salze bekannter     p-Aminobenzolsulfonamide;

       beispielsweise zeigt das     Natriumsalz    des     N-          (4-Aminobenzolsulfon)        -N'-benzylharnstoffes     in 5%iger     wässriger    Lösung ein p$ von<B>8,5</B>     2,          während    die     Natriumsalze    des     2-(p-Amino-          benzolsulfamido)-pyridins,    des     p-Aminoben-:

            zolsuHamino-2-thiazols    und des     2-Sulfanil-          amido-pyrimidins        pH-Werte    von 11,2, 10,0       bezw.    9,6-9,7 (je in 2     %iger        Lösung)    auf  weisen.  



  Als Basen kommen für die Herstellung  der Salze des     N-(4-Aminobenzolsulfon)-N'-          benzylharnstGffes    Alkalien in Frage, z. B.  Natronlauge,     Alkalicarbonate        und        -bicarbo-          nate,        Magnesiumhydrogyd,        Erdalkalihy-          drogyde    oder auch organische Basen wie  z. B.     Diäthylamin,        Morpholin,        Aminoäthanol,          Ä.thylendiamin    usw.  



  Gegenstand vorliegenden Patentes ist ein  Verfahren zur Herstellung     eines    Salzes des  N - (4.-     Amino-benzolsulfon)    - N'-     benzylharn.-          stoffes.    Das Verfahren ist dadurch gekenn-    zeichnet, dass man -1     Mol        einer    Verbindung  der Formel  
EMI0001.0056     
    mit 1     Mol    einer     Natriumverbindung    der For  mel     Na-Y,        worin    X und Y bei der     Reaktion     sich     abspaltende    Reste bedeuten,.

       umsetzt.     Die erhaltene neue Verbindung, das Natrium  salz des     N-(4-Amino-benzolsulfon)-N'-ben-          zylharnstoffes,        kristallisiert    in feinen Pris  men und     schmilzt    bei 248 . Sie soll therapeu  tische     Verwendung    finden.  



       Beispiel:     101 Teile     N-(4-Amino-benzolsulfon)-N'-          benzylharnstoff    werden     in    333     Volumteilen     wässriger,     reiner        n-Natronlauge    gelöst, fil  triert und im Vakuum auf etwa 200     Teile     eingedampft. Die     konzentrierte    warme Lö  sung     wird        sofort    mit 2000 Teilen Alkohol  versetzt. Nach einigem Stehen kristallisiert  das     Natriumsalz    in     feinen    Prismen aus, die  bei 248  schmelzen.



      Process for the preparation of a salt of N- (4-aminobenzenesulfone) -N'-benzylurea. Solutions of salts of the 4-amino-benzenesulfonamides are often used for injections, provided they do not have a strongly alkaline reaction. For this purpose, however, it is important that the solutions react as neutrally as possible, otherwise there is a risk of necrosis.

   It has now been found that the salts of N- (4-aminobenzenesulfone) -N'-benzylurea have a much less alkaline reaction than the comparable salts of known p-aminobenzenesulfonamides;

       For example, the sodium salt of N- (4-aminobenzene sulfone) -N'-benzylurea in 5% aqueous solution has a p $ of <B> 8.5 </B> 2, while the sodium salts of 2- (p-amino- benzenesulfamido) pyridine, des p-aminoben-:

            zolsuHamino-2-thiazole and des 2-sulfanilamido-pyrimidine pH values of 11.2, 10.0, respectively. 9.6-9.7 (each in a 2% solution).



  Bases that can be used for the preparation of the salts of N- (4-aminobenzene sulfone) -N'-benzyluric acid are alkalis, e.g. B. caustic soda, alkali carbonates and bicarbonates, magnesium hydrogen, alkaline earth metal or organic bases such. B. diethylamine, morpholine, aminoethanol, ethylene diamine etc.



  The present patent relates to a process for the preparation of a salt of N - (4.-Amino-benzenesulfone) - N'-benzylur.- substance. The process is characterized in that -1 mol of a compound of the formula
EMI0001.0056
    with 1 mol of a sodium compound of the formula Na-Y, in which X and Y are radicals which are split off during the reaction.

       implements. The new compound obtained, the sodium salt of N- (4-amino-benzenesulfone) -N'-benzylurea, crystallizes in fine prisms and melts at 248. It should find therapeutic use.



       Example: 101 parts of N- (4-amino-benzenesulfone) -N'-benzylurea are dissolved in 333 parts by volume of pure aqueous n-sodium hydroxide solution, filtered and evaporated to about 200 parts in vacuo. The concentrated warm solution is immediately mixed with 2000 parts of alcohol. After standing for a while, the sodium salt crystallizes out in fine prisms which melt at 248.

 

Claims (1)

PATENTANSPRUCH: Verfahren zur Herstellung eines Salzes des N - (4-Amino-benzolsulfon) - N'-benzyl- harnstoffes, dadurch gekennzeichnet, dass man 1 Mol einer Verbindung der Formel EMI0001.0088 mit 1 Mol einer Natriumverbindung der For mel Na-Y, worin X und Y bei der Reaktion sieh abspaltende Reste bedeuten, umsetzt. Die erhaltene neue Verbindung, das Natrium salz des N-(4-Amino-benzolsulfon) Claim: Process for the preparation of a salt of N - (4-amino-benzenesulfone) - N'-benzyl urea, characterized in that 1 mol of a compound of the formula EMI0001.0088 with 1 mol of a sodium compound of the formula Na-Y, in which X and Y in the reaction are radicals which are split off. The new compound obtained, the sodium salt of N- (4-amino-benzenesulfone) -N'=ben- zylharnstof f es, kristallisiert in feinen Pris men und schmilzt bei 248 . -N '= benzylurea f es, crystallizes in fine prisms and melts at 248.
CH247123D 1944-12-28 1944-12-28 Process for the preparation of a salt of N- (4-amino-benzenesulfone) -N'-benzyl urea. CH247123A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CH247123T 1944-12-28

Publications (1)

Publication Number Publication Date
CH247123A true CH247123A (en) 1947-02-15

Family

ID=4466008

Family Applications (1)

Application Number Title Priority Date Filing Date
CH247123D CH247123A (en) 1944-12-28 1944-12-28 Process for the preparation of a salt of N- (4-amino-benzenesulfone) -N'-benzyl urea.

Country Status (1)

Country Link
CH (1) CH247123A (en)

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