KR950703673A - 폴리프로필렌 연질 섬유용 중합체 조성물(polymeric composition for soft polypropylene fibers) - Google Patents
폴리프로필렌 연질 섬유용 중합체 조성물(polymeric composition for soft polypropylene fibers) Download PDFInfo
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- KR950703673A KR950703673A KR1019950701345A KR19950701345A KR950703673A KR 950703673 A KR950703673 A KR 950703673A KR 1019950701345 A KR1019950701345 A KR 1019950701345A KR 19950701345 A KR19950701345 A KR 19950701345A KR 950703673 A KR950703673 A KR 950703673A
- Authority
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- South Korea
- Prior art keywords
- group
- polyester
- filament
- ester forming
- forming functional
- Prior art date
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- 239000000835 fiber Substances 0.000 title claims abstract 12
- 239000000203 mixture Substances 0.000 title claims 2
- -1 POLYPROPYLENE Polymers 0.000 title 1
- 239000004743 Polypropylene Substances 0.000 title 1
- 229920001155 polypropylene Polymers 0.000 title 1
- 229920000728 polyester Polymers 0.000 claims abstract 9
- 150000002148 esters Chemical class 0.000 claims abstract 6
- 125000000524 functional group Chemical group 0.000 claims abstract 6
- 125000000217 alkyl group Chemical group 0.000 claims abstract 3
- 125000004435 hydrogen atom Chemical group [H]* 0.000 claims abstract 3
- 239000002131 composite material Substances 0.000 claims abstract 2
- 150000001875 compounds Chemical class 0.000 claims 2
- 238000007334 copolymerization reaction Methods 0.000 claims 2
- 229920000642 polymer Polymers 0.000 claims 1
- 206010011732 Cyst Diseases 0.000 abstract 1
- 208000031513 cyst Diseases 0.000 abstract 1
- 238000004043 dyeing Methods 0.000 abstract 1
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 abstract 1
Classifications
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B27/00—Layered products comprising a layer of synthetic resin
- B32B27/12—Layered products comprising a layer of synthetic resin next to a fibrous or filamentary layer
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B27/00—Layered products comprising a layer of synthetic resin
- B32B27/32—Layered products comprising a layer of synthetic resin comprising polyolefins
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B5/00—Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts
- B32B5/02—Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts characterised by structural features of a fibrous or filamentary layer
- B32B5/022—Non-woven fabric
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
- C08L23/02—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
- C08L23/10—Homopolymers or copolymers of propene
- C08L23/12—Polypropene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
- C08L23/02—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
- C08L23/16—Elastomeric ethene-propene or ethene-propene-diene copolymers, e.g. EPR and EPDM rubbers
-
- D—TEXTILES; PAPER
- D01—NATURAL OR MAN-MADE THREADS OR FIBRES; SPINNING
- D01F—CHEMICAL FEATURES IN THE MANUFACTURE OF ARTIFICIAL FILAMENTS, THREADS, FIBRES, BRISTLES OR RIBBONS; APPARATUS SPECIALLY ADAPTED FOR THE MANUFACTURE OF CARBON FILAMENTS
- D01F6/00—Monocomponent artificial filaments or the like of synthetic polymers; Manufacture thereof
- D01F6/44—Monocomponent artificial filaments or the like of synthetic polymers; Manufacture thereof from mixtures of polymers obtained by reactions only involving carbon-to-carbon unsaturated bonds as major constituent with other polymers or low-molecular-weight compounds
- D01F6/46—Monocomponent artificial filaments or the like of synthetic polymers; Manufacture thereof from mixtures of polymers obtained by reactions only involving carbon-to-carbon unsaturated bonds as major constituent with other polymers or low-molecular-weight compounds of polyolefins
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B2262/00—Composition or structural features of fibres which form a fibrous or filamentary layer or are present as additives
- B32B2262/02—Synthetic macromolecular fibres
- B32B2262/0253—Polyolefin fibres
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B2307/00—Properties of the layers or laminate
- B32B2307/70—Other properties
- B32B2307/718—Weight, e.g. weight per square meter
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2203/00—Applications
- C08L2203/12—Applications used for fibers
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2205/00—Polymer mixtures characterised by other features
- C08L2205/02—Polymer mixtures characterised by other features containing two or more polymers of the same C08L -group
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2205/00—Polymer mixtures characterised by other features
- C08L2205/03—Polymer mixtures characterised by other features containing three or more polymers in a blend
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2205/00—Polymer mixtures characterised by other features
- C08L2205/03—Polymer mixtures characterised by other features containing three or more polymers in a blend
- C08L2205/035—Polymer mixtures characterised by other features containing three or more polymers in a blend containing four or more polymers in a blend
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2207/00—Properties characterising the ingredient of the composition
- C08L2207/02—Heterophasic composition
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
- C08L23/02—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
- C08L23/04—Homopolymers or copolymers of ethene
- C08L23/08—Copolymers of ethene
- C08L23/0807—Copolymers of ethene with unsaturated hydrocarbons only containing more than three carbon atoms
- C08L23/0815—Copolymers of ethene with aliphatic 1-olefins
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
- C08L23/02—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
- C08L23/10—Homopolymers or copolymers of propene
- C08L23/14—Copolymers of propene
- C08L23/142—Copolymers of propene at least partially crystalline copolymers of propene with other olefins
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2314/00—Polymer mixtures characterised by way of preparation
- C08L2314/02—Ziegler natta catalyst
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
- Y10T442/00—Fabric [woven, knitted, or nonwoven textile or cloth, etc.]
- Y10T442/60—Nonwoven fabric [i.e., nonwoven strand or fiber material]
- Y10T442/637—Including strand or fiber material which is a monofilament composed of two or more polymeric materials in physically distinct relationship [e.g., sheath-core, side-by-side, islands-in-sea, fibrils-in-matrix, etc.] or composed of physical blend of chemically different polymeric materials or a physical blend of a polymeric material and a filler material
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
- Y10T442/00—Fabric [woven, knitted, or nonwoven textile or cloth, etc.]
- Y10T442/60—Nonwoven fabric [i.e., nonwoven strand or fiber material]
- Y10T442/674—Nonwoven fabric with a preformed polymeric film or sheet
- Y10T442/678—Olefin polymer or copolymer sheet or film [e.g., polypropylene, polyethylene, ethylene-butylene copolymer, etc.]
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- Chemical & Material Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Engineering & Computer Science (AREA)
- Textile Engineering (AREA)
- Health & Medical Sciences (AREA)
- Polymers & Plastics (AREA)
- Organic Chemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Artificial Filaments (AREA)
- Compositions Of Macromolecular Compounds (AREA)
- Nonwoven Fabrics (AREA)
- Multicomponent Fibers (AREA)
- Materials For Medical Uses (AREA)
Abstract
본 발명은 일반식(1)의 공단량체 성분을 2 내지 20몰% 함유하는 폴리에스테르로부터 제조한 섬유; 상기 섬유가 사용된 사, 즉 수측율이 상이한 필라멘트로 구성된 혼방사 및 혼방스테이플사; 및 한 성붐으로서 사이 폴리에스테르를 함유하는 복합섬유에 관한 것이다. 본 발명의 섬유는 복굴절도가 낮고 염색성 및 심색 효과도 우수하다. 추가로 연신조건에 따라 고수축율 뿐만 아니라 고수축 응력 및 매우 우수한 광결뢰도를 갖기 때문에 기존의 고수축성 섬유의 대용품으로서 유용하다.
상기식에서, R1내지 R10은 각각 에스테르 형성 작용성 그룹, 수소원자 및 알킬 그룹으로 이루어진 그룹중에서 선택된 그룹을 나타내며, 단 R1내지 R10중의 1개 또는 2개의 에스테르 형성 작용성 그룹이고, x는 0 또는 1이며, y는 조건 1 ≤ x+y ≤3을 충족시키는 정수이다.
Description
본 내용은 요부공개 건이므로 전문내용을 수록하지 않았음
Claims (5)
- 다음 일반식(1)의 화합물을 공중합 성분으로서 2 내지 20몰% 함유하는 폴리에스테르를 포함하는 폴리에스테르 섬유.상기식에서, R1내지 R10은 각각 에스테르 형성 작용성 그룹, 수소원자 및 알킬 그룹으로 이루어진 그룹중에서 선택된 그룹을 나타내며, 단 R1내지 R10중의 1개 또는 2개의 에스테르 형성 작용성 그룹이고, x는 0 또는 1이며, y는 조건 1 ≤ x+y ≤3을 충족시키는 정수이다.
- 제1항에 따르는 폴리에스테르 필라멘트로 이루어진 필라멘트 그룹과 기타의 필라멘트로 이루어진 그룹을 포함하는 수축성이 상이한 필라멘트들로 이루어지며, 98℃에서의 습열 수축율이 10 내지 55% 이고, 폴리에스테르 필라멘트 그룹과 기타의 필라멘트 그룹 사이의 필라멘트 길이의 차이가 4% 이상인 이수축성 혼합물 필라멘트사.
- 쉬쓰 사에 의해 피복된, 제1항에 따르는 폴리에스테르 필라멘트를 포함하는 코어 필라멘트사를 포함하는 쉬쓰-코어(sheath-core)가공사.
- 제1항에 따르는 폴리에스테르 섬유와 기타의 합성 섬유 또는 천연섬유를 포함하는 스테이플 섬유를 포함하는 혼방사.
- 다음 일반식(1)의 화합물을 공중합 성분으로서 2 내지 20몰% 함유하는 폴리에스테르와 기타의 섬유 형성 중합체를 포함하는 복합섬유.상기식에서, R1내지 R10은 각각 에스테르 형성 작용성 그룹, 수소원자 및 알킬 그룹으로 이루어진 그룹중에서 선택된 그룹을 나타내며, 단 R1내지 R10중의 1개 또는 2개의 에스테르 형성 작용성 그룹이고, x는 0 또는 1이며, y는 조건 1 ≤ x+y ≤3을 충족시키는 정수이다.※ 참고사항 : 최초출원 내용에 의하여 공개하는 것임.
Applications Claiming Priority (4)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
ITM192A002324 | 1992-10-09 | ||
ITMI92A0002324 | 1992-10-09 | ||
ITMI922324A IT1256157B (it) | 1992-10-09 | 1992-10-09 | Composizione polimerica per fibre polipropileniche soffici, fibre ottenute da tale composizione e manufatti derivati da dette fibre |
PCT/EP1993/002744 WO1994009193A1 (en) | 1992-10-09 | 1993-10-07 | Polymeric composition for soft polypropylene fibers |
Publications (2)
Publication Number | Publication Date |
---|---|
KR950703673A true KR950703673A (ko) | 1995-09-20 |
KR100292172B1 KR100292172B1 (ko) | 2001-10-24 |
Family
ID=11364083
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
KR1019950701345A KR100292172B1 (ko) | 1992-10-09 | 1993-10-07 | 연질폴리프로필렌섬유 |
Country Status (11)
Country | Link |
---|---|
US (2) | US5514751A (ko) |
EP (1) | EP0663965B2 (ko) |
JP (1) | JP3347328B2 (ko) |
KR (1) | KR100292172B1 (ko) |
AT (1) | ATE156872T1 (ko) |
AU (1) | AU682012B2 (ko) |
DE (1) | DE69313124T3 (ko) |
DK (1) | DK0663965T4 (ko) |
ES (1) | ES2107053T5 (ko) |
IT (1) | IT1256157B (ko) |
WO (1) | WO1994009193A1 (ko) |
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IT1264841B1 (it) * | 1993-06-17 | 1996-10-17 | Himont Inc | Fibre adatte per la produzione di tessuti non tessuti con migliorate caratteristiche di tenacita' e sofficita' |
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US5942452A (en) * | 1996-05-03 | 1999-08-24 | Amoco Corporation | Antiskid fabric |
EP0878567B1 (de) * | 1997-05-14 | 2004-09-29 | Borealis GmbH | Polyolefinfasern und Polyolefingarne und daraus hergestellte textile Flächengebilde |
IT1299169B1 (it) * | 1998-04-29 | 2000-02-29 | Meraklon S R L | Fibra in fiocco da miscele di resine polipropileniche con polietilene per la produzione di tessuto-non-tessuto termosaldato. |
EP1126053A1 (en) * | 2000-02-18 | 2001-08-22 | Atofina Research S.A. | Polypropylene fibres |
DE10009248C2 (de) * | 2000-02-28 | 2002-06-27 | Freudenberg Carl Kg | Medizinisches Verbandsmaterial |
US20040110443A1 (en) * | 2002-12-05 | 2004-06-10 | Pelham Matthew C. | Abrasive webs and methods of making the same |
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WO2007071496A1 (en) * | 2005-12-20 | 2007-06-28 | Basell Poliolefine Italia S.R.L. | Soft non-woven fabrics |
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WO2014114638A1 (en) * | 2013-01-22 | 2014-07-31 | Total Research & Technology Feluy | High-tenacity drawn fibers of a polypropylene composition with improved elongational properties and nonwovens |
US20170001412A1 (en) * | 2015-06-30 | 2017-01-05 | The Procter & Gamble Company | Fibrous Structures and Method for Making Same |
EP3649192B1 (en) | 2017-07-07 | 2023-11-22 | Basell Poliolefine Italia S.r.l. | Polyolefin compositon for fibers |
WO2021110762A1 (en) * | 2019-12-03 | 2021-06-10 | Basell Polyolefine Gmbh | Polyethylene composition for filaments or fibers |
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JP2682130B2 (ja) † | 1989-04-25 | 1997-11-26 | 三井石油化学工業株式会社 | 柔軟な長繊維不織布 |
US5108827A (en) † | 1989-04-28 | 1992-04-28 | Fiberweb North America, Inc. | Strong nonwoven fabrics from engineered multiconstituent fibers |
IT1230133B (it) * | 1989-04-28 | 1991-10-14 | Himont Inc | Composizioni polipropileniche plasto-elastiche |
IT1240417B (it) * | 1990-02-28 | 1993-12-15 | Himont Inc | Procedimento per la produzione di film e corpi laminari polipropilenici e prodotti cosi' ottenuti |
GB2244058B (en) * | 1990-05-01 | 1993-03-24 | Courtaulds Films & Packaging | Packaging materials |
IT1243188B (it) * | 1990-08-01 | 1994-05-24 | Himont Inc | Composizioni poliolefiniche elastoplastiche |
US5212246A (en) * | 1990-09-28 | 1993-05-18 | Himont Incorporated | Olefin polymer films |
IT1254202B (it) * | 1992-02-06 | 1995-09-14 | Himont Inc | Manufatti accoppiati comprendenti un tessuto-non-tessuto e un film in materiali poliolefinici e procedimento per la loro preparazione |
-
1992
- 1992-10-09 IT ITMI922324A patent/IT1256157B/it active IP Right Grant
-
1993
- 1993-10-07 ES ES93922525T patent/ES2107053T5/es not_active Expired - Lifetime
- 1993-10-07 JP JP50958294A patent/JP3347328B2/ja not_active Expired - Fee Related
- 1993-10-07 DE DE69313124T patent/DE69313124T3/de not_active Expired - Fee Related
- 1993-10-07 EP EP93922525A patent/EP0663965B2/en not_active Expired - Lifetime
- 1993-10-07 AU AU51495/93A patent/AU682012B2/en not_active Ceased
- 1993-10-07 KR KR1019950701345A patent/KR100292172B1/ko not_active IP Right Cessation
- 1993-10-07 DK DK93922525T patent/DK0663965T4/da active
- 1993-10-07 WO PCT/EP1993/002744 patent/WO1994009193A1/en active IP Right Grant
- 1993-10-07 AT AT93922525T patent/ATE156872T1/de not_active IP Right Cessation
- 1993-10-08 US US08/133,968 patent/US5514751A/en not_active Expired - Fee Related
-
1996
- 1996-03-06 US US08/611,799 patent/US5585172A/en not_active Expired - Fee Related
Also Published As
Publication number | Publication date |
---|---|
AU682012B2 (en) | 1997-09-18 |
DK0663965T3 (da) | 1997-09-01 |
EP0663965B1 (en) | 1997-08-13 |
ES2107053T5 (es) | 2000-12-16 |
KR100292172B1 (ko) | 2001-10-24 |
DE69313124D1 (de) | 1997-09-18 |
EP0663965B2 (en) | 2000-07-12 |
ES2107053T3 (es) | 1997-11-16 |
ITMI922324A1 (it) | 1994-04-09 |
DK0663965T4 (da) | 2000-11-13 |
DE69313124T3 (de) | 2001-07-12 |
AU5149593A (en) | 1994-05-09 |
US5514751A (en) | 1996-05-07 |
JP3347328B2 (ja) | 2002-11-20 |
ITMI922324A0 (it) | 1992-10-09 |
WO1994009193A1 (en) | 1994-04-28 |
US5585172A (en) | 1996-12-17 |
EP0663965A1 (en) | 1995-07-26 |
IT1256157B (it) | 1995-11-29 |
JPH08502311A (ja) | 1996-03-12 |
ATE156872T1 (de) | 1997-08-15 |
DE69313124T2 (de) | 1998-02-26 |
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