KR101539282B1 - Myrrha oil and manufacturing method therof - Google Patents

Abstract

A manufacturing method of myrrh oil using a myrrh resin is disclosed. Provided is myrrh oil, as a manufacturing method of myrrh oil, which can be used in various fields such as a food or a medicine, and a composition for beauty treatment with high stability and little change in configuration or precipitation phenomenon of myrrh oil, and which comprises: a drying and crushing step of cooling the dried myrrh resin at -15 to -20°C; an aging step for aging the myrrh resin powder; a second crushing step for drying the aged myrrh resin powder and crushing the same again; an oil mixing step for mixing the crushed myrrh resin powder with liquid oil; and a stirring step for evenly mixing the myrrh resin powder and oil to make myrrh oil.

Description

FIELD OF THE INVENTION [0001] The present invention relates to a myrrh oil,

The present invention relates to a method for producing a myrrh oil using a myrrh resin, and more particularly, to a method for producing a myrrh oil which can be used in various fields such as foods, medicines and cosmetic compositions, .

Most of the myrrh is composed of sesquiterpene. The main components of sesquiterpene are the Furanossequat pen from Utezman and Guanian. Sesquiterpenes are chain or cyclic hydrocarbons and derivatives thereof composed of 15 carbon atoms in terpenes contained in plant essential oils. The hydrocarbons of sesquiterpene are, for example, beta and delta-alpha-, beta -bromobenzene, beta-califolene, hufuran and elephant.

Some of the pnanosese quetiepenes are characterized by pharmacological myrrhics and are classified as substances with potent analgesic effects and there are a number of research papers on myrrh.

On the other hand, in spite of its useful antimicrobial activity, the myrrh resin has not been dissolved or dispersed in water itself, and thus it has not been easy to use it, and thus it has been limitedly commercialized (the related product using the myrrh-medicinal efficacy is' guggulsterone '), which is a lump with a diameter of 1 to 3 cm or more solidified by a solid body.

Until now, the use of myrrh had been processed into oil and added to toothpaste or soap, or was also used as a hot-dip method in one room. It is also used as an additive for ointment for surgical treatment or as an aroma oil.

For example, in relation to the use of myrrh, Korea Patent Publication No. 10-2011-0108654 discloses a health food using olive tree sap and a method for producing the same, wherein the myrrh ingredient is obtained from olive tree sap, . Korean Patent Laid-Open No. 10-2010-0071606 discloses a composition for skin whitening comprising a herbal extract, which is an example of a skin whitening composition containing myrrh as an active ingredient. In addition, the composition for oral use (Korean Patent Application No. 10-2008-0086780) containing the natural extract and the method of extracting fragrance, oil and concentrated liquid from myrrh (Korean Patent Application No. 10-2011-0142311) Have been proposed.

However, the myrrh oil containing the conventional myrrh resin or various myrrh extracts has a low amount of the myrrh component dissolved in the oil, so that it is difficult to expect the effect of the myrrh. And the inclusion of a large amount of oil caused the impurities contained in the myrrh.

Patent Document 1. Korean Patent Publication No. 10-2011-0108654 Patent Document 2: Korean Patent Publication No. 10-2010-0071606

It is an object of the present invention to provide a method for producing a high-purity myrrh oil which comprises myrrh as a main component and an oil as a subcomponent.

Another object of the present invention is to provide a myrrh oil which has less deterioration of components such as sedimentation, color deterioration and the like and which is stable in use over time.

The present invention also relates to the production of myrrh oil which can be used for a wide range of purposes in medical and household goods which are closely related to real life such as food and medicine, surgical medicine field, cosmetics field.

According to another aspect of the present invention, there is provided a method for manufacturing a mrs. Oil, comprising: removing impurities from a mrs. Resin; A drying and first grinding step of drying the washed myrrh resin and cooling the dried myrrh resin to -15 to -20 DEG C and cooling the myrrh resin to obtain a myrrh resin powder using a commonly used grinding method; The mulberry resin powder obtained in the above-mentioned drying and first pulverization step is mixed with individual flower, dandelion flower, stem, chinese herb, oriental herb, and blue barley uniformly and then mixed with water, ethanol or fermented liquor, Or a cold extraction method; A first aging step of aging the myrrh resin powder by mixing any one selected from an enzyme and a solvent; A second aging step of aging the myrrh resin powder by adding water or an aqueous solvent selected from the alcohol or the fermentation alcohol to the myrrh powder of the resin subjected to the first aging step; A second milling step of milling the aged myrrh resin powder through the first and second aging steps and re-grinding the dried myrrh powder; An oil mixing step of mixing the myrrh resin powder, which has been aged, dried and pulverized, with a liquid oil through the steps; Mixing the myrrh resin powder and the oil evenly to oil the myrrh; And a stabilization step of stabilizing the stirred myrrh oil through the stirring step, wherein the oil used in the oil mixing step is selected from the group consisting of soybean oil, corn oil, vegetable oil, mono- or di-glyceride of oleic acid, Propyl myristate, isopropyl palmitate, ethyl linoleate, and ethyl oleate. ≪ IMAGE >
The present invention provides a method for producing myrrh oil, which is a natural drying method in which the myristic resin drying method performed in the drying step and the first pulverization step is in contact with air in the atmosphere, and the pulverized myrrh powder particle size is 100 to 150 mesh.

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The present invention provides a method for producing myrrh oil, wherein the complex extract is added to the myrrh powder of the resin in the aging step or the first ripening step using the complex extract and then mixed for 10 to 15 hours at 40 to 60 ° C to increase the safety of the myrrh oil do.

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The present invention provides a method for producing myrrh oil, wherein the amount of the complex extract used in the aging step or the first ripening step is 200 to 400 g per 1 kg of the myrrh resin powder.

The present invention relates to a method for producing a myrrh powder which comprises adding 200 to 500 g of water or a water-soluble or fermented water-soluble solvent per 1 kg of the myrrh resin powder subjected to the first aging step in the second aging step, and then aging at a temperature of 50 to 60 ° C for 60 to 120 minutes A method for producing an oil is provided.

The present invention is characterized in that in the second aging step, the aqueous solvent added to the myrrhic resin powder is at least one selected from the group consisting of water, a myrrh oil which is aged by adding one or more aqueous solvents selected from ethanol, grainy alcohols and ethyl hydroxides, And a manufacturing method thereof.

The present invention provides a method for producing myrrh oil, wherein the agglomerated myrrh resin aged in the second milling step or aged through the first and second aging steps is pulverized into particles having a size ranging from 200 to 300 meshes.

The present invention relates to a method for producing a myristic resin composition, which comprises adding a myrrh resin powder aged in an oil mixing step to an oil and heating and stirring the mixture, and adding the small amount of the aged myrrh resin powder obtained when the oil temperature reaches 50 캜 in the heating stirring step Wherein the mulberry resin powder is added in a ratio of 1: 50 or 1: 80 to the oil mass and the stirring speed is maintained in the range of 600 to 700 rpm using a stirrer.

The present invention provides a method for producing myrrh oil, wherein stirring of the myrrh oil is performed at a temperature of 80 to 120 ° C. and at a temperature of 1000 to 1200 rpm for 60 to 120 minutes after the addition of the myrrh powder is aged do.

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According to the embodiment of the present invention, in the stabilization step of stabilizing the myrrh oil after the stirring, the myrrh oil which has been agitated is stabilized by stirring without heating the myrrh oil, and the stirring speed is about 700 To 900 rpm. ≪ / RTI >
According to the embodiment of the present invention, in the stabilization step of the myrrh oil, mash stick liquid, which is an exudate of pistacia lentiscus, is added in order to add flavor and flavor of the oil, and the addition amount of the mastic oil is 0.1% 20% by weight based on the total weight of the composition.
According to an embodiment of the present invention, there is provided a myrrh oil wherein the content of the pure myrrh component in the myrrh oil is 1 to 99% by weight based on 100% by weight of the myrrh oil.

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The present invention has the effect of providing a commercially available myrrh oil by various methods by preparing high purity myrrh oil having myrrh as a main component and oil as a subcomponent.

The myrrh oil prepared according to the embodiment of the present invention is effective to provide a high quality myrrh oil with high stability of use because it does not change shape such as precipitation and color change even after a long time.

The myrrh oil produced according to the embodiment of the present invention can be used for a wide range of applications such as food and medicine, medical and surgical products, cosmetics and the like, which are closely related to real life.

Figure 1 is a general external view of a moult.
2 is a flow chart of a process for manufacturing myrrh oil according to the first embodiment of the present invention;
3 is a block diagram showing the composition of myrrh oil according to the first embodiment of the present invention.
4 is a flow chart of a process for manufacturing myrrh oil according to a second embodiment of the present invention;
5 is a block diagram showing a myrrh oil composition according to a second embodiment of the present invention.
6 is a flow chart of a myrrh oil manufacturing process according to a third embodiment of the present invention.
7 is a block diagram showing the composition of a myrrh oil according to a third embodiment of the present invention.

Hereinafter, embodiments of the present invention will be described in detail with reference to the drawings.

Myrrh is known to have a powerful analgesic effect on its own components. The main components are Furanoeudesman-1, 3-diene, Lindestrenee, Furanodiene, 2-methoxyfuranodiene, 2-acetoxyfuranodiene and Insofuranogermancrene. In general, most of the myrrh is composed of sesquiterpene.

Myrrh was approved as a safe natural spice material by the US FDA in 1992 and registered as food raw material in the Korea Food and Drug Administration (KFDA) (2000), Kim Changmin et al., 'The Korean Herbal Medicine Illustrated Book', Academy Book 307p (2001), 'The Raw Materials of Processed Foods', Journal of the Korean Society of Food Science and Nutrition A study on the range of flora and fauna that can be used ', Korea Food Research Institute Korea Food Research Institute 144p (1994)).

The registration items for the myrrh-related foods / medicines are registered in the Korea Food and Drug Administration (KFDA) Food Ingredients (raw material name, 'myrrha', 'myrrha' myrrha) and herbal medicine registration (registered name, 'Myrrh' It is listed in the FDA Food Additives Registration (registered name, 'MYRRH') and in the pharmacopoeia (name, 'MYRRH'), Australian Pharmacopoeia (name 'Myrrh') and European Pharmacopoeia (EUROPEAN PHARMACOPOEIA 5.3. 2069 p.

The Korean Food and Drug Administration's registration for myrrh (herbal medicine) is marked and named as myrrh-没 药 -Myrrha (ミ ラ ラ). In the context of the literature, 'this herb is a rubber resin obtained from the sum index Commiphoa molmol Engler or from the myrrh, Commiphoa myrrha Engler (Olive Burseraceae). The former is called the gum opoponax, and the latter is called the natural myrrh Gum Myrrha. ' Regarding the properties, it is described as "the drug is an irregular granule or lumpy shape with rubber resin."

The effect of myrrh for the treatment of cirrhosis of the uterine cervix was investigated. The results of this study were as follows: 1) The effect of myrrh on the gout of white rats induced by Monosodium Urate (Korean Journal of Oriental Internal Medicine. V.27, no.3 pp715 ~ (Korean Journal of Oriental Obstetrics and Gynecology, v18m, no.2 pp70 ~ 84, 2005), 'Structure Identification and Food Application of Inhibitors of Microbial Growth of Food Poisoning Mulberry' (Korean Journal of Food Science and Nutrition v.33, no.4, pp401 ~ 408, 2001), 'The effect of myrrh solution on cultivated sphagnum gupo (Korean Journal of Veterinary Medicine, v.27, no.3 pp715 ~ 721, 2006).

On the other hand, myrrh had a limited commercialization due to the fact that the myrrh resin itself is not easily dissolved or dispersed in water, despite its useful antimicrobial activity (the related product using the pharmacodynamic efficacy of myrrh was called guggulsterone ), Which is a lump with a diameter of 1 ~ 3 cm or more solidified by a solid body.

In the present invention, the pulverized myrrh resin powder is mixed with oil and is converted into a high-purity myrrh oil. The meaning of the modification is not to mean the modification of the molluscule itself but to mix it with other materials and change the physical properties by mixing with the oil.

According to the method for producing myrrh oil according to the embodiment of the present invention, first, a myrrh resin close to a natural state is processed into a powdery powder, and a mixture with other substances is formed in a proper treatment atmosphere, and after aging, the myrrh resin powder and oil To give a myrrh oil. Myrrh oil itself offers many values that are not available in solid lumps of myrrh in use and application, as compared to untreated myrrh, which has a solid lump appearance.

The conventional myrrhyl resin oil may cause sedimentation and color change over time. However, since the myrrhyl resin oil produced by the production method of the present invention has little change in morphology or sedimentation and is safe, it can be used as food or soft capsule, toothpaste, And the like. In particular, it is known that myrrh resin has antibacterial effect against various bacteria including bacteria that cause strong analgesic effect, immunity enhancing effect, irritable bowel and periodontitis. Therefore, it is possible to use myrrh resin oil for a composition for treating and preventing various diseases, Composition and functional food.

A method for producing myrrh oil according to an embodiment of the present invention will be described in detail as follows.

FIG. 2 is a flow chart of the manufacturing process of the myrrh resin oil according to the first embodiment of the present invention. 3 is a block diagram showing the composition of myrrh oil according to the first embodiment of the present invention.

As shown in FIG. 2 and FIG. 3, the manufacturing process of the myristic resin oil according to the first embodiment of the present invention removes impurities adhered to the myristic resin, and removes impurities and cleans the myrrh resin (S 101).

In step S101, the removal and washing of the impurities may be carried out in different manners depending on the degree of management of the myrrh, which is the base material, so that the impurities can be eliminated and the washing can be omitted in some cases. However, . Therefore, depending on the cleanliness of the myrrh, removal of impurities or washing may be omitted, but this may be a necessary course. Impurity removal and cleaning of the myrrhic resins described herein are excluded from the technical process of meaning.

After removing the impurities and washing, the myrrh resin is naturally dried. After the natural drying is completed, the myrrh resin is cooled to -15 to -20 ° C, and the cooled myrrh resin is pulverized by a commonly used grinding method Followed by drying and a first grinding step (S102). Natural drying is selected as a drying method suitable for preserving and preserving the intrinsic components of myrrh as compared with freeze drying or hot drying. In the processing after the drying, that is, the cooling of the myrrh at a temperature of -15 to -20 ° C, And the like, and is advantageously granulated into a powdery state in a stable state. The drying performed in step S102 and the first grinding step are naturally dried in contact with air in the atmosphere as described above, and the particle size of the myrrh powder is preferably adjusted to a range of about 100 to 150 mesh .

Thereafter, the mulch resin powder obtained in the drying and first pulverization step (S102) is mixed with either the complex extract or any one selected from enzymes and solvents to perform aging (S103) in which the myrrh resin powder is aged.

Here, in order to mature the myrrh resin powder, it can be aged using a complex extract as shown in the drawing chart of FIG. In the aging of the myrrh resin powder, it may be selected from any one or more substances selected from a complex extract or an enzyme and a solvent suitable for decomposing or weakening the binding of the myrrh resin.

Since enzymes and solvents have their own resolving power, when they are mixed with myrrh, they usually break down the binding of the myrrh component to break down the bond. Such breakdown or decomposition accelerates the aging of the myrrh resin. Complex extracts have similar resolution.

Composite extracts can be selected from natural sources such as individual flowers, dandelion flowers and stalks, fresh chrysanthemum, orchard, and blue barley mixed together and then mixed with one or more of water or ethanol or fermented liquor And extracted with a method selected from the heat extraction method or the cooling extraction method, and the resultant mixture is mixed with the myrrh resin powder to mature the myrrh resin powder.

Here, since aging can shorten the aging time by selecting among the substances having high fermentation performance, it is possible to select and adjust the aging time depending on the material selection. It is predicted that the enzyme can regulate the time and amount depending on the amount used. It is expected that the complex extracts will be difficult to control the aging and control of myrrh in comparison with the simple solvents and enzymes of the former, which are harmless to the human body. However, individual flowers, dandelion flowers and stems, Both have the advantage of having environmentally benign stability when mixed with myrrh resin powder.

The aging of the myrrh resin powder may vary depending on the material properties, but the selection of the solvent may be appropriately selected according to the need. The degree of aging may be controlled by time or by mixing appropriate solvents A satisfactory ripening state can be obtained from the use. Therefore, if the mulching treatment process in step S103 is carried out, the property of the mulch, which is made of the solidified material of the liquid extracted from the wood, is almost insoluble in water, is modified by a pretreatment and aging process. The stage of aging of the myrrh resin powder is an important treatment step to ensure the safety and uniformity of the myrrh oil, that is, the precipitation does not occur over time. Complex extracts, enzymes or those treated with a solvent.

Representative examples of composition composition of the complex extract according to the first embodiment Raw material (scientific name) Mixing ratio (%) Remarks (extraction method) Individual flowers (Pseudostellaria heterophylla) 30 Extraction of complex extracts mixed with raw materials by hot or cold extraction method evenly mixing or mixing individual raw materials in semi-dry state. The mixing ratio can be adjusted. Dandelion flower and stem (Taraxacum platycarpum Dahlst) 20 Angelica keiskei 20 Houttuynia cordata 15 Blue barley (Hordeum vulgare var. Hexastichon) 15

The appropriate amount of the complex extract used for aging the myrrh resin powder is suitably, for example, 200 to 400 g per 1 kg of the myrrh powder.

In the step of aging S103, it is preferable to add myrrhic resin powder and complex extract, and warm-aged at 40 to 60 DEG C for 10 to 15 hours. In the temperature range below 40 ℃, the ripening time was long and the degree of ripening was low. In the temperature range exceeding 60 ℃, the water evaporation was much higher than expected.

After the aging step of S103, the aged myrrh resin powder is treated with a second grinding step in which the dried and dried myrrh resin powder is pulverized (S104). Here, when the aged myrrh resin is dried, it is solidified into a lump-shaped myrrh resin. The dried lump-like myrrh resin is pulverized by a general pulverizing method. The size of the pulverized particles is preferably maintained at about 200 to 300 mesh.

The drying in the second crushing step of S104 may be selected from natural drying or artificial drying. For controlling the drying time, artificial drying is preferably carried out. Otherwise, natural drying and pulverization are preferred.

Thereafter, the myrrh powder is aged, dried and pulverized through steps S103 to S104 (S105).

The aging milled particles The method of mixing the mullet resin powder with the oil is carried out by adding an appropriate amount of aged mulch resin powder to the oil and heating and stirring the mixture. Preferably, when the temperature of the oil reaches a temperature of 50 DEG C, the obtained aged myrrh resin powder is added in small quantities. At this time, it is preferable that the myrrh resin powder is added at a ratio of about 1:50 or 1: 80 to the oil mass and the stirring speed is maintained at about 600 to 700 rpm. The oil to be added is preferably selected from among soybean oil, corn oil, vegetable oil, mono- or di-glyceride of isoleic acid, isopropyl myristate, isopropyl palmitate, ethyl linoleate and ethyl oleate .

Thereafter, the myrrh resin powder and the oil are uniformly mixed with the S105 oil mixing step to stir the myrrh oil (S106) to obtain a myrrh oil (S107).

The stirring step of S106 is a step of performing high temperature high-speed stirring when the addition of the myrrh powder of the resin aged in oil is completed. The stirring at this stage is carried out at a temperature of 80 to 120 DEG C at 1000 to 1200 rpm for 60 to 120 minutes at a relatively high temperature High-speed stirring process. The myrrh resin powder and the oil are prepared as a brown myrrh oil which is stabilized by dense particle bonding with little decomposition when subjected to such a relatively high-temperature high-speed stirring process.

In the mixing of materials, the heating temperature affects the affinity binding of the material and the spin rotation affects the degree of mixing by reducing intergranular porosity. In general, the temperature atmosphere of the stirrer at an operating speed of 900 to 1100 rpm and the temperature of the stirrer at a temperature of about 60 to 100 ° C reduces the interfacial boundary and particle voids constituting the myristic resin mixture (components of the myrrh resin powder, the aqueous solvent used) In order to have the same effect.

The processing step of S106 relating to oil mixing and heating stirring is a step of performing heating stirring until the aged myrrh powder is completely mixed with the oil. After heating and stirring, the mulberry medicament service finally required or targeted is obtained (S107).

Since the myrrh oil thus prepared contains the myrrh component as a main component in a high purity, the myrrh oil itself has the general efficacy of the myrrh. For example, it has a strong analgesic effect, an immunity-enhancing effect, a bacterium killing effect causing cavities and periodontitis, and an antibacterial effect against various bacteria. Therefore, it can be used as a myrrh oil as a therapeutic drug for various types of diseases and various purposes. It can also be used as a therapeutic agent for the prevention of diseases, a therapeutic agent for skin beauty and a beauty agent, and can be widely used in medical and food fields.

The production of the myrrh oil according to the first embodiment as described above can be produced by other methods. 4 is a flow chart of the manufacturing process of the myrrh resin oil according to the second embodiment of the present invention. 5 is a block diagram showing the composition of myrrh oil according to the second embodiment of the present invention.

The method for producing myrrh oil according to the second embodiment of the present invention may be partly or partly carried out in the method for producing myrrh oil according to the first embodiment of the present invention or may be carried out continuously continuously. Hereinafter, in the description of the method for producing myrrh oil according to the second embodiment of the present invention, matters related to the production of the myrrh oil according to the first embodiment will be briefly described or omitted.

Comparison chart of the production methods of myrrh oil according to the first and second embodiments First Embodiment Second Embodiment Second Manufacturing Method Addition Step S101, Impurity removal and cleaning S201, Impurity removal and cleaning
Second Age S102, drying and first grinding S202, drying and first grinding S103, aging S203, 1st ripening S104, the second crushing S204, 2nd ripening S105, oil mixing S205, the second crush S106, oil mixing stirring S206, Oil Mix S107, obtain myrrh oil S207, oil mixing stirring
S208, obtain myrrh oil

The method of manufacturing myrrh oil according to Table 2 is performed in steps S201 to S208, and the manufacturing sequence corresponds to the steps S101 to S107 of the myrrh oil production method according to the first embodiment of the present invention, or alternatively, .

4 and 5, the process for manufacturing a myrrh oil according to a second embodiment of the present invention will be described with reference to FIGS. 4 and 5. FIG. , The foreign substances and impurities attached to the myristic resin are first removed and washed (S201).

In step S201, impurities can be removed and washed depending on the degree of management of the myrrh, which is a base material. In this case, it is generally preferable to remove the impurities and remove the impurities when using the natural agent. . Therefore, depending on the cleanliness of the myrrh, removal of impurities or washing may be omitted, but this may be a necessary course. Impurity removal and cleaning of the myrrhic resins described herein are excluded from the technical process of meaning.

After removing the impurities and washing, the myrrh resin is naturally dried. After the natural drying is completed, the myrrh resin is cooled to -15 to -20 ° C, and the cooled myrrh resin is pulverized by a commonly used grinding method Followed by drying and first grinding (S202). Natural drying is selected as a drying method suitable for preserving and preserving the intrinsic components of myrrh as compared with freeze drying or hot drying. In the processing after the drying, that is, the cooling of the myrrh at a temperature of -15 to -20 ° C, And the like, and is advantageously granulated into a powdery state in a stable state. Drying and drying performed in the first milling step (S202) are naturally dried in contact with atmospheric air as described above, and it is preferable that the particle size of the myrrh powder is adjusted to about 100 to 150 mesh .

Thereafter, a first aging process is performed in which the mulch resin powder obtained in the drying step and the first pulverization step (S202) is mixed with a complex extract or any one selected from enzymes or solvents to mature the myrrh resin powder (S203).

Here, in order to mature the myrrh resin powder, it is possible to mature using a complex extract as shown in the drawing of FIG. In the aging of the myrrh resin powder, it may be selected from any one or more substances selected from a complex extract or an enzyme and a solvent suitable for decomposing or weakening the binding of the myrrh resin.

Since enzymes and solvents have their own resolving power, when they are mixed with myrrh, they usually break down the binding of the myrrh component to break down the bond. Such breakdown or decomposition accelerates the aging of the myrrh resin. Complex extracts have similar resolution.

Composite extracts can be selected from natural sources such as individual flowers, dandelion flowers and stalks, fresh chrysanthemum, orchard, and blue barley mixed together and then mixed with one or more of water or ethanol or fermented liquor And extracted with a method selected from the heat extraction method or the cooling extraction method, and the resultant mixture is mixed with the myrrh resin powder to mature the myrrh resin powder.

Here, since aging can shorten the aging time by selecting among the substances having high fermentation performance, it is possible to select and adjust the aging time depending on the material selection. It is predicted that the enzyme can regulate the time and amount depending on the amount used. It is expected that the complex extracts will be difficult to control the aging and control of myrrh in comparison with the simple solvents and enzymes of the former, which are harmless to the human body. However, individual flowers, dandelion flowers and stems, Both have the advantage of having environmentally benign stability when mixed with myrrh resin powder.

The aging of the myrrh resin powder may vary depending on the material properties, but the selection of the solvent may be appropriately selected according to the need. The degree of aging may be controlled by time or by mixing appropriate solvents A satisfactory ripening state can be obtained from the use.

Therefore, when the first aging treatment step of step S203 is performed, the characteristic of the mulch, which is a substance in which the liquid extracted from wood is solidified, hardly dissolves in water itself, do.

Representative example of composition composition of the complex extract according to the second embodiment Raw material (scientific name) Mixing ratio (%) Remarks (extraction method) Individual flowers (Pseudostellaria heterophylla) 30 Extraction of complex extracts mixed with raw materials by hot or cold extraction method evenly mixing or mixing individual raw materials in semi-dry state. The mixing ratio can be adjusted. Dandelion flower and stem (Taraxacum platycarpum Dahlst) 20 Angelica keiskei 20 Houttuynia cordata 15 Blue barley (Hordeum vulgare var. Hexastichon) 15

The appropriate amount of the complex extract used for aging the myrrh resin powder is suitably, for example, 200 to 400 g per 1 kg of the myrrh powder.

In the first ripening step of S203, it is preferable to add the myrrh powder and the complex extract and then mature the mixture at 40 to 60 DEG C for 10 to 15 hours. In the temperature range below 40 ℃, the ripening time was long and the degree of ripening was low. In the temperature range exceeding 60 ℃, the water evaporation was much higher than expected.

Then, a second aging step (S204) is performed in which water is added to the myrrh resin powder which has been subjected to the first aging step (S203), or an aqueous solvent selected from the alcohol or the fermentation alcohol, to mature the myrrh resin powder.

In the second aging step of S204, 200 to 500 g of water or a water-soluble or fermented water-soluble organic solvent is added per 1 kg of the myrrh resin powder which has undergone the first aging step (S203), and the mixture is heated at a temperature of 50 to 60 DEG C for 60 to 120 minutes It is preferable to aged. In the second aging step (S204), the aqueous solvent to be added to the myristic resin powder can be aged by adding water or one or more aqueous solvents selected from ethanol, grained alcohol and ethyl hydroxide including water or alcohol or fermented alcohol have.

After the first and second aging steps of S203 and S204, the aged myrrh resin powder is dried (S205), and the dried myrrh resin powder is treated again with the second mill. Here, when the aged myrrh resin is dried, it is solidified into a lump-shaped myrrh resin. The dried lump-like myrrh resin is pulverized by a general pulverizing method. The size of the pulverized particles is preferably maintained at about 200 to 300 mesh.

The drying in the second pulverization step of S205 may be selected from natural drying or an artificial drying. In order to control the drying time, artificial drying is preferably carried out. Otherwise, natural drying and pulverization are preferred.

Thereafter, the myrrh powder is aged, dried, and pulverized through the steps S203 to S205 (S206).

The aging milled particles The method of mixing the mullet resin powder with the oil is carried out by adding an appropriate amount of aged mulch resin powder to the oil and heating and stirring the mixture. Preferably, when the temperature of the oil reaches a temperature of 50 DEG C, the obtained aged myrrh resin powder is added in small quantities. At this time, it is preferable that the myrrh resin powder is added at a ratio of about 1:50 or 1: 80 to the oil mass and the stirring speed is maintained at about 600 to 700 rpm. The oil to be added is preferably selected from among soybean oil, corn oil, vegetable oil, mono- or di-glyceride of isoleic acid, isopropyl myristate, isopropyl palmitate, ethyl linoleate and ethyl oleate .

After mixing the myrrh resin powder and the oil through the S206 oil mixing step, the stirring step (S207) for oiling the myrrh was performed to obtain a myrrh oil (S208).

The stirring step of S207 is a step of performing high-temperature high-speed stirring when the addition of the myrrh powder powder aged in oil is completed, wherein stirring at this stage is carried out at a temperature of 80 to 120 DEG C at 1000 to 1200 rpm for 60 to 120 minutes at a relatively high temperature High-speed stirring process. The myrrh resin powder and the oil are prepared as a brown myrrh oil which is stabilized by dense particle bonding with little decomposition when subjected to such a relatively high-temperature high-speed stirring process.

In the mixing of materials, the heating temperature affects the affinity binding of the material and the spin rotation affects the degree of mixing by reducing intergranular porosity. In general, the temperature atmosphere of the stirrer at an operating speed of 900 to 1100 rpm and the temperature of the stirrer at a temperature of about 60 to 100 ° C reduces the interfacial boundary and particle voids constituting the myristic resin mixture (components of the myrrh resin powder, the aqueous solvent used) In order to have the same effect.

The processing step of S207 for mixing and heating the oil is a step of performing heating and stirring until the first and second aged myristic resin powders are completely mixed with the oil. After heating and stirring, a finally required or targeted myrrh oil is obtained (S208).

Since the myrrh oil thus prepared contains the myrrh component as a main component in a high purity, the myrrh oil itself has the general efficacy of the myrrh. For example, it has a strong analgesic effect, an immunity-enhancing effect, a bacterium killing effect causing cavities and periodontitis, and an antibacterial effect against various bacteria. Therefore, it can be used as a myrrh oil as a therapeutic agent for various types of diseases and various purposes, and can be used as a therapeutic agent for treating diseases, beauty treatments and cosmetics, and can be used in a wide range of fields such as medicine and food.

The production of the myrrh oil according to the first and second embodiments as described above can be produced by other methods. FIG. 6 is a flow chart of the manufacturing process of the myrrh oil according to the third embodiment of the present invention. 7 is a block diagram showing the composition of myrrh oil according to the third embodiment of the present invention.

The method for producing myrrh oil according to the third embodiment of the present invention may be partly or partly carried out by the method for producing myrrh oil according to the first and second embodiments of the present invention or may be carried out continuously continuously. For reference, in the description of the method for producing myrrh oil according to the third embodiment of the present invention, matters related to the production of the myrrh oil according to the first and second embodiments described above will be briefly described or omitted.

Comparison charts of manufacturing methods of myrrh oil according to the first to third embodiments First Embodiment Second Embodiment Third Embodiment Third Embodiment [ S101, Impurity removal and cleaning S201, Impurity removal and cleaning S301, Impurity removal and cleaning Second Age
Myrrh oil stabilization







S102, drying and first grinding S202, drying and first grinding S302, drying and first grinding S103, aging S203, 1st ripening S303, 1st ripening S104, the second crushing S204, 2nd ripening S304, 2nd ripening S105, oil mixing S205, the second crush S305, the second crushing S106, oil mixing stirring S206, Oil Mix S306, oil mixing S107, Myrtle resin oil obtained S207, oil mixing stirring S307, oil mixing stirring
208, obtained myrrh oil S308, myrrh oil stabilization S309, obtain myrrh oil

As shown in Table 4, the method for producing myrrh oil is performed in steps S301 to S309, and the manufacturing sequence corresponds to steps S201 to S208 of the method for producing myrrh oil according to the second embodiment of the present invention, or alternatively .

6 and 7, a process for manufacturing a myrrh oil according to a third embodiment of the present invention will be described with reference to FIGS. 6 and 7. FIG. The foreign substances and impurities attached to the myristic resin are first removed and washed (S301).

In step S301, the removal and washing of impurities may be omitted depending on the degree of management of the myrrh, which is the base material, by eliminating impurities and washing depending on the degree of management. However, in general, starting with removing residual impurities when using a natural agent . Therefore, depending on the cleanliness of the myrrh, removal of impurities or washing may be omitted, but this may be a necessary course. Impurity removal and cleaning of the myrrhic resins described herein are excluded from the technical process of meaning.

After removing the impurities and washing, the myrrh resin is naturally dried. After the natural drying is completed, the myrrh resin is cooled to -15 to -20 ° C, and the cooled myrrh resin is pulverized by a commonly used grinding method Followed by drying and first grinding (S302). Natural drying is selected as a drying method suitable for preserving and preserving the intrinsic components of myrrh as compared with freeze drying or hot drying. In the processing after the drying, that is, the cooling of the myrrh at a temperature of -15 to -20 ° C, And the like, and is advantageously granulated into a powdery state in a stable state. Drying and drying performed in the first milling step (S302) are naturally dried in contact with atmospheric air as described above, and it is preferable that the particle size of the myrrh powder is adjusted to a range of about 100 to 150 mesh .

Thereafter, a first aging process is performed in which the mulch resin powder obtained in the drying step (S302) and the complex extract or any one selected from enzymes or solvents are mixed to agitate the myrrh resin powder (S303).

Here, in order to mature the myrrh resin powder, it is possible to mature using a complex extract as shown in the drawing of FIG. In the aging of the myrrh resin powder, it may be selected from any one or more substances selected from a complex extract or an enzyme and a solvent suitable for decomposing or weakening the binding of the myrrh resin.

Since enzymes and solvents have their own resolving power, when they are mixed with myrrh, they usually break down the binding of the myrrh component to break down the bond. Such breakdown or decomposition accelerates the aging of the myrrh resin. Complex extracts have similar resolution.

Composite extracts can be selected from natural sources such as individual flowers, dandelion flowers and stalks, fresh chrysanthemum, orchard, and blue barley mixed together and then mixed with one or more of water or ethanol or fermented liquor And extracted with a method selected from the heat extraction method or the cooling extraction method, and the resultant mixture is mixed with the myrrh resin powder to mature the myrrh resin powder.

Here, since aging can shorten the aging time by selecting among the substances having high fermentation performance, it is possible to select and adjust the aging time depending on the material selection. It is predicted that the enzyme can regulate the time and amount depending on the amount used. It is expected that the complex extracts will be difficult to control the aging and control of myrrh in comparison with the simple solvents and enzymes of the former, which are harmless to the human body. However, individual flowers, dandelion flowers and stems, Both have the advantage of having environmentally benign stability when mixed with myrrh resin powder.

The aging of the myrrh resin powder may vary depending on the material properties, but the selection of the solvent may be appropriately selected according to the need. The degree of aging may be controlled by time or by mixing appropriate solvents A satisfactory ripening state can be obtained from the use.

Therefore, when the first aging treatment process of step S303 is performed, the characteristic of the mulch, which is a substance in which the liquid extracted from the wood is solidified, hardly dissolves in water itself, do.

Representative examples of composition composition of the complex extract according to the third embodiment Raw material (scientific name) Mixing ratio (%) Remarks (extraction method) Individual flowers (Pseudostellaria heterophylla) 30 Extraction of complex extracts mixed with raw materials by hot or cold extraction method evenly mixing or mixing individual raw materials in semi-dry state. The mixing ratio can be adjusted. Dandelion flower and stem (Taraxacum platycarpum Dahlst) 20 Angelica keiskei 20 Houttuynia cordata 15 Blue barley (Hordeum vulgare var. Hexastichon) 15

The appropriate amount of the complex extract used for aging the myrrh resin powder is suitably, for example, 200 to 400 g per 1 kg of the myrrh powder.

In the first ripening step of S303, it is preferable to add myrrhic resin powder and complex extract, and then mature the mixture at 40 to 60 DEG C for 10 to 15 hours. In the temperature range below 40 ℃, the ripening time was long and the degree of ripening was low. In the temperature range exceeding 60 ℃, the water evaporation was much higher than expected.

Then, a second aging step (S304) is performed in which water is added to the myrrh resin powder which has undergone the first aging step (S303), or an aqueous solvent selected from the alcohol or the fermentation alcohol is aged.

In the second aging step of S304, 200 to 500 g of water or a spirits or fermented water-soluble solvent is added per 1 kg of the myrrh resin powder which has undergone the first aging step (S303), and the mixture is heated at a temperature of 50 to 60 DEG C for 60 to 120 minutes It is preferable to aged. In the second aging step (S304), the aqueous solvent to be added to the myrrh resin powder may be aged by adding water or any one or more aqueous solvents selected from ethanol, grainy alcohol and ethyl hydroxide, including water or alcohol or fermented alcohol have.

Then, the aged myrrh resin powder is subjected to the first and second aging steps S303 and S304, and the dried and dried myrrh resin powder is treated with the second milling (S305). Here, when the aged myrrh resin is dried, it is solidified into a lump-shaped myrrh resin. The dried lump-like myrrh resin is pulverized by a general pulverizing method. The size of the pulverized particles is preferably maintained at about 200 to 300 mesh.

The drying in the second pulverization step of S305 may be selected from natural drying or artificial drying. In order to control the drying time, artificial drying is preferably performed. Otherwise, natural drying and pulverization are preferred.

Thereafter, the myrrh powder is aged, dried, and pulverized through the steps S303 to S305 (S306).

The aging milled particles The method of mixing the mullet resin powder with the oil is carried out by adding an appropriate amount of aged mulch resin powder to the oil and heating and stirring the mixture. Preferably, when the temperature of the oil reaches a temperature of 50 DEG C, the obtained aged myrrh resin powder is added in small quantities. At this time, it is preferable that the myrrh resin powder is added at a ratio of about 1:50 or 1: 80 to the oil mass and the stirring speed is maintained at about 600 to 700 rpm. The oil to be added is preferably selected from among soybean oil, corn oil, vegetable oil, mono- or di-glyceride of isoleic acid, isopropyl myristate, isopropyl palmitate, ethyl linoleate and ethyl oleate .
Thereafter, the stirring step (S307) in which the myrrh resin powder and oil mixed through the S206 oil mixing step are mixed uniformly to oil the myrrh is performed.

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The stirring step of S307 is a step of performing high temperature high-speed stirring when the addition of the myrrh powder powder aged in oil is completed, wherein stirring at this stage is performed at a temperature of 80 to 120 DEG C at 1000 to 1200 rpm for 60 to 120 minutes at a relatively high temperature High-speed stirring process. The myrrh resin powder and the oil are prepared as a brown myrrh oil which is stabilized by dense particle bonding with little decomposition when subjected to such a relatively high-temperature high-speed stirring process.

In the mixing of materials, the heating temperature affects the affinity binding of the material and the spin rotation affects the degree of mixing by reducing intergranular porosity. In general, the temperature atmosphere of the stirrer at an operating speed of 900 to 1100 rpm and the temperature of the stirrer at a temperature of about 60 to 100 ° C reduces the interfacial boundary and particle voids constituting the myristic resin mixture (components of the myrrh resin powder, the aqueous solvent used) In order to have the same effect. The processing step of S307 for oil mixing and heating stirring is a step of performing heating and stirring until the first and second aged mullig resin powders are completely mixed with the oil.

The myrrh oil subjected to the heating and stirring at the high temperature of S307 is subjected to stabilization so as to stabilize it continuously (S308). In the stabilization treatment, the myristic resin and the oil are stabilized after the completion of the mixing and heating and agitation, without adding the temperature.

In the stabilization process (S308), stirring is performed at a relatively low speed of 700 to 900 rpm through a stirrer until the temperature reaches 50 to 60 占 폚. In step S308, the mastic liquid, which is an exudate of the pistacia lentiscus, may be added to add the flavor and aroma of the oil. At this time, the addition amount of the mastic solution may be about 0.1% to 20%. Mastic is a resin extracted from the tree of pistacia lentiscus and used for the health promotion, especially the digestive organs health maintenance purpose. The mastic was announced to the institute that it has strong antibacterial activity against Helicobacter pylori as well as digestive system. It has also been reported that gastritis, duodenal ulcer, and periodontitis are effective, and various studies are underway.

S308 for stabilization treatment is performed to obtain the finally required or targeted myrrh oil (S309). The myrrh oil obtained at this time is a myrrh oil to which a mastic has been added to add flavor and flavor, and can be usefully used in a product directly related to the taste and skin contact of the human body such as foods and cosmetics.

In addition, the myrrh oil prepared in this way contains the myrrh component as its main component in a high purity, and thus has the general efficacy of the myrrh as it is. For example, it has a strong analgesic effect, an immunity-enhancing effect, a bacterium killing effect causing cavities and periodontitis, and an antibacterial effect against various bacteria. Therefore, it can be used as a myrrh oil as a therapeutic agent for various types of diseases and various purposes, and can be used as a therapeutic agent for treating diseases, beauty treatments and cosmetics, and can be used in a wide range of fields such as medicine and food.

The myrrh oil prepared according to the embodiment of the present invention can freely produce a myrrh oil having a myrrh content ranging from 1 to 99% with respect to 100% by weight of the myrrh oil. Therefore, a high purity myrrh oil can be produced relatively simply and stably.

The myrrh oil prepared according to an embodiment of the present invention can be used as a food additive or a food additive. In this case, the myrrh oil exhibited different texture but did not affect the general function of the food, and when the myrrh oil added with the mash stick solution was applied to the food, the flavor and taste of the mast stick solution doubled. Thus, it is possible to use myrrh oil as an additive or a main ingredient in foodstuffs such as foods and the like, and to provide effective ingredients and potency of myrrh without affecting the physical properties and sensory properties of foodstuffs.

The myrrh oil prepared according to the embodiment of the present invention may be added to any one selected from toothpaste or oral cleanser in an amount of 1 to 20% by weight to obtain a dentifrice or oral cleanser product.

A toothpaste was prepared in the same manner as in the control group except that toothpaste was prepared as a general toothpaste as a control group and 2.1 wt% of myrrh oil was added as an experimental group. The effect of myrrh oil on overall acceptability and texture was investigated by the conventional sensory test method. According to the sensory evaluation results, there was no significant difference in the overall acceptability and texture when the myrrh oil was added to toothpaste. Therefore, it was confirmed that the addition of myrrh oil did not affect the sensory properties of the toothpaste. Thus, the addition of myrrh oil to dentifrices and oral cleansers can impart beneficial effects of myrrhic resins, including antimicrobial activity, to toothpastes and mouthwashes without affecting the sensory properties.

In addition, the myrrh oil obtained according to the embodiment of the present invention can be mixed with any one selected from cosmetics or skin cosmetics to obtain a cosmetic product containing myrrh oil and a product for skin care, and also a product obtained according to the embodiment of the present invention The myrrh oil may be mixed with either a soft capsule or a hard capsule to obtain a soft capsule and a hard capsule product. In the case of products containing such a myrrh oil, the myrrh oil was included as a constituent of the whole product and did not affect the sensory properties or taste, but it was possible to obtain the result that the effective functional effect of the myrrh was included as a constituent of the product.

As described above, the myrrh oil prepared according to the embodiment of the present invention can be circulated in the semi-finished product or the finished product according to the purpose of use and can be manufactured to contain a large amount of myrrh resin as a main component, As it is. For example, it has a strong analgesic effect, an immunity-enhancing effect, a bacterium killing effect causing cavities and periodontitis, and an antibacterial effect against various bacteria. Therefore, it can be used as an oil state for various types of diseases and therapeutic drugs for various purposes, and can be used as a therapeutic agent and a cosmetic agent for prevention of disease, skin care, and can be widely used in the fields of medicine and food and beverage, And as additives and drinks in the food sector.

The present invention is not limited to the embodiments but can be modified and modified without departing from the gist of the present invention, and modifications and variations are included in the technical idea of the present invention.

S101 to S107: Manufacturing method of the first embodiment
S201 to S208: Manufacturing method of the second embodiment
S301 to S309: Manufacturing method of the third embodiment

Claims (19)

A step of removing impurities and cleaning the myrrh resin by removing impurities attached to the myrrh resin;
A drying and first grinding step of drying the washed myrrh resin and cooling the dried myrrh resin to -15 to -20 DEG C and cooling the myrrh resin to obtain a myrrh resin powder using a commonly used grinding method;
The mulberry resin powder obtained in the above-mentioned drying and first pulverization step is mixed with individual flower, dandelion flower, stem, chinese herb, oriental herb, and blue barley uniformly and then mixed with water, ethanol or fermented liquor, Or a cold extraction method; A first aging step of aging the myrrh resin powder by mixing any one selected from an enzyme and a solvent;
A second aging step of aging the myrrh resin powder by adding water or an aqueous solvent selected from the alcohol or the fermentation alcohol to the myrrh powder of the resin subjected to the first aging step;
A second milling step of milling the aged myrrh resin powder through the first and second aging steps and re-grinding the dried myrrh powder;
An oil mixing step of mixing the myrrh resin powder, which has been aged, dried and pulverized, with a liquid oil through the steps;
Mixing the myrrh resin powder and the oil evenly to oil the myrrh; And a stabilization step of stabilizing the stirred myrrh oil through the stirring step,
The oil used in the oil mixing step may be any one selected from soybean oil, corn oil, vegetable oil, mono- or di-glyceride of isoleic acid, isopropyl myristate, isopropyl palmitate, ethyl linoleate and ethyl oleate ≪ / RTI > delete delete The method of claim 1, wherein the drying performed in the drying step and the first pulverizing step is naturally dried in contact with air in the atmosphere, and the size of the pulverized myrrh powder powder is 100 to 150 mesh. delete The method according to claim 1, wherein the complex extract is added to the myrrh resin powder in the first ripening step using the complex extract, followed by mixing for 10-15 hours at 40 to 60 ° C to increase the safety of the myrrh oil. [2] The method according to claim 1, wherein the amount of the complex extract used in the first ripening step is 200 to 400 g per 1 kg of the myrrh powder. The method according to claim 1, wherein, in the second aging step, 200 to 500 g of water or a water-soluble or fermented water-soluble organic solvent is added per 1 kg of the myrrh resin powder which has been subjected to the first aging step, A method for producing a myrrh oil which is miniscule. The method according to claim 1, wherein the aqueous solvent added to the myristic resin powder in the second aging step is one or more aqueous solvents selected from the group consisting of water, ethanol, grainy alcohol and ethyl hydroxide including water or a fermented alcohol, Method of manufacturing myrrh oil for aging. The method according to claim 1, wherein in the second milling step, the agglomerated myrrh resin aged through the first and second aging steps is pulverized into particles having a size ranging from 200 to 300 mesh. 2. The method according to claim 1, wherein in the oil mixing step, the aged mullite resin powder is added to oil and the mixture is heated and agitated. When the oil temperature reaches the temperature of 50 ° C in the heating agitation step, In a proportion of 1: 50 or 1: 80 to the oil mass, and the stirring speed using a stirrer is maintained in the range of 600 to 700 rpm. delete The method according to claim 1, wherein the stirring step for oiling the myrrh oil is performed by stirring the myrrh oil powder at a temperature of 80 to 120 DEG C at 1000 to 1200 rpm for 60 to 120 minutes, Gt; The process according to claim 1, wherein the stabilizing step of stabilizing the stirred myrrh oil is to stabilize the myrrh oil by stirring without heating the stirred myrrh oil, and stirring the mixture at a stirring speed of from 700 to 900 rpm ≪ / RTI > with stirring. The method according to claim 1, wherein in the step of stabilizing the myrrh oil, a mastic liquid, which is an exudate of pistacia lentiscus, is added to add the flavor and aroma of the oil, and the amount of the mastic liquid added is 0.1% to 20% % ≪ / RTI > by weight. A method for producing a myrrhic oil, which comprises, by weight, 100% by weight of a myrrh oil obtained by the process according to any one of claims 1, 4, 6 to 11, 13 and 14, To 99% by weight of a myrrh oil.






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