JP6863861B2 - エーテルを含む水性電解液及び当該電解液を使用した電池 - Google Patents
エーテルを含む水性電解液及び当該電解液を使用した電池 Download PDFInfo
- Publication number
- JP6863861B2 JP6863861B2 JP2017165193A JP2017165193A JP6863861B2 JP 6863861 B2 JP6863861 B2 JP 6863861B2 JP 2017165193 A JP2017165193 A JP 2017165193A JP 2017165193 A JP2017165193 A JP 2017165193A JP 6863861 B2 JP6863861 B2 JP 6863861B2
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- Prior art keywords
- lithium
- ether
- group
- formula
- glycol dimethyl
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
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- RTZKZFJDLAIYFH-UHFFFAOYSA-N Diethyl ether Chemical compound CCOCC RTZKZFJDLAIYFH-UHFFFAOYSA-N 0.000 title claims description 40
- 239000003792 electrolyte Substances 0.000 title claims description 29
- 229910001416 lithium ion Inorganic materials 0.000 claims description 42
- HBBGRARXTFLTSG-UHFFFAOYSA-N Lithium ion Chemical compound [Li+] HBBGRARXTFLTSG-UHFFFAOYSA-N 0.000 claims description 38
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 claims description 29
- XTHFKEDIFFGKHM-UHFFFAOYSA-N Dimethoxyethane Chemical compound COCCOC XTHFKEDIFFGKHM-UHFFFAOYSA-N 0.000 claims description 25
- WYURNTSHIVDZCO-UHFFFAOYSA-N Tetrahydrofuran Chemical compound C1CCOC1 WYURNTSHIVDZCO-UHFFFAOYSA-N 0.000 claims description 20
- 229910003002 lithium salt Inorganic materials 0.000 claims description 19
- 150000001450 anions Chemical class 0.000 claims description 17
- 239000008151 electrolyte solution Substances 0.000 claims description 17
- 159000000002 lithium salts Chemical class 0.000 claims description 17
- -1 anion lithium salt Chemical class 0.000 claims description 15
- 229920001223 polyethylene glycol Polymers 0.000 claims description 15
- ZUHZGEOKBKGPSW-UHFFFAOYSA-N tetraglyme Chemical compound COCCOCCOCCOCCOC ZUHZGEOKBKGPSW-UHFFFAOYSA-N 0.000 claims description 15
- 150000003839 salts Chemical class 0.000 claims description 14
- WHXSMMKQMYFTQS-UHFFFAOYSA-N Lithium Chemical compound [Li] WHXSMMKQMYFTQS-UHFFFAOYSA-N 0.000 claims description 12
- 150000004292 cyclic ethers Chemical class 0.000 claims description 12
- 229910052744 lithium Inorganic materials 0.000 claims description 12
- 239000002202 Polyethylene glycol Substances 0.000 claims description 10
- SBZXBUIDTXKZTM-UHFFFAOYSA-N diglyme Chemical compound COCCOCCOC SBZXBUIDTXKZTM-UHFFFAOYSA-N 0.000 claims description 10
- ACFSQHQYDZIPRL-UHFFFAOYSA-N lithium;bis(1,1,2,2,2-pentafluoroethylsulfonyl)azanide Chemical compound [Li+].FC(F)(F)C(F)(F)S(=O)(=O)[N-]S(=O)(=O)C(F)(F)C(F)(F)F ACFSQHQYDZIPRL-UHFFFAOYSA-N 0.000 claims description 10
- QSZMZKBZAYQGRS-UHFFFAOYSA-N lithium;bis(trifluoromethylsulfonyl)azanide Chemical compound [Li+].FC(F)(F)S(=O)(=O)[N-]S(=O)(=O)C(F)(F)F QSZMZKBZAYQGRS-UHFFFAOYSA-N 0.000 claims description 10
- MCVFFRWZNYZUIJ-UHFFFAOYSA-M lithium;trifluoromethanesulfonate Chemical compound [Li+].[O-]S(=O)(=O)C(F)(F)F MCVFFRWZNYZUIJ-UHFFFAOYSA-M 0.000 claims description 10
- YLQBMQCUIZJEEH-UHFFFAOYSA-N tetrahydrofuran Natural products C=1C=COC=1 YLQBMQCUIZJEEH-UHFFFAOYSA-N 0.000 claims description 10
- YFNKIDBQEZZDLK-UHFFFAOYSA-N triglyme Chemical compound COCCOCCOCCOC YFNKIDBQEZZDLK-UHFFFAOYSA-N 0.000 claims description 10
- 238000009830 intercalation Methods 0.000 claims description 9
- 239000000463 material Substances 0.000 claims description 9
- 125000004432 carbon atom Chemical group C* 0.000 claims description 7
- 238000009831 deintercalation Methods 0.000 claims description 7
- 125000005010 perfluoroalkyl group Chemical group 0.000 claims description 7
- 150000003949 imides Chemical class 0.000 claims description 5
- 125000001153 fluoro group Chemical group F* 0.000 claims description 4
- 125000004170 methylsulfonyl group Chemical group [H]C([H])([H])S(*)(=O)=O 0.000 claims description 4
- 229910015643 LiMn 2 O 4 Inorganic materials 0.000 claims description 3
- 230000002687 intercalation Effects 0.000 claims description 3
- 229910012851 LiCoO 2 Inorganic materials 0.000 claims description 2
- 229910011281 LiCoPO 4 Inorganic materials 0.000 claims description 2
- 229910011573 LiFe Inorganic materials 0.000 claims description 2
- 229910002099 LiNi0.5Mn1.5O4 Inorganic materials 0.000 claims description 2
- 125000003709 fluoroalkyl group Chemical group 0.000 claims description 2
- 229910014089 LiMn1/3Ni1/3Co1/3O2 Inorganic materials 0.000 claims 1
- 125000000472 sulfonyl group Chemical group *S(*)(=O)=O 0.000 claims 1
- 239000000203 mixture Substances 0.000 description 16
- 239000011230 binding agent Substances 0.000 description 8
- 229920001577 copolymer Polymers 0.000 description 8
- 238000000034 method Methods 0.000 description 7
- PXHVJJICTQNCMI-UHFFFAOYSA-N nickel Substances [Ni] PXHVJJICTQNCMI-UHFFFAOYSA-N 0.000 description 6
- 229920002981 polyvinylidene fluoride Polymers 0.000 description 6
- 239000010405 anode material Substances 0.000 description 5
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 4
- 229920001780 ECTFE Polymers 0.000 description 4
- 239000002033 PVDF binder Substances 0.000 description 4
- 229910052799 carbon Inorganic materials 0.000 description 4
- 239000002245 particle Substances 0.000 description 4
- 229920002493 poly(chlorotrifluoroethylene) Polymers 0.000 description 4
- 239000005023 polychlorotrifluoroethylene (PCTFE) polymer Substances 0.000 description 4
- 229920001343 polytetrafluoroethylene Polymers 0.000 description 4
- 239000004810 polytetrafluoroethylene Substances 0.000 description 4
- 229920005989 resin Polymers 0.000 description 4
- 239000011347 resin Substances 0.000 description 4
- 239000010406 cathode material Substances 0.000 description 3
- 239000010949 copper Substances 0.000 description 3
- 238000004519 manufacturing process Methods 0.000 description 3
- 229910052759 nickel Inorganic materials 0.000 description 3
- 239000010936 titanium Substances 0.000 description 3
- RYGMFSIKBFXOCR-UHFFFAOYSA-N Copper Chemical compound [Cu] RYGMFSIKBFXOCR-UHFFFAOYSA-N 0.000 description 2
- 239000004698 Polyethylene Substances 0.000 description 2
- 239000011149 active material Substances 0.000 description 2
- 229910052782 aluminium Inorganic materials 0.000 description 2
- XAGFODPZIPBFFR-UHFFFAOYSA-N aluminium Chemical compound [Al] XAGFODPZIPBFFR-UHFFFAOYSA-N 0.000 description 2
- 239000006182 cathode active material Substances 0.000 description 2
- 229910052802 copper Inorganic materials 0.000 description 2
- 238000000354 decomposition reaction Methods 0.000 description 2
- QHSJIZLJUFMIFP-UHFFFAOYSA-N ethene;1,1,2,2-tetrafluoroethene Chemical compound C=C.FC(F)=C(F)F QHSJIZLJUFMIFP-UHFFFAOYSA-N 0.000 description 2
- 229920006242 ethylene acrylic acid copolymer Polymers 0.000 description 2
- 229920000840 ethylene tetrafluoroethylene copolymer Polymers 0.000 description 2
- 238000011156 evaluation Methods 0.000 description 2
- 229910052751 metal Inorganic materials 0.000 description 2
- 239000002184 metal Substances 0.000 description 2
- 239000004570 mortar (masonry) Substances 0.000 description 2
- 239000002105 nanoparticle Substances 0.000 description 2
- 229920000573 polyethylene Polymers 0.000 description 2
- 229920000642 polymer Polymers 0.000 description 2
- 239000002002 slurry Substances 0.000 description 2
- 239000002904 solvent Substances 0.000 description 2
- 229910001220 stainless steel Inorganic materials 0.000 description 2
- 239000010935 stainless steel Substances 0.000 description 2
- 229920003048 styrene butadiene rubber Polymers 0.000 description 2
- BFKJFAAPBSQJPD-UHFFFAOYSA-N tetrafluoroethene Chemical group FC(F)=C(F)F BFKJFAAPBSQJPD-UHFFFAOYSA-N 0.000 description 2
- 229920001169 thermoplastic Polymers 0.000 description 2
- 229920001187 thermosetting polymer Polymers 0.000 description 2
- 239000004416 thermosoftening plastic Substances 0.000 description 2
- 229910015645 LiMn Inorganic materials 0.000 description 1
- 229910017267 Mo 6 S 8 Inorganic materials 0.000 description 1
- 239000004721 Polyphenylene oxide Substances 0.000 description 1
- NINIDFKCEFEMDL-UHFFFAOYSA-N Sulfur Chemical compound [S] NINIDFKCEFEMDL-UHFFFAOYSA-N 0.000 description 1
- FDLZQPXZHIFURF-UHFFFAOYSA-N [O-2].[Ti+4].[Li+] Chemical compound [O-2].[Ti+4].[Li+] FDLZQPXZHIFURF-UHFFFAOYSA-N 0.000 description 1
- 239000007864 aqueous solution Substances 0.000 description 1
- 230000001351 cycling effect Effects 0.000 description 1
- 239000003365 glass fiber Substances 0.000 description 1
- 229910052987 metal hydride Inorganic materials 0.000 description 1
- 239000011255 nonaqueous electrolyte Substances 0.000 description 1
- 230000008520 organization Effects 0.000 description 1
- 230000033116 oxidation-reduction process Effects 0.000 description 1
- 229920000570 polyether Polymers 0.000 description 1
- 239000000126 substance Substances 0.000 description 1
- KKEYFWRCBNTPAC-UHFFFAOYSA-L terephthalate(2-) Chemical compound [O-]C(=O)C1=CC=C(C([O-])=O)C=C1 KKEYFWRCBNTPAC-UHFFFAOYSA-L 0.000 description 1
Images
Classifications
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M10/00—Secondary cells; Manufacture thereof
- H01M10/36—Accumulators not provided for in groups H01M10/05-H01M10/34
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M10/00—Secondary cells; Manufacture thereof
- H01M10/05—Accumulators with non-aqueous electrolyte
- H01M10/052—Li-accumulators
- H01M10/0525—Rocking-chair batteries, i.e. batteries with lithium insertion or intercalation in both electrodes; Lithium-ion batteries
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M10/00—Secondary cells; Manufacture thereof
- H01M10/05—Accumulators with non-aqueous electrolyte
- H01M10/056—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes
- H01M10/0564—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes the electrolyte being constituted of organic materials only
- H01M10/0566—Liquid materials
- H01M10/0567—Liquid materials characterised by the additives
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M10/00—Secondary cells; Manufacture thereof
- H01M10/05—Accumulators with non-aqueous electrolyte
- H01M10/056—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes
- H01M10/0564—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes the electrolyte being constituted of organic materials only
- H01M10/0566—Liquid materials
- H01M10/0568—Liquid materials characterised by the solutes
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M10/00—Secondary cells; Manufacture thereof
- H01M10/05—Accumulators with non-aqueous electrolyte
- H01M10/056—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes
- H01M10/0564—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes the electrolyte being constituted of organic materials only
- H01M10/0566—Liquid materials
- H01M10/0569—Liquid materials characterised by the solvents
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M2220/00—Batteries for particular applications
- H01M2220/20—Batteries in motive systems, e.g. vehicle, ship, plane
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M2300/00—Electrolytes
- H01M2300/0002—Aqueous electrolytes
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/10—Energy storage using batteries
Landscapes
- Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Manufacturing & Machinery (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Electrochemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Inorganic Chemistry (AREA)
- General Physics & Mathematics (AREA)
- Condensed Matter Physics & Semiconductors (AREA)
- Physics & Mathematics (AREA)
- Materials Engineering (AREA)
- Secondary Cells (AREA)
- Battery Electrode And Active Subsutance (AREA)
Applications Claiming Priority (2)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| US15/252,513 | 2016-08-31 | ||
| US15/252,513 US10193188B2 (en) | 2016-08-31 | 2016-08-31 | Aqueous electrolyte with ethers and batteries using the electrolyte |
Publications (3)
| Publication Number | Publication Date |
|---|---|
| JP2018049819A JP2018049819A (ja) | 2018-03-29 |
| JP2018049819A5 JP2018049819A5 (enExample) | 2019-07-18 |
| JP6863861B2 true JP6863861B2 (ja) | 2021-04-21 |
Family
ID=61243594
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| JP2017165193A Active JP6863861B2 (ja) | 2016-08-31 | 2017-08-30 | エーテルを含む水性電解液及び当該電解液を使用した電池 |
Country Status (2)
| Country | Link |
|---|---|
| US (1) | US10193188B2 (enExample) |
| JP (1) | JP6863861B2 (enExample) |
Families Citing this family (7)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US11133523B2 (en) * | 2017-07-28 | 2021-09-28 | Toyota Motor Engineering & Manufacturing North America, Inc. | Aqueous electrolytes with protonic ionic liquid and batteries using the electrolyte |
| US10868340B2 (en) * | 2018-03-23 | 2020-12-15 | Kabushiki Kaisha Toshiba | Secondary battery, battery pack, vehicle, and stationary power supply |
| CN111477977B (zh) * | 2019-01-23 | 2022-07-01 | 北京理工大学 | 一种锂离子电池用水-醚类混合电解液及其制备方法 |
| CN114243127A (zh) * | 2022-02-21 | 2022-03-25 | 浙江金羽新能源科技有限公司 | 一种低溶解氧的水系电解液、其制备方法以及水系离子电池 |
| JP7613434B2 (ja) * | 2022-08-29 | 2025-01-15 | トヨタ自動車株式会社 | 水系カリウムイオン電池 |
| KR102821116B1 (ko) * | 2022-09-26 | 2025-06-17 | 한국화학연구원 | 수계 전해질, 그 제조방법 및 이를 포함하는 리튬이차전지 |
| CN115275208B (zh) * | 2022-09-27 | 2023-02-07 | 宇恒电池股份有限公司 | 一种高比能水系锂离子电池及其制备方法 |
Family Cites Families (13)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| JP2001052747A (ja) | 1999-08-06 | 2001-02-23 | Matsushita Electric Ind Co Ltd | リチウム二次電池 |
| US6344293B1 (en) * | 2000-04-18 | 2002-02-05 | Moltech Corporation | Lithium electrochemical cells with enhanced cycle life |
| JP5218406B2 (ja) | 2007-07-11 | 2013-06-26 | 株式会社豊田中央研究所 | 水系リチウム二次電池 |
| EP2270917B1 (en) * | 2008-04-28 | 2014-06-25 | Asahi Glass Company, Limited | Non-aqueous electrolyte for secondary cell and secondary cell comprising the same |
| JP2011154783A (ja) | 2010-01-26 | 2011-08-11 | Equos Research Co Ltd | 電気化学デバイス用電解液の製造方法 |
| WO2012163300A1 (zh) | 2011-06-03 | 2012-12-06 | 苏州宝时得电动工具有限公司 | 电池 |
| US8828574B2 (en) | 2011-11-15 | 2014-09-09 | Polyplus Battery Company | Electrolyte compositions for aqueous electrolyte lithium sulfur batteries |
| US9660265B2 (en) | 2011-11-15 | 2017-05-23 | Polyplus Battery Company | Lithium sulfur batteries and electrolytes and sulfur cathodes thereof |
| US8828575B2 (en) | 2011-11-15 | 2014-09-09 | PolyPlus Batter Company | Aqueous electrolyte lithium sulfur batteries |
| BR112016006399A2 (pt) * | 2013-09-25 | 2017-08-01 | Univ Tokyo | solução eletrolítica, para dispositivos de armazenagem elétrica tais como baterias e capacitores, contendo sais cujo cátion é um metal alcalino, metal alcalinoterroso, ou alumínio, e sol-vente orgânico tendo heteroelemento, método para produção da referida solução eletrolítica, e capaci-tor incluindo a referida solução eletrolítica |
| WO2015045389A1 (ja) * | 2013-09-25 | 2015-04-02 | 国立大学法人東京大学 | アルカリ金属、アルカリ土類金属又はアルミニウムをカチオンとする塩と、ヘテロ元素を有する有機溶媒とを含む、電池、キャパシタ等の蓄電装置用電解液、及びその製造方法、並びに当該電解液を具備するキャパシタ |
| JP6423453B2 (ja) * | 2015-01-14 | 2018-11-14 | 国立大学法人 東京大学 | 蓄電装置用水系電解液、及び当該水系電解液を含む蓄電装置 |
| JP6421778B2 (ja) * | 2016-03-23 | 2018-11-14 | トヨタ自動車株式会社 | リチウムイオン二次電池 |
-
2016
- 2016-08-31 US US15/252,513 patent/US10193188B2/en not_active Expired - Fee Related
-
2017
- 2017-08-30 JP JP2017165193A patent/JP6863861B2/ja active Active
Also Published As
| Publication number | Publication date |
|---|---|
| US10193188B2 (en) | 2019-01-29 |
| US20180062205A1 (en) | 2018-03-01 |
| JP2018049819A (ja) | 2018-03-29 |
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