JP6342905B2 - 有機光起電力におけるアクセプタおよびドナーのエネルギー感光化 - Google Patents

有機光起電力におけるアクセプタおよびドナーのエネルギー感光化 Download PDF

Info

Publication number
JP6342905B2
JP6342905B2 JP2015535864A JP2015535864A JP6342905B2 JP 6342905 B2 JP6342905 B2 JP 6342905B2 JP 2015535864 A JP2015535864 A JP 2015535864A JP 2015535864 A JP2015535864 A JP 2015535864A JP 6342905 B2 JP6342905 B2 JP 6342905B2
Authority
JP
Japan
Prior art keywords
acceptor
photoreceptor
organic
layer
donor
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
JP2015535864A
Other languages
English (en)
Japanese (ja)
Other versions
JP2015530761A (ja
Inventor
トンプソン，マーク，イー．
トリン，コン
ジューロビッチ，ピーター，アイ．
コンロン，サラ，エム．
Original Assignee
ユニバーシティ オブ サザン カリフォルニア
ユニバーシティ オブ サザン カリフォルニア
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by ユニバーシティ オブ サザン カリフォルニア, ユニバーシティ オブ サザン カリフォルニア filed Critical ユニバーシティ オブ サザン カリフォルニア
Publication of JP2015530761A publication Critical patent/JP2015530761A/ja
Application granted granted Critical
Publication of JP6342905B2 publication Critical patent/JP6342905B2/ja
Expired - Fee Related legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09B—ORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B47/00—Porphines; Azaporphines
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B82—NANOTECHNOLOGY
    • B82Y—SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES; MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES; MANUFACTURE OR TREATMENT OF NANOSTRUCTURES
    • B82Y10/00—Nanotechnology for information processing, storage or transmission, e.g. quantum computing or single electron logic
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09B—ORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B57/00—Other synthetic dyes of known constitution
    • C09B57/10—Metal complexes of organic compounds not being dyes in uncomplexed form
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K30/00—Organic devices sensitive to infrared radiation, light, electromagnetic radiation of shorter wavelength or corpuscular radiation
    • H10K30/20—Organic devices sensitive to infrared radiation, light, electromagnetic radiation of shorter wavelength or corpuscular radiation comprising organic-organic junctions, e.g. donor-acceptor junctions
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K85/00—Organic materials used in the body or electrodes of devices covered by this subclass
    • H10K85/20—Carbon compounds, e.g. carbon nanotubes or fullerenes
    • H10K85/211—Fullerenes, e.g. C60
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K85/00—Organic materials used in the body or electrodes of devices covered by this subclass
    • H10K85/30—Coordination compounds
    • H10K85/321—Metal complexes comprising a group IIIA element, e.g. Tris (8-hydroxyquinoline) gallium [Gaq3]
    • H10K85/322—Metal complexes comprising a group IIIA element, e.g. Tris (8-hydroxyquinoline) gallium [Gaq3] comprising boron
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K85/00—Organic materials used in the body or electrodes of devices covered by this subclass
    • H10K85/30—Coordination compounds
    • H10K85/341—Transition metal complexes, e.g. Ru(II)polypyridine complexes
    • H10K85/342—Transition metal complexes, e.g. Ru(II)polypyridine complexes comprising iridium
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K85/00—Organic materials used in the body or electrodes of devices covered by this subclass
    • H10K85/30—Coordination compounds
    • H10K85/381—Metal complexes comprising a group IIB metal element, e.g. comprising cadmium, mercury or zinc
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K2101/00—Properties of the organic materials covered by group H10K85/00
    • H10K2101/30—Highest occupied molecular orbital [HOMO], lowest unoccupied molecular orbital [LUMO] or Fermi energy values
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K2101/00—Properties of the organic materials covered by group H10K85/00
    • H10K2101/40—Interrelation of parameters between multiple constituent active layers or sublayers, e.g. HOMO values in adjacent layers
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K30/00—Organic devices sensitive to infrared radiation, light, electromagnetic radiation of shorter wavelength or corpuscular radiation
    • H10K30/50—Photovoltaic [PV] devices
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K30/00—Organic devices sensitive to infrared radiation, light, electromagnetic radiation of shorter wavelength or corpuscular radiation
    • H10K30/80—Constructional details
    • H10K30/81—Electrodes
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K50/00—Organic light-emitting devices
    • H10K50/10—OLEDs or polymer light-emitting diodes [PLED]
    • H10K50/11—OLEDs or polymer light-emitting diodes [PLED] characterised by the electroluminescent [EL] layers
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K85/00—Organic materials used in the body or electrodes of devices covered by this subclass
    • H10K85/20—Carbon compounds, e.g. carbon nanotubes or fullerenes
    • H10K85/211—Fullerenes, e.g. C60
    • H10K85/215—Fullerenes, e.g. C60 comprising substituents, e.g. PCBM
    • H—ELECTRICITY
    • H10—SEMICONDUCTOR DEVICES; ELECTRIC SOLID-STATE DEVICES NOT OTHERWISE PROVIDED FOR
    • H10K—ORGANIC ELECTRIC SOLID-STATE DEVICES
    • H10K85/00—Organic materials used in the body or electrodes of devices covered by this subclass
    • H10K85/30—Coordination compounds
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E10/00—Energy generation through renewable energy sources
    • Y02E10/50—Photovoltaic [PV] energy
    • Y02E10/549—Organic PV cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Nanotechnology (AREA)
  • Inorganic Chemistry (AREA)
  • Organic Chemistry (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Physics & Mathematics (AREA)
  • Mathematical Physics (AREA)
  • Theoretical Computer Science (AREA)
  • Electromagnetism (AREA)
  • Photovoltaic Devices (AREA)
  • Photoreceptors In Electrophotography (AREA)
  • Electroluminescent Light Sources (AREA)
  • Pyridine Compounds (AREA)
  • Pyrrole Compounds (AREA)
JP2015535864A 2012-10-05 2013-10-07 有機光起電力におけるアクセプタおよびドナーのエネルギー感光化 Expired - Fee Related JP6342905B2 (ja)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
US201261710504P 2012-10-05 2012-10-05
US61/710,504 2012-10-05
PCT/US2013/063661 WO2014055976A1 (en) 2012-10-05 2013-10-07 Energy sensitization of acceptors and donors in organic photovoltaics

Related Child Applications (1)

Application Number Title Priority Date Filing Date
JP2018051592A Division JP6734315B2 (ja) 2012-10-05 2018-03-19 有機光起電力におけるアクセプタおよびドナーのエネルギー感光化

Publications (2)

Publication Number Publication Date
JP2015530761A JP2015530761A (ja) 2015-10-15
JP6342905B2 true JP6342905B2 (ja) 2018-06-13

Family

ID=49382646

Family Applications (2)

Application Number Title Priority Date Filing Date
JP2015535864A Expired - Fee Related JP6342905B2 (ja) 2012-10-05 2013-10-07 有機光起電力におけるアクセプタおよびドナーのエネルギー感光化
JP2018051592A Expired - Fee Related JP6734315B2 (ja) 2012-10-05 2018-03-19 有機光起電力におけるアクセプタおよびドナーのエネルギー感光化

Family Applications After (1)

Application Number Title Priority Date Filing Date
JP2018051592A Expired - Fee Related JP6734315B2 (ja) 2012-10-05 2018-03-19 有機光起電力におけるアクセプタおよびドナーのエネルギー感光化

Country Status (11)

Country Link
US (2) US10367157B2 (https=)
EP (1) EP2904649B1 (https=)
JP (2) JP6342905B2 (https=)
KR (1) KR102160497B1 (https=)
CN (1) CN104904028A (https=)
AU (1) AU2013326799A1 (https=)
CA (1) CA2887101A1 (https=)
IL (1) IL238124A0 (https=)
IN (1) IN2015DN03049A (https=)
TW (2) TWI638476B (https=)
WO (1) WO2014055976A1 (https=)

Families Citing this family (31)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
TWI612704B (zh) * 2012-10-11 2018-01-21 史蒂芬Ｒ 佛瑞斯特 利用方酸施體添加物的聚合物光伏打裝置
MY162427A (en) * 2013-02-14 2017-06-15 Daicel Corp Curable resin composition and cured product thereof, encapsulant, and semiconductor device
JP6387410B2 (ja) * 2013-07-24 2018-09-05 アイメック・ヴェーゼットウェーＩｍｅｃ Ｖｚｗ 改良された光電流を有する有機太陽電池
JP2019216256A (ja) * 2014-05-13 2019-12-19 ソニーセミコンダクタソリューションズ株式会社 光電変換膜、固体撮像素子、および電子機器
JP6567276B2 (ja) * 2014-05-13 2019-08-28 ソニーセミコンダクタソリューションズ株式会社 固体撮像素子、および電子機器
KR102903774B1 (ko) 2015-05-29 2025-12-24 소니 세미컨덕터 솔루션즈 가부시키가이샤 광전변환 소자 및 고체 촬상 장치
EP3327810B1 (en) * 2015-07-17 2022-11-02 Sony Group Corporation Imaging element, multilayer imaging element and solid-state imaging device
US11341426B2 (en) * 2015-11-27 2022-05-24 Photonic Inc. Systems, devices, and methods to interact with quantum information stored in spins
WO2017159610A1 (ja) * 2016-03-18 2017-09-21 日本化薬株式会社 有機化合物、近赤外吸収色素、光電変換素子及びその光センサー、撮像素子
CN105732593A (zh) * 2016-04-20 2016-07-06 江苏大学 一种咔唑二吡咯甲烷金属配合物及其制备方法
US10665803B2 (en) * 2016-04-22 2020-05-26 The Trusteees Of Princeton University Solid-state organic intermediate-band photovoltaic devices
JP2018014396A (ja) * 2016-07-20 2018-01-25 ソニーセミコンダクタソリューションズ株式会社 光電変換素子および固体撮像装置
US11158675B2 (en) * 2016-07-20 2021-10-26 Sony Corporation Solid-state imaging element and solid-state imaging apparatus
EP3496147A4 (en) * 2016-08-03 2019-08-14 Sony Corporation IMAGING ELEMENT, MULTILAYER IMAGING ELEMENT AND SOLID STATE IMAGING DEVICE
WO2018147202A1 (ja) * 2017-02-07 2018-08-16 キヤノン株式会社 光電変換素子、及びこれを用いた光エリアセンサ、撮像素子、撮像装置
JP7039285B2 (ja) * 2017-02-07 2022-03-22 キヤノン株式会社 光電変換素子、及びこれを用いた光エリアセンサ、撮像素子、撮像装置
EP3582275B1 (en) 2017-02-07 2023-09-06 Canon Kabushiki Kaisha Photoelectric conversion element, optical area sensor using same, imaging element, and imaging device
JP7086573B2 (ja) * 2017-11-17 2022-06-20 キヤノン株式会社 光電変換素子、及びこれを用いた光エリアセンサ、撮像素子、撮像装置
KR102250191B1 (ko) * 2017-03-06 2021-05-10 삼성전자주식회사 발광 장치
US10903438B2 (en) 2017-06-16 2021-01-26 Ubiquitous Energy, Inc. Visibly transparent, ultraviolet-absorbing photovoltaic devices
US11152581B2 (en) * 2017-06-16 2021-10-19 Ubiquitous Energy, Inc. Visibly transparent, near-infrared-absorbing donor/acceptor photovoltaic devices
CN110944986A (zh) * 2017-06-16 2020-03-31 无处不在能量公司 可见透明的近红外吸收性和紫外吸收性光伏装置
US11545635B2 (en) 2017-06-16 2023-01-03 Ubiquitous Energy, Inc. Visibly transparent, near-infrared-absorbing boron-containing photovoltaic devices
US11778896B2 (en) 2017-06-16 2023-10-03 Ubiquitous Energy, Inc. Visibly transparent, near-infrared-absorbing metal-complex photovoltaic devices
KR102235223B1 (ko) * 2017-11-28 2021-04-02 주식회사 엘지화학 광활성층 및 이를 포함하는 유기태양전지
CN108336231B (zh) * 2018-03-14 2021-08-27 南京邮电大学 一种宽光谱响应的有机光电探测器
CN108807683B (zh) * 2018-07-05 2021-04-30 南京邮电大学 一种宽光谱响应的倍增型有机光电探测器
JP7224158B2 (ja) * 2018-11-30 2023-02-17 住友化学株式会社 光電変換素子
CN114981277B (zh) * 2020-03-04 2024-06-11 株式会社Lg化学 化合物和包含其的光学膜
EP4012794B1 (en) * 2020-12-11 2026-03-04 Julius-Maximilians-Universität Würzburg Emission of electromagnetic radiation and control of properties of the emitted electromagnetic radiation
KR20240055181A (ko) * 2022-10-18 2024-04-29 삼성디스플레이 주식회사 유기 광다이오드 및 이를 포함하는 전자 장치

Family Cites Families (21)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
AU8783998A (en) * 1997-08-15 1999-03-08 Uniax Corporation Organic diodes with switchable photosensitivity
US6451415B1 (en) 1998-08-19 2002-09-17 The Trustees Of Princeton University Organic photosensitive optoelectronic device with an exciton blocking layer
US6352777B1 (en) 1998-08-19 2002-03-05 The Trustees Of Princeton University Organic photosensitive optoelectronic devices with transparent electrodes
US7332599B2 (en) * 2003-06-06 2008-02-19 North Carolina State University Methods and intermediates for the synthesis of dipyrrin-substituted porphyrinic macrocycles
US8357849B2 (en) 2004-09-22 2013-01-22 The Trustees Of Princeton University Organic photosensitive devices
DE102005010979A1 (de) 2005-03-04 2006-09-21 Technische Universität Dresden Photoaktives Bauelement mit organischen Schichten
US7230269B2 (en) 2005-06-13 2007-06-12 The Trustees Of Princeton University Organic photosensitive cells having a reciprocal-carrier exciton blocking layer
JP4238324B2 (ja) 2005-11-09 2009-03-18 国立大学法人北陸先端科学技術大学院大学 太陽電池
US20070272918A1 (en) 2006-05-25 2007-11-29 Barry Rand Organic photosensitive devices using subphthalocyanine compounds
JP2008109097A (ja) * 2006-09-28 2008-05-08 Toray Ind Inc 光起電力素子用材料および光起電力素子
JP5258037B2 (ja) * 2008-09-08 2013-08-07 国立大学法人京都大学 光電変換素子、その製造方法、及び太陽電池
US20100065112A1 (en) * 2008-09-15 2010-03-18 Thompson Mark E Organic Photosensitive Devices Comprising a Squaraine Containing Organoheterojunction and Methods of Making Same
WO2010036963A1 (en) * 2008-09-26 2010-04-01 The Regents Of The University Of Michigan Organic tandem solar cells
CN102282694B (zh) 2008-10-27 2015-02-25 密歇根大学董事会 倒置有机光敏器件
WO2010075512A1 (en) * 2008-12-23 2010-07-01 Michigan Technological University Polymers with bodipy-based backbone for solar cells
AU2010236973A1 (en) 2009-01-12 2011-08-11 The Regents Of The University Of Michigan Enhancement of organic photovoltaic cell open circuit voltage using electron/hole blocking exciton blocking layers
CN102473843A (zh) * 2009-08-04 2012-05-23 三菱化学株式会社 光电转换元件及使用该元件的太阳能电池
EP2385556B1 (de) * 2010-05-04 2021-01-20 Heliatek GmbH Photoaktives Bauelement mit organischen Schichten
CN105037246A (zh) 2011-02-09 2015-11-11 密歇根大学董事会 包含芳基方酸化合物的有机光敏器件及其制造方法
EP3751629B1 (en) 2011-02-21 2024-05-01 The Regents of the University of Michigan Organic photovoltaic cell incorporating electron conducting exciton blocking layers
CN102382117A (zh) * 2011-09-07 2012-03-21 四川大学 一类新型5，15-二烷基取代卟啉的制备及其在光电器件领域中应用

Also Published As

Publication number Publication date
JP6734315B2 (ja) 2020-08-05
TWI638476B (zh) 2018-10-11
JP2018121068A (ja) 2018-08-02
WO2014055976A1 (en) 2014-04-10
JP2015530761A (ja) 2015-10-15
EP2904649A1 (en) 2015-08-12
KR102160497B1 (ko) 2020-09-28
IN2015DN03049A (https=) 2015-10-02
KR20150060810A (ko) 2015-06-03
CA2887101A1 (en) 2014-04-10
US12239015B2 (en) 2025-02-25
TW201417378A (zh) 2014-05-01
EP2904649B1 (en) 2021-12-08
TW201916458A (zh) 2019-04-16
US20200203638A1 (en) 2020-06-25
IL238124A0 (en) 2015-05-31
AU2013326799A1 (en) 2015-04-30
TWI709265B (zh) 2020-11-01
CN104904028A (zh) 2015-09-09
US10367157B2 (en) 2019-07-30
US20150270501A1 (en) 2015-09-24

Similar Documents

Publication Publication Date Title
JP6734315B2 (ja) 有機光起電力におけるアクセプタおよびドナーのエネルギー感光化
AU2005271663B2 (en) Stacked organic photosensitive devices
US7196366B2 (en) Stacked organic photosensitive devices
JP7281216B2 (ja) 有機光起電装置のためのハイブリッド平面混合ヘテロ接合
US7326955B2 (en) Stacked organic photosensitive devices
KR20110069085A (ko) 스쿠아레인 함유 유기이종접합을 포함하는 유기 감광성 디바이스 및 이의 제조 방법
AU2011202560B2 (en) Stacked organic photosensitive devices

Legal Events

Date Code Title Description
A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20151016

A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20151016

A621 Written request for application examination

Free format text: JAPANESE INTERMEDIATE CODE: A621

Effective date: 20160906

A977 Report on retrieval

Free format text: JAPANESE INTERMEDIATE CODE: A971007

Effective date: 20170831

A131 Notification of reasons for refusal

Free format text: JAPANESE INTERMEDIATE CODE: A131

Effective date: 20170919

A601 Written request for extension of time

Free format text: JAPANESE INTERMEDIATE CODE: A601

Effective date: 20171013

A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20180319

TRDD Decision of grant or rejection written
A01 Written decision to grant a patent or to grant a registration (utility model)

Free format text: JAPANESE INTERMEDIATE CODE: A01

Effective date: 20180424

A61 First payment of annual fees (during grant procedure)

Free format text: JAPANESE INTERMEDIATE CODE: A61

Effective date: 20180517

R150 Certificate of patent or registration of utility model

Ref document number: 6342905

Country of ref document: JP

Free format text: JAPANESE INTERMEDIATE CODE: R150

R250 Receipt of annual fees

Free format text: JAPANESE INTERMEDIATE CODE: R250

R250 Receipt of annual fees

Free format text: JAPANESE INTERMEDIATE CODE: R250

R250 Receipt of annual fees

Free format text: JAPANESE INTERMEDIATE CODE: R250

R250 Receipt of annual fees

Free format text: JAPANESE INTERMEDIATE CODE: R250

LAPS Cancellation because of no payment of annual fees