JP2008179802A - ガス化触媒担持石炭の製造方法 - Google Patents
ガス化触媒担持石炭の製造方法 Download PDFInfo
- Publication number
- JP2008179802A JP2008179802A JP2007334081A JP2007334081A JP2008179802A JP 2008179802 A JP2008179802 A JP 2008179802A JP 2007334081 A JP2007334081 A JP 2007334081A JP 2007334081 A JP2007334081 A JP 2007334081A JP 2008179802 A JP2008179802 A JP 2008179802A
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- JP
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- Prior art keywords
- calcium
- coal
- biomass
- raw material
- gasification
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- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Pending
Links
- 239000003245 coal Substances 0.000 title claims abstract description 211
- 238000002309 gasification Methods 0.000 title claims abstract description 158
- 238000004519 manufacturing process Methods 0.000 title claims description 20
- 239000002028 Biomass Substances 0.000 claims abstract description 256
- 239000011575 calcium Substances 0.000 claims abstract description 160
- 229910052791 calcium Inorganic materials 0.000 claims abstract description 160
- OYPRJOBELJOOCE-UHFFFAOYSA-N Calcium Chemical compound [Ca] OYPRJOBELJOOCE-UHFFFAOYSA-N 0.000 claims abstract description 159
- 239000007788 liquid Substances 0.000 claims abstract description 140
- 239000002994 raw material Substances 0.000 claims abstract description 92
- 239000003054 catalyst Substances 0.000 claims abstract description 61
- 239000007864 aqueous solution Substances 0.000 claims abstract description 47
- AXCZMVOFGPJBDE-UHFFFAOYSA-L calcium dihydroxide Chemical compound [OH-].[OH-].[Ca+2] AXCZMVOFGPJBDE-UHFFFAOYSA-L 0.000 claims abstract description 45
- 239000000920 calcium hydroxide Substances 0.000 claims abstract description 43
- 229910001861 calcium hydroxide Inorganic materials 0.000 claims abstract description 43
- 230000002378 acidificating effect Effects 0.000 claims abstract description 42
- 239000000243 solution Substances 0.000 claims abstract description 32
- 239000010794 food waste Substances 0.000 claims abstract description 31
- 238000010000 carbonizing Methods 0.000 claims abstract description 25
- VTYYLEPIZMXCLO-UHFFFAOYSA-L Calcium carbonate Chemical compound [Ca+2].[O-]C([O-])=O VTYYLEPIZMXCLO-UHFFFAOYSA-L 0.000 claims description 50
- ODINCKMPIJJUCX-UHFFFAOYSA-N calcium oxide Inorganic materials [Ca]=O ODINCKMPIJJUCX-UHFFFAOYSA-N 0.000 claims description 27
- BRPQOXSCLDDYGP-UHFFFAOYSA-N calcium oxide Chemical compound [O-2].[Ca+2] BRPQOXSCLDDYGP-UHFFFAOYSA-N 0.000 claims description 26
- 239000000292 calcium oxide Substances 0.000 claims description 26
- 229910000019 calcium carbonate Inorganic materials 0.000 claims description 25
- 239000010883 coal ash Substances 0.000 claims description 8
- 238000006243 chemical reaction Methods 0.000 description 53
- 239000012738 dissolution medium Substances 0.000 description 35
- 238000000034 method Methods 0.000 description 32
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 28
- 241000196324 Embryophyta Species 0.000 description 27
- 239000000463 material Substances 0.000 description 24
- QTBSBXVTEAMEQO-UHFFFAOYSA-N Acetic acid Chemical compound CC(O)=O QTBSBXVTEAMEQO-UHFFFAOYSA-N 0.000 description 21
- 239000002956 ash Substances 0.000 description 21
- CURLTUGMZLYLDI-UHFFFAOYSA-N Carbon dioxide Chemical compound O=C=O CURLTUGMZLYLDI-UHFFFAOYSA-N 0.000 description 20
- 241000218645 Cedrus Species 0.000 description 20
- 241000209094 Oryza Species 0.000 description 20
- 235000007164 Oryza sativa Nutrition 0.000 description 20
- 235000009566 rice Nutrition 0.000 description 20
- 239000007789 gas Substances 0.000 description 19
- 235000017166 Bambusa arundinacea Nutrition 0.000 description 18
- 235000017491 Bambusa tulda Nutrition 0.000 description 18
- 241001330002 Bambuseae Species 0.000 description 18
- 235000015334 Phyllostachys viridis Nutrition 0.000 description 18
- 239000011425 bamboo Substances 0.000 description 18
- 239000010903 husk Substances 0.000 description 18
- 238000005259 measurement Methods 0.000 description 16
- OKKJLVBELUTLKV-UHFFFAOYSA-N Methanol Chemical compound OC OKKJLVBELUTLKV-UHFFFAOYSA-N 0.000 description 15
- 238000000926 separation method Methods 0.000 description 15
- 238000001035 drying Methods 0.000 description 14
- 230000000694 effects Effects 0.000 description 14
- 238000005470 impregnation Methods 0.000 description 14
- 238000010438 heat treatment Methods 0.000 description 11
- 238000010248 power generation Methods 0.000 description 11
- 239000001569 carbon dioxide Substances 0.000 description 10
- 229910002092 carbon dioxide Inorganic materials 0.000 description 10
- 238000002474 experimental method Methods 0.000 description 10
- 239000011269 tar Substances 0.000 description 10
- DGAQECJNVWCQMB-PUAWFVPOSA-M Ilexoside XXIX Chemical compound C[C@@H]1CC[C@@]2(CC[C@@]3(C(=CC[C@H]4[C@]3(CC[C@@H]5[C@@]4(CC[C@@H](C5(C)C)OS(=O)(=O)[O-])C)C)[C@@H]2[C@]1(C)O)C)C(=O)O[C@H]6[C@@H]([C@H]([C@@H]([C@H](O6)CO)O)O)O.[Na+] DGAQECJNVWCQMB-PUAWFVPOSA-M 0.000 description 9
- ZLMJMSJWJFRBEC-UHFFFAOYSA-N Potassium Chemical compound [K] ZLMJMSJWJFRBEC-UHFFFAOYSA-N 0.000 description 9
- 238000003763 carbonization Methods 0.000 description 9
- 238000002485 combustion reaction Methods 0.000 description 9
- 229910052700 potassium Inorganic materials 0.000 description 9
- 239000011591 potassium Substances 0.000 description 9
- 229910052708 sodium Inorganic materials 0.000 description 9
- 239000011734 sodium Substances 0.000 description 9
- 230000003197 catalytic effect Effects 0.000 description 8
- 230000008569 process Effects 0.000 description 8
- 239000007787 solid Substances 0.000 description 8
- KWYUFKZDYYNOTN-UHFFFAOYSA-M Potassium hydroxide Chemical compound [OH-].[K+] KWYUFKZDYYNOTN-UHFFFAOYSA-M 0.000 description 6
- HEMHJVSKTPXQMS-UHFFFAOYSA-M Sodium hydroxide Chemical compound [OH-].[Na+] HEMHJVSKTPXQMS-UHFFFAOYSA-M 0.000 description 6
- 238000001816 cooling Methods 0.000 description 6
- 239000000446 fuel Substances 0.000 description 6
- 239000000523 sample Substances 0.000 description 6
- 238000011068 loading method Methods 0.000 description 5
- 239000000843 powder Substances 0.000 description 5
- 238000000197 pyrolysis Methods 0.000 description 5
- CDBYLPFSWZWCQE-UHFFFAOYSA-L Sodium Carbonate Chemical compound [Na+].[Na+].[O-]C([O-])=O CDBYLPFSWZWCQE-UHFFFAOYSA-L 0.000 description 4
- 239000012300 argon atmosphere Substances 0.000 description 4
- 230000005587 bubbling Effects 0.000 description 4
- 239000011261 inert gas Substances 0.000 description 4
- BWHMMNNQKKPAPP-UHFFFAOYSA-L potassium carbonate Chemical compound [K+].[K+].[O-]C([O-])=O BWHMMNNQKKPAPP-UHFFFAOYSA-L 0.000 description 4
- 238000002360 preparation method Methods 0.000 description 4
- 230000009257 reactivity Effects 0.000 description 4
- 238000011084 recovery Methods 0.000 description 4
- 241000894007 species Species 0.000 description 4
- 238000005979 thermal decomposition reaction Methods 0.000 description 4
- 239000013585 weight reducing agent Substances 0.000 description 4
- MWUXSHHQAYIFBG-UHFFFAOYSA-N Nitric oxide Chemical compound O=[N] MWUXSHHQAYIFBG-UHFFFAOYSA-N 0.000 description 3
- 150000001339 alkali metal compounds Chemical class 0.000 description 3
- 238000009835 boiling Methods 0.000 description 3
- 239000003795 chemical substances by application Substances 0.000 description 3
- 235000013399 edible fruits Nutrition 0.000 description 3
- 125000000524 functional group Chemical group 0.000 description 3
- 230000006872 improvement Effects 0.000 description 3
- 238000005342 ion exchange Methods 0.000 description 3
- 239000000203 mixture Substances 0.000 description 3
- 239000002245 particle Substances 0.000 description 3
- XKRFYHLGVUSROY-UHFFFAOYSA-N Argon Chemical compound [Ar] XKRFYHLGVUSROY-UHFFFAOYSA-N 0.000 description 2
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 description 2
- VYPSYNLAJGMNEJ-UHFFFAOYSA-N Silicium dioxide Chemical compound O=[Si]=O VYPSYNLAJGMNEJ-UHFFFAOYSA-N 0.000 description 2
- QAOWNCQODCNURD-UHFFFAOYSA-N Sulfuric acid Chemical compound OS(O)(=O)=O QAOWNCQODCNURD-UHFFFAOYSA-N 0.000 description 2
- 239000002253 acid Substances 0.000 description 2
- -1 alkaline earth metal carbonates Chemical class 0.000 description 2
- OEERIBPGRSLGEK-UHFFFAOYSA-N carbon dioxide;methanol Chemical compound OC.O=C=O OEERIBPGRSLGEK-UHFFFAOYSA-N 0.000 description 2
- 125000003178 carboxy group Chemical group [H]OC(*)=O 0.000 description 2
- 150000003841 chloride salts Chemical class 0.000 description 2
- 238000010586 diagram Methods 0.000 description 2
- 229910001873 dinitrogen Inorganic materials 0.000 description 2
- 239000005457 ice water Substances 0.000 description 2
- 239000003960 organic solvent Substances 0.000 description 2
- 229910000027 potassium carbonate Inorganic materials 0.000 description 2
- 230000035484 reaction time Effects 0.000 description 2
- 230000009467 reduction Effects 0.000 description 2
- 230000008929 regeneration Effects 0.000 description 2
- 238000011069 regeneration method Methods 0.000 description 2
- 229910000029 sodium carbonate Inorganic materials 0.000 description 2
- 238000003746 solid phase reaction Methods 0.000 description 2
- 239000000126 substance Substances 0.000 description 2
- 230000004580 weight loss Effects 0.000 description 2
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 1
- GRYLNZFGIOXLOG-UHFFFAOYSA-N Nitric acid Chemical compound O[N+]([O-])=O GRYLNZFGIOXLOG-UHFFFAOYSA-N 0.000 description 1
- 239000012494 Quartz wool Substances 0.000 description 1
- 240000000111 Saccharum officinarum Species 0.000 description 1
- 235000007201 Saccharum officinarum Nutrition 0.000 description 1
- 244000269722 Thea sinensis Species 0.000 description 1
- 239000002250 absorbent Substances 0.000 description 1
- 230000002745 absorbent Effects 0.000 description 1
- 238000010521 absorption reaction Methods 0.000 description 1
- 239000012445 acidic reagent Substances 0.000 description 1
- 239000003929 acidic solution Substances 0.000 description 1
- 230000009471 action Effects 0.000 description 1
- 230000004931 aggregating effect Effects 0.000 description 1
- 229910052783 alkali metal Inorganic materials 0.000 description 1
- 150000008044 alkali metal hydroxides Chemical class 0.000 description 1
- 229910052784 alkaline earth metal Inorganic materials 0.000 description 1
- PNEYBMLMFCGWSK-UHFFFAOYSA-N aluminium oxide Inorganic materials [O-2].[O-2].[O-2].[Al+3].[Al+3] PNEYBMLMFCGWSK-UHFFFAOYSA-N 0.000 description 1
- 229910052786 argon Inorganic materials 0.000 description 1
- 239000012298 atmosphere Substances 0.000 description 1
- 238000009529 body temperature measurement Methods 0.000 description 1
- 150000001669 calcium Chemical class 0.000 description 1
- VSGNNIFQASZAOI-UHFFFAOYSA-L calcium acetate Chemical compound [Ca+2].CC([O-])=O.CC([O-])=O VSGNNIFQASZAOI-UHFFFAOYSA-L 0.000 description 1
- 239000001639 calcium acetate Substances 0.000 description 1
- 235000011092 calcium acetate Nutrition 0.000 description 1
- 229960005147 calcium acetate Drugs 0.000 description 1
- 150000004649 carbonic acid derivatives Chemical class 0.000 description 1
- 239000003610 charcoal Substances 0.000 description 1
- 239000007795 chemical reaction product Substances 0.000 description 1
- 239000003034 coal gas Substances 0.000 description 1
- 230000000052 comparative effect Effects 0.000 description 1
- 238000011109 contamination Methods 0.000 description 1
- 238000007796 conventional method Methods 0.000 description 1
- 238000005260 corrosion Methods 0.000 description 1
- 230000007797 corrosion Effects 0.000 description 1
- 230000007423 decrease Effects 0.000 description 1
- 238000007598 dipping method Methods 0.000 description 1
- TXKMVPPZCYKFAC-UHFFFAOYSA-N disulfur monoxide Inorganic materials O=S=S TXKMVPPZCYKFAC-UHFFFAOYSA-N 0.000 description 1
- 239000002737 fuel gas Substances 0.000 description 1
- 230000005484 gravity Effects 0.000 description 1
- 238000001027 hydrothermal synthesis Methods 0.000 description 1
- 125000002887 hydroxy group Chemical group [H]O* 0.000 description 1
- 238000000622 liquid--liquid extraction Methods 0.000 description 1
- 150000007522 mineralic acids Chemical class 0.000 description 1
- 238000012986 modification Methods 0.000 description 1
- 230000004048 modification Effects 0.000 description 1
- 229910017604 nitric acid Inorganic materials 0.000 description 1
- 239000012299 nitrogen atmosphere Substances 0.000 description 1
- 238000001556 precipitation Methods 0.000 description 1
- 239000000047 product Substances 0.000 description 1
- 238000004064 recycling Methods 0.000 description 1
- 239000013074 reference sample Substances 0.000 description 1
- 238000011160 research Methods 0.000 description 1
- 238000004904 shortening Methods 0.000 description 1
- 239000000377 silicon dioxide Substances 0.000 description 1
- 238000000638 solvent extraction Methods 0.000 description 1
- 239000011550 stock solution Substances 0.000 description 1
- 239000010902 straw Substances 0.000 description 1
- XTQHKBHJIVJGKJ-UHFFFAOYSA-N sulfur monoxide Chemical compound S=O XTQHKBHJIVJGKJ-UHFFFAOYSA-N 0.000 description 1
- 229910021381 transition metal chloride Inorganic materials 0.000 description 1
- 238000010792 warming Methods 0.000 description 1
- 239000002699 waste material Substances 0.000 description 1
Classifications
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E20/00—Combustion technologies with mitigation potential
- Y02E20/16—Combined cycle power plant [CCPP], or combined cycle gas turbine [CCGT]
- Y02E20/18—Integrated gasification combined cycle [IGCC], e.g. combined with carbon capture and storage [CCS]
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
- Y02P20/00—Technologies relating to chemical industry
- Y02P20/50—Improvements relating to the production of bulk chemicals
- Y02P20/52—Improvements relating to the production of bulk chemicals using catalysts, e.g. selective catalysts
Landscapes
- Catalysts (AREA)
Priority Applications (1)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| JP2007334081A JP2008179802A (ja) | 2006-12-27 | 2007-12-26 | ガス化触媒担持石炭の製造方法 |
Applications Claiming Priority (2)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| JP2006352184 | 2006-12-27 | ||
| JP2007334081A JP2008179802A (ja) | 2006-12-27 | 2007-12-26 | ガス化触媒担持石炭の製造方法 |
Publications (2)
| Publication Number | Publication Date |
|---|---|
| JP2008179802A true JP2008179802A (ja) | 2008-08-07 |
| JP2008179802A5 JP2008179802A5 (https=) | 2009-05-07 |
Family
ID=39723940
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| JP2007334081A Pending JP2008179802A (ja) | 2006-12-27 | 2007-12-26 | ガス化触媒担持石炭の製造方法 |
Country Status (1)
| Country | Link |
|---|---|
| JP (1) | JP2008179802A (https=) |
Cited By (4)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| WO2010109798A1 (ja) | 2009-03-25 | 2010-09-30 | 財団法人電力中央研究所 | ガス化システム及びガス化方法 |
| JP2013011377A (ja) * | 2011-06-28 | 2013-01-17 | Central Research Institute Of Electric Power Industry | 石炭燃焼方法及び石炭燃焼システム |
| WO2015010448A1 (zh) * | 2013-07-25 | 2015-01-29 | 易高环保能源研究院有限公司 | 一种由固体有机物水蒸气气化制取富氢气体的方法 |
| CN115404091A (zh) * | 2022-09-01 | 2022-11-29 | 西安石油大学 | 一种提高共热解焦气化反应性的方法 |
Citations (1)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| JPH0975890A (ja) * | 1995-09-08 | 1997-03-25 | Mitsubishi Heavy Ind Ltd | 石炭灰の処理方法 |
-
2007
- 2007-12-26 JP JP2007334081A patent/JP2008179802A/ja active Pending
Patent Citations (1)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| JPH0975890A (ja) * | 1995-09-08 | 1997-03-25 | Mitsubishi Heavy Ind Ltd | 石炭灰の処理方法 |
Non-Patent Citations (3)
| Title |
|---|
| JPN6013005444; 二宮善彦、外２名: 'バイオマスの部分酸化によって製造した酢酸カルシウムによる石炭の高温乾式脱硫に関する研究' 日本エネルギー学会石炭科学会議発表論文集 ｖｏｌ．４０, 20031023, ｐ．７４-７５, 日本エネルギー学会 * |
| JPN6013005445; Ｒｏｂｅｒｔ Ｊ． Ｌａｎｇ、Ｒｉｃｈａｒｄ Ｃ． Ｎｅａｖｅｌ: 'Ｂｅｈａｖｉｏｕｒ ｏｆ ｃａｌｃｉｕｍ ａｓ ａ ｓｔｅａｍ ｇａｓｉｆｉｃａｔｉｏｎｃａｔａｌｙｓｔ' ＦＵＥＬ ｖｏｌ．６１, 198207, ｐ．６２０-６２６, Ｅｌｓｅｖｉｅｒ * |
| JPN6013005447; 岸野正裕、外２名: 'ワンドアン炭急速熱分解チャ-の性状に対する穏和な前処理の効果' 日本エネルギー学会誌 ｖｏｌ．７６，Ｎｏ．５, 199705, ｐ．４０５-４１１, 日本エネルギー学会 * |
Cited By (9)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| WO2010109798A1 (ja) | 2009-03-25 | 2010-09-30 | 財団法人電力中央研究所 | ガス化システム及びガス化方法 |
| JP2010222517A (ja) * | 2009-03-25 | 2010-10-07 | Central Res Inst Of Electric Power Ind | ガス化システム及びガス化方法 |
| CN102227492A (zh) * | 2009-03-25 | 2011-10-26 | 财团法人电力中央研究所 | 气化系统及气化方法 |
| AU2010228721B2 (en) * | 2009-03-25 | 2013-06-27 | Central Research Institute Of Electric Power Industry | Gasification system and gasification process |
| JP2013011377A (ja) * | 2011-06-28 | 2013-01-17 | Central Research Institute Of Electric Power Industry | 石炭燃焼方法及び石炭燃焼システム |
| WO2015010448A1 (zh) * | 2013-07-25 | 2015-01-29 | 易高环保能源研究院有限公司 | 一种由固体有机物水蒸气气化制取富氢气体的方法 |
| US9809770B2 (en) | 2013-07-25 | 2017-11-07 | Eco Environmental Energy Research Institute Limited | Method for preparing hydrogen-rich gas by gasification of solid organic substance and steam |
| CN115404091A (zh) * | 2022-09-01 | 2022-11-29 | 西安石油大学 | 一种提高共热解焦气化反应性的方法 |
| CN115404091B (zh) * | 2022-09-01 | 2024-02-27 | 西安石油大学 | 一种提高共热解焦气化反应性的方法 |
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