ES8609156A1 - Un reactor para reformado de hidrocarburos - Google Patents

Un reactor para reformado de hidrocarburos

Info

Publication number
ES8609156A1
ES8609156A1 ES546154A ES546154A ES8609156A1 ES 8609156 A1 ES8609156 A1 ES 8609156A1 ES 546154 A ES546154 A ES 546154A ES 546154 A ES546154 A ES 546154A ES 8609156 A1 ES8609156 A1 ES 8609156A1
Authority
ES
Spain
Prior art keywords
reformer
heat transfer
enhanced heat
transfer reformer
hydrocarbons
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
ES546154A
Other languages
English (en)
Other versions
ES546154A0 (es
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Air Products and Chemicals Inc
Original Assignee
Air Products and Chemicals Inc
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Air Products and Chemicals Inc filed Critical Air Products and Chemicals Inc
Publication of ES546154A0 publication Critical patent/ES546154A0/es
Publication of ES8609156A1 publication Critical patent/ES8609156A1/es
Expired legal-status Critical Current

Links

Classifications

    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J8/00—Chemical or physical processes in general, conducted in the presence of fluids and solid particles; Apparatus for such processes
    • B01J8/02—Chemical or physical processes in general, conducted in the presence of fluids and solid particles; Apparatus for such processes with stationary particles, e.g. in fixed beds
    • B01J8/06—Chemical or physical processes in general, conducted in the presence of fluids and solid particles; Apparatus for such processes with stationary particles, e.g. in fixed beds in tube reactors; the solid particles being arranged in tubes
    • B01J8/067—Heating or cooling the reactor
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J8/00—Chemical or physical processes in general, conducted in the presence of fluids and solid particles; Apparatus for such processes
    • B01J8/02—Chemical or physical processes in general, conducted in the presence of fluids and solid particles; Apparatus for such processes with stationary particles, e.g. in fixed beds
    • B01J8/06—Chemical or physical processes in general, conducted in the presence of fluids and solid particles; Apparatus for such processes with stationary particles, e.g. in fixed beds in tube reactors; the solid particles being arranged in tubes
    • B01J8/062—Chemical or physical processes in general, conducted in the presence of fluids and solid particles; Apparatus for such processes with stationary particles, e.g. in fixed beds in tube reactors; the solid particles being arranged in tubes being installed in a furnace
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
    • C01B3/382—Multi-step processes
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
    • C01B3/384—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts the catalyst being continuously externally heated
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2208/00—Processes carried out in the presence of solid particles; Reactors therefor
    • B01J2208/00008—Controlling the process
    • B01J2208/00017—Controlling the temperature
    • B01J2208/00026—Controlling or regulating the heat exchange system
    • B01J2208/00035—Controlling or regulating the heat exchange system involving measured parameters
    • B01J2208/00088—Flow rate measurement
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2208/00—Processes carried out in the presence of solid particles; Reactors therefor
    • B01J2208/00008—Controlling the process
    • B01J2208/00017—Controlling the temperature
    • B01J2208/00106—Controlling the temperature by indirect heat exchange
    • B01J2208/00265—Part of all of the reactants being heated or cooled outside the reactor while recycling
    • B01J2208/00274—Part of all of the reactants being heated or cooled outside the reactor while recycling involving reactant vapours
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2208/00—Processes carried out in the presence of solid particles; Reactors therefor
    • B01J2208/00008—Controlling the process
    • B01J2208/00017—Controlling the temperature
    • B01J2208/00106—Controlling the temperature by indirect heat exchange
    • B01J2208/00309—Controlling the temperature by indirect heat exchange with two or more reactions in heat exchange with each other, such as an endothermic reaction in heat exchange with an exothermic reaction
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2208/00—Processes carried out in the presence of solid particles; Reactors therefor
    • B01J2208/00008—Controlling the process
    • B01J2208/00017—Controlling the temperature
    • B01J2208/00477—Controlling the temperature by thermal insulation means
    • B01J2208/00495—Controlling the temperature by thermal insulation means using insulating materials or refractories
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2208/00—Processes carried out in the presence of solid particles; Reactors therefor
    • B01J2208/00008—Controlling the process
    • B01J2208/00017—Controlling the temperature
    • B01J2208/00504—Controlling the temperature by means of a burner
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2208/00—Processes carried out in the presence of solid particles; Reactors therefor
    • B01J2208/00008—Controlling the process
    • B01J2208/00017—Controlling the temperature
    • B01J2208/0053—Controlling multiple zones along the direction of flow, e.g. pre-heating and after-cooling
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08—Methods of heating or cooling
    • C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0811—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08—Methods of heating or cooling
    • C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0811—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel
    • C01B2203/0816—Heating by flames
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08—Methods of heating or cooling
    • C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0811—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel
    • C01B2203/0822—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel the fuel containing hydrogen
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08—Methods of heating or cooling
    • C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0811—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel
    • C01B2203/0827—Methods of heating the process for making hydrogen or synthesis gas by combustion of fuel at least part of the fuel being a recycle stream
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08—Methods of heating or cooling
    • C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0838—Methods of heating the process for making hydrogen or synthesis gas by heat exchange with exothermic reactions, other than by combustion of fuel
    • C01B2203/0844—Methods of heating the process for making hydrogen or synthesis gas by heat exchange with exothermic reactions, other than by combustion of fuel the non-combustive exothermic reaction being another reforming reaction as defined in groups C01B2203/02 - C01B2203/0294
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08—Methods of heating or cooling
    • C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0866—Methods of heating the process for making hydrogen or synthesis gas by combination of different heating methods
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/14—Details of the flowsheet
    • C01B2203/141—At least two reforming, decomposition or partial oxidation steps in parallel
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/14—Details of the flowsheet
    • C01B2203/146—At least two purification steps in series
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00—Technologies relating to chemical industry
    • Y02P20/10—Process efficiency

Abstract

EQUIPO PARA EL REFORMADO DE HIDROCARBUROS, FORMADO POR TUBOS RELLENOS DE CATALIZADOR UNICO, EN EL QUE SE UTILIZA EL CALOR PRODUCIDO EN LA REACCION PARA EFECTUAR EL REFORMADO DE LOS HIDROCARBUROS QUE PASAN A TRAVES DEL REFORMADOR. EL REACTOR TIENE UNA CARCASA EXTERIOR CON UNA ENTRADA PARA EL REACCIONANTE, UNA PARA EL PRODUCTO Y UNA SALIDA PARA EL PRODUCTO, VARIOS TUBOS DE REACCION RELLENOS DE CATALIZADOR DE REFORMADO Y UN MEDIO DE INTERCAMBIO DE CALOR QUE PUEDE ESTAR CONSTITUIDO POR TUBOS DE ALETAS, ANILLOS RASCHIG, BOLAS DE CERAMICA O BOLAS DE UNA COMPOSICION DE ALUMINIO. SE PRODUCE MENOR VAPOR DE AGUA EN EL METODO CONVENCIONAL.
ES546154A 1984-08-16 1985-08-14 Un reactor para reformado de hidrocarburos Expired ES8609156A1 (es)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US06/641,819 US4919844A (en) 1984-08-16 1984-08-16 Enhanced heat transfer reformer and method

Publications (2)

Publication Number Publication Date
ES546154A0 ES546154A0 (es) 1986-09-01
ES8609156A1 true ES8609156A1 (es) 1986-09-01

Family

ID=24573973

Family Applications (2)

Application Number Title Priority Date Filing Date
ES546154A Expired ES8609156A1 (es) 1984-08-16 1985-08-14 Un reactor para reformado de hidrocarburos
ES551793A Expired ES8706566A1 (es) 1984-08-16 1986-02-10 Un metodo para reformar hidrocarburos.

Family Applications After (1)

Application Number Title Priority Date Filing Date
ES551793A Expired ES8706566A1 (es) 1984-08-16 1986-02-10 Un metodo para reformar hidrocarburos.

Country Status (6)

Country Link
US (1) US4919844A (es)
EP (1) EP0171786B1 (es)
JP (1) JPS6158801A (es)
KR (1) KR890001963B1 (es)
DE (1) DE3576678D1 (es)
ES (2) ES8609156A1 (es)

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US5202057A (en) * 1988-09-14 1993-04-13 Air Products And Chemicals, Inc. Production of ammonia synthesis gas
US5164163A (en) * 1988-09-19 1992-11-17 Kabushiki Kaisha Kobe Seiko Sho Hydrocarbon reforming apparatus
US5068058A (en) * 1989-05-04 1991-11-26 Air Products And Chemicals, Inc. Production of ammonia synthesis gas
US5112012A (en) * 1989-10-26 1992-05-12 Yuan Mark S Tilting momentum wheel for spacecraft
GB9000389D0 (en) * 1990-01-08 1990-03-07 Ici Plc Steam reforming
CA2054260A1 (en) * 1990-11-01 1992-05-02 Gregory D. Snyder Combined prereformer and convetive heat transfer reformer
US5264202A (en) * 1990-11-01 1993-11-23 Air Products And Chemicals, Inc. Combined prereformer and convective heat transfer reformer
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US6114400A (en) * 1998-09-21 2000-09-05 Air Products And Chemicals, Inc. Synthesis gas production by mixed conducting membranes with integrated conversion into liquid products
US6641625B1 (en) 1999-05-03 2003-11-04 Nuvera Fuel Cells, Inc. Integrated hydrocarbon reforming system and controls
DE19954871A1 (de) * 1999-09-07 2001-03-15 Caloric Anlagenbau Gmbh Verfahren zur Wasserstofferzeugung
US6397790B1 (en) 2000-04-03 2002-06-04 R. Kirk Collier, Jr. Octane enhanced natural gas for internal combustion engine
US6508209B1 (en) 2000-04-03 2003-01-21 R. Kirk Collier, Jr. Reformed natural gas for powering an internal combustion engine
US6405720B1 (en) 2000-04-03 2002-06-18 R. Kirk Collier, Jr. Natural gas powered engine
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KR100445183B1 (ko) * 2001-11-29 2004-08-21 주식회사 경동도시가스 플레이트형 수증기 개질장치
US20030162846A1 (en) 2002-02-25 2003-08-28 Wang Shoou-L Process and apparatus for the production of synthesis gas
US6739125B1 (en) 2002-11-13 2004-05-25 Collier Technologies, Inc. Internal combustion engine with SCR and integrated ammonia production
US6796369B1 (en) 2003-04-04 2004-09-28 Air Products And Chemicals, Inc. Method and apparatus to prevent metal dusting
JP4603251B2 (ja) * 2003-08-07 2010-12-22 千代田化工建設株式会社 水蒸気改質炉
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JP4477432B2 (ja) * 2004-06-29 2010-06-09 東洋エンジニアリング株式会社 改質器
BRPI0515031A (pt) * 2004-09-09 2008-07-01 Haldor Topsoe As processo para produção de gás rico em hidrogênio e/ou monóxido de carbono e processo para a preparação de metanol a partir de matéria-prima de hidrocarboneto gasoso ou lìquido
GB0508740D0 (en) * 2005-04-29 2005-06-08 Johnson Matthey Plc Steam reforming
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US7501078B2 (en) * 2007-01-10 2009-03-10 Air Products And Chemicals, Inc. Process for generating synthesis gas using catalyzed structured packing
US8287815B2 (en) * 2008-05-02 2012-10-16 General Electric Company Methods and systems for controlling temperature in a vessel
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US8287763B2 (en) 2010-10-28 2012-10-16 Air Products And Chemicals, Inc. Steam-hydrocarbon reforming with limited steam export
FR2979257B1 (fr) * 2011-08-26 2013-08-16 Ifp Energies Now Reacteur echangeur pour la production d'hydrogene avec faisceau de generation vapeur integre
US8545775B2 (en) * 2011-10-20 2013-10-01 Kellogg Brown & Root Llc Reforming exchanger system with intermediate shift conversion
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ITUB20150576A1 (it) * 2015-04-24 2016-10-24 Hexsol Italy Srl Scambiatore di calore a fascio tubiero e struttura perfezionata
CN105295967B (zh) * 2015-11-12 2017-12-26 盐城工学院 一种高湿碳基原料外热式热解反应器
EP3551576A1 (en) 2016-12-08 2019-10-16 Technip France Scalable heat exchanger reformer for syngas production
RU2664063C1 (ru) * 2017-08-08 2018-08-14 Публичное акционерное общество "Нефтяная компания "Роснефть" (ПАО "НК "Роснефть") Способ переработки природного/попутного газа в синтез-газ автотермическим риформингом
RU2664138C1 (ru) * 2017-08-08 2018-08-15 Публичное акционерное общество "Нефтяная компания "Роснефть" (ПАО "НК "Роснефть") Компактный реактор для получения синтез-газа из природного/попутного газа в процессе автотермического риформинга
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Also Published As

Publication number Publication date
EP0171786A2 (en) 1986-02-19
DE3576678D1 (de) 1990-04-26
JPS6158801A (ja) 1986-03-26
KR860001868A (ko) 1986-03-24
EP0171786B1 (en) 1990-03-21
US4919844A (en) 1990-04-24
ES551793A0 (es) 1987-07-01
ES546154A0 (es) 1986-09-01
ES8706566A1 (es) 1987-07-01
KR890001963B1 (ko) 1989-06-05
EP0171786A3 (en) 1987-01-07

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