EP0244433A1 - Verfahren zum trennen und rückgewinnen von metallen aus mischungen metallischer schwefelverbindungen, wie bleierzen - Google Patents

Verfahren zum trennen und rückgewinnen von metallen aus mischungen metallischer schwefelverbindungen, wie bleierzen

Info

Publication number
EP0244433A1
EP0244433A1 EP86905847A EP86905847A EP0244433A1 EP 0244433 A1 EP0244433 A1 EP 0244433A1 EP 86905847 A EP86905847 A EP 86905847A EP 86905847 A EP86905847 A EP 86905847A EP 0244433 A1 EP0244433 A1 EP 0244433A1
Authority
EP
European Patent Office
Prior art keywords
lead
solution
silver
metals
mixture
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
EP86905847A
Other languages
English (en)
French (fr)
Inventor
Patrick Noual
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Extramet SA
Original Assignee
Extramet SA
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Extramet SA filed Critical Extramet SA
Publication of EP0244433A1 publication Critical patent/EP0244433A1/de
Ceased legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C25ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25CPROCESSES FOR THE ELECTROLYTIC PRODUCTION, RECOVERY OR REFINING OF METALS; APPARATUS THEREFOR
    • C25C1/00Electrolytic production, recovery or refining of metals by electrolysis of solutions
    • C25C1/18Electrolytic production, recovery or refining of metals by electrolysis of solutions of lead
    • CCHEMISTRY; METALLURGY
    • C22METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
    • C22BPRODUCTION AND REFINING OF METALS; PRETREATMENT OF RAW MATERIALS
    • C22B13/00Obtaining lead
    • C22B13/04Obtaining lead by wet processes
    • CCHEMISTRY; METALLURGY
    • C22METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
    • C22BPRODUCTION AND REFINING OF METALS; PRETREATMENT OF RAW MATERIALS
    • C22B3/00Extraction of metal compounds from ores or concentrates by wet processes
    • C22B3/04Extraction of metal compounds from ores or concentrates by wet processes by leaching
    • C22B3/06Extraction of metal compounds from ores or concentrates by wet processes by leaching in inorganic acid solutions, e.g. with acids generated in situ; in inorganic salt solutions other than ammonium salt solutions
    • C22B3/10Hydrochloric acid, other halogenated acids or salts thereof
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02PCLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P10/00Technologies related to metal processing
    • Y02P10/20Recycling

Definitions

  • the present invention relates to a new process for treating mixtures of metal sulfides which facilitates the recovery of different metals by selective precipitation, because it previously ensures the simultaneous dissolution of the different sulfides corresponding to a single operation.
  • the conditions suitable for the dissolution of all the metals to be recovered, in particular in the treatment of natural lead ores, are met in particular the oxidizing nature of the attack solution is provided by the redox couple suitably chosen from the known redox couples.
  • the other metals which may be present in the initial mixture of sulphides it is in particular possible to successively extract the copper, iron and zinc from the sulphide attack filtrate, by proceeding by displacement using iron and / or metallic zinc to precipitate the copper, possibly present, then after filtration, by precipitation of the iron possibly present in the filtrate, with sodium hydroxide and air bubbling then, after filtration of the goethite formed, by precipitation with sulphide sodium or hydrogen sulphide of the zinc possibly present and filtration of the zinc sulphide formed.
  • the hydrogen sulfide used there can be obtained from the residue.
  • the attack solution of the mixture of sulphides contains a minimal amount, even a trace, of hydrochloric acid, and if for a sulphide concentration of 90 to 100 g / l for example, it contains from 80 to 100 g / l of fluosilicic acid and 30 to 40 g / l of nitric acid, 10 to 50 g / l of ferric iron.
  • FIG. 1 The succession of the different stages of the process, completed in a particular implementation mode, is illustrated by FIG. 1.
  • the leaching stage is shown diagrammatically in 1, at which level a sulfur concentrate to be treated is admitted in 2.
  • the oxidizing agent, with recirculation in 4 an aqueous hydrochloric acid solution and in 5 air, optionally enriched in oxygen. Fluosilicic acid is recycled at this stage in 6.
  • a precipitate is recovered by filtration. which is subjected in 8 to a step of dissolution with a hydrochloric solution of fluosilicic acid and of calcium chloride recirculated in 9.
  • the precipitate formed is separated, which contains calcium sulphate, sulfur and residues d attack of sulphides, the assembly being eliminated at 11.
  • the collected solution is subjected at 12 to a displacement step with lead introduced at 13 and the precipitated silver is collected at 14.
  • the remaining filtrate is treated by electrolysis at 15 so as to collect the lead at 16, while the electrolysis is recycled to the dissolving step at 8.
  • the filtrate separated from the sulfates at 7 is treated at 17 by displacement of the copper by means of iron and / or zinc introduced in 18, according to methods which are in themselves conventional, the precipitated copper being recovered in 19.
  • the filtrate is then subjected to a precipitation step in 20 by means of a solution of soda 21, under air bubbling 22, which makes it possible to cause the precipitation of iron by techniques in themselves conventional, which is collected at 23.
  • a subsequent precipitation, carried out at 24 by means of hydrogen sulfide at 25, allows the precipitation of zinc, collected at 26 in the form of zinc sulfide.
  • the filtrate is reused in leaching step 1.
  • the progress of the reaction is checked by taking samples after 30, 60, 90, 120 and 240 minutes.
  • the etching solution contains only 0.17 g / l of copper.
  • the recovery of the attack precipitate consisting mainly of lead sulphate (Pb SO 4 ) with calcium chloride in a fluosilicic acid medium gives a solution containing 25 g / l of lead, which can be treated for recovery of lead , especially by electrolysis.
  • Pb SO 4 lead sulphate
  • the solution contains 112.5 g / l of dissolved lead, 80 g / l of fluosilicic acid and 320 g / l of calcium chloride.
  • the anode compartment contains only an aqueous solution containing 400 g / l of fluosicilic acid.
  • Electrolysis is carried out at 30 ° C. at 3.29 volts and 0.27 amperes with a stainless steel cathode of

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Electrochemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Inorganic Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Environmental & Geological Engineering (AREA)
  • General Life Sciences & Earth Sciences (AREA)
  • Geochemistry & Mineralogy (AREA)
  • Geology (AREA)
  • Manufacture And Refinement Of Metals (AREA)
  • Electrolytic Production Of Metals (AREA)
EP86905847A 1985-09-27 1986-09-26 Verfahren zum trennen und rückgewinnen von metallen aus mischungen metallischer schwefelverbindungen, wie bleierzen Ceased EP0244433A1 (de)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
FR8514325A FR2589885B1 (fr) 1985-09-27 1985-09-27 Procede de separation et de recuperation de metaux, dans des melanges de sulfures metalliques, tels que des minerais de plomb
FR8514325 1985-09-27

Publications (1)

Publication Number Publication Date
EP0244433A1 true EP0244433A1 (de) 1987-11-11

Family

ID=9323299

Family Applications (1)

Application Number Title Priority Date Filing Date
EP86905847A Ceased EP0244433A1 (de) 1985-09-27 1986-09-26 Verfahren zum trennen und rückgewinnen von metallen aus mischungen metallischer schwefelverbindungen, wie bleierzen

Country Status (9)

Country Link
EP (1) EP0244433A1 (de)
JP (1) JPS63501023A (de)
AU (1) AU586507B2 (de)
BR (1) BR8606886A (de)
ES (1) ES2001803A6 (de)
FR (1) FR2589885B1 (de)
MA (1) MA20776A1 (de)
PT (1) PT83433B (de)
WO (1) WO1987002068A1 (de)

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US7902472B2 (en) 2006-02-09 2011-03-08 Siemens Aktiengesellschaft Arrangement, in particular, for activating a transport pawl and clamping device for a spring energy store of an electric switch comprising such an arrangement

Families Citing this family (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2636939B1 (fr) * 1988-09-06 1991-08-30 Inst Nat Rech Chimique Procede perfectionne d'obtention de composes de ta et (ou) nb exempts d'impuretes a partir de materiaux contenant ces metaux
IT201800003369A1 (it) * 2018-03-08 2019-09-08 Engitec Tech S P A Procedimento per recuperare il piombo da un pastello di piombo e relativo uso in un procedimento di recupero dei componenti di accumulatori al piombo-acido.
WO2020110198A1 (ja) * 2018-11-27 2020-06-04 株式会社ジェーエフシーテック 鉛の製造方法および製造設備
CN111705216B (zh) * 2020-06-16 2021-12-03 云南锡业股份有限公司锡业分公司 一种焊锡电解阳极泥的处理工艺

Family Cites Families (13)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR320097A (fr) * 1902-04-01 1902-12-01 Betts Perfectionnements dans et relatifs au raffinage électrolytique du plomb et des alliages de plomb
FR1474663A (fr) * 1966-04-06 1967-03-24 Electrolyt Zinc Australasia Procédé d'extraction de métaux
US4026776A (en) * 1970-12-02 1977-05-31 Mitsui Mining & Smelting Co., Ltd. Method for producing high purity lead
US3960681A (en) * 1974-02-21 1976-06-01 Mitsui Mining & Smelting Co., Ltd. Method for producing electrolytic high purity lead using large-sized electrodes
NZ181123A (en) * 1975-06-30 1979-12-11 Univ Melbourne Treatment of mineralcontaining materials with an acid in the presence of fluoride ion
US3972790A (en) * 1975-09-26 1976-08-03 Uop Inc. Production of metallic lead
US4189461A (en) * 1977-11-30 1980-02-19 Kennecott Copper Corporation Metal leaching from concentrates using nitrogen dioxide in acids
FR2446863A1 (fr) * 1979-01-22 1980-08-14 Uop Inc Procede perfectionne de recuperation de plomb
FR2453906A1 (fr) * 1979-04-12 1980-11-07 Uop Inc Procede de preparation hydrometallurgique de plomb a l'aide d'une extraction par voie electrochimique
US4229271A (en) * 1979-05-24 1980-10-21 Rsr Corporation Method of recovering lead values from battery sludge
FR2505876A1 (en) * 1981-05-12 1982-11-19 Noual Patrick Selective winning of lead from sulphide ores - by leaching with hot aq. hydro:fluorosilicic acid soln. contg. hydrogen peroxide and air so only lead is dissolved
FI850334L (fi) * 1983-05-25 1985-01-25 Oa Brand Pty Limited Foerfarande foer extrahering av metaller ur malm.
US4500398A (en) * 1984-06-20 1985-02-19 The United States Of America As Represented By The Secretary Of The Interior Production of lead from sulfides

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
See references of WO8702068A1 *

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US7902472B2 (en) 2006-02-09 2011-03-08 Siemens Aktiengesellschaft Arrangement, in particular, for activating a transport pawl and clamping device for a spring energy store of an electric switch comprising such an arrangement

Also Published As

Publication number Publication date
BR8606886A (pt) 1987-11-03
PT83433B (fr) 1988-01-08
FR2589885B1 (fr) 1988-01-15
AU6405186A (en) 1987-04-24
MA20776A1 (fr) 1987-04-01
FR2589885A1 (fr) 1987-05-15
AU586507B2 (en) 1989-07-13
ES2001803A6 (es) 1988-06-16
JPS63501023A (ja) 1988-04-14
PT83433A (fr) 1986-10-01
WO1987002068A1 (fr) 1987-04-09

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Inventor name: NOUAL, PATRICK