DK2161076T3 - Fremgangsmåde til selektiv hydrogenering under anvendelse af en sulfidkatalysator med en specifik sammensætning - Google Patents

Fremgangsmåde til selektiv hydrogenering under anvendelse af en sulfidkatalysator med en specifik sammensætning Download PDF

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DK2161076T3
DK2161076T3 DK09290579.3T DK09290579T DK2161076T3 DK 2161076 T3 DK2161076 T3 DK 2161076T3 DK 09290579 T DK09290579 T DK 09290579T DK 2161076 T3 DK2161076 T3 DK 2161076T3
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catalyst
metal
group vib
group viii
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Maxime Montillet
Elodie Devers
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Ifp Energies Now
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    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper
    • B01J23/76—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
    • B01J23/84—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36 with arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
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    • C10G45/00—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
    • C10G45/02—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing
    • C10G45/04—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used
    • C10G45/06—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used containing nickel or cobalt metal, or compounds thereof
    • C10G45/08—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used containing nickel or cobalt metal, or compounds thereof in combination with chromium, molybdenum, or tungsten metals, or compounds thereof
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    • C10G45/00—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
    • C10G45/02—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing
    • C10G45/04—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used
    • C10G45/06—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used containing nickel or cobalt metal, or compounds thereof
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    • B01J23/16—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
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    • B01J23/76—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
    • B01J23/84—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36 with arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • B01J23/85—Chromium, molybdenum or tungsten
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    • C10G45/00—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
    • C10G45/02—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing
    • C10G45/04—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used
    • C10G45/12—Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds to eliminate hetero atoms without changing the skeleton of the hydrocarbon involved and without cracking into lower boiling hydrocarbons; Hydrofinishing characterised by the catalyst used containing crystalline alumino-silicates, e.g. molecular sieves
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    • B01J21/00—Catalysts comprising the elements, oxides, or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium, or hafnium
    • B01J21/02—Boron or aluminium; Oxides or hydroxides thereof
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    • B—PERFORMING OPERATIONS; TRANSPORTING
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    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
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    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
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    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2400/00—Products obtained by processes covered by groups C10G9/00 - C10G69/14
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  • Materials Engineering (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • General Chemical & Material Sciences (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Catalysts (AREA)
  • Production Of Liquid Hydrocarbon Mixture For Refining Petroleum (AREA)
  • Low-Molecular Organic Synthesis Reactions Using Catalysts (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Claims (15)

1. Fremgangsmåde til selektiv hydrogenering af polyumættede forbindelser til monoumættede forbindelser, som samtidigt gør det muligt at gøre lette, mættede svovlholdige forbindelser tungere ved reaktion med de umættede forbindelser, der er indeholdt i FCC-benzin, hvilken fremgangsmåde anvender en katalysator, der indeholder mindst et gruppe VIb-metal og mindst ikke-ædelt gruppe Vlll-metal afsat på en bærer, og i hvilken • vægtindholdet af oxid af gruppe VIb-grundstoffet ligger på mellem 4 og 20 %, • vægtindholdet af oxid af gruppe VIII-grundstoffet er lavere end 15 vægt-%, • sulfideringsgraden af metallerne, der udgør katalysatoren, er højere end 80 %, • molforholdet mellem det ikke-ædle gruppe Vlll-metal og gruppe VIb-metallet ligger på mellem 1,0 og 2,5 mol/mol, • tætheden af gruppe VIb-grundstof pr. overfladeenhed af katalysatoren er strengt lavere end 7.10-4 gram oxider af gruppe VIb-grundstof pr. m2 katalysator.
2. Fremgangsmåde ifølge krav 1, hvor katalysatoren omfatter et gruppe VIb-metal valgt blandt molybden og wolfram.
3. Fremgangsmåde ifølge krav 2, hvor gruppe VIb-metallet er molybden.
4. Fremgangsmåde ifølge krav 1, hvor katalysatoren omfatter et ikke-ædelt gruppe Vlll-metal valgt blandt nikkel, cobalt og j ern.
5. Fremgangsmåde ifølge krav 4, hvor det ikke-ædle gruppe Vlll-metal er nikkel.
6. Fremgangsmåde ifølge et af de foregående krav, hvor katalysatoren omfatter et vægtindhold af oxid af gruppe VIII-grundstoffet på mellem 1 og 10 vægt-%. Ί. Fremgangsmåde ifølge krav 1, hvor molforholdet mellem det ikke-ædle gruppe VIII-metal og gruppe VIb-metallet ligger på mellem 1 og 2 mol/mol.
8. Fremgangsmåde ifølge et af de foregående krav, hvor katalysatoren har et totalt porevolumen på over 0,3 cm3/g.
9. Fremgangsmåde ifølge krav 8, hvor katalysatoren har et totalt porevolumen på mellem 0,4 cm3/g og 1,4 cm3/g.
10. Fremgangsmåde ifølge et af de foregående krav, hvor katalysatorens specifikke overflade er mindre end 300 m2/g.
11. Fremgangsmåde ifølge krav 1, hvor katalysatorens bærer er et porøst metaloxid valgt blandt aluminiumoxid, silica, siliciumcarbid og en blanding af disse oxider.
12. Fremgangsmåde ifølge krav 11, hvor katalysatorens bærer er udgjort af rent aluminiumoxid.
13. Fremgangsmåde ifølge et af kravene 11 eller 12, hvor bæreren er udgjort af kubisk gamma-aluminiumoxid eller delta-aluminiumoxid.
14. Fremgangsmåde ifølge et af kravene 11 til 13, hvor katalysatorens bærer har et totalt porevolumen på mellem 0,4 og 1,4 cm3/g.
15. Fremgangsmåde ifølge krav 14, hvor katalysatorens bærer har et porevolumen på mellem 0,5 og 1,3 cm3/g.
16. Fremgangsmåde til selektiv hydrogenering ifølge et af de foregående krav, hvor føden bringes i kontakt med katalysatoren ved en temperatur på mellem 80 °C og 220 °C, en flydende rumhastighed på mellem 1 h_1 og 10 h_1 og et tryk på mellem 0,5 og 5 MPa.
DK09290579.3T 2008-09-04 2009-07-21 Fremgangsmåde til selektiv hydrogenering under anvendelse af en sulfidkatalysator med en specifik sammensætning DK2161076T3 (da)

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FR0804842A FR2935389B1 (fr) 2008-09-04 2008-09-04 Procede d'hydrogenation selective mettant en oeuvre un catalyseur sulfure de composition specifique

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EP (1) EP2161076B1 (da)
JP (1) JP5563259B2 (da)
KR (1) KR101668481B1 (da)
CN (2) CN106867575A (da)
BR (1) BRPI0902949B1 (da)
DK (1) DK2161076T3 (da)
FR (1) FR2935389B1 (da)
SG (1) SG159489A1 (da)
TW (1) TWI492788B (da)

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CN103145516B (zh) 2011-12-06 2015-01-21 中国石油天然气股份有限公司 一种使不饱和化合物选择加氢的方法
FR2986799B1 (fr) 2012-02-15 2015-02-06 IFP Energies Nouvelles Procede de conversion d'une charge lourde, mettant en oeuvre une unite de craquage catalytique et une etape d'hydrogenation selective de l'essence issue du craquage catalytique
FR2988732B1 (fr) 2012-03-29 2015-02-06 IFP Energies Nouvelles Procede d'hydrogenation selective d'une essence
FR2993569B1 (fr) * 2012-07-17 2015-12-04 IFP Energies Nouvelles Procede de desulfuration d'une essence
FR2997415B1 (fr) * 2012-10-29 2015-10-02 IFP Energies Nouvelles Procede de production d'une essence a basse teneur en soufre
FR3014896B1 (fr) 2013-12-18 2018-07-27 IFP Energies Nouvelles Procede d'hydrodesulfuration de coupes d'hydrocarbures
FR3030563B1 (fr) * 2014-12-18 2018-06-29 IFP Energies Nouvelles Procede d'adoucissement en composes du type sulfure d'une essence olefinique
FR3035117B1 (fr) 2015-04-15 2019-04-19 IFP Energies Nouvelles Procede d'adoucissement en composes du type sulfure d'une essence olefinique
US9828093B2 (en) * 2015-05-27 2017-11-28 First Principles, Inc. System for recharging remotely controlled aerial vehicle, charging station and rechargeable remotely controlled aerial vehicle, and method of use thereof
US9714012B1 (en) 2016-01-22 2017-07-25 International Business Machines Corporation Power source element replacement during vehicle operation
FR3049955B1 (fr) 2016-04-08 2018-04-06 IFP Energies Nouvelles Procede de traitement d'une essence
FR3057578B1 (fr) 2016-10-19 2018-11-16 IFP Energies Nouvelles Procede d'hydrodesulfuration d'une essence olefinique.
FR3109899B1 (fr) 2020-05-07 2023-11-24 Ifp Energies Now Catalyseur d’hydrogénation comprenant un support et un ratio NiMo spécifique
FR3109897B1 (fr) 2020-05-07 2023-11-24 Ifp Energies Now Catalyseur d’hydrogénation sélective comprenant un support spécifique en partie sous forme aluminate

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KR20100028502A (ko) 2010-03-12
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JP5563259B2 (ja) 2014-07-30
TWI492788B (zh) 2015-07-21
EP2161076B1 (fr) 2018-04-25
BRPI0902949B1 (pt) 2022-09-20
CN106867575A (zh) 2017-06-20
TW201016318A (en) 2010-05-01
FR2935389B1 (fr) 2012-05-11
JP2010090366A (ja) 2010-04-22
FR2935389A1 (fr) 2010-03-05

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