DE112004000920B8 - Protonenleitende Membran enthaltend ein Copolymerisationsprodukt aus mindestens einem ersten Silan und einem zweiten Silan und deren Verwendung, sowie Silanverbindung und Verfahren zu deren Herstellung - Google Patents

Protonenleitende Membran enthaltend ein Copolymerisationsprodukt aus mindestens einem ersten Silan und einem zweiten Silan und deren Verwendung, sowie Silanverbindung und Verfahren zu deren Herstellung Download PDF

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Publication number
DE112004000920B8
DE112004000920B8 DE112004000920.0T DE112004000920T DE112004000920B8 DE 112004000920 B8 DE112004000920 B8 DE 112004000920B8 DE 112004000920 T DE112004000920 T DE 112004000920T DE 112004000920 B8 DE112004000920 B8 DE 112004000920B8
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Germany
Prior art keywords
silane
proton
preparation
membrane containing
conducting membrane
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Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
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DE112004000920.0T
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English (en)
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DE112004000920B4 (de
DE112004000920T5 (de
Inventor
Siwen Li
Meilin Liu
Qunhui Sun
Wen Li
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Toyota Motor Corp
Georgia Tech Research Corp
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Toyota Technical Center USA Inc
Georgia Tech Research Institute
Georgia Tech Research Corp
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Publication of DE112004000920B8 publication Critical patent/DE112004000920B8/de
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Expired - Fee Related legal-status Critical Current

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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D71/00—Semi-permeable membranes for separation processes or apparatus characterised by the material; Manufacturing processes specially adapted therefor
    • B01D71/06—Organic material
    • B01D71/70—Polymers having silicon in the main chain, with or without sulfur, nitrogen, oxygen or carbon only
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D67/00—Processes specially adapted for manufacturing semi-permeable membranes for separation processes or apparatus
    • B01D67/0002—Organic membrane manufacture
    • B01D67/0006—Organic membrane manufacture by chemical reactions
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D67/00—Processes specially adapted for manufacturing semi-permeable membranes for separation processes or apparatus
    • B01D67/0039—Inorganic membrane manufacture
    • B01D67/0044—Inorganic membrane manufacture by chemical reaction
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D67/00—Processes specially adapted for manufacturing semi-permeable membranes for separation processes or apparatus
    • B01D67/0039—Inorganic membrane manufacture
    • B01D67/0048—Inorganic membrane manufacture by sol-gel transition
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D71/00—Semi-permeable membranes for separation processes or apparatus characterised by the material; Manufacturing processes specially adapted therefor
    • B01D71/06—Organic material
    • B01D71/76—Macromolecular material not specifically provided for in a single one of groups B01D71/08 - B01D71/74
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D71/00—Semi-permeable membranes for separation processes or apparatus characterised by the material; Manufacturing processes specially adapted therefor
    • B01D71/06—Organic material
    • B01D71/76—Macromolecular material not specifically provided for in a single one of groups B01D71/08 - B01D71/74
    • B01D71/78—Graft polymers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/04—Polysiloxanes
    • C08G77/38—Polysiloxanes modified by chemical after-treatment
    • C08G77/382—Polysiloxanes modified by chemical after-treatment containing atoms other than carbon, hydrogen, oxygen or silicon
    • C08G77/392—Polysiloxanes modified by chemical after-treatment containing atoms other than carbon, hydrogen, oxygen or silicon containing sulfur
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218—Synthetic macromolecular compounds
    • C08J5/2256—Synthetic macromolecular compounds based on macromolecular compounds obtained by reactions other than those involving carbon-to-carbon bonds, e.g. obtained by polycondensation
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L83/00—Compositions of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon only; Compositions of derivatives of such polymers
    • C08L83/04—Polysiloxanes
    • C08L83/08—Polysiloxanes containing silicon bound to organic groups containing atoms other than carbon, hydrogen and oxygen
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1037—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having silicon, e.g. sulfonated crosslinked polydimethylsiloxanes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1072—Polymeric electrolyte materials characterised by the manufacturing processes by chemical reactions, e.g. insitu polymerisation or insitu crosslinking
    • H01M8/1074—Sol-gel processes
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D2323/00—Details relating to membrane preparation
    • B01D2323/30—Cross-linking
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D2325/00—Details relating to properties of membranes
    • B01D2325/26—Electrical properties
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2379/00—Characterised by the use of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing nitrogen with or without oxygen, or carbon only, not provided for in groups C08J2361/00 - C08J2377/00
    • C08J2379/04—Polycondensates having nitrogen-containing heterocyclic rings in the main chain; Polyhydrazides; Polyamide acids or similar polyimide precursors
    • C08J2379/06—Polyhydrazides; Polytriazoles; Polyamino-triazoles; Polyoxadiazoles
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0082—Organic polymers
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0088—Composites
    • H01M2300/0091—Composites in the form of mixtures
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • General Chemical & Material Sciences (AREA)
  • Inorganic Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Dispersion Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Electrochemistry (AREA)
  • Materials Engineering (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Conductive Materials (AREA)
  • Silicon Polymers (AREA)
  • Fuel Cell (AREA)
  • Manufacture Of Macromolecular Shaped Articles (AREA)
  • Separation Using Semi-Permeable Membranes (AREA)
DE112004000920.0T 2003-05-28 2004-05-28 Protonenleitende Membran enthaltend ein Copolymerisationsprodukt aus mindestens einem ersten Silan und einem zweiten Silan und deren Verwendung, sowie Silanverbindung und Verfahren zu deren Herstellung Expired - Fee Related DE112004000920B8 (de)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
US47395703P 2003-05-28 2003-05-28
US60/473,957 2003-05-28
PCT/US2004/016897 WO2004107477A2 (en) 2003-05-28 2004-05-28 Conductive membranes formed from silanes having functional groups

Publications (3)

Publication Number Publication Date
DE112004000920T5 DE112004000920T5 (de) 2008-03-13
DE112004000920B4 DE112004000920B4 (de) 2019-04-11
DE112004000920B8 true DE112004000920B8 (de) 2019-05-29

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DE112004000920.0T Expired - Fee Related DE112004000920B8 (de) 2003-05-28 2004-05-28 Protonenleitende Membran enthaltend ein Copolymerisationsprodukt aus mindestens einem ersten Silan und einem zweiten Silan und deren Verwendung, sowie Silanverbindung und Verfahren zu deren Herstellung

Country Status (5)

Country Link
US (1) US7851580B2 (de)
JP (1) JP5085132B2 (de)
CN (1) CN1809606B (de)
DE (1) DE112004000920B8 (de)
WO (1) WO2004107477A2 (de)

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US7576165B2 (en) 2004-01-27 2009-08-18 Georgia Institute Of Technology Heterocycle grafted monomers and related polymers and hybrid inorganic-organic polymer membranes
US7259230B2 (en) * 2004-06-07 2007-08-21 Battelle Energy Alliance, Llc Polybenzimidazole compounds, polymeric media, and methods of post-polymerization modifications
JP2006244920A (ja) * 2005-03-04 2006-09-14 Fujitsu Ltd 固体電解質組成物および高分子型燃料電池
US8043762B2 (en) * 2005-07-15 2011-10-25 Jsr Corporation Polyphenylene-containing electrode paste
DE102005044433A1 (de) * 2005-09-16 2007-03-22 Universität Bremen Katalytisch aktive Zusammensetzung, Membran-Elektroden-Einheit mit der Zusammensetzung und Katalysator mit/aus der Zusammensetzung
KR101193164B1 (ko) 2006-02-21 2012-10-19 삼성에스디아이 주식회사 술폰산기 함유 유기 고분자 실록산 화합물 및 이를포함하는 연료전지
CN100518914C (zh) * 2006-10-27 2009-07-29 中国科学技术大学 有机-无机杂化阴离子交换膜的制备方法
US7964651B2 (en) * 2006-12-21 2011-06-21 Toyota Motor Engineering & Manufacturing North America, Inc. Sulfonyl grafted heterocycle materials for proton conducting electrolytes
US10788608B2 (en) 2007-08-12 2020-09-29 Toyota Jidosha Kabushiki Kaisha Non-color shifting multilayer structures
US10690823B2 (en) 2007-08-12 2020-06-23 Toyota Motor Corporation Omnidirectional structural color made from metal and dielectric layers
US10870740B2 (en) 2007-08-12 2020-12-22 Toyota Jidosha Kabushiki Kaisha Non-color shifting multilayer structures and protective coatings thereon
US10048415B2 (en) 2007-08-12 2018-08-14 Toyota Motor Engineering & Manufacturing North America, Inc. Non-dichroic omnidirectional structural color
US8586259B2 (en) 2008-05-29 2013-11-19 Georgia Tech Research Corporation Proton exchange membranes based on heterocycles and acids through an organic-inorganic hybrid process
US7947410B2 (en) 2008-08-22 2011-05-24 Toyota Motor Engineering & Manufacturing North America, Inc. Fuel cell electrodes with triazole modified polymers and membrane electrode assemblies incorporating same
KR101746868B1 (ko) * 2009-03-31 2017-06-14 도레이 카부시키가이샤 복합 반투막 및 그의 제조 방법
JP5750436B2 (ja) 2010-05-14 2015-07-22 株式会社Kri 修飾金属酸化物ゾル
JP2014009190A (ja) * 2012-06-29 2014-01-20 Shikoku Chem Corp イミダゾールシラン化合物、合成方法及びその利用
US9658375B2 (en) 2012-08-10 2017-05-23 Toyota Motor Engineering & Manufacturing North America, Inc. Omnidirectional high chroma red structural color with combination metal absorber and dielectric absorber layers
US9664832B2 (en) 2012-08-10 2017-05-30 Toyota Motor Engineering & Manufacturing North America, Inc. Omnidirectional high chroma red structural color with combination semiconductor absorber and dielectric absorber layers
US9678260B2 (en) 2012-08-10 2017-06-13 Toyota Motor Engineering & Manufacturing North America, Inc. Omnidirectional high chroma red structural color with semiconductor absorber layer
DE112015001639B4 (de) 2014-04-01 2023-12-14 Toyota Jidosha Kabushiki Kaisha Nicht-farbverschiebende mehrschichtige strukturen
WO2016011412A1 (en) 2014-07-17 2016-01-21 Ada Technologies, Inc. Extreme long life, high energy density batteries and method of making and using the same
US9810824B2 (en) 2015-01-28 2017-11-07 Toyota Motor Engineering & Manufacturing North America, Inc. Omnidirectional high chroma red structural colors
WO2016209460A2 (en) 2015-05-21 2016-12-29 Ada Technologies, Inc. High energy density hybrid pseudocapacitors and method of making and using the same
WO2017023797A1 (en) 2015-07-31 2017-02-09 Ada Technologies, Inc. High energy and power electrochemical device and method of making and using same
FR3041350B1 (fr) * 2015-09-21 2019-05-10 Commissariat A L'energie Atomique Et Aux Energies Alternatives Electrolyte solide pour generateur electrochimique
US11024846B2 (en) 2017-03-23 2021-06-01 Ada Technologies, Inc. High energy/power density, long cycle life, safe lithium-ion battery capable of long-term deep discharge/storage near zero volt and method of making and using the same

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EP0054426A2 (de) * 1980-12-15 1982-06-23 M & T Chemicals, Inc. Siloxane
US5283310A (en) * 1991-09-13 1994-02-01 Saint-Gobain Vitrage International Proton conducting polymer, and application thereof as electrolyte in electrochemical devices
US6310110B1 (en) * 1999-07-30 2001-10-30 Michael A. Markowitz Molecularly-imprinted material made by template-directed synthesis
US6531539B2 (en) * 2000-04-08 2003-03-11 Degussa Ag Organosilicon compounds
US6390102B1 (en) * 2000-07-14 2002-05-21 General Electric Company Silicone compositions for personal care products and method for making
US6713643B2 (en) * 2001-05-24 2004-03-30 Board Of Trustees Of Michigan State University Ultrastable organofunctional microporous to mesoporous silica compositions

Also Published As

Publication number Publication date
JP2007504637A (ja) 2007-03-01
US7851580B2 (en) 2010-12-14
CN1809606A (zh) 2006-07-26
JP5085132B2 (ja) 2012-11-28
CN1809606B (zh) 2010-10-27
WO2004107477A2 (en) 2004-12-09
US20070099035A1 (en) 2007-05-03
WO2004107477A3 (en) 2005-02-10
DE112004000920B4 (de) 2019-04-11
DE112004000920T5 (de) 2008-03-13

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