CN115590238A

CN115590238A - Cigarette additive with herb fragrance and preparation method and application thereof

Info

Publication number: CN115590238A
Application number: CN202211376052.XA
Authority: CN
Inventors: 曹毅; 叶远青; 钱建财; 赵才能; 朱怀远; 秦艳华; 伍鹏霖
Original assignee: China Tobacco Jiangsu Industrial Co Ltd
Current assignee: China Tobacco Jiangsu Industrial Co Ltd
Priority date: 2022-11-04
Filing date: 2022-11-04
Publication date: 2023-01-13

Abstract

The invention provides a cigarette additive with a medicinal herb fragrance, and a preparation method and application thereof. The cigarette additive with the herbal fragrance provided by the invention has the effects of inducing resuscitation, relieving pain, relieving cough, eliminating phlegm, clearing lung, moistening dryness, clearing heat, detoxifying and the like, and can effectively relieve symptoms of throat discomfort, lung dryness, excessive phlegm and the like of consumers caused by smoking. The cigarette additive with the medicinal herb aroma provided by the invention is applied to cigarette formula tobacco shreds, can soften smoke, harmonize the tobacco aroma, has remarkable style characteristics, can obviously sense the medicinal herb aroma and the tobacco aroma, has the effects of resuscitation inducing, body fluid production promoting, sweetening, cough relieving and lung moistening, can meet the physiological requirements of consumers on cigarette products, and can play a health care role on the consumers.

Description

Cigarette additive with herb fragrance and preparation method and application thereof

Technical Field

The invention belongs to the technical field of tobacco, and particularly relates to a cigarette additive with a medicinal and herbal aroma and a preparation method and application thereof.

Background

The tobacco leaf is used as the main raw material of cigarette and is derived from the leaf of Nicotiana tabacum L. According to records in the Chinese herbal medicine assembly, the tobacco is warm in nature, sweet in taste and toxic, has the effects of reducing swelling, detoxifying and killing insects and is mainly used for treating symptoms such as furuncle, pyogenic infection, tinea capitis, tinea alba, tinea capitis, venomous snake bite and the like. Modern pharmacological research finds that the traditional Chinese medicine composition has good effects on the central nervous system, such as refreshing, calming and the like. From the point of view of the classification and initial application of tobacco, tobacco is homologous to Chinese herbs. The tobacco is a special Chinese herbal medicine, and according to history, the tobacco is applied to treating diseases at first and gradually develops into a hobby product in human life later. Therefore, the tobacco and the Chinese herbal medicine are communicated, the traditional effects confirmed by the Chinese herbal medicine can be fully utilized, the advantage that the Chinese herbal medicine has fragrance is brought into play, and the tobacco smoking quality is improved by adding the Chinese herbal medicine into the tobacco.

The Chinese herbal medicine contains substances with aromatic odor such as volatile oil, and multiple polysaccharide moisture-keeping components, and can increase fragrance and reduce discomfort after smoking when added into tobacco. The medicinal and edible Chinese herbal medicine has rich resources and different properties and flavor effects, is unique to China, contains thousands of years of health preserving ideas and practical experiences of Chinese nations, and has the functions of preventing and treating diseases and rehabilitation and health care.

Patent CN106235393A provides a traditional Chinese medicine extract additive for cigarette, which is used in combination with flos Eriocauli, semen Fagopyri Esculenti, folium Mori, fructus Cannabis, flos Sophorae Immaturus, semen Oroxyli, herba Eupatorii, and radix Asteris in the formula, and can reduce the content of harmful substances such as ammonia, phenol, carbon monoxide and nitrosamine in mainstream smoke and reduce the influence on human health in the process of smoking cigarette.

In patent CN106418659A, puffball, sword bean and other Chinese medicinal materials are adopted to be compatible with taurine, sodium glutamate, radix tetrastigme, sodium aluminosilicate and ethyl p-hydroxybenzoate, and the prepared composite additive can increase the fragrance of the tobacco sheet, reduce miscellaneous gas and irritation, is moderate in strength and comfortable in aftertaste, and obviously improves the smoking quality of the tobacco sheet.

The patent CN106868926A combines the agilawood powder and the mint leaf powder together to be used as a traditional Chinese medicine composition for preparing the cigarette paper, so that the cigarette paper has cool fragrance, smoke released by the cigarette paper in the combustion process can be smooth and tense, the health care cigarette has the advantages of making people feel happy, helping sleep, playing a good health care role, enriching the fragrance in the smoke, increasing the smoke concentration, coordinating and reducing the miscellaneous gas and reducing the irritation.

The Chinese herbal medicine has the treatment and health care effects, and can provide unique fragrance and lasting appeal simultaneously. The reasonable construction of the Chinese herbal medicine compound, effective extraction of key components and harmony of cigarette aroma are the key points for developing cigarettes with herb aroma.

Disclosure of Invention

Aiming at the defects of the prior art, the invention aims to provide a cigarette additive with a medicinal herb fragrance and a preparation method and application thereof. The cigarette additive with the aroma of the medicinal herbs provided by the invention has the health-care effects of inducing resuscitation, relieving pain, relieving cough, eliminating phlegm, clearing lung, moistening dryness, clearing heat, detoxifying and the like for smokers.

In order to achieve the purpose, the invention adopts the following technical scheme:

in a first aspect, the invention provides a cigarette additive with a medicinal herb aroma, which is prepared from Chinese herbal medicine compound extracts and a flavoring liquid, wherein the Chinese herbal medicine compound extracts are prepared from platycodon grandiflorum, mulberry leaves, epimedium and dogbane leaves.

In the invention, the mass ratio of the Chinese herbal medicine compound extract to the flavoring liquid is (8-9.9): (2-0.1) (wherein, 8-9.9 can be 8, 8.3, 8.6, 8.9, 9, 9.2, 9.4, 9.6, 9.8, 9.9, etc., and 2-0.1 can be 2, 1.5, 1.3, 1, 0.5, 0.3, 0.1, etc.).

In the invention, the raw materials for preparing the Chinese herbal medicine compound extract comprise, by weight, 10-25 parts of platycodon grandiflorum (for example, 10 parts, 12 parts, 14 parts, 16 parts, 18 parts, 20 parts, 22 parts, 24 parts, 25 parts and the like), 1-7 parts of mulberry leaves (for example, 1 part, 2 parts, 3 parts, 4 parts, 5 parts, 6 parts, 7 parts and the like), 10-25 parts of epimedium (for example, 10 parts, 12 parts, 14 parts, 16 parts, 18 parts, 20 parts, 22 parts, 24 parts, 25 parts and the like), and 1-3 parts of dogbane leaves (for example, 1 part, 1.5 parts, 2 parts, 2.5 parts, 3 parts and the like).

In the invention, the raw materials for preparing the Chinese herbal medicine compound extract also comprise any one or the combination of at least two of green tangerine orange peel, albizia flower, airpotato yam rhizome, perilla leaf or ligusticum chuanxiong hort.

In the invention, the raw materials for preparing the Chinese herbal medicine compound extract also comprise green tangerine orange peel, albizia flower, airpotato yam rhizome, perilla leaf and ligusticum chuanxiong hort.

Preferably, the raw materials for preparing the Chinese herbal medicine compound extract further include, by weight, 9-25 parts of pericarpium citri reticulatae viride (for example, 9 parts, 10 parts, 13 parts, 16 parts, 19 parts, 22 parts, 25 parts, etc.), 1-7 parts of flos albiziae (for example, 1 part, 2 parts, 3 parts, 4 parts, 5 parts, 6 parts, 7 parts, etc.), 1-5 parts of airpotato yam (for example, 1 part, 2 parts, 3 parts, 4 parts, 5 parts, etc.), 1-3 parts of perilla leaf (for example, 1 part, 1.5 parts, 2 parts, 2.5 parts, 3 parts, etc.), and 8-45 parts of ligusticum chuanxiong hort (for example, 8 parts, 10 parts, 15 parts, 20 parts, 25 parts, 30 parts, 35 parts, 40 parts, 45 parts, etc.).

The functions of the components of the Chinese herbal medicine compound are as follows:

and (3) platycodon root: has effects in dispersing lung qi, clearing away heat and toxic materials, expelling phlegm, relieving cough, and expelling pus;

mulberry leaf: has good effects of dispelling wind heat, clearing liver heat, moistening lung dryness, etc.;

herba epimedii: it enters liver and kidney meridians due to its warm nature. Has effects in invigorating kidney, supporting yang, protecting cardiovascular system, and preventing anemia;

and (3) dogbane leaf: has effects of suppressing hyperactive liver, tranquilizing mind, clearing heat, promoting diuresis, and lowering blood pressure and blood lipid.

Albizzia flower: has effects in relieving depression, tranquilizing mind, regulating qi, stimulating appetite, activating collaterals, relieving pain, and clearing away summer-heat;

green tangerine peel: has effects of dispersing stagnated liver qi, relieving qi stagnation, and removing blood stasis;

ligusticum wallichii: has effects in promoting blood circulation, dispelling blood stasis, expelling pathogenic wind, and relieving pain;

radix Polygoni Ciliinerve: has effects in removing toxic materials, relieving swelling, dissipating phlegm, resolving masses, cooling blood, and stopping bleeding;

perilla leaf: dispelling cold, dispersing lung qi, promoting qi circulation, and eliminating phlegm.

In the invention, the flavoring liquid comprises any one of or a combination of at least two of sage oil, vetiver oil, eucalyptol, storax extract or thyme oil.

Preferably, the flavoring liquid comprises sage oil, vetiver oil, eucalyptol, storax extract and thyme oil.

Preferably, the flavoring liquid comprises 2-20 parts (such as 2 parts, 5 parts, 8 parts, 11 parts, 14 parts, 17 parts, 20 parts and the like) of sage oil, 2-15 parts (such as 2 parts, 5 parts, 8 parts, 11 parts, 13 parts, 15 parts and the like) of vetiver oil, 10-40 parts (such as 10 parts, 15 parts, 20 parts, 25 parts, 30 parts, 35 parts, 40 parts and the like) of cineole, 12-30 parts (such as 12 parts, 15 parts, 18 parts, 20 parts, 23 parts, 26 parts, 29 parts, 30 parts and the like) of storax extract and 20-50 parts (such as 20 parts, 25 parts, 30 parts, 35 parts, 40 parts, 45 parts, 50 parts and the like) of red thyme oil by weight.

In a second aspect, the present invention provides a method for preparing the cigarette additive with herbal aroma according to the first aspect, wherein the preparation method comprises the following steps: extracting each Chinese herbal medicine raw material of the Chinese herbal medicine compound to obtain a Chinese herbal medicine compound extract; and then mixing the Chinese herbal medicine compound extract with the flavoring liquid to obtain the cigarette additive with the herbal medicine fragrance.

In the present invention, the extraction solvent used for the extraction includes an aqueous ethanol solution.

Preferably, the volume ratio of ethanol to water in the ethanol aqueous solution is (3-9): 1 (wherein, "3-9" can be 3, 4, 5, 6, 7, 8, 9, etc.).

Preferably, the solid-to-liquid ratio of the Chinese herbal medicine compound and the extraction solvent is 1 (3-6) g/mL (wherein, 3-6 can be 3, 4, 5, 6, etc.).

In the invention, the extraction mode comprises any one of ultrasonic heating extraction, heating reflux extraction or distillation condensation extraction.

Preferably, the extraction temperature is 70-90 deg.C (such as 70 deg.C, 73 deg.C, 76 deg.C, 79 deg.C, 83 deg.C, 86 deg.C, 89 deg.C, 90 deg.C, etc.), and the extraction time is 3-10h (such as 3h, 4h, 5h, 6h, 7h, 8h, 9h, 10h, etc.).

Preferably, the Chinese herbal medicine raw materials are ground before extraction, and the grain size of the Chinese herbal medicine powder obtained after grinding is 40-100 meshes (for example, 40 meshes, 50 meshes, 60 meshes, 70 meshes, 80 meshes, 90 meshes, 100 meshes and the like can be obtained).

Preferably, centrifugation is carried out after the extraction, and supernatant is collected to obtain the Chinese herbal medicine compound extract.

Preferably, the rotation speed of the centrifugation is 6000-10000rpm (such as 6000rpm, 7000rpm, 8000rpm, 9000rpm, 10000rpm, etc.), and the time of the centrifugation is 3-15min (such as 3min, 5min, 7min, 9min, 11min, 13min, 15min, etc.).

Preferably, the mixing further comprises a polyol comprising any one of glycerol, 1,2-propanediol, or 1,3-butanediol, or a combination of at least two.

Preferably, the volume ratio of the sum of the volumes of the Chinese herbal medicine compound extract and the flavoring liquid to the polyol is 1 (0.5-2) (wherein, the '0.5-2' can be 0.5, 0.7, 0.9, 1.1, 1.3, 1.5, 1.7, 1.9, 2, etc.).

In a third aspect, the invention provides a cigarette comprising cut tobacco and the cigarette additive with herbal aroma of the first aspect.

Preferably, the cigarette additive with the herb note accounts for 0.05-0.5% (for example, 0.05%, 0.1%, 0.2%, 0.3%, 0.4%, 0.5%, etc.) of the total mass of the cut tobacco.

Preferably, the preparation raw materials of the tobacco shreds comprise Yunnan tobacco leaves, fujian tobacco leaves, guizhou tobacco leaves, hunan tobacco leaves, zimbabwe tobacco leaves and Argentina tobacco leaves.

In the invention, the tobacco shreds with a specific formula are matched with the cigarette additive with the herb fragrance, so that the cigarette has more obvious herb fragrance.

Preferably, the mass ratio of the Yunnan tobacco leaves, the Fujian tobacco leaves, the Guizhou tobacco leaves, the Hunan tobacco leaves, the Zimbabwe tobacco leaves and the Argentina tobacco leaves is (3.5-4.5): (1.5-2.5): (0.5-1.5): (0.2-0.7);

wherein "3.5-4.5" can be 3.5, 3.7, 3.9, 4.1, 4.3, 4.5, etc.;

"1.5-2.5" can be 1.5, 1.7, 1.9, 2.1, 2.3, 2.5, etc.;

"0.5-1.5" can be 0.5, 0.7, 0.9, 1.1, 1.3, 1.5, etc.;

"0.2-0.7" may be 0.2, 0.3, 0.4, 0.5, 0.6, 0.7, etc.

Preferably, the cigarette is prepared by the following method, and the method comprises the following steps: and spraying the cigarette additive on tobacco shreds, and matching with cigarette paper, tipping paper and a filter tip to obtain the cigarette.

According to the normal cigarette production process, the tobacco shreds sprayed with the cigarette additives are matched with cigarette materials such as cigarette paper, tipping paper, filter tips and the like to prepare cigarettes by using cigarette production equipment, so that the cigarettes are obtained.

Compared with the prior art, the invention has the following beneficial effects:

1. the cigarette additive with the aroma of the medicinal herbs provided by the invention has the effects of inducing resuscitation, relieving pain, relieving cough, eliminating phlegm, clearing lung, moistening dryness, clearing heat, detoxifying and the like, and can effectively relieve symptoms of throat discomfort, lung dryness, excessive phlegm and the like caused by smoking of consumers.

2. The cigarette additive with the herbal aroma provided by the invention is applied to cigarette formula tobacco shreds, has the advantages of soft smoke, harmonious tobacco aroma, obvious style characteristics, obvious perception of the herbal aroma and the tobacco aroma, and the effects of resuscitation inducing, body fluid production promoting, sweet returning, cough relieving and lung moistening, and can meet the physiological requirements of consumers on cigarette products and play a role in health care for the consumers. The cigarette additive with the herb fragrance provided by the invention has important practical significance for accelerating scientific and technological progress of the tobacco industry, fully exploiting functions and applications of Chinese herbal medicines and improving cigarette brand value.

Detailed Description

The technical solution of the present invention is further explained by the following embodiments. It should be understood by those skilled in the art that the examples are only for the understanding of the present invention and should not be construed as the specific limitations of the present invention.

The following examples each component of the flavoring solution (sage oil, vetiver oil, eucalyptol, storax extract and thyme oil) was purchased from Zhengzhou tobacco institute.

Example 1

The embodiment provides a cigarette additive with a herbal aroma, and the preparation method of the cigarette additive with the herbal aroma comprises the following steps:

(1) After 2.0g of platycodon grandiflorum, 0.2g of mulberry leaf, 0.2g of albizia flower, 1.8g of green tangerine peel, 2.0g of epimedium herb, 1.6g of ligusticum wallichii, 0.2g of airpotato yam rhizome, 0.2g of perilla leaf and 0.2g of dogbane leaf are mixed, the obtained Chinese herbal medicine compound is fully ground to prepare 40-mesh Chinese herbal medicine compound powder.

(2) Uniformly mixing the Chinese herbal medicine compound powder obtained in the step (1) with 75% ethanol water solution according to the solid-to-liquid ratio of 1:3, and carrying out ultrasonic heating extraction at the water bath temperature of 70 ℃ for 3h. Centrifuging the extracted mixed solution at 6000r/min for 10min, and collecting supernatant to obtain Chinese herbal medicine compound extract.

(3) Uniformly mixing 0.1g of sage oil, 0.05g of vetiver oil, 0.3g of cineole, 0.26g of storax extract and 0.47g of thyme oil to obtain the flavoring liquid.

(4) And (3) uniformly mixing the Chinese herbal medicine compound extract obtained in the step (2) with the flavoring liquid obtained in the step (3) according to the mass ratio of 8:2, and then uniformly mixing with glycerol according to the volume ratio of 1.

Example 2

The embodiment provides a cigarette additive with a medicinal herb flavor, and a preparation method of the cigarette additive with the medicinal herb flavor comprises the following steps:

(1) After 3.6g of platycodon grandiflorum, 1.4g of mulberry leaf, 1.4g of albizia flower, 3.2g of green tangerine peel, 4.0g of epimedium herb, 9.0g of ligusticum wallichii, 1.0g of airpotato yam rhizome, 0.6g of perilla leaf and 0.6g of dogbane leaf are mixed, the obtained Chinese herbal medicine compound is fully ground to prepare 60-mesh Chinese herbal medicine compound powder.

(2) Uniformly mixing the Chinese herbal medicine compound powder obtained in the step (1) with 80% ethanol water solution according to the solid-to-liquid ratio of 1:4, heating and refluxing for extraction, wherein the water bath temperature is 80 ℃, and the extraction time is 5 hours. Centrifuging the extracted mixed solution at 8000r/min for 5min, and collecting supernatant to obtain Chinese medicinal compound extract.

(3) Uniformly mixing 0.2g of sage oil, 0.1g of vetiver oil, 0.35g of cineole, 0.2g of storax extract and 0.5g of thyme oil to obtain the flavoring liquid.

(4) And (3) uniformly mixing the Chinese herbal medicine compound extract obtained in the step (2) with the flavoring liquid obtained in the step (3) according to the mass ratio of 9:1, and then uniformly mixing the mixture with 1,3-butanediol according to the volume ratio of 1:1 to obtain the cigarette additive with the aroma of the herbal medicines.

Example 3

(1) After 3.0g of platycodon grandiflorum, 1.0g of mulberry leaf, 1.0g of albizia flower, 3.0g of green tangerine peel, 3.0g of epimedium herb, 8.0g of ligusticum wallichii, 0.6g of airpotato yam rhizome, 0.4g of perilla leaf and 0.4g of dogbane leaf are mixed, the obtained Chinese herbal medicine compound is fully ground to prepare the 80-mesh Chinese herbal medicine compound powder.

(2) Uniformly mixing the Chinese herbal medicine compound powder obtained in the step (1) with 85% ethanol water solution according to the solid-to-liquid ratio of 1:5, heating and refluxing for extraction, wherein the water bath temperature is 85 ℃, and the extraction time is 8 hours. Centrifuging the extracted mixed solution at 10000r/min for 3min, and collecting supernatant to obtain Chinese herbal medicine compound extract.

(3) Uniformly mixing 0.15g of sage oil, 0.15g of vetiver oil, 0.2g of cineole, 0.3g of storax extract and 0.4g of thyme oil to obtain the flavoring liquid.

(4) And (3) uniformly mixing the Chinese herbal medicine compound extract obtained in the step (2) with the flavoring liquid obtained in the step (3) according to the mass ratio of 9.9.

Example 4

(1) 2.5g of platycodon grandiflorum, 0.8g of mulberry leaf, 0.8g of albizia julibrissin, 2.4g of green tangerine peel, 2.5g of epimedium herb, 5.0g of ligusticum wallichii, 0.4g of airpotato yam rhizome, 0.3g of perilla leaf and 0.3g of dogbane leaf are mixed, and the obtained compound is fully ground to prepare 100-mesh Chinese herbal medicine compound powder.

(2) Uniformly mixing the Chinese herbal medicine compound powder obtained in the step (1) with 90% ethanol water solution according to the solid-to-liquid ratio of 1:6, distilling, condensing and extracting, wherein the water bath temperature is 90 ℃, and the extraction time is 10 hours. Centrifuging the extracted mixed solution at 8000r/min for 5min, and collecting supernatant to obtain Chinese herbal compound extract.

(3) Uniformly mixing 0.05g of sage oil, 0.1g of vetiver oil, 0.35g of cineole, 0.4g of storax extract and 0.45g of thyme oil to obtain the flavoring liquid.

(4) And (3) uniformly mixing the Chinese herbal medicine compound extract obtained in the step (2) with the flavoring liquid obtained in the step (3) according to the mass ratio of 9.5.

Example 5

(1) After 3.2g of platycodon grandiflorum, 1.2g of mulberry leaf, 1.2g of albizia flower, 3.1g of green tangerine peel, 3.5g of epimedium herb, 8.5g of ligusticum wallichii, 0.8g of airpotato yam rhizome, 0.5g of perilla leaf and 0.5g of dogbane leaf are mixed, the obtained Chinese herbal medicine compound is fully ground to prepare the 80-mesh Chinese herbal medicine compound powder.

(2) Uniformly mixing the Chinese herbal medicine compound powder obtained in the step (1) with 85% ethanol water solution according to the solid-to-liquid ratio of 1:5, heating and refluxing for extraction, wherein the water bath temperature is 85 ℃, and the extraction time is 6 hours. Centrifuging the extracted mixed solution at 8000r/min for 10min, and collecting supernatant to obtain Chinese herbal compound extract.

(3) Uniformly mixing 0.15g of sage oil, 0.2g of vetiver oil, 0.3g of cineole, 0.45g of storax extract and 0.35g of thyme oil to obtain the flavoring liquid.

(4) And (3) uniformly mixing the Chinese herbal medicine compound extract obtained in the step (2) with the flavor blending liquid obtained in the step (3) according to the mass ratio of 9:1, and then uniformly mixing the mixture with 1,3-butanediol according to the volume ratio of 1.

Example 6

The present example provides a cigarette additive with herbal flavor, which is different from example 3 only in that the cigarette additive does not contain mulberry leaves, the sum of the mass of the albizia flower, the airpotato yam rhizome, the perilla leaf and the dogbane leaf is increased by 3.4g, the mass ratio of the albizia flower, the airpotato yam rhizome, the perilla leaf and the dogbane leaf is kept unchanged, and the other preparation methods are the same as example 3.

Example 7

The present example provides a cigarette additive with herbal flavor, which is different from example 3 only in that albizia flower is not contained, the sum of the mass of mulberry leaves, airpotato yam seeds, perilla leaves and dogbane leaves is increased by 3.4g, the mass ratio of the mulberry leaves, the airpotato yam seeds, the perilla leaves and the dogbane leaves is kept unchanged, and the other preparation methods are the same as example 3.

Example 8

The present example provides a cigarette additive with herbal flavor, which is different from example 3 only in that it does not contain airpotato yam, the sum of the mass of mulberry leaves, silktree albizzia flowers, perilla leaves and dogbane leaves is increased by 3.4g, the mass ratio of the mulberry leaves, silktree albizzia flowers, perilla leaves and dogbane leaves is kept unchanged, and the other preparation methods are the same as example 3.

Example 9

The present example provides a cigarette additive with herbal flavor, which is different from example 3 only in that it does not contain perilla leaves, the sum of the mass of mulberry leaves, flos albiziae, airpotato yam and dogbane leaves is increased by 3.4g, the mass ratio of the mulberry leaves, the flos albiziae, the airpotato yam and the dogbane leaves is kept unchanged, and the other preparation methods are the same as example 3.

Example 10

The present example provides a cigarette additive with herbal flavor, which is different from example 3 only in that it does not contain dogbane leaf, the sum of the mass of mulberry leaf, albizia flower, airpotato yam and perilla leaf is increased by 3.4g, the mass ratio of mulberry leaf, albizia flower, airpotato yam and perilla leaf is kept unchanged, and the other preparation methods are the same as example 3.

Example 11

This example provides a cigarette additive with herbal aroma, which is different from example 3 only in that the additive does not contain sage oil, the sum of the mass of vetiver oil, eucalyptol, storax extract and red thyme oil is increased to 1.2g, and the mass ratio of the vetiver oil, eucalyptol, storax extract and red thyme oil is kept unchanged, and other preparation methods are the same as example 3.

Example 12

This example provides a cigarette additive with herbal note, which is different from example 3 only in that, without vetiver oil, the sum of the mass of sage oil, eucalyptol, storax extract and red thyme oil is increased to 1.2g, and the mass ratio of sage oil, eucalyptol, storax extract and red thyme oil is kept unchanged, and other preparation methods are the same as example 3.

Example 13

This example provides a cigarette additive with herbal note, which is different from example 3 only in that, without eucalyptol, the sum of the mass of sage oil, vetiver oil, storax extract and thyme oil red is increased to 1.2g, and the mass ratio of sage oil, vetiver oil, storax extract and thyme oil red is kept unchanged, and other preparation methods are the same as example 3.

Example 14

This example provides a cigarette additive with herbal note, which is different from example 3 only in that, without containing styrax extract, the sum of the mass of sage oil, vetiver oil, eucalyptol and red thyme oil is increased to 1.2g, and the mass ratio of the sage oil, vetiver oil, eucalyptol and red thyme oil is kept unchanged, and other preparation methods are the same as example 3.

Example 15

This example provides a cigarette additive with herbal note, which is different from example 3 only in that, without thyme oil, the sum of the mass of sage oil, vetiver oil, eucalyptol and styrax extract is increased to 1.2g, and the mass ratio of sage oil, vetiver oil, eucalyptol and styrax extract is kept unchanged, and other preparation methods are the same as example 3.

Comparative example 1

The comparative example provides a cigarette additive with a herbal and herbaceous scent, which is different from example 3 only in that platycodon grandiflorum is not contained, the sum of the mass of pericarpium citri reticulatae viride, epimedium and ligusticum chuanxiong hort is increased to 17g, the mass ratio of the pericarpium citri reticulatae viride, the epimedium and the ligusticum chuanxiong hort is kept unchanged, and other preparation methods are the same as example 3.

Comparative example 2

The comparative example provides a cigarette additive with a herbal and herbaceous scent, which is different from example 3 only in that the cigarette additive does not contain green tangerine orange peels, the sum of the mass of platycodon grandiflorum, epimedium and ligusticum chuanxiong hort is increased to 17g, the mass ratio of the platycodon grandiflorum, the epimedium and the ligusticum chuanxiong hort remains unchanged, and other preparation methods are the same as example 3.

Comparative example 3

The comparative example provides a cigarette additive with a herbal fragrance, which is different from example 3 only in that epimedium is not contained, the sum of the mass of platycodon grandiflorum, green tangerine orange peel and ligusticum chuanxiong hort is increased to 17g, the mass ratio of the platycodon grandiflorum, the green tangerine orange peel and the ligusticum chuanxiong hort remains unchanged, and other preparation methods are the same as example 3.

Comparative example 4

The comparative example provides a cigarette additive with a herbal fragrance, which is different from example 3 only in that the cigarette additive does not contain ligusticum chuanxiong hort, the mass sum of platycodon grandiflorum, pericarpium citri reticulatae viride and herba epimedii is increased to 17g, the mass ratio of the platycodon grandiflorum, the pericarpium citri reticulatae viride and the herba epimedii is kept unchanged, and the other preparation methods are the same as example 3.

Application example 1

The application example provides a cigarette with a herbal aroma, and the preparation method of the cigarette with the herbal aroma comprises the following steps:

(1) The formula tobacco shreds are prepared from Yunnan tobacco leaves, fujian tobacco leaves, guizhou tobacco leaves, hunan tobacco leaves, zimbabwe tobacco leaves and Argentina tobacco leaves according to the mass ratio of 4;

(2) The cigarette additive with the herb fragrance provided in the example 1 with accurate mass is uniformly sprayed to the cut tobacco in the formula, the spraying mass ratio is 0.05%, and the cigarette with the herb fragrance is prepared by using cigarette production equipment and matching cigarette paper, tipping paper and a filter tip according to a normal cigarette production process.

Application example 2

(2) The cigarette additive with the herb fragrance provided in the example 2 with accurate mass is uniformly sprayed to the cut tobacco in the formula, the spraying mass ratio is 0.1%, and the cigarette with the herb fragrance is prepared by using cigarette production equipment and matching cigarette paper, tipping paper and a filter tip according to a normal cigarette production process.

Application example 3

(1) The formula tobacco shreds are prepared from Yunnan tobacco leaves, fujian tobacco leaves, guizhou tobacco leaves, hunan tobacco leaves, zimbabwe tobacco leaves and Argentina tobacco leaves according to the mass ratio of 4.

(2) The cigarette additive with the herb fragrance provided by the embodiment 3 with accurate mass is uniformly sprayed to the cut tobacco in the formula, the spraying mass ratio is 0.2%, and the cigarette with the herb fragrance is prepared by using cigarette production equipment and matching cigarette paper, tipping paper and a filter tip according to a normal cigarette production process.

Application example 4

The application example provides a cigarette with a herbal aroma, and the preparation method of the cigarette with the herbal aroma comprises the following steps

(2) The cigarette additive with the herb fragrance provided in the example 4 with accurate mass is uniformly sprayed to the cut tobacco in the formula, the spraying mass ratio is 0.3%, and the cigarette with the herb fragrance is prepared by using cigarette production equipment and matching cigarette paper, tipping paper and a filter tip according to a normal cigarette production process.

Application example 5

(2) The cigarette additive with the herb note provided by the embodiment 5 with accurate mass is uniformly sprayed to the cut tobacco with the formula, the spraying mass ratio is 0.5%, and according to the normal cigarette production process, cigarette paper, tipping paper and a filter tip are matched by cigarette production equipment to prepare the cigarette with the herb note.

Application examples 6 to 15

Application examples 6 to 15 respectively provide cigarettes with herbal and herbal flavors, and the difference from the application example 3 is only that the cigarette additives with herbal and herbal flavors provided in the application examples 6 to 15 are respectively adopted, and other preparation methods are the same as those in the application example 3.

Comparative application examples 1 to 4

Comparative application examples 1 to 4 respectively provide cigarettes with herbal aroma, and the difference from application example 3 is that the cigarette additives with herbal aroma provided in comparative examples 1 to 4 are respectively adopted, and other preparation methods are the same as application example 3.

Comparative application example 5

The comparative application example provides a cigarette with a herbal aroma, and the preparation method of the cigarette with the herbal aroma comprises the following steps:

(1) Uniformly mixing 0.1g of sage oil, 0.05g of vetiver oil, 0.3g of cineole, 0.26g of storax extract and 0.47g of thyme oil to obtain the flavoring liquid.

(2) And (3) uniformly mixing the flavoring liquid obtained in the step (1) with glycerol according to the volume ratio of 1.5, and thus obtaining the cigarette additive.

(3) The formula tobacco shreds are prepared from Yunnan tobacco leaves, fujian tobacco leaves, guizhou tobacco leaves, hunan tobacco leaves, zimbabwe tobacco leaves and Argentina tobacco leaves according to the mass ratio of 4.

(4) Uniformly spraying the cigarette additive obtained in the step (2) with accurate mass to the cut tobacco in the formula, wherein the spraying mass ratio is 0.05%, and preparing the cigarette with the herb fragrance.

Comparative application example 6

(1) Uniformly mixing 0.15g of sage oil, 0.15g of vetiver oil, 0.2g of cineole, 0.3g of storax extract and 0.4g of thyme oil red to obtain the flavoring liquid.

(2) And (3) uniformly mixing the flavoring liquid obtained in the step (1) with 1,2-propylene glycol according to the volume ratio of 1:1 to prepare the cigarette additive.

(4) And (3) uniformly spraying the cigarette additive with the accurate mass obtained in the step (2) to the cut tobacco in the formula, wherein the spraying mass ratio is 0.2%, and preparing the cigarette with the herb fragrance.

Test example 1

Component detection

The cigarette additive with the herb flavor provided in the embodiment 3 is subjected to gas chromatography/mass spectrometry, and the main components are as follows:

alpha-pinene, camphene, sabinene, beta-pinene, myrcene, phellandrene, 3-carene, terpinene, 4-isopropyltoluene (p-cymene), limonene, eucalyptol, gamma-terpinene, linalool, 2,3-dihydro-3,5 dihydroxy-6-methyl-4 (H) -pyran-4-one, 4-terpene alcohol, alpha-terpineol, 5-hydroxymethylfurfural, citronellol, geraniol, 4-vinyl-2-methoxyphenol, iso 3763 zxf3763 acetate, p-hydroxybenzaldehyde, alpha-copal, beta-elemene, beta-caryophyllene, geranylacetone, beta-farnesene, alpha-humulene, myrcene, gercene, beta-bisabolene, gamma-cadinene, borneol, terpinene, ylarene, benzoic acid, gallic acid, vanillic acid, and the like.

Test example 2

Sensory evaluation

Testing a sample: the cigarettes provided in application examples 1-15 and comparative application examples 1-6 have herbal notes.

The test method comprises the following steps: referring to GB 5606.4-2005 cigarette part 4: the sensory technical requirements of the cigarette evaluation are scored, 15 persons with cigarette sensory evaluation qualification rate score the aroma (full score of 32), harmony (full score of 6), offensive odor (full score of 12), irritation (full score of 20), aftertaste (full score of 25) and herb note (full score of 5), and the test result is taken as the average value of each group.

The test results are shown in table 1 below:

TABLE 1

The data in table 2 show that the cigarette with the herbal aroma provided by the invention has the advantages that various components are matched with each other and synergized, the cigarette has a full-bodied herbal aroma, the harmony and harmony of the aroma are obviously improved, the aftertaste is improved, and the irritation and the offensive odor are also greatly reduced.

Test example 3

Efficacy testing

Testing a sample: the cigarettes with the herbal note provided in application examples 3, 6-10 and comparative application examples 1-4, 6.

1. Test objects: aiming at the current smoking population, the selection meets the requirements of patients with dizziness, cough, throat discomfort, lung dryness and excessive phlegm caused by long-term smoking. 220 volunteers with adverse symptoms and smoking history are selected, and divided into 4 groups (respectively a dizziness group, a cough group, a throat discomfort group and a lung dryness and excessive phlegm group) according to main symptoms, wherein 55 volunteers are selected in each group; each large group was subdivided into 11 groups of 5 persons each, and each group smoked the cigarettes with the herbal notes provided in application examples 3, 6-10 and comparative application examples 1-4, 6, respectively.

2. The sucking method comprises the following steps: five cigarettes with the herb note were smoked every day, and the effect evaluation was performed for 30 days.

3. The treatment effect evaluation standard is as follows:

the method has the following advantages: the problems of dizziness, cough, throat discomfort, lung dryness and excessive phlegm are improved.

And (4) invalidation: there was no change in symptom signs before and after treatment.

4. And (4) counting results: the number of persons in each group (5 persons) who considered the cigarettes with herb notes provided by the present invention to be effective against the disease was counted.

The test results are shown in table 2 below:

TABLE 2

Note: the statistics did not include clinical symptoms caused by other diseases and complications, and all volunteers had physical discomfort due to long-term smoking.

As can be seen from the data in Table 2, the cigarette with the herbal fragrance provided by the invention has the effects of inducing resuscitation, relieving pain, relieving cough, eliminating phlegm, clearing lung, moistening dryness, clearing heat, removing toxicity and the like, and can effectively relieve the symptoms of throat discomfort, lung dryness, excessive phlegm and the like of consumers caused by smoking. And the smoking frequency of the patient is obviously reduced, and the smoking amount of the smoker to the cigarettes can be effectively reduced.

The applicant states that the present invention is illustrated by the above examples to show the cigarette additive with herb note and its preparation method and application, but the present invention is not limited by the above examples, i.e. it does not mean that the present invention must rely on the above examples to be implemented. It should be understood by those skilled in the art that any modification of the present invention, equivalent substitutions of the raw materials of the product of the present invention, addition of auxiliary components, selection of specific modes, etc., are within the scope and disclosure of the present invention.

Claims

1. The cigarette additive with the herbal aroma is characterized in that the cigarette additive with the herbal aroma is prepared from Chinese herbal medicine compound extracts and flavoring liquid, wherein the Chinese herbal medicine compound extracts are prepared from platycodon grandiflorum, mulberry leaves, epimedium and dogbane leaves.

2. The cigarette additive with herbal note of claim 1, wherein the mass ratio of the herbal compound extract to the flavoring liquid is (8-9.9): 2-0.1;

preferably, the preparation raw materials of the Chinese herbal medicine compound extract comprise, by weight, 10-25 parts of platycodon grandiflorum, 1-7 parts of mulberry leaf, 10-25 parts of epimedium and 1-3 parts of dogbane leaf.

3. The cigarette additive with herbal flavor according to claim 1 or 2, wherein the raw materials for preparing the herbal compound extract further comprise any one or a combination of at least two of green tangerine orange peel, albizia flower, airpotato yam, perilla leaf or ligusticum chuanxiong hort;

preferably, the raw materials for preparing the Chinese herbal medicine compound extract also comprise green tangerine peel, flos albiziae, airpotato yam rhizome, perilla leaf and ligusticum chuanxiong hort;

preferably, the preparation raw materials of the Chinese herbal medicine compound extract also comprise 9-25 parts of green tangerine orange peel, 1-7 parts of albizia flower, 1-5 parts of airpotato yam rhizome, 1-3 parts of perilla leaf and 8-45 parts of ligusticum chuanxiong hort according to parts by weight.

4. The cigarette additive with herbal note according to any one of claims 1-3, wherein the flavoring liquid comprises any one or a combination of at least two of sage oil, vetivermectin, eucalyptol, storax extract or thyme oil red;

preferably, the flavoring liquid comprises sage oil, vetiver oil, eucalyptol, storax extract and thyme oil red;

preferably, the flavoring liquid comprises, by weight, 2-20 parts of sage oil, 2-15 parts of vetiver oil, 10-40 parts of cineole, 12-30 parts of storax extract and 20-50 parts of thyme oil.

5. A method for preparing the cigarette additive with herbal note according to any one of claims 1-4, characterized in that the preparation method comprises the following steps: extracting each Chinese herbal medicine raw material of the Chinese herbal medicine compound to obtain a Chinese herbal medicine compound extract; and then mixing the Chinese herbal medicine compound extract with the flavoring liquid to obtain the cigarette additive with the herbal medicine fragrance.

6. The method according to claim 5, wherein the extraction solvent used for the extraction comprises an aqueous ethanol solution;

preferably, the volume ratio of the ethanol to the water in the ethanol water solution is (3-9): 1;

preferably, the solid-liquid ratio of the Chinese herbal medicine compound and the extraction solvent is 1 (3-6) g/mL.

7. The preparation method according to claim 5 or 6, wherein the extraction manner comprises any one of ultrasonic heating extraction, heating reflux extraction or distillation condensation extraction;

preferably, the extraction temperature is 70-90 ℃, and the extraction time is 3-10h;

preferably, the Chinese herbal medicine raw materials are ground before extraction, and the grain size of the Chinese herbal medicine powder obtained after grinding is 40-100 meshes;

preferably, centrifugation is carried out after the extraction, and supernatant is collected to obtain the Chinese herbal medicine compound extract;

preferably, the rotating speed of the centrifugation is 6000-10000rpm, and the time of the centrifugation is 3-15min.

8. The method of any one of claims 5-7, wherein the mixing further comprises a polyol comprising any one of glycerol, 1,2-propanediol, or 1,3-butanediol, or a combination of at least two thereof;

preferably, the volume ratio of the sum of the volumes of the Chinese herbal medicine compound extract and the flavoring liquid to the polyol is 1 (0.5-2).

9. A cigarette, characterized in that it comprises cut tobacco and a cigarette additive with a medicinal herb note according to any one of claims 1 to 4;

preferably, the cigarette additive with the herb fragrance accounts for 0.05-0.5% of the total mass of the tobacco shreds.

10. The cigarette according to claim 9, wherein the preparation raw material of tobacco shreds comprises Yunnan tobacco leaves, fujian tobacco leaves, guizhou tobacco leaves, hunan tobacco leaves, zimbabwe tobacco leaves and Argentina tobacco leaves;

preferably, the cigarette is prepared by the following method, and the method comprises the following steps: and spraying the cigarette additive with the herb fragrance on tobacco shreds, and matching with cigarette paper, tipping paper and a filter tip to obtain the cigarette.