CN110437872A - 一种利用生物油催化裂化改善油品质量和提高低碳烯烃收率的方法 - Google Patents
一种利用生物油催化裂化改善油品质量和提高低碳烯烃收率的方法 Download PDFInfo
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- CN110437872A CN110437872A CN201910828885.7A CN201910828885A CN110437872A CN 110437872 A CN110437872 A CN 110437872A CN 201910828885 A CN201910828885 A CN 201910828885A CN 110437872 A CN110437872 A CN 110437872A
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- Prior art keywords
- oil
- improving
- catalytic cracking
- bio
- molecular sieve
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- 239000003921 oil Substances 0.000 title claims abstract description 79
- 238000000034 method Methods 0.000 title claims abstract description 72
- 239000012075 bio-oil Substances 0.000 title claims abstract description 68
- 238000004523 catalytic cracking Methods 0.000 title claims abstract description 51
- 150000001336 alkenes Chemical class 0.000 title claims abstract description 19
- 238000006243 chemical reaction Methods 0.000 claims abstract description 37
- 229910052799 carbon Inorganic materials 0.000 claims abstract description 23
- 150000002430 hydrocarbons Chemical class 0.000 claims abstract description 15
- 229930195733 hydrocarbon Natural products 0.000 claims abstract description 13
- 239000004215 Carbon black (E152) Substances 0.000 claims abstract description 12
- 235000019198 oils Nutrition 0.000 claims description 76
- 239000003054 catalyst Substances 0.000 claims description 74
- 239000002808 molecular sieve Substances 0.000 claims description 35
- URGAHOPLAPQHLN-UHFFFAOYSA-N sodium aluminosilicate Chemical compound [Na+].[Al+3].[O-][Si]([O-])=O.[O-][Si]([O-])=O URGAHOPLAPQHLN-UHFFFAOYSA-N 0.000 claims description 33
- PNEYBMLMFCGWSK-UHFFFAOYSA-N aluminium oxide Inorganic materials [O-2].[O-2].[O-2].[Al+3].[Al+3] PNEYBMLMFCGWSK-UHFFFAOYSA-N 0.000 claims description 18
- VYPSYNLAJGMNEJ-UHFFFAOYSA-N Silicium dioxide Chemical compound O=[Si]=O VYPSYNLAJGMNEJ-UHFFFAOYSA-N 0.000 claims description 16
- 229910052739 hydrogen Inorganic materials 0.000 claims description 12
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 claims description 11
- 239000001257 hydrogen Substances 0.000 claims description 11
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 claims description 9
- 238000005336 cracking Methods 0.000 claims description 9
- 239000011230 binding agent Substances 0.000 claims description 8
- 239000000377 silicon dioxide Substances 0.000 claims description 8
- 229910052593 corundum Inorganic materials 0.000 claims description 7
- 229910052760 oxygen Inorganic materials 0.000 claims description 7
- 229910001845 yogo sapphire Inorganic materials 0.000 claims description 7
- 235000019482 Palm oil Nutrition 0.000 claims description 6
- 238000006555 catalytic reaction Methods 0.000 claims description 6
- 239000000571 coke Substances 0.000 claims description 6
- 239000001301 oxygen Substances 0.000 claims description 6
- 239000002540 palm oil Substances 0.000 claims description 6
- 235000010469 Glycine max Nutrition 0.000 claims description 5
- 244000068988 Glycine max Species 0.000 claims description 5
- 235000019483 Peanut oil Nutrition 0.000 claims description 5
- 230000008859 change Effects 0.000 claims description 5
- 239000000312 peanut oil Substances 0.000 claims description 5
- OAICVXFJPJFONN-UHFFFAOYSA-N Phosphorus Chemical compound [P] OAICVXFJPJFONN-UHFFFAOYSA-N 0.000 claims description 4
- 239000011159 matrix material Substances 0.000 claims description 4
- 229910052698 phosphorus Inorganic materials 0.000 claims description 4
- 239000011574 phosphorus Substances 0.000 claims description 4
- 229910052761 rare earth metal Inorganic materials 0.000 claims description 4
- 150000002910 rare earth metals Chemical class 0.000 claims description 3
- 238000000926 separation method Methods 0.000 claims description 3
- 230000006641 stabilisation Effects 0.000 claims description 3
- 230000009471 action Effects 0.000 claims description 2
- 229910052784 alkaline earth metal Inorganic materials 0.000 claims description 2
- 150000001342 alkaline earth metals Chemical class 0.000 claims description 2
- 239000004927 clay Substances 0.000 claims description 2
- 230000006837 decompression Effects 0.000 claims description 2
- 238000000605 extraction Methods 0.000 claims description 2
- 238000011069 regeneration method Methods 0.000 claims description 2
- 210000004243 sweat Anatomy 0.000 claims description 2
- MYMOFIZGZYHOMD-UHFFFAOYSA-N Dioxygen Chemical compound O=O MYMOFIZGZYHOMD-UHFFFAOYSA-N 0.000 claims 1
- 239000003502 gasoline Substances 0.000 abstract description 14
- TVMXDCGIABBOFY-UHFFFAOYSA-N octane Chemical compound CCCCCCCC TVMXDCGIABBOFY-UHFFFAOYSA-N 0.000 abstract description 3
- QQONPFPTGQHPMA-UHFFFAOYSA-N propylene Natural products CC=C QQONPFPTGQHPMA-UHFFFAOYSA-N 0.000 abstract description 3
- 125000004805 propylene group Chemical group [H]C([H])([H])C([H])([*:1])C([H])([H])[*:2] 0.000 abstract description 3
- 239000002002 slurry Substances 0.000 description 24
- 230000008569 process Effects 0.000 description 22
- NLYAJNPCOHFWQQ-UHFFFAOYSA-N kaolin Chemical compound O.O.O=[Al]O[Si](=O)O[Si](=O)O[Al]=O NLYAJNPCOHFWQQ-UHFFFAOYSA-N 0.000 description 12
- 239000005995 Aluminium silicate Substances 0.000 description 11
- 235000012211 aluminium silicate Nutrition 0.000 description 11
- 229910001593 boehmite Inorganic materials 0.000 description 11
- FAHBNUUHRFUEAI-UHFFFAOYSA-M hydroxidooxidoaluminium Chemical compound O[Al]=O FAHBNUUHRFUEAI-UHFFFAOYSA-M 0.000 description 11
- 239000002994 raw material Substances 0.000 description 10
- 238000011049 filling Methods 0.000 description 9
- 239000003225 biodiesel Substances 0.000 description 8
- 230000000052 comparative effect Effects 0.000 description 8
- 239000002283 diesel fuel Substances 0.000 description 8
- 238000004519 manufacturing process Methods 0.000 description 8
- 238000005299 abrasion Methods 0.000 description 7
- 230000003197 catalytic effect Effects 0.000 description 7
- 239000007789 gas Substances 0.000 description 7
- 239000002028 Biomass Substances 0.000 description 6
- OKKJLVBELUTLKV-UHFFFAOYSA-N Methanol Chemical compound OC OKKJLVBELUTLKV-UHFFFAOYSA-N 0.000 description 6
- 238000013019 agitation Methods 0.000 description 6
- 239000008367 deionised water Substances 0.000 description 6
- 229910021641 deionized water Inorganic materials 0.000 description 6
- -1 ethylene, propylene Chemical group 0.000 description 6
- HYBBIBNJHNGZAN-UHFFFAOYSA-N furfural Chemical compound O=CC1=CC=CO1 HYBBIBNJHNGZAN-UHFFFAOYSA-N 0.000 description 6
- 239000003208 petroleum Substances 0.000 description 6
- 239000004033 plastic Substances 0.000 description 6
- 238000007493 shaping process Methods 0.000 description 6
- 239000007787 solid Substances 0.000 description 6
- 239000007921 spray Substances 0.000 description 6
- 238000003756 stirring Methods 0.000 description 6
- 239000000126 substance Substances 0.000 description 6
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Chemical compound O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 6
- 239000001993 wax Substances 0.000 description 6
- 229910052782 aluminium Inorganic materials 0.000 description 5
- XAGFODPZIPBFFR-UHFFFAOYSA-N aluminium Chemical compound [Al] XAGFODPZIPBFFR-UHFFFAOYSA-N 0.000 description 5
- 150000004945 aromatic hydrocarbons Chemical class 0.000 description 5
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 description 5
- 229910052681 coesite Inorganic materials 0.000 description 5
- 229910052906 cristobalite Inorganic materials 0.000 description 5
- 229920005610 lignin Polymers 0.000 description 5
- 239000000463 material Substances 0.000 description 5
- 238000002360 preparation method Methods 0.000 description 5
- 229910001404 rare earth metal oxide Inorganic materials 0.000 description 5
- 229910052682 stishovite Inorganic materials 0.000 description 5
- 229910052905 tridymite Inorganic materials 0.000 description 5
- 238000005984 hydrogenation reaction Methods 0.000 description 4
- PXHVJJICTQNCMI-UHFFFAOYSA-N nickel Substances [Ni] PXHVJJICTQNCMI-UHFFFAOYSA-N 0.000 description 4
- 230000008901 benefit Effects 0.000 description 3
- 230000032050 esterification Effects 0.000 description 3
- 238000005886 esterification reaction Methods 0.000 description 3
- 238000002474 experimental method Methods 0.000 description 3
- 239000004519 grease Substances 0.000 description 3
- 239000003350 kerosene Substances 0.000 description 3
- 229910052751 metal Inorganic materials 0.000 description 3
- 239000002184 metal Substances 0.000 description 3
- 150000003839 salts Chemical class 0.000 description 3
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 description 2
- LFQSCWFLJHTTHZ-UHFFFAOYSA-N Ethanol Chemical compound CCO LFQSCWFLJHTTHZ-UHFFFAOYSA-N 0.000 description 2
- 150000001335 aliphatic alkanes Chemical class 0.000 description 2
- 239000001913 cellulose Substances 0.000 description 2
- 229920002678 cellulose Polymers 0.000 description 2
- 239000003795 chemical substances by application Substances 0.000 description 2
- 238000002485 combustion reaction Methods 0.000 description 2
- 239000000539 dimer Substances 0.000 description 2
- 239000000446 fuel Substances 0.000 description 2
- 239000000295 fuel oil Substances 0.000 description 2
- 239000007788 liquid Substances 0.000 description 2
- 239000002480 mineral oil Substances 0.000 description 2
- 235000010446 mineral oil Nutrition 0.000 description 2
- 239000000178 monomer Substances 0.000 description 2
- ISWSIDIOOBJBQZ-UHFFFAOYSA-N phenol group Chemical group C1(=CC=CC=C1)O ISWSIDIOOBJBQZ-UHFFFAOYSA-N 0.000 description 2
- 238000012545 processing Methods 0.000 description 2
- 238000002407 reforming Methods 0.000 description 2
- 238000012216 screening Methods 0.000 description 2
- 238000001179 sorption measurement Methods 0.000 description 2
- 239000002699 waste material Substances 0.000 description 2
- 241000196324 Embryophyta Species 0.000 description 1
- 229910021536 Zeolite Inorganic materials 0.000 description 1
- 230000029936 alkylation Effects 0.000 description 1
- 239000012620 biological material Substances 0.000 description 1
- 238000003442 catalytic alkylation reaction Methods 0.000 description 1
- 238000009903 catalytic hydrogenation reaction Methods 0.000 description 1
- 238000007233 catalytic pyrolysis Methods 0.000 description 1
- 238000004587 chromatography analysis Methods 0.000 description 1
- 239000003245 coal Substances 0.000 description 1
- 239000010941 cobalt Substances 0.000 description 1
- 229910017052 cobalt Inorganic materials 0.000 description 1
- GUTLYIVDDKVIGB-UHFFFAOYSA-N cobalt atom Chemical compound [Co] GUTLYIVDDKVIGB-UHFFFAOYSA-N 0.000 description 1
- 150000001875 compounds Chemical class 0.000 description 1
- 238000001514 detection method Methods 0.000 description 1
- HNPSIPDUKPIQMN-UHFFFAOYSA-N dioxosilane;oxo(oxoalumanyloxy)alumane Chemical compound O=[Si]=O.O=[Al]O[Al]=O HNPSIPDUKPIQMN-UHFFFAOYSA-N 0.000 description 1
- 238000004821 distillation Methods 0.000 description 1
- 238000009826 distribution Methods 0.000 description 1
- 230000000694 effects Effects 0.000 description 1
- 238000005516 engineering process Methods 0.000 description 1
- 230000007613 environmental effect Effects 0.000 description 1
- 235000019441 ethanol Nutrition 0.000 description 1
- 125000004494 ethyl ester group Chemical group 0.000 description 1
- 238000011156 evaluation Methods 0.000 description 1
- 235000019387 fatty acid methyl ester Nutrition 0.000 description 1
- 239000003317 industrial substance Substances 0.000 description 1
- 229910052622 kaolinite Inorganic materials 0.000 description 1
- 238000005360 mashing Methods 0.000 description 1
- 230000013011 mating Effects 0.000 description 1
- 229910044991 metal oxide Inorganic materials 0.000 description 1
- 150000004706 metal oxides Chemical class 0.000 description 1
- 239000000203 mixture Substances 0.000 description 1
- 230000004048 modification Effects 0.000 description 1
- 238000012986 modification Methods 0.000 description 1
- 150000002751 molybdenum Chemical class 0.000 description 1
- 229910052759 nickel Inorganic materials 0.000 description 1
- 229910052757 nitrogen Inorganic materials 0.000 description 1
- 229910000510 noble metal Inorganic materials 0.000 description 1
- JRZJOMJEPLMPRA-UHFFFAOYSA-N olefin Natural products CCCCCCCC=C JRZJOMJEPLMPRA-UHFFFAOYSA-N 0.000 description 1
- 239000012188 paraffin wax Substances 0.000 description 1
- 238000005504 petroleum refining Methods 0.000 description 1
- 230000029553 photosynthesis Effects 0.000 description 1
- 238000010672 photosynthesis Methods 0.000 description 1
- 238000006116 polymerization reaction Methods 0.000 description 1
- 238000003672 processing method Methods 0.000 description 1
- 238000000197 pyrolysis Methods 0.000 description 1
- 230000009257 reactivity Effects 0.000 description 1
- 238000011160 research Methods 0.000 description 1
- 238000005245 sintering Methods 0.000 description 1
- 239000002689 soil Substances 0.000 description 1
- 239000011973 solid acid Substances 0.000 description 1
- 238000010998 test method Methods 0.000 description 1
- 238000012360 testing method Methods 0.000 description 1
- YLQBMQCUIZJEEH-UHFFFAOYSA-N tetrahydrofuran Natural products C=1C=COC=1 YLQBMQCUIZJEEH-UHFFFAOYSA-N 0.000 description 1
- 125000000383 tetramethylene group Chemical group [H]C([H])([*:1])C([H])([H])C([H])([H])C([H])([H])[*:2] 0.000 description 1
- WFKWXMTUELFFGS-UHFFFAOYSA-N tungsten Chemical compound [W] WFKWXMTUELFFGS-UHFFFAOYSA-N 0.000 description 1
- 229910052721 tungsten Inorganic materials 0.000 description 1
- 239000010937 tungsten Substances 0.000 description 1
- 239000002023 wood Substances 0.000 description 1
- 239000010457 zeolite Substances 0.000 description 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
- C10G55/00—Treatment of hydrocarbon oils, in the absence of hydrogen, by at least one refining process and at least one cracking process
- C10G55/02—Treatment of hydrocarbon oils, in the absence of hydrogen, by at least one refining process and at least one cracking process plural serial stages only
- C10G55/06—Treatment of hydrocarbon oils, in the absence of hydrogen, by at least one refining process and at least one cracking process plural serial stages only including at least one catalytic cracking step
Landscapes
- Chemical & Material Sciences (AREA)
- Oil, Petroleum & Natural Gas (AREA)
- Engineering & Computer Science (AREA)
- Chemical Kinetics & Catalysis (AREA)
- General Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Production Of Liquid Hydrocarbon Mixture For Refining Petroleum (AREA)
Abstract
Description
生物油 | 碳/氧摩尔比 | 氢/碳摩尔比 |
棕榈油 | 8.24 | 1.80 |
花生油 | 9.21 | 1.90 |
豆油 | 8.93 | 1.81 |
地沟油 | 9.06 | 1.82 |
糠醛 | 2.50 | 0.80 |
Claims (10)
Priority Applications (3)
Application Number | Priority Date | Filing Date | Title |
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CN201910828885.7A CN110437872A (zh) | 2019-09-03 | 2019-09-03 | 一种利用生物油催化裂化改善油品质量和提高低碳烯烃收率的方法 |
PCT/CN2020/110823 WO2021043018A1 (zh) | 2019-09-03 | 2020-08-24 | 一种利用生物油催化裂化改善油品质量和提高低碳烯烃收率的方法 |
US17/056,426 US20220306942A1 (en) | 2019-09-03 | 2020-08-24 | Method for Improving Oil Quality and Increasing Yield of Low-carbon Olefins by Utilizing Bio-Oil Catalytic Cracking |
Applications Claiming Priority (1)
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CN201910828885.7A CN110437872A (zh) | 2019-09-03 | 2019-09-03 | 一种利用生物油催化裂化改善油品质量和提高低碳烯烃收率的方法 |
Publications (1)
Publication Number | Publication Date |
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CN110437872A true CN110437872A (zh) | 2019-11-12 |
Family
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Family Applications (1)
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CN201910828885.7A Pending CN110437872A (zh) | 2019-09-03 | 2019-09-03 | 一种利用生物油催化裂化改善油品质量和提高低碳烯烃收率的方法 |
Country Status (1)
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CN (1) | CN110437872A (zh) |
Cited By (3)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN111748367A (zh) * | 2020-06-01 | 2020-10-09 | 四川润和催化新材料股份有限公司 | 利用生物油催化裂解/热裂解提高乙烯和丙烯产率的方法 |
WO2021043017A1 (zh) * | 2019-09-03 | 2021-03-11 | 四川润和催化新材料股份有限公司 | 一种降油浆和多产低碳烯烃的助剂及其制备方法与应用 |
WO2021043018A1 (zh) * | 2019-09-03 | 2021-03-11 | 四川润和催化新材料股份有限公司 | 一种利用生物油催化裂化改善油品质量和提高低碳烯烃收率的方法 |
Citations (5)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN1916135A (zh) * | 2006-09-06 | 2007-02-21 | 湖南长岭石化科技开发有限公司 | 一种由生物油脂生产燃料油的方法 |
CN101092318A (zh) * | 2006-06-21 | 2007-12-26 | 中国科学院大连化学物理研究所 | 一种用植物油脂和动物油脂制烯烃的方法 |
CN101314724A (zh) * | 2007-05-31 | 2008-12-03 | 中国石油化工股份有限公司 | 一种生物油脂和矿物油组合催化转化方法 |
CN105925381A (zh) * | 2016-04-14 | 2016-09-07 | 淮阴师范学院 | 地沟油高值化利用方法 |
CN109694725A (zh) * | 2017-10-20 | 2019-04-30 | 中国石油化工股份有限公司 | 一种生产高辛烷值汽油的催化裂化方法 |
-
2019
- 2019-09-03 CN CN201910828885.7A patent/CN110437872A/zh active Pending
Patent Citations (5)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN101092318A (zh) * | 2006-06-21 | 2007-12-26 | 中国科学院大连化学物理研究所 | 一种用植物油脂和动物油脂制烯烃的方法 |
CN1916135A (zh) * | 2006-09-06 | 2007-02-21 | 湖南长岭石化科技开发有限公司 | 一种由生物油脂生产燃料油的方法 |
CN101314724A (zh) * | 2007-05-31 | 2008-12-03 | 中国石油化工股份有限公司 | 一种生物油脂和矿物油组合催化转化方法 |
CN105925381A (zh) * | 2016-04-14 | 2016-09-07 | 淮阴师范学院 | 地沟油高值化利用方法 |
CN109694725A (zh) * | 2017-10-20 | 2019-04-30 | 中国石油化工股份有限公司 | 一种生产高辛烷值汽油的催化裂化方法 |
Cited By (3)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
WO2021043017A1 (zh) * | 2019-09-03 | 2021-03-11 | 四川润和催化新材料股份有限公司 | 一种降油浆和多产低碳烯烃的助剂及其制备方法与应用 |
WO2021043018A1 (zh) * | 2019-09-03 | 2021-03-11 | 四川润和催化新材料股份有限公司 | 一种利用生物油催化裂化改善油品质量和提高低碳烯烃收率的方法 |
CN111748367A (zh) * | 2020-06-01 | 2020-10-09 | 四川润和催化新材料股份有限公司 | 利用生物油催化裂解/热裂解提高乙烯和丙烯产率的方法 |
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Address after: 614000 group 3, Miaoer village, Jinsu Town, Wutongqiao District, Leshan City, Sichuan Province Applicant after: Runhe catalyst Co.,Ltd. Address before: 614803 group 3, Miaoer village, Jinsu Town, Wutongqiao District, Leshan City, Sichuan Province Applicant before: REZEL CATALYSTS Corp. |
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TA01 | Transfer of patent application right | ||
TA01 | Transfer of patent application right |
Effective date of registration: 20210826 Address after: 201208 room 118, building 20, No. 1-42, Lane 83, Hongxiang North Road, Lingang New Area, China (Shanghai) pilot Free Trade Zone, Pudong New Area, Shanghai Applicant after: Runhe Kehua catalyst (Shanghai) Co.,Ltd. Address before: 614000 group 3, Miaoer village, Jinsu Town, Wutongqiao District, Leshan City, Sichuan Province Applicant before: Runhe catalyst Co.,Ltd. |
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RJ01 | Rejection of invention patent application after publication | ||
RJ01 | Rejection of invention patent application after publication |
Application publication date: 20191112 |