CN101258635B - 调湿燃料电池用膜电极组件的方法 - Google Patents

调湿燃料电池用膜电极组件的方法 Download PDF

Info

Publication number
CN101258635B
CN101258635B CN200680032891.2A CN200680032891A CN101258635B CN 101258635 B CN101258635 B CN 101258635B CN 200680032891 A CN200680032891 A CN 200680032891A CN 101258635 B CN101258635 B CN 101258635B
Authority
CN
China
Prior art keywords
polymer
different
oneself
monokaryon
multinuclear
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
CN200680032891.2A
Other languages
English (en)
Chinese (zh)
Other versions
CN101258635A (zh
Inventor
欧默尔·乌恩萨尔
约阿基姆·基弗
伊沙贝尔·孔德勒
马蒂亚斯·韦伯
克利斯托弗·帕德贝格
托马斯·施密特
约亨·鲍尔梅斯特
戈登·卡伦丹恩
格伦·霍普斯
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
BASF Fuel Cell GmbH
Original Assignee
BASF Fuel Cell GmbH
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by BASF Fuel Cell GmbH filed Critical BASF Fuel Cell GmbH
Publication of CN101258635A publication Critical patent/CN101258635A/zh
Application granted granted Critical
Publication of CN101258635B publication Critical patent/CN101258635B/zh
Expired - Fee Related legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
    • H01M8/04223—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids during start-up or shut-down; Depolarisation or activation, e.g. purging; Means for short-circuiting defective fuel cells
    • H01M8/04238—Depolarisation
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2287—After-treatment
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0289—Means for holding the electrolyte
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/08—Fuel cells with aqueous electrolytes
    • H01M8/083—Alkaline fuel cells
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1004—Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1023—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having only carbon, e.g. polyarylenes, polystyrenes or polybutadiene-styrenes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1027—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having carbon, oxygen and other atoms, e.g. sulfonated polyethersulfones [S-PES]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/103—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having nitrogen, e.g. sulfonated polybenzimidazoles [S-PBI], polybenzimidazoles with phosphoric acid, sulfonated polyamides [S-PA] or sulfonated polyphosphazenes [S-PPh]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1032—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having sulfur, e.g. sulfonated-polyethersulfones [S-PES]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1041—Polymer electrolyte composites, mixtures or blends
    • H01M8/1044—Mixtures of polymers, of which at least one is ionically conductive
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1072—Polymeric electrolyte materials characterised by the manufacturing processes by chemical reactions, e.g. in situ polymerisation or in situ crosslinking
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Electrochemistry (AREA)
  • Sustainable Development (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Energy (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Materials Engineering (AREA)
  • Composite Materials (AREA)
  • Fuel Cell (AREA)
  • Conductive Materials (AREA)
  • Inert Electrodes (AREA)
CN200680032891.2A 2005-09-10 2006-09-08 调湿燃料电池用膜电极组件的方法 Expired - Fee Related CN101258635B (zh)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
DE102005043127.5 2005-09-10
DE102005043127A DE102005043127A1 (de) 2005-09-10 2005-09-10 Verfahren zur Konditionierung von Membran-Elektroden-Einheiten für Brennstoffzellen
PCT/EP2006/008759 WO2007028626A1 (de) 2005-09-10 2006-09-08 Verfahren zur konditionierung von membran-elektroden-einheiten fur brennstoffzellen

Related Child Applications (1)

Application Number Title Priority Date Filing Date
CN2013100459126A Division CN103172888A (zh) 2005-09-10 2006-09-08 调湿燃料电池用膜电极组件的方法

Publications (2)

Publication Number Publication Date
CN101258635A CN101258635A (zh) 2008-09-03
CN101258635B true CN101258635B (zh) 2014-11-26

Family

ID=37708433

Family Applications (2)

Application Number Title Priority Date Filing Date
CN200680032891.2A Expired - Fee Related CN101258635B (zh) 2005-09-10 2006-09-08 调湿燃料电池用膜电极组件的方法
CN2013100459126A Pending CN103172888A (zh) 2005-09-10 2006-09-08 调湿燃料电池用膜电极组件的方法

Family Applications After (1)

Application Number Title Priority Date Filing Date
CN2013100459126A Pending CN103172888A (zh) 2005-09-10 2006-09-08 调湿燃料电池用膜电极组件的方法

Country Status (9)

Country Link
EP (1) EP1927151B1 (https=)
JP (2) JP5675048B2 (https=)
KR (1) KR20080042123A (https=)
CN (2) CN101258635B (https=)
AT (1) ATE521101T1 (https=)
CA (1) CA2619258A1 (https=)
DE (1) DE102005043127A1 (https=)
RU (1) RU2008113388A (https=)
WO (1) WO2007028626A1 (https=)

Families Citing this family (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE102007024619B4 (de) 2007-05-24 2013-01-10 Technische Universität Darmstadt Verfahren zur Herstellung eines geträgerten Katalysators für die Oxidation von Kohlenmonoxid, dieser geträgerte Katalysator sowie ein Verfahren zur Oxidation von Kohlenmonoxid
DE102010039846A1 (de) 2010-08-26 2012-03-01 Bayer Materialscience Aktiengesellschaft Sauerstoffverzehrelektrode und Verfahren zu ihrer Herstellung
RU2487442C1 (ru) * 2012-02-28 2013-07-10 Федеральное государственное бюджетное учреждение науки Физико-технический институт им. А.Ф. Иоффе Российской академии наук Способ активации мембранно-электродного блока
US20130317141A1 (en) 2012-05-24 2013-11-28 Sabic Innovative Plastics Ip B.V. Flame retardant polycarbonate compositions, methods of manufacture thereof and articles comprising the same
US9023922B2 (en) 2012-05-24 2015-05-05 Sabic Global Technologies B.V. Flame retardant compositions, articles comprising the same and methods of manufacture thereof
DE102014205035A1 (de) 2014-03-18 2015-09-24 Volkswagen Ag Verfahren zum Herstellen einer Membran-Elektroden-Einheit, Membran-Elektroden-Einheit, Brennstoffzelle und Kraftfahrzeug mit Brennstoffzelle
EP3760683B1 (de) 2019-07-04 2024-04-03 Heraeus Precious Metals GmbH & Co. KG Verfahren zur herstellung einer katalysator-beschichteten membran

Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2005506901A (ja) * 2001-10-19 2005-03-10 スーペリア　マイクロパウダーズ　リミテッド　ライアビリティ　カンパニー 電子部品堆積用テープ組成物
CN1649944A (zh) * 2002-03-05 2005-08-03 佩密斯股份有限公司 用于高温应用中的质导电解质膜及其在燃料电池中的应用

Family Cites Families (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP1523053A3 (en) * 1999-09-09 2010-04-28 Danish Power Systems APS Polymer electrolyte membrane fuel cells
DE10340928A1 (de) * 2003-09-04 2005-04-07 Celanese Ventures Gmbh Mit einer Katalysatorschicht beschichtete protonenleitende Polymermembran enthaltend Phosphonensäuregruppen umfassende Polymere, Membran-Elektroden-Einheit und deren Anwendung in Brennstoffzellen
KR100513541B1 (ko) * 2003-11-27 2005-09-07 현대자동차주식회사 고체 고분자 연료 전지의 초기 활성화 방법
DE10361833A1 (de) * 2003-12-30 2005-08-04 Celanese Ventures Gmbh Protonenleitende Membran und deren Verwendung
DE102004034139A1 (de) * 2004-07-15 2006-02-02 Pemeas Gmbh Verfahren zur Herstellung von Membran-Elektroden-Einheiten

Patent Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2005506901A (ja) * 2001-10-19 2005-03-10 スーペリア　マイクロパウダーズ　リミテッド　ライアビリティ　カンパニー 電子部品堆積用テープ組成物
CN1649944A (zh) * 2002-03-05 2005-08-03 佩密斯股份有限公司 用于高温应用中的质导电解质膜及其在燃料电池中的应用

Also Published As

Publication number Publication date
JP2013175466A (ja) 2013-09-05
EP1927151A1 (de) 2008-06-04
CA2619258A1 (en) 2007-03-15
CN101258635A (zh) 2008-09-03
KR20080042123A (ko) 2008-05-14
JP5675048B2 (ja) 2015-02-25
ATE521101T1 (de) 2011-09-15
DE102005043127A1 (de) 2007-03-15
JP2009508296A (ja) 2009-02-26
WO2007028626A1 (de) 2007-03-15
CN103172888A (zh) 2013-06-26
EP1927151B1 (de) 2011-08-17
RU2008113388A (ru) 2009-10-20
JP5698289B2 (ja) 2015-04-08

Similar Documents

Publication Publication Date Title
CN100448086C (zh) 包括含乙烯基的膦酸的混合物、含聚乙烯膦酸的聚合物电解质膜及其在燃料电池中的应用
CN100408616C (zh) 用于高温应用中的质导电解质膜及其在燃料电池中的应用
KR100993157B1 (ko) 감소된 메탄올 투과성을 갖는 양성자 전도성 전해질 막 및연료 전지에서의 이의 용도
CN100544104C (zh) 包括含有磺酸基团的聚合物的质子导电聚合物膜及其在燃料电池中的应用
CN100385724C (zh) 包括含有膦酸基团的聚合物的质子导电聚合物膜及其在燃料电池中的应用
CN100530801C (zh) 接枝聚合物电解质膜、制备方法及其在燃料电池中的应用
US20060166067A1 (en) Polymer electrolyte membrane, method for the production thereof, and application thereof in fuel cells
CN1318484C (zh) 包括含乙烯基的磺酸的混合物、含聚乙烯磺酸的聚合物电解质膜及其在燃料电池中的应用
JP5698289B2 (ja) 燃料電池用の膜電極接合体のコンディショニング方法
JP2008507082A (ja) 膜−電極ユニットの製造方法
JP2009293045A (ja) スルホン酸基含有ポリマーを含むプロトン伝導性ポリマー膜および燃料電池におけるその使用
US20150125779A1 (en) Method for conditioning membrane-electrode-units for fuel cells
KR20070015156A (ko) 고성능 막전극 유닛 및 연료 전지에서 그의 용도
US9130208B2 (en) Membrane electrode assemblies and fuel cells with long lifetime
US20070055045A1 (en) Proton-conducting polymer membrane containing polymers with sulfonic acid groups that are covalently bonded to aromatic groups, membrane electrode unit, and use thereof in fuel cells
US20070202415A1 (en) Proton-Conducting Polymer Membrane Comprising At Least One Porous Carrier Material, And Use Thereof In Fuel Cells
US9325025B2 (en) Membrane electrode assemblies and fuel cells with long lifetime
WO2013167950A1 (en) Improved membrane electrode assemblies and fuel cells with long lifetime
KR20050018679A (ko) 그라프트화된 중합체 전해질 막, 이의 제조 방법, 및 연료전지에서의 이의 용도

Legal Events

Date Code Title Description
C06 Publication
PB01 Publication
C10 Entry into substantive examination
SE01 Entry into force of request for substantive examination
C14 Grant of patent or utility model
GR01 Patent grant
CF01 Termination of patent right due to non-payment of annual fee

Granted publication date: 20141126

Termination date: 20150908

EXPY Termination of patent right or utility model