WO2009053746A1 - Cooling device - Google Patents
Cooling device Download PDFInfo
- Publication number
- WO2009053746A1 WO2009053746A1 PCT/GB2008/050984 GB2008050984W WO2009053746A1 WO 2009053746 A1 WO2009053746 A1 WO 2009053746A1 GB 2008050984 W GB2008050984 W GB 2008050984W WO 2009053746 A1 WO2009053746 A1 WO 2009053746A1
- Authority
- WO
- WIPO (PCT)
- Prior art keywords
- cooling device
- electrodes
- cooling
- high voltage
- spark gap
- Prior art date
Links
Classifications
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F25—REFRIGERATION OR COOLING; COMBINED HEATING AND REFRIGERATION SYSTEMS; HEAT PUMP SYSTEMS; MANUFACTURE OR STORAGE OF ICE; LIQUEFACTION SOLIDIFICATION OF GASES
- F25B—REFRIGERATION MACHINES, PLANTS OR SYSTEMS; COMBINED HEATING AND REFRIGERATION SYSTEMS; HEAT PUMP SYSTEMS
- F25B21/00—Machines, plants or systems, using electric or magnetic effects
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F25—REFRIGERATION OR COOLING; COMBINED HEATING AND REFRIGERATION SYSTEMS; HEAT PUMP SYSTEMS; MANUFACTURE OR STORAGE OF ICE; LIQUEFACTION SOLIDIFICATION OF GASES
- F25B—REFRIGERATION MACHINES, PLANTS OR SYSTEMS; COMBINED HEATING AND REFRIGERATION SYSTEMS; HEAT PUMP SYSTEMS
- F25B2321/00—Details of machines, plants or systems, using electric or magnetic effects
- F25B2321/003—Details of machines, plants or systems, using electric or magnetic effects by using thermionic electron cooling effects
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02B—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO BUILDINGS, e.g. HOUSING, HOUSE APPLIANCES OR RELATED END-USER APPLICATIONS
- Y02B30/00—Energy efficient heating, ventilation or air conditioning [HVAC]
Definitions
- This invention relates to the field of temperature regulation and, in particular, to a device for cooling enclosed or confined spaces.
- Cooling devices for maintaining a room, car or other enclosed space at a comfortable temperature are well known. The majority are based on forced air systems that may incorporate some form of cooling of the air. Cooling is generally based on the thermodynamics of condensation and evaporation of a refrigerant gas. On condensation of a gas to a liquid, heat is rejected to the environment and on evaporation of a liquid, heat is absorbed. The evaporation / condensation cycle is driven by compression. In conventional air conditioning units the compression is driven by mechanical work that is normally provided by an electrical motor. Alternatively, sorption devices are driven by the adsorption or absorption of the refrigerant gas (or sorbate), such as ammonia, by a solid or solid / liquid sorbent.
- the refrigerant gas or sorbate
- a further problem presented by prior art cooling devices is the potentially hazardous nature of the refrigerant gas used. Ammonia, alcohols, hydrogen, hydrocarbons, hydrofluorocarbons and carbon dioxide have all been used in cooling systems. The potential risks from employing such substances are of course more significant if using in a confined space, such as an underground room or carriage. Most prior art cooling devices also suffer from high CO 2 emissions, which further harm the environment.
- the present invention provides a cooling device comprising a high voltage source connected to a spark gap and controlled by a timing means, wherein the source and timing means are arranged to generate unidirectional high voltage pulses which are discharged in short and regular impulses across the spark gap and the device also includes an emitter located in the vicinity of an electrode of the spark gap and electrically isolated therefrom.
- a device creates a source of high voltage direct current pulses which are discharged in very short impulses, preferably less than 100 ns duration, through a spark gap. As a result of this process, heat is withdrawn from the atmosphere surrounding the spark gap.
- the cooling effect is highly localised around the discharge spark and so the emitter is used to provide a means of delocalisation. That is, the emitter distributes the cooling effect over a larger volume.
- a cooling device that operates according to this principle is radically different from those known in the prior art. Whereas prior art devices are based on a refrigerant condensation / evaporation cycle, the present device is based on a cooling effect produced by a high voltage electrical discharge.
- a cooling device based on this principle advantageously achieves cooling without the use of potentially hazardous refrigerant. Moreover, the power required to generate a suitable electrical discharge is far less than that required to operate conventional cooling devices. A device can readily be constructed that consumes less than 1 % of the energy used by current air cooling technology to achieve the same effect.
- Such a device has numerous applications, primarily in the field of air conditioning.
- the device of the present invention may be far smaller than currently available air conditioning units. This renders it even more attractive to applications on mobile or non-permanent locations such as trains, cars, boats and caravans.
- the high voltage source is arranged to provide a voltage of at least 3 kV and, more preferably, at least 4 kV.
- the high voltage source may comprise a medium voltage source, timing control means for timing power output from said source in medium voltage pulses, a transformer arranged to convert the medium voltage pulses to high voltage pulses and a rectifier arranged to convert the high voltage pulses to a unidirectional signal.
- a medium voltage source timing control means for timing power output from said source in medium voltage pulses
- a transformer arranged to convert the medium voltage pulses to high voltage pulses
- a rectifier arranged to convert the high voltage pulses to a unidirectional signal.
- the medium voltage source itself may comprise a storage device for storing charge at medium voltage and which is discharged by operation of the timing control means.
- the storage device may be a capacitor or a bank of capacitors.
- a suitable capacitance may be in the region of 50 ⁇ F, and preferably around 47 ⁇ F. It may alternatively be an inductor.
- the capacitor is preferably charged by a circuit comprising a low voltage source, a pulse generator arranged to produce an alternating signal from the low voltage source, a second transformer arranged to convert low voltage input to a medium voltage output and a rectifier arranged to rectify alternating signal input to direct current output.
- the spark gap preferably comprises first and second electrodes sealed within a chamber and separated by an insulating gap. The sealing chamber prevents the electrodes from becoming contaminated, which may inhibit generation of a discharge spark.
- the electrodes are preferably dome shaped, which discourages localisation of spark emissions at a particular point on their surface and hence may prolong their useable life.
- the electrodes are made of chrome- or nickel- coated steel.
- the chamber may be filled with argon or other suitably inert gas.
- the emitter may comprise inner and outer thin-walled coaxial tubes, which are coaxially mounted about an electrode connection lead.
- the tubes should be good electrical conductors and are therefore preferably metallic or made from ceramic materials with high conductivity. Metals are generally cheaper and therefore preferred.
- the tubes preferably have internal diameters in the range 6 mm to 14 mm and lengths in the range 7 mm to 20 mm.
- the present invention provides a method of generating a cooling effect, the method comprising the steps of:- (a) Repeatedly applying a high-voltage, unidirectional pulse of electricity between a pair of electrodes in a gaseous environment, thereby causing sparking between the electrodes; and (b) Diffusing a cooling effect resulting from the sparking by means of an emitter located in the vicinity of the electrodes.
- the pulse is preferably of voltage higher than 4 kV and of duration shorter than 100 ns.
- Figure 1 is an overview of the process by which a spark that is capable of effecting an environmental cooling is generated.
- Figure 2 is a schematic of a circuit design, suitable for generating a cooling discharge.
- FIG. 3 is a detailed drawing of a spark gap and emitter.
- Figure 4 is a detailed circuit design for generating a spark that is suitable for effecting cooling.
- a unidirectional medium direct current voltage of around 225V
- a control capacitor 2-6 Figure 2 .
- a bank of capacitors may be used.
- the capacitor 2-6 is discharged into the primary coil of a first step up transformer 2-9 ( Figure 2) under control of a timer circuit 2-8 to create alternating pulses at around 4500 V.
- the 4.5 kV output from the first step up transformer 2-9 is rectified to create high voltage unidirectional pulses.
- the pulses are discharged in very short impulses, of less than 100 ns duration, through a spark gap 2-13 located in the vicinity of an emitter 2-12.
- the emitter 2-12 spreads or extends a cooling effect that is stimulated by the impulsed discharge. This therefore withdraws heat from the emitter / spark gap environment, which lowers the surrounding temperature.
- a device containing the emitter 2-12 and spark gap 2-13 would be placed in a room and the effect used to cool the air within the room.
- FIG. 2 illustrates a schematic of a circuit design, suitable for generating a spark in conjunction with an emitter that may be used to produce a cooling device in accordance with this invention. It is the discharging of the control capacitor 2-6 that is central to the generation of a suitable discharge spark.
- a low voltage direct current power supply, 2-1 such as a regulated mains adaptor or battery, powers a square wave generator 2-2 whose output is in turn connected to a second step up transformer 2-3.
- a bridge rectifier 2-4 takes its input from the transformer 2-3 output, and has a diode 2-5 and the control capacitor 2-6 connected in parallel across its output.
- the low voltage direct current supply 2-1 typically provides around 50OmA at 9V.
- the square wave generator 2-2 converts this signal to a square wave, which is applied across the second step up transformer 2-3.
- This transformer 2-3 is arranged to convert 9V input to a medium voltage output of around 225V.
- the output signal from the transformer 2-3 is therefore an alternating signal, at around 225V.
- the bridge rectifier 2-4 converts this signal to a direct current, maintaining the medium voltage level, reversals of current being prevented by the diode 2-5.
- the medium voltage unidirectional direct current is stored in the capacitor (or bank of capacitors) 2-6. Typically, the capacitance provided by this capacitor or bank is around 47 ⁇ F.
- a timing control circuit 2-8 and the input to the first transformer 2-9 are connected in series across the output of the capacitor 2-6.
- the timing circuit 2-8 thereby regulates the capacitor discharge into the primary coil of the transformer 2-9. If the timing circuit 2-8 is on, current is discharged from the capacitor 2-6 and input to the first step up transformer 2-9. If the timing circuit 2-8 is off, the control capacitor 2-6 is allowed to recharge, as described above.
- the timing circuit 2-8 is typically a transistor switch with on / off timing controlled by an integrated circuit timer, which is set to permit discharging of the capacitor 2-6 for a period of the order 15 ⁇ s or less.
- the first step up transformer 2-9 is arranged to raise the medium level input voltage to a high voltage output of around 4500 V. Under control of the timing circuit 2-8, this output is pulsed.
- the high voltage alternating current pulses, output from the second step up transformer 2-9 are input to a second rectifier 2-10, which in this embodiment is a diode.
- the pulses are thereby converted into a high-voltage dc signal, in the region of 4.5 kV.
- the spark gap 2-13 is connected across the rectified output from the first transformer 2-9 in parallel with a second capacitor 2-11.
- the rectified signal is then discharged into the spark gap 2-13 in short impulses, whose duration is controlled by circuit parameters, primarily the inductance of the transformer 2-9 and the value of capacitor 2-11.
- the impulse duration should be no more than 100 ns.
- the capacitor 2-11 should have capacitance in the region of 22 pF for satisfactory operation.
- the emitter 2-12 is located in the vicinity of the spark gap 2-13 and electrically isolated therefrom. As a result of the discharging impulses in the spark gap 2-13, the emitter experiences electro-static energy fluctuations, and the surrounding area is cooled.
- Figure 3 is a diagram showing suitable designs of spark gap 2-13 and emitter 2-12 for use with this invention.
- Figure 3a shows a side illustration, Figure 3b a cross-section along line AA and Figure 3c a cross-section along line BB.
- the spark gap 2-13 is formed by first 3-1 a and second 3-1 b electrodes separated by a gap, which is typically in the region of 0.7 mm.
- the electrodes 3-1 a, b are dome-shaped and typically made of steel and coated with nickel or chrome.
- the electrodes are sealed in a ceramic chamber containing an argon environment. Other inert gases, in addition to air, are also suitable.
- the spark gap should however be hermetically sealed in order to prevent the accumulation of material on the electrodes, which may impede the discharge of impulses.
- a voltage of over 3000V is required to cause a discharge current to flow through the surrounding gas, resulting in a sparking between the ends of the electrodes 3-1 a, b.
- the dome shape is advantageous as it allows sparks to extend across the gap between the electrodes without being restricted to a base position on the electrode. This extends the life of the electrodes.
- the emitter 2-12 abuts the first electrode 3-1 a and is electrically isolated therefrom. It consists of inner 3-2 and outer 3-4 thin-walled metal tubes that are coaxially mounted about the electrode lead, at the opposite side of the electrode to the spark gap 2-13. Plastic end caps 3-3 located at both ends of the tubes 3-2, 3-4 serve to isolate electrically the tubes from the electrode and its lead.
- the tubes 3-2 and 3-4 are typically made from electro-plated copper or stainless steel.
- the inner tube 3-2 has an external diameter of around 8mm and length of around 9mm.
- the outer tube 3-4 has an external diameter of around 12mm and length of about 13mm.
- the radial gap between the electrode 3-1 a and the internal walls of inner tube 3-2 is usually at least 2mm to prevent sparks developing within the emitter.
- the plastic end caps 3-3 extend beyond the circumference of the outer metal tube 3-4 to prevent sparks developing between the outer walls of the emitter and the dome shaped head of the electrode 3-1 a.
- the emitter tubes 3-2 and 3-4 become charged electro-statically as a result of the impulse discharges across the spark gap 2-13.
- the tubes produce a cooling effect that withdraws natural heat from the surrounding environment, typically air.
- the impulse voltage applied across the spark gap 2-13 has certain properties.
- it must be a direct current impulse of at least 3 kV and preferably 4 kV. This voltage should be discharged in a timescale of not longer than 100 ns. With these characteristics an impulse will electro-statically charge an emitter 2-12 located in the vicinity of, but electrically isolated from, the spark gap 2-13.
- FIG. 4 is a detailed circuit design for a printed circuit board for the cooling device of this invention.
- the low voltage direct current power supply 2-1 may be connected to this circuit at CN2. As stated previously, this supply is conveniently provided by a regulated switched mode mains adaptor or by batteries. Pads P1 and P2 allow an external switch to be fitted to control the power to the circuit.
- the square wave generator is indicated by integrated circuit U1. Resistors R1 , R2, R3 and R4, capacitors C1 , C3 and C4, diodes D3 and D4 and transistor Q1 control the square wave produced by U1. As will be apparent to one skilled in the art, if the values of these components are selected appropriately, transistor Q1 will not overheat.
- the values indicated in Figure 4 provide one example of a suitable combination that ensures transistor Q1 will not normally overheat.
- the second step up transformer 2-3 is represented in this circuit diagram by T1 , which is a 1 :25 step up transformer.
- the square wave generated by U1 is therefore raised (step 1 , Figure 1 ) to medium voltage by T1.
- the medium voltage current is rectified by bridge rectifier BR1 (2-4).
- Current reversals are prevented by diode D1 (2-5).
- These components, enclosed in the diagram by box 4-1 govern the charging, at medium voltage, of control capacitor 2-6 (C7 in Figure 4).
- the medium voltage unidirectional direct current is stored in capacitor(s) C7 and converted into short pulses of energy at a regular frequency by switch circuit 2-8, transistor Q2 of Figure 4.
- Resistors 2-7 (R8 and R9) ensure that capacitor 2-6 (C7) is discharged when the circuit is switched off.
- Integrated circuits U2 and U3, resistors R5, R6 and R7, capacitors C4, C5, C8, C9 and C10, diodes D9 and D10 control the switching of transistor Q2. This corresponds to step 2, as shown in Figure 1.
- the short pulses (of around 15 ⁇ s duration) discharged from the capacitor 2-6 (C7) are raised to high voltage by the first step up transformer 2-9 (T2), which, in this embodiment, is a 1 :20 transformer.
- the high voltage current is half rectified by diode 2-10 (D2) to create high voltage pulses.
- the high voltage pulses are discharged in impulses, controlled by capacitor 2-11 (C6), of less than 100 ns in spark gap 2-13 (FS1 ).
- the discharging of capacitor 2-6 (C7) and subsequent raising to high voltage impulses is controlled by the components shown in box 4-2 in Figure 4.
- Diode D2 should be encapsulated in a polyurethane or silicone sealant to prevent the development of high voltage coronas.
- the circuit shown in Figure 4 is encased and connected to a source of power. Once the device is operated, impulses are discharged across the spark gap 2-13 at a rate of around 300 Hz.
- circuit parameters can be adjusted to vary the spark discharge characteristics, which in turn affects the cooling that can be achieved. It is important however in considering changes to the circuit to ensure that there is enough energy stored in the control capacitor 2-6 to drive the spark emissions at the rate and voltages required. That is, the charging part of the circuit 4-1 must be capable of providing the energy demanded by the discharging part 4-2. For example, increasing the discharge frequency across the spark gap should increase the cooling that can be achieved. As a consequence however of the control capacitor 2-6 being required to power the discharge sparks more frequently the total energy stored (/4CV 2 ) should be increased. Care must be taken in increasing this energy that the transformers 2-3, 2-9 are not saturated, with consequent reduction in performance.
- a threshold voltage of at least 3 kV is required to generate a spark that is capable of providing cooling. Increasing this voltage generally improves cooling performance, but this effect appears to become saturated at around 4.5 - 5 kV.
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- Engineering & Computer Science (AREA)
- Physics & Mathematics (AREA)
- Mechanical Engineering (AREA)
- Thermal Sciences (AREA)
- General Engineering & Computer Science (AREA)
- Generation Of Surge Voltage And Current (AREA)
- Other Air-Conditioning Systems (AREA)
- Plasma Technology (AREA)
Abstract
Description
Claims
Priority Applications (5)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
CN2008801225058A CN101910755B (en) | 2007-10-24 | 2008-10-23 | Cooling device |
AU2008315755A AU2008315755A1 (en) | 2007-10-24 | 2008-10-23 | Cooling device |
JP2010530563A JP2011502238A (en) | 2007-10-24 | 2008-10-23 | Air conditioner |
EP08806791A EP2245390A1 (en) | 2007-10-24 | 2008-10-23 | Cooling device |
US12/739,237 US20100242498A1 (en) | 2007-10-24 | 2008-10-23 | Cooling Device |
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
GB0720939.8 | 2007-10-24 | ||
GBGB0720939.8A GB0720939D0 (en) | 2007-10-24 | 2007-10-24 | Coolign device |
Publications (1)
Publication Number | Publication Date |
---|---|
WO2009053746A1 true WO2009053746A1 (en) | 2009-04-30 |
Family
ID=38829919
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
PCT/GB2008/050984 WO2009053746A1 (en) | 2007-10-24 | 2008-10-23 | Cooling device |
Country Status (7)
Country | Link |
---|---|
US (1) | US20100242498A1 (en) |
EP (1) | EP2245390A1 (en) |
JP (1) | JP2011502238A (en) |
CN (1) | CN101910755B (en) |
AU (1) | AU2008315755A1 (en) |
GB (1) | GB0720939D0 (en) |
WO (1) | WO2009053746A1 (en) |
Families Citing this family (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US9429344B2 (en) * | 2014-06-17 | 2016-08-30 | Palo Alto Research Center Incorporated | Electrocaloric system with active regeneration |
Citations (4)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
GB1110575A (en) * | 1965-08-04 | 1968-04-18 | Inter Probe | Method and apparatus for lowering the temperature of a heated body |
US3938345A (en) * | 1973-10-06 | 1976-02-17 | Agency Of Industrial Science & Technology | Cooling method by use of corona discharge |
US20060130489A1 (en) * | 2004-12-17 | 2006-06-22 | Weaver Stanton E Jr | Thermal transfer device and system and method incorporating same |
US20070053394A1 (en) * | 2005-09-06 | 2007-03-08 | Cox Isaiah W | Cooling device using direct deposition of diode heat pump |
Family Cites Families (19)
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US1959374A (en) * | 1932-10-01 | 1934-05-22 | Int Precipitation Co | Method and apparatus for electrical precipitation |
US2433755A (en) * | 1942-06-12 | 1947-12-30 | Vickers Electrical Co Ltd | Spark gap electrical apparatus |
JPS5326471B2 (en) * | 1972-03-15 | 1978-08-02 | ||
JPS50143171A (en) * | 1974-05-07 | 1975-11-18 | ||
US4563608A (en) * | 1982-11-08 | 1986-01-07 | The United States Of America As Represented By The United States Department Of Energy | Gas flow stabilized megavolt spark gap for repetitive pulses |
DE3513422C2 (en) * | 1985-04-15 | 1993-10-28 | Beru Werk Ruprecht Gmbh Co A | Ignition system for internal combustion engines |
CN1055594A (en) * | 1991-04-05 | 1991-10-23 | 北京理工大学 | Unit-construction water cooler for radio-frequency discharge electrodes |
CN1097387A (en) * | 1993-03-29 | 1995-01-18 | 谢经湟 | Rectifying and filtering device of air anion generator of automobile and tractor |
CN2201629Y (en) * | 1994-04-29 | 1995-06-21 | 肖立云 | Differential temp electrical refrigerating unit with plasmd gas producer |
JPH10215526A (en) * | 1996-12-01 | 1998-08-11 | Hiroyuki Matsuda | Power conversion increasing unit |
US6069314A (en) * | 1997-05-16 | 2000-05-30 | Varela; Manuel Domingo | Emitter of ions for a lightning rod with a parabolic reflector |
JP3345318B2 (en) * | 1997-10-17 | 2002-11-18 | 株式会社岡村研究所 | Capacitor power storage device |
CN2390351Y (en) * | 1999-09-13 | 2000-08-02 | 中国科学院安徽光学精密机械研究所 | Voltage-regulated pulse laser power supply |
CN1271834A (en) * | 1999-12-24 | 2000-11-01 | 石运达 | Pulse heat transfer unit with contact capacitor |
JP2002052392A (en) * | 2000-08-09 | 2002-02-19 | Masaaki Takarada | Optical water treatment apparatus and water |
CN2468449Y (en) * | 2000-12-07 | 2002-01-02 | 张征宇 | Means for regulating head temp. |
ATE401963T1 (en) * | 2002-04-11 | 2008-08-15 | Floppy Sprinkler Proprietary L | OUTPUT HOSE FOR IRRIGATION SYSTEM |
JP2005160259A (en) * | 2003-11-28 | 2005-06-16 | Sanyo Electric Co Ltd | High-voltage power circuit |
JP4457021B2 (en) * | 2005-01-24 | 2010-04-28 | 日本特殊陶業株式会社 | Spark plug |
-
2007
- 2007-10-24 GB GBGB0720939.8A patent/GB0720939D0/en not_active Ceased
-
2008
- 2008-10-23 EP EP08806791A patent/EP2245390A1/en not_active Ceased
- 2008-10-23 WO PCT/GB2008/050984 patent/WO2009053746A1/en active Application Filing
- 2008-10-23 JP JP2010530563A patent/JP2011502238A/en active Pending
- 2008-10-23 CN CN2008801225058A patent/CN101910755B/en not_active Expired - Fee Related
- 2008-10-23 AU AU2008315755A patent/AU2008315755A1/en not_active Abandoned
- 2008-10-23 US US12/739,237 patent/US20100242498A1/en not_active Abandoned
Patent Citations (4)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
GB1110575A (en) * | 1965-08-04 | 1968-04-18 | Inter Probe | Method and apparatus for lowering the temperature of a heated body |
US3938345A (en) * | 1973-10-06 | 1976-02-17 | Agency Of Industrial Science & Technology | Cooling method by use of corona discharge |
US20060130489A1 (en) * | 2004-12-17 | 2006-06-22 | Weaver Stanton E Jr | Thermal transfer device and system and method incorporating same |
US20070053394A1 (en) * | 2005-09-06 | 2007-03-08 | Cox Isaiah W | Cooling device using direct deposition of diode heat pump |
Also Published As
Publication number | Publication date |
---|---|
AU2008315755A1 (en) | 2009-04-30 |
GB0720939D0 (en) | 2007-12-05 |
JP2011502238A (en) | 2011-01-20 |
US20100242498A1 (en) | 2010-09-30 |
CN101910755B (en) | 2013-05-29 |
EP2245390A1 (en) | 2010-11-03 |
CN101910755A (en) | 2010-12-08 |
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