WO2002013302A8 - Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it - Google Patents

Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it

Info

Publication number
WO2002013302A8
WO2002013302A8 PCT/NL2001/000621 NL0100621W WO0213302A8 WO 2002013302 A8 WO2002013302 A8 WO 2002013302A8 NL 0100621 W NL0100621 W NL 0100621W WO 0213302 A8 WO0213302 A8 WO 0213302A8
Authority
WO
WIPO (PCT)
Prior art keywords
electrode
mixed oxide
oxide material
approximately
electrochemical cell
Prior art date
Application number
PCT/NL2001/000621
Other languages
French (fr)
Other versions
WO2002013302A1 (en
Inventor
Heuveln Frederik Hendrik Van
Lambertus Plomp
Gerard Douwe Elzinga
Original Assignee
Energieonderzoek Ct Nederland
Heuveln Frederik Hendrik Van
Lambertus Plomp
Gerard Douwe Elzinga
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Priority claimed from NL1015886A external-priority patent/NL1015886C2/en
Priority claimed from NL1017632A external-priority patent/NL1017632C1/en
Priority claimed from NL1018266A external-priority patent/NL1018266C1/en
Priority to JP2002518555A priority Critical patent/JP2004506302A/en
Priority to EP01972803A priority patent/EP1320906A1/en
Priority to HU0302080A priority patent/HUP0302080A2/en
Priority to PL36043701A priority patent/PL360437A1/en
Priority to KR10-2003-7001740A priority patent/KR20030038687A/en
Application filed by Energieonderzoek Ct Nederland, Heuveln Frederik Hendrik Van, Lambertus Plomp, Gerard Douwe Elzinga filed Critical Energieonderzoek Ct Nederland
Priority to NZ523942A priority patent/NZ523942A/en
Priority to US10/344,083 priority patent/US20040089540A1/en
Priority to IL15420401A priority patent/IL154204A0/en
Priority to AU2001292443A priority patent/AU2001292443A1/en
Priority to CA002417013A priority patent/CA2417013A1/en
Publication of WO2002013302A1 publication Critical patent/WO2002013302A1/en
Publication of WO2002013302A8 publication Critical patent/WO2002013302A8/en

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    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G51/00—Compounds of cobalt
    • C01G51/40—Cobaltates
    • C01G51/66—Cobaltates containing alkaline earth metals, e.g. SrCoO3
    • C01G51/68—Cobaltates containing alkaline earth metals, e.g. SrCoO3 containing rare earth, e.g. La0.3Sr0.7CoO3
    • C—CHEMISTRY; METALLURGY
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    • C04B35/00—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products
    • C04B35/01—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES, LIGHT-SENSITIVE OR TEMPERATURE-SENSITIVE DEVICES OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/22—Electrodes
    • H01G11/30—Electrodes characterised by their material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES, LIGHT-SENSITIVE OR TEMPERATURE-SENSITIVE DEVICES OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/22—Electrodes
    • H01G11/30—Electrodes characterised by their material
    • H01G11/46—Metal oxides
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES, LIGHT-SENSITIVE OR TEMPERATURE-SENSITIVE DEVICES OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/84—Processes for the manufacture of hybrid or EDL capacitors, or components thereof
    • H01G11/86—Processes for the manufacture of hybrid or EDL capacitors, or components thereof specially adapted for electrodes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H—ELECTRICITY
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    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
    • H—ELECTRICITY
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    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
    • H01M4/9025—Oxides specially used in fuel cell operating at high temperature, e.g. SOFC
    • H01M4/9033—Complex oxides, optionally doped, of the type M1MeO3, M1 being an alkaline earth metal or a rare earth, Me being a metal, e.g. perovskites
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    • C01P2002/30—Three-dimensional structures
    • C01P2002/34—Three-dimensional structures perovskite-type (ABO3)
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    • C01P2002/54—Solid solutions containing elements as dopants one element only
    • C—CHEMISTRY; METALLURGY
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3205—Alkaline earth oxides or oxide forming salts thereof, e.g. beryllium oxide
    • C04B2235/3213—Strontium oxides or oxide-forming salts thereof
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
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    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3224—Rare earth oxide or oxide forming salts thereof, e.g. scandium oxide
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
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    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/327—Iron group oxides, their mixed metal oxides, or oxide-forming salts thereof
    • C04B2235/3272—Iron oxides or oxide forming salts thereof, e.g. hematite, magnetite
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/327—Iron group oxides, their mixed metal oxides, or oxide-forming salts thereof
    • C04B2235/3275—Cobalt oxides, cobaltates or cobaltites or oxide forming salts thereof, e.g. bismuth cobaltate, zinc cobaltite
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3289—Noble metal oxides
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3296—Lead oxides, plumbates or oxide forming salts thereof, e.g. silver plumbate
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES, LIGHT-SENSITIVE OR TEMPERATURE-SENSITIVE DEVICES OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/04—Hybrid capacitors
    • H01G11/06—Hybrid capacitors with one of the electrodes allowing ions to be reversibly doped thereinto, e.g. lithium ion capacitors [LIC]
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    • H01M12/00—Hybrid cells; Manufacture thereof
    • H01M12/04—Hybrid cells; Manufacture thereof composed of a half-cell of the fuel-cell type and of a half-cell of the primary-cell type
    • H01M12/06—Hybrid cells; Manufacture thereof composed of a half-cell of the fuel-cell type and of a half-cell of the primary-cell type with one metallic and one gaseous electrode
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    • H01M4/00—Electrodes
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    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/13—Energy storage using capacitors
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    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
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    • Y02E60/30—Hydrogen technology
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    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T29/00—Metal working
    • Y10T29/49—Method of mechanical manufacture
    • Y10T29/49002—Electrical device making

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  • Engineering & Computer Science (AREA)
  • Chemical & Material Sciences (AREA)
  • Materials Engineering (AREA)
  • Power Engineering (AREA)
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  • Microelectronics & Electronic Packaging (AREA)
  • General Chemical & Material Sciences (AREA)
  • Electrochemistry (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Ceramic Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • General Life Sciences & Earth Sciences (AREA)
  • Geology (AREA)
  • Structural Engineering (AREA)
  • Electric Double-Layer Capacitors Or The Like (AREA)
  • Battery Electrode And Active Subsutance (AREA)
  • Inert Electrodes (AREA)
  • Fuel Cell (AREA)
  • Conductive Materials (AREA)
  • Compositions Of Oxide Ceramics (AREA)
  • Hybrid Cells (AREA)
  • Inorganic Compounds Of Heavy Metals (AREA)

Abstract

The invention relates to a mixed oxide material with a high electron conductivity, of empirical formula ABOY, where y ≠ 3 and where A comprises at least one metal selected from Na, K, Rb, Ca, Ba, La, Pr, Sr, Ce, Nb, Pb, Nd, Sm and Gd, and B comprises at least one metal selected from the group consisting of Cu, Mg, Ti, V, Cr, Mn, Fe, Co, Nb, Mo, W and Zr, where A and B cannot both be Nb and where the compound SrVO2.5 is excluded. The material may be a perovskite-type material, in which y = 3-δ and δ ≠ 0, with values for δ in the range from approximately -0.2 to approximately -0.05 or in the range from +0.05 to +0.7. The material may also be a Brown-Millerite-type material, for which y = 2.5-κ and κ has a value in the range from approximately -0.2 to approximately -0.05 or in the range from +0.05 to approximately 0.3. The invention also describes an electrode for an electrochemical cell which can be produced from a mixed oxide material of this type, a method for producing an electrode from a mixed oxide material and an electrochemical cell which comprises at least one electrode of this type made from mixed oxide material according to the invention.
PCT/NL2001/000621 2000-08-07 2001-07-26 Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it WO2002013302A1 (en)

Priority Applications (10)

Application Number Priority Date Filing Date Title
CA002417013A CA2417013A1 (en) 2000-08-07 2001-07-26 Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it
AU2001292443A AU2001292443A1 (en) 2000-08-07 2001-07-26 Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it
IL15420401A IL154204A0 (en) 2000-08-07 2001-07-26 Mixed oxide active material, electrode and method of manufacturing the electrode and electrochemical cell comprising it
EP01972803A EP1320906A1 (en) 2000-08-07 2001-07-26 Mixed oxide active material, electrode and method of manufacturing the electrode and electrochemical cell comprising it
HU0302080A HUP0302080A2 (en) 2000-08-07 2001-07-26 Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it
PL36043701A PL360437A1 (en) 2000-08-07 2001-07-26 Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it
KR10-2003-7001740A KR20030038687A (en) 2000-08-07 2001-07-26 Mixed oxide material, electrode and method of manufacturing the eletrode and electrochemical cell comprising it
JP2002518555A JP2004506302A (en) 2000-08-07 2001-07-26 Mixed oxide material, electrode, method for manufacturing the electrode, and electrochemical cell including the same
NZ523942A NZ523942A (en) 2000-08-07 2001-07-26 Mixed oxide material of formula ABOy, an electrode comprising said material, and method of manufacturing said electrode for use in an electrochemical cell
US10/344,083 US20040089540A1 (en) 2000-08-07 2001-07-26 Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it

Applications Claiming Priority (6)

Application Number Priority Date Filing Date Title
NL1015886 2000-08-07
NL1015886A NL1015886C2 (en) 2000-08-07 2000-08-07 Mixed oxide material with high electron conductivity, used in production of electrode for electrochemical cell, does not contain metals from platinum group
NL1017632A NL1017632C1 (en) 2001-03-19 2001-03-19 Mixed oxide material with high electron conductivity, used in production of electrode for electrochemical cell, does not contain metals from platinum group
NL1017632 2001-03-19
NL1018266 2001-06-12
NL1018266A NL1018266C1 (en) 2001-06-12 2001-06-12 Mixed oxide material with high electron conductivity, used in production of electrode for electrochemical cell, does not contain metals from platinum group

Publications (2)

Publication Number Publication Date
WO2002013302A1 WO2002013302A1 (en) 2002-02-14
WO2002013302A8 true WO2002013302A8 (en) 2002-05-16

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PCT/NL2001/000621 WO2002013302A1 (en) 2000-08-07 2001-07-26 Mixed oxide material, electrode and method of manufacturing the electrode and electrochemical cell comprising it

Country Status (12)

Country Link
US (1) US20040089540A1 (en)
EP (1) EP1320906A1 (en)
JP (1) JP2004506302A (en)
KR (1) KR20030038687A (en)
AU (1) AU2001292443A1 (en)
CA (1) CA2417013A1 (en)
CZ (1) CZ2003246A3 (en)
HU (1) HUP0302080A2 (en)
IL (1) IL154204A0 (en)
NZ (1) NZ523942A (en)
PL (1) PL360437A1 (en)
WO (1) WO2002013302A1 (en)

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