US3880772A - Composition for ring passivation - Google Patents

Composition for ring passivation Download PDF

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Publication number
US3880772A
US3880772A US278867A US27886772A US3880772A US 3880772 A US3880772 A US 3880772A US 278867 A US278867 A US 278867A US 27886772 A US27886772 A US 27886772A US 3880772 A US3880772 A US 3880772A
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United States
Prior art keywords
chromium
calculated
composition
zinc
boron
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US278867A
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English (en)
Inventor
Romualdes Vatslovovic Rekertas
Romas Romovich Sharmaitis
Juozas Juozovich Matulis
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    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C22/00Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals
    • C23C22/05Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions
    • C23C22/06Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions using aqueous acidic solutions with pH less than 6
    • C23C22/24Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions using aqueous acidic solutions with pH less than 6 containing hexavalent chromium compounds
    • C23C22/30Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions using aqueous acidic solutions with pH less than 6 containing hexavalent chromium compounds containing also trivalent chromium

Definitions

  • trivalent chromium compound (as calculated for chromium): 5.0-20.0 hexavalent chromium compound (as calculated for chromium): 0.1-2.0 nitric acid salt (as calculated for N0 10.0-25.0 boron-containing compound (as calculated for boron): 1.8-6.0
  • the invention is applicable in metal-working industry.
  • the present invention relates to finishing metal parts and has particular reference to a dry composition for the preparation of a solution for bright dipping and colourless passivation of zinc to increase the anticorrosive properties of the zinc-coated parts such as zinc-based alloys, zinc casting, and especially zinc-plated parts.
  • Zinc is known to rapidly corrode under the effects of atmospheric moisture. In order to lengthen the service life and preserve the esthetic appearance of zinccoated parts, such parts may be passivated in acid solutions of trior hexavalent chromium. Prior art liquid aqueous solutions are known for the colourless zinc; passivation which comprise a trivalent chromium compound and nitric acid, or triand hexavalent chromium compounds.
  • Said methods are instrumental in obtaining colourless ornamental films on the zinc surface.
  • incipient traces of corrosion on the zinc surface when tested with a S-percent neutral solution of sodium chloride are found to appear as early as within 10-20 hours of the test period.
  • hexavalent chromium compound (as calculated for chromium): 0.1-2.0; nitric acid salt (as calculated for N 10.0-25.0; boron compound (as calculated for boron): 1.8-6.0.
  • Trivalent chromium compounds are the principal passivating agent. In the present zinc-passivating composition trivalent chromium must be present in an amount of from 50-200 weight parts.
  • a hexavalent chromium compound is an auxiliary passivating substance; its concentration in the passivating composition must be within 0.1 to 2.0 weight parts.
  • Nitric acid salts render oxidating and brightening effects; their concentration in the composition, as calculated the N0 ions is to be maintained within 10.0 to 25.0 weight parts.
  • the boron compounds impart polishing and brightening properties to the present composition; their concentration in the zinc-passivating compositions of the invention, as calculated for boron, should be within 1.8 to 6.0 weight parts.
  • One of the optimum variants of the colourless zinc passivating composition may one incorporating the following constituents (parts by weight):
  • cording to the invention is essentially a mixture of tri- H O. etc. for instance.
  • chromium trioxide ammonium chromates. beryllium chromates. potassium chromates, cadmium chromates, lithium chromates, magnesium chromates, sodium chromates, zinc chromates, bichromates of ammonium, beryllium, potassium, cadmium, lithium, magnesium, sodium, zinc. or mixtures of the afore-mentioned compounds may be used.
  • the nitric acid salts present in the proposed zincpassivating composition may be nitrates of ammonium, beryllium, potassium, cadmium, lithium, magnesium. sodium, zinc, or as mixtures of the abovesaid salts.
  • the sources of boron compounds may be orthoboric acid, magnesium orthoborate, polyborates of ammonium, beryllium, potassium, lithium, magnesium, sodium, as well as a diversity of combinations of the abovementioned compounds.
  • the proposed zinc-passivating composition is a mixture of non-volatile solid chemicals and therefore is distinguished for by its simplicity of preparation, transportation, storage and application.
  • the preparations simplicity resides in an easily obtained passivating solution, and correction and control of the composition thereof. Correction of the passivating solution during its use consists in merely adding chemicals to the zincpassivatin g composition.
  • the present zinc-passivating composition may be prepared, in case of necessity, by conventional mechanical intermixing of the parent components thereof at the site of application.
  • the resultant colourless passive films possess good corrosion resistance.
  • the incipient traces of corrosion on a zinc surface exposed to the effects of a S-percent neutral solution of sodium chloride at 35 1 1C may 1 appear only after from 40-60 testing hours.
  • passivation may be carried out in manual or automatic plants of both the stationary or the rotary type.
  • the passivating composition is prepared by thoroughly mixing the parent substances until a homogeneous mass is obtained. Then the zinc-passivating composition is dissolved in a definite amount of distilled or de- 7 ionized water taking into consideration that the concentration of the trivalent chromium in the resultant passivating solution should be from 3-6 g/l. Acidity of the freshly prepared solution should be within the pH value of 2.1 i 0.3; during the operation the acidity may be corrected by adding some acid, e.g., sulphuric.
  • Objects made from the fine (unalloyed) zinc or zinc casting, or zinc plated are passivated by dipping or spraying same for from 10120s, optimum 30 s at a temperature of to 35C, optimum C, washed with water and dried.
  • a zinc-passivating composition is prepared containing (in parts by weight): chromium sulphate (as calculated for chromium): 10.4 chromium trioxide (as calculated for chromium): 1.1
  • chromium-potassium alum (as calculated for chromium): 10.2
  • chromium trioxide (as calculated for chromium): 1.0
  • ammonium nitrate (as calculated for N0 10.5
  • magnesium orthoborate (as calculated for boron): 4.3
  • the corrosion resistance time of the zinc surface as
  • Example 3 Following the conditions of Example 1 following passivating composition was prepared (in party by weight): chromium nitrate (as calculated for chromium): 10.0 chromium-potassium alum (as calculated for chromium): 10.0 sodium monochromate (as calculated for chromium):
  • EXAMPLE 4 Following the conditions of Example 1. the following passivating composition was prepared (in parts by weight): chromium-potassium alum (as calculated for chromium): 5.0 potassium mono'chromate (as calculated for chromium): 2.0 cadmium nitrate (as calculated for N0 10.0 boric acid (as calculated for boron): 6.0
  • EXAMPLE 5 Following the conditions of Example 1. the following passivating composition was prepared (in parts by weight): chromium-potassium alum (as calculated for chromium): 8.0 sodiumbichromate (as calculated for chromium): 1.0 beryllium nitrate (as calculated for N0 25.0 sodium tetraborate (as calculated for boron): 1.8
  • EXAMPLE 6 Following the conditions of Example 1, the following passivating composition was prepared (in parts by weight): chromium sulphate (as calculated for chromium): 10.5 lithium chromate (as calculated for chromium): 0.5 ammonium bichromate (as calculated for chromium):
  • a composition for passivating zinc comprising a mixture of the following components, in parts by weight of from 5.0 to 20.0 of trivalent chromium compounds, as calculated for the chromium; from 0.1-2.0 hexavalent chromium, as calculated for the chromium; from 10.0 to 25.0 of inorganic salts of nitric acid, as
  • composition for passivating zinc as claimed in claim 1 wherein the mixture comprises a mixture. in parts by weight, of from 8.0 to 13.0 of trivalent chromium compounds, as calculated for the chromium; from 0.7 1.1 of hexavalent chromium, as calculated for the chromium; from 13.0 to 16.0 of of inorganic salts of nitric acid, as calculated for N0 and from 2.5 to 4.5 of boron containing compounds, as calculated for the boron.
  • composition for passivating zinc wherein the mixture consists essentially of the components as claimed in claim 1, and wherein the salts of nitric acid are selected from the group consisting of nitrates of ammonium, of beryllium, of potassium, of cadmium, of lithium, of magnesium, of sodium, of zinc, and of mixtures of said salts.
  • composition as claimed in claim 4, wherein the boron component is selected from the group consisting of orthoboric acid, magnesium orthoborate, polyborates of ammonium, beryllium, potassium, lithium, magnesium, sodium, and mixtures thereof.
  • composition as claimed in claim 1, wherein the trivalent chromium component is selected from the group consisting of chromic sulfates, chromic nitrates, and mixtures thereof.
  • composition as claimed in claim 1, wherein the hexavalent chromium component is selected from the group consisting of chromium trioxide; the chromates and bichromates of ammonium, beryllium, potassium, cadmium, sodium, magnesium, lithium, and

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  • Chemical & Material Sciences (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Chemical Treatment Of Metals (AREA)
US278867A 1971-10-05 1972-08-08 Composition for ring passivation Expired - Lifetime US3880772A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
SU7101702264A SU427614A1 (ru) 1971-10-05 1971-10-05 Состав дл пассисировани цинка

Publications (1)

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US3880772A true US3880772A (en) 1975-04-29

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US278867A Expired - Lifetime US3880772A (en) 1971-10-05 1972-08-08 Composition for ring passivation

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US (1) US3880772A (cs)
CS (1) CS171853B1 (cs)
DD (1) DD99182A1 (cs)
DE (1) DE2244489B2 (cs)
FR (1) FR2156579B1 (cs)
GB (1) GB1358216A (cs)
HU (1) HU164916B (cs)
IT (1) IT965190B (cs)
PL (1) PL84468B1 (cs)
SU (1) SU427614A1 (cs)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3213384A1 (de) * 1981-04-16 1982-12-09 Hooker Chemicals & Plastics Corp., 48089 Warren, Mich. Waessrige saure loesung und verfahren fuer die behandlung aufnahmefaehiger metallsubstrate zur verleihung eines passivierungsfilms
US4756805A (en) * 1985-11-01 1988-07-12 Nihon Parkerizing Co., Ltd. Treatment of galvanized steel

Families Citing this family (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3423990A1 (de) * 1983-07-19 1985-01-31 Omi International Corp., Warren, Mich. Peroxidfreie chrom(iii)-passivierungsloesung und verfahren zum passivieren von substraten mit dieser loesung
ES2046921B1 (es) * 1991-05-13 1994-09-01 Enthone Omi Inc Procedimiento de sellado de revestimientos de conversion de cromato sobre cinc electrodepositado.

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3553034A (en) * 1967-04-20 1971-01-05 Lysaght Australia Ltd Composition and process for inhibiting corrosion of zinc surfaces
US3582368A (en) * 1968-12-30 1971-06-01 Borden Inc Corrosion-inhibiting composition
US3620777A (en) * 1968-07-24 1971-11-16 Hooker Chemical Corp Chromate chemical coating solution for zinc alloy
US3706603A (en) * 1967-06-14 1972-12-19 Albright & Wilson Metal coatings comprising hexavalent chromium,trivalent chromium,silica or a silicate and an alkali metal cation

Family Cites Families (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3121032A (en) * 1960-09-27 1964-02-11 M & T Chemicals Inc Process for applying a protective transparent coating to zinc and cadmium and composition therefor
US3404046A (en) * 1964-09-25 1968-10-01 Hooker Chemical Corp Chromating of zinc and aluminum and composition therefor

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3553034A (en) * 1967-04-20 1971-01-05 Lysaght Australia Ltd Composition and process for inhibiting corrosion of zinc surfaces
US3706603A (en) * 1967-06-14 1972-12-19 Albright & Wilson Metal coatings comprising hexavalent chromium,trivalent chromium,silica or a silicate and an alkali metal cation
US3620777A (en) * 1968-07-24 1971-11-16 Hooker Chemical Corp Chromate chemical coating solution for zinc alloy
US3582368A (en) * 1968-12-30 1971-06-01 Borden Inc Corrosion-inhibiting composition

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3213384A1 (de) * 1981-04-16 1982-12-09 Hooker Chemicals & Plastics Corp., 48089 Warren, Mich. Waessrige saure loesung und verfahren fuer die behandlung aufnahmefaehiger metallsubstrate zur verleihung eines passivierungsfilms
US4756805A (en) * 1985-11-01 1988-07-12 Nihon Parkerizing Co., Ltd. Treatment of galvanized steel

Also Published As

Publication number Publication date
IT965190B (it) 1974-01-31
CS171853B1 (cs) 1976-11-29
DD99182A1 (cs) 1973-07-20
SU427614A1 (ru) 1977-11-05
FR2156579B1 (cs) 1976-08-13
GB1358216A (en) 1974-07-03
PL84468B1 (cs) 1976-04-30
DE2244489A1 (de) 1973-04-12
DE2244489B2 (de) 1979-11-15
FR2156579A1 (cs) 1973-06-01
HU164916B (cs) 1974-05-28

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