RU99111591A - Способ выработки электрической энергии - Google Patents

Способ выработки электрической энергии Download PDF

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RU99111591A
RU99111591A RU99111591/09A RU99111591A RU99111591A RU 99111591 A RU99111591 A RU 99111591A RU 99111591/09 A RU99111591/09 A RU 99111591/09A RU 99111591 A RU99111591 A RU 99111591A RU 99111591 A RU99111591 A RU 99111591A
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Рави ПРАСАД (US)
Рави Прасад
Кристиан Фридрих ГОТТЦМАНН (US)
Кристиан Фридрих ГОТТЦМАНН
Нитин Рамеш КЕСКАР (US)
Нитин Рамеш Кескар
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Праксайр Текнолоджи
Праксайр Текнолоджи, Инк.
Инк. (US)
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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/36—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using oxygen or mixtures containing oxygen as gasifying agents
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
    • B01D53/32—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols by electrical effects other than those provided for in group B01D61/00
    • B01D53/326—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols by electrical effects other than those provided for in group B01D61/00 in electrochemical cells
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B13/00—Oxygen; Ozone; Oxides or hydroxides in general
    • C01B13/02—Preparation of oxygen
    • C01B13/0229—Purification or separation processes
    • C01B13/0248—Physical processing only
    • C01B13/0251—Physical processing only by making use of membranes
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
    • C01B3/386—Catalytic partial combustion
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/06—Combination of fuel cells with means for production of reactants or for treatment of residues
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/06—Combination of fuel cells with means for production of reactants or for treatment of residues
    • H01M8/0662—Treatment of gaseous reactants or gaseous residues, e.g. cleaning
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/1231—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte with both reactants being gaseous or vaporised
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2210/00—Purification or separation of specific gases
    • C01B2210/0043—Impurity removed
    • C01B2210/0046—Nitrogen
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2210/00—Purification or separation of specific gases
    • C01B2210/0043—Impurity removed
    • C01B2210/0051—Carbon dioxide
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2210/00—Purification or separation of specific gases
    • C01B2210/0043—Impurity removed
    • C01B2210/0062—Water
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0068—Solid electrolytes inorganic
    • H01M2300/0071—Oxides
    • H01M2300/0074—Ion conductive at high temperature
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
    • H01M8/04007—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids related to heat exchange
    • H01M8/04014—Heat exchange using gaseous fluids; Heat exchange by combustion of reactants
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
    • H01M8/04007—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids related to heat exchange
    • H01M8/04014—Heat exchange using gaseous fluids; Heat exchange by combustion of reactants
    • H01M8/04022—Heating by combustion
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00—Technologies relating to chemical industry
    • Y02P20/10—Process efficiency
    • Y02P20/129—Energy recovery, e.g. by cogeneration, H2recovery or pressure recovery turbines

Claims (10)

1. Способ выработки электрической энергии и потока газообразного продукта из смеси потока кислородосодержашего газа и первого потока газообразного топлива, в котором изготавливают твердооксидный топливный элемент, имеющий образующую первый катод сторону и образующую первый анод сторону и первый реактор для переноса ионов с расположенной в нем кислородоизбирательной мембраной для переноса ионов, которая имеет образующую второй катод сторону и образующую второй анод сторону; вводят поток кислородосодержащего газа в контакт с образующей первый катод стороной и вводят первый поток газообразного топлива в контакт с образующей первой анод стороной; осуществляют перенос первой части кислорода из указанного потока кислородосодержащего газа от образующей первый катод стороны к образующей первый анод стороне; вводят первую часть кислорода в реакцию с первым потоком газообразного топлива на образующей первый анод стороне с образованием потока электронов от образующей первый анод стороны к образующей первый катод стороне, который используют в качестве электрической энергии; остальную часть потока кислородосодержащего газа направляют в виде первого потока удержанного вещества от образующей первый катод стороны к образующей второй катод стороне; вводят указанный первый поток удержанного вещества в контакт с образующей второй катод стороной и направляют вторую часть кислорода от образующей второй катод стороны к образующей второй анод стороне; и отводят поток газа в качестве потока газообразного продукта, по меньшей мере, от образующей первый катод стороны, образующей первый анод стороны, образующей второй катод стороны и образующей второй анод стороны.
2. Способ по п. 1, в котором поток кислородосодержащего газа включает в себя воздух.
3. Способ по п. 2, в котором дополнительно сжимают воздух перед введением его в контакт с образующей первый катод стороной.
4. Способ по п. 3, в котором дополнительно улавливают кислород в качестве потока газообразного продукта от образующей второй анод стороны.
5. Способ по п. 4, в котором дополнительно вводят поток газообразного удержанного вещества, отходящего от образующей второй катод стороны, в реакцию со вторым потоком газообразного топлива для образования продуктов горения.
6. Способ по п. 5, в котором продукты горения используют для приведения в действие турбины.
7. Способ по п. 2, в котором с помощью рекуперативного теплообменника осуществляют передачу тепла, по меньшей мере, от одного потока - после контактирования потока, по меньшей мере, с одной из образующих первый и второй катоды и образующих первый и второй аноды сторон - к воздуху и к первому потоку газообразного топлива до твердооксидного топливного элемента (по ходу движения потоков).
8. Способ по п. 2, в котором дополнительно омывают образующую второй анод сторону паром при повышенном давлении, в результате чего поток газообразного пропущенного вещества, отходящий от образующей второй анод стороны, содержит смесь пара и кислорода.
9. Способ по п. 8, в котором дополнительно регулируют отношение пара к кислороду в потоке газообразного пропущенного вещества от образующей второй анод стороны до молярного отношения, эффективного для газификации угля.
10. Способ по п. 9, в котором для обеспечения регулирования разделяют поток газообразного пропущенного вещества от образующей второй анод стороны на первую часть и вторую часть, охлаждают вторую часть, удаляют воду из второй части путем конденсации, сжимают оставшийся газ из второй части обратно до давления потока газообразного пропущенного вещества и затем объединяют первую часть и вторую часть.
RU99111591/09A 1998-06-03 1999-06-02 Способ выработки электрической энергии RU99111591A (ru)

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US09/089,513 US6017646A (en) 1998-06-03 1998-06-03 Process integrating a solid oxide fuel cell and an ion transport reactor
US09/089,513 1998-06-03

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US (1) US6017646A (ru)
EP (1) EP0964466B2 (ru)
JP (1) JP3592581B2 (ru)
KR (1) KR100397365B1 (ru)
CN (1) CN1156930C (ru)
AU (1) AU750689B2 (ru)
BR (1) BR9901777A (ru)
CA (1) CA2273550C (ru)
DE (1) DE69900079T2 (ru)
ES (1) ES2155726T3 (ru)
ID (1) ID23281A (ru)
RU (1) RU99111591A (ru)
ZA (1) ZA993721B (ru)

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BR9901777A (pt) 2000-01-04
AU750689B2 (en) 2002-07-25
CA2273550C (en) 2003-10-14
CA2273550A1 (en) 1999-12-03
DE69900079T2 (de) 2001-09-13
EP0964466A1 (en) 1999-12-15
JP3592581B2 (ja) 2004-11-24
EP0964466B1 (en) 2001-04-11
KR20000005651A (ko) 2000-01-25
EP0964466B2 (en) 2008-09-03
US6017646A (en) 2000-01-25
JP2000003719A (ja) 2000-01-07
CN1239333A (zh) 1999-12-22
ES2155726T3 (es) 2001-05-16
AU3238199A (en) 1999-12-16
ID23281A (id) 2000-04-05
ZA993721B (en) 1999-12-02
DE69900079D1 (de) 2001-05-17
CN1156930C (zh) 2004-07-07
KR100397365B1 (ko) 2003-09-13

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