RU2003113528A - RUBBER MIXTURE CONTAINING A BINDING AGENT POLYFUNCTIONAL ORGANOSILANE - Google Patents

RUBBER MIXTURE CONTAINING A BINDING AGENT POLYFUNCTIONAL ORGANOSILANE

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RU2003113528A
RU2003113528A RU2003113528/04A RU2003113528A RU2003113528A RU 2003113528 A RU2003113528 A RU 2003113528A RU 2003113528/04 A RU2003113528/04 A RU 2003113528/04A RU 2003113528 A RU2003113528 A RU 2003113528A RU 2003113528 A RU2003113528 A RU 2003113528A
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composition according
hydroxysilane
radicals
function
different
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Жан-Клод ТАРДИВА
Сальваторе Пагано
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Сосьете Де Текнолоджи Мишлен
Мишлен Решерш Э Текник С.А.
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1. Эластомерная композиция на основе по меньшей мере одного диенового эластомера, неорганического наполнителя в качестве усиливающего наполнителя, полифункционального органосилана в качестве связывающего агента (для системы неорганический наполнитель/диеновый эластомер), имеющего по меньшей мере две функциональные группы, обозначаемые X и Y, который может быть привит, с одной стороны, к эластомеру с помощью функции Х и, с другой стороны, к неорганическому наполнителю с помощью функции Y, отличающаяся тем, что названная функция Y является гидроксисилильной функцией (≡Si-OH).1. An elastomeric composition based on at least one diene elastomer, an inorganic filler as a reinforcing filler, a polyfunctional organosilane as a binding agent (for the inorganic filler / diene elastomer system) having at least two functional groups, X and Y, which can be grafted, on the one hand, to an elastomer using function X and, on the other hand, to an inorganic filler using function Y, characterized in that said function Y is r hydroxy-silyl function (≡ Si-OH). 2. Композиция по п.1, для которой диеновый эластомер выбирают из группы, в которую входят полибутадиены, натуральный каучук, синтетические полиизопрены, сополимеры бутадиена, сополимеры изопрена и смеси этих сополимеров.2. The composition according to claim 1, for which the diene elastomer is selected from the group consisting of polybutadiene, natural rubber, synthetic polyisoprene, butadiene copolymers, isoprene copolymers and mixtures of these copolymers. 3. Композиция по п.2, для которой сополимеры бутадиена и сополимеры изопрена выбирают из бутадиен-стирольных сополимеров, бутадиен-изопреновых сополимеров, изопрен-стирольных сополимеров, бутадиен-акрилонитрильных сополимеров, бутадиен-стирол-изопреновых сополимеров и смесей этих сополимеров.3. The composition according to claim 2, for which the butadiene copolymers and isoprene copolymers are selected from styrene-butadiene copolymers, isoprene-styrene copolymers, styrene-butadiene copolymers, butadiene-styrene-isoprene copolymers and mixtures thereof. 4. Композиция по любому из пп.1-3, содержащая от 10 до 200 (вес. частей на 100 вес. частей эластомера) неорганического усиливающего наполнителя.4. The composition according to any one of claims 1 to 3, containing from 10 to 200 (wt. Parts per 100 wt. Parts of elastomer) inorganic reinforcing filler. 5. Композиция по любому из пп.1-4, в которой количество гидроксисилана находится в пределах от 1 до 20.5. The composition according to any one of claims 1 to 4, in which the amount of hydroxysilane is in the range from 1 to 20. 6. Композиция по любому из пп.1-5, в которой гидроксисилан имеет серусодержащую группу в качестве функции Х и преимущественно является полисульфидом гидроксисилана.6. The composition according to any one of claims 1 to 5, in which the hydroxysilane has a sulfur-containing group as a function of X and is preferably a hydroxysilane polysulfide. 7. Композиция по п.6, в которой гидроксисилан отвечает общей формуле7. The composition according to claim 6, in which hydroxysilane meets the General formula
Figure 00000001
Figure 00000001
 в которой радикалы R, одинаковые или разные, означают углеводородные группы, содержащие преимущественно от 1 до 15 атомов углерода;in which the radicals R, identical or different, mean hydrocarbon groups containing mainly from 1 to 15 carbon atoms; радикалы R’, одинаковые или разные, означают двухвалентные связывающие группы, содержащие преимущественно от 1 до 18 атомов углерода;R ’radicals, identical or different, mean divalent linking groups containing predominantly from 1 to 18 carbon atoms; а и b, одинаковые или разные, равны 1 или 2;a and b, the same or different, are equal to 1 or 2; x больше или равен 2.x is greater than or equal to 2. 8. Композиция по любому из пп.1-7, в которой гидроксисиланом является моногидроксисилан (a=b=1).8. The composition according to any one of claims 1 to 7, in which the hydroxysilane is monohydroxysilane (a = b = 1). 9. Композиция по п.7 или 8, в которой радикалы R выбирают из C1-С6-алкилов, С5С8-циклоалкилов и радикала фенила, а радикалы R’ выбирают из С1-С18-алкиленов и С6-С12-ариленов.9. The composition according to claim 7 or 8, in which the radicals R are selected from C 1 -C 6 -alkyls, C 5 C 8 -cycloalkyls and a phenyl radical, and the radicals R 'are selected from C 1 -C 18 -alkylenes and C 6 -C 12 arylenes. 10. Композиция по п.9, в которой радикалы R выбирают из C1-С6-алкилов, а радикалы R’ из C1-С10-алкиленов.10. The composition according to claim 9, in which the radicals R are selected from C 1 -C 6 -alkyls, and the radicals R 'from C 1 -C 10 -alkylene. 11. Композиция по п.10, в которой гидроксисилан является полисульфидом моногидроксисилана формулы (II)11. The composition of claim 10, in which the hydroxysilane is a polysulfide monohydroxysilane of the formula (II)
Figure 00000002
Figure 00000002
 в которой радикалы R означают C1-С3-алкилы, преимущественно метил;in which R radicals are C 1 -C 3 alkyl, preferably methyl; радикалы R’ означают С1-С4-алкилены, преимущественно метилен, этилен или пропилен;R 'radicals are C 1 -C 4 alkylene, preferably methylene, ethylene or propylene; x больше или равен 2.x is greater than or equal to 2. 12. Композиция по п.11, в которой гидроксисилан является полисульфидом бис(пропилдиметилсиланола) формулы (II-2)12. The composition according to claim 11, in which the hydroxysilane is a polysulfide of bis (propyldimethylsilanol) of the formula (II-2)
Figure 00000003
Figure 00000003
 13. Композиция по любому из пп.1-12, в которой количество гидроксисилана составляет от 0,5 до 20 мас.% от количества неорганического усиливающего наполнителя.13. The composition according to any one of claims 1 to 12, in which the amount of hydroxysilane is from 0.5 to 20 wt.% The amount of inorganic reinforcing filler. 14. Композиция по любому из пп.1-13, в которой преобладающую часть неорганического усиливающего наполнителя составляет кремнезем.14. The composition according to any one of claims 1 to 13, in which the predominant part of the inorganic reinforcing filler is silica. 15. Композиция по любому из пп.1-14, в которой неорганический усиливающий наполнитель составляет все количество усиливающего наполнителя.15. The composition according to any one of claims 1 to 14, in which the inorganic reinforcing filler is the entire amount of reinforcing filler. 16. Композиция по любому из пп.1-14, содержащая, кроме того, углеродную сажу.16. The composition according to any one of claims 1 to 14, containing, in addition, carbon black. 17. Композиция по п.16, в которой углеродная сажа содержится в количестве от 2 до 20 чсэ.17. The composition according to clause 16, in which carbon black is contained in an amount of from 2 to 20 hours. 18. Композиция по п.17, в которой углеродная сажа содержится в количестве от 5 до 15.18. The composition according to 17, in which the carbon black is contained in an amount of from 5 to 15. 19. Композиция по любому из пп.2-18, в которой диеновым эластомером является бутадиен-стирольный сополимер (SBR) с содержанием стирола в пределах от 20 до 30 мас.%, содержанием виниловых связей в бутадиеновой части в пределах от 15 до 65%, содержанием связей транс-1,4 в пределах от 20 до 75% и температурой стеклования в пределах от -20 до -55°С.19. The composition according to any one of claims 2 to 18, in which the diene elastomer is a styrene butadiene copolymer (SBR) with a styrene content in the range from 20 to 30 wt.%, Vinyl content in the butadiene portion in the range from 15 to 65% , the content of trans-1,4 bonds in the range from 20 to 75% and the glass transition temperature in the range from -20 to -55 ° C. 20. Композиция по п.19, в которой бутадиен-стирольный сополимер является сополимером, полученным в растворе.20. The composition according to claim 19, in which the styrene-butadiene copolymer is a copolymer obtained in solution. 21. Композиция по п.19 или 20, в которой бутадиен-стирольный сополимер применяют в смеси с полибутадиеном.21. The composition according to claim 19 or 20, in which the styrene-butadiene copolymer is used in a mixture with polybutadiene. 22. Композиция по п.21, в которой полибутадиен имеет 90% связей цис-1,4.22. The composition of claim 21, wherein the polybutadiene has 90% cis-1,4 bonds. 23. Композиция по любому из пп.2-18, в которой диеновым эластомером является изопреновый эластомер, преимущественно синтетический полиизопрен или натуральный каучук.23. The composition according to any one of claims 2 to 18, in which the diene elastomer is an isoprene elastomer, preferably synthetic polyisoprene or natural rubber. 24. Композиция по любому из пп.1-23, отличающаяся тем, что она находится в вулканизованном состоянии.24. The composition according to any one of claims 1 to 23, characterized in that it is in a vulcanized state. 25. Способ получения эластомерной композиции с улучшенной кинетикой вулканизации, отличающийся тем, что в по меньшей мере один диеновый эластомер вводят по меньшей мере один неорганический наполнитель в качестве усиливающего наполнителя и полифункциональный органосилан в качестве связывающего агента (для системы неорганический наполнитель/диеновый эластомер), имеющий по меньшей мере две функциональные группы, обозначаемые X и Y, который может быть привит, с одной стороны, к эластомеру с помощью функции Х и, с другой стороны, к неорганическому наполнителю с помощью функции У, которая является гидроксисилильной функцией (≡Si-OH), и что полученную смесь перемешивают термомеханически в одну или две стадии до достижения максимальной температуры от 110 до 190°С.25. A method of obtaining an elastomeric composition with improved kinetics of vulcanization, characterized in that at least one diene elastomer is injected with at least one inorganic filler as a reinforcing filler and polyfunctional organosilane as a binding agent (for the inorganic filler / diene elastomer system), having at least two functional groups, denoted by X and Y, which can be grafted, on the one hand, to the elastomer using function X and, on the other hand, to inorganic to the filler using function Y, which is a hydroxysilyl function (≡Si-OH), and that the resulting mixture is thermomechanically mixed in one or two stages until a maximum temperature of 110 to 190 ° C is reached. 26. Способ по п.25, в котором органосиланом является серусодержащий гидроксисилан, преимущественно полисульфид гидроксисилана.26. The method according A.25, in which the organosilane is a sulfur-containing hydroxysilane, mainly polysulfide hydroxysilane. 27. Способ по п.26, в котором полисульфид гидроксисилана отвечает общей формуле (I)27. The method according to p, in which the hydroxysilane polysulfide meets the General formula (I)
Figure 00000004
Figure 00000004
 в которой радикалы R, одинаковые или разные, означают углеводородные группы, содержащие преимущественно от 1 до 15 атомов углерода;in which the radicals R, identical or different, mean hydrocarbon groups containing mainly from 1 to 15 carbon atoms; радикалы R’, одинаковые или разные, означают двухвалентные связывающие группы, содержащие преимущественно от 1 до 18 атомов углерода;R ’radicals, identical or different, mean divalent linking groups containing predominantly from 1 to 18 carbon atoms; а и b, одинаковые или разные, равны 1 или 2;a and b, the same or different, are equal to 1 or 2; x больше или равен 2.x is greater than or equal to 2. 28. Способ по п.27, в котором гидроксисиланом является моногидроксисилан (a=b=1).28. The method according to item 27, in which the hydroxysilane is monohydroxysilane (a = b = 1). 29. Применение каучуковой композиции по любому из пп.1-24 для производства пневмошин или для производства полупродуктов, предназначенных для этих пневмошин, причем эти полупродукты относятся, в частности, к группе, в которую входят протекторы, подслои, верхние слои, боковины, каркасные слои, закраины, защитные слои, воздушные камеры и внутренние уплотнительные резины для бескамерных пневмошин.29. The use of the rubber composition according to any one of claims 1 to 24 for the manufacture of pneumatic tires or for the production of intermediates intended for these pneumatic tires, and these intermediates belong, in particular, to the group of treads, sublayers, upper layers, sidewalls, carcasses layers, flanges, protective layers, air chambers and internal sealing rubbers for tubeless pneumatic tires. 30. Пневмошина, содержащая каучуковую композицию по любому из пп.1-24.30. A pneumatic tire containing a rubber composition according to any one of claims 1 to 24. 31. Полупродукт для пневмошины, содержащий каучуковую композицию по любому из пп.1-24, относящийся, в частности, к группе, в которую входят протекторы, подслои для протекторов, верхние слои, боковины, каркасные слои, закраины, защитные слои, воздушные камеры и внутренняя уплотнительная резина для бескамерных пневмошин.31. The intermediate product for the pneumatic tire containing the rubber composition according to any one of claims 1 to 24, relating, in particular, to the group of treads, underlayers for treads, upper layers, sidewalls, carcass layers, flanges, protective layers, air chambers and internal sealing rubber for tubeless pneumatic tires. 32. Полупродукт по п.31, представляющий собой протектор для пневмошины.32. The intermediate product of claim 31, which is a tread for a pneumatic tire. 33. Протектор для пневмошины описанный в п.32, изготовленный из каучуковой композиции по любому из пп.19-23.33. A tread for a pneumatic tire described in clause 32, made of a rubber composition according to any one of paragraphs 19-23. 34. Пневмошина, содержащая протектор по п.33.34. A pneumatic tire comprising a tread according to claim 33. 35. Применение (для системы неорганический наполнитель/диеновый эластомер) в композиции на основе диенового эластомера, усиленного неорганическим наполнителем, полифункционального органосилана, имеющего по меньшей мере две функции, обозначаемые X и Y, который может быть привит, с одной стороны, к эластомеру с помощью функции Х и, с другой стороны, к неорганическому наполнителю с помощью функции Y, которая является гидроксисилильной функцией (≡Si-OH), в качестве связующего агента.35. The use (for the inorganic filler / diene elastomer system) in a composition based on a diene elastomer reinforced with an inorganic filler, a multifunctional organosilane having at least two functions, designated X and Y, which can be grafted, on the one hand, to an elastomer with using function X and, on the other hand, to an inorganic filler using function Y, which is a hydroxysilyl function (≡ Si-OH), as a binding agent. 36. Применение по п.35, в котором органосиланом является серусодержащий гидроксисилан, преимущественно полисульфид гидроксисилана.36. The use of claim 35, wherein the organosilane is a sulfur-containing hydroxysilane, preferably a hydroxysilane polysulfide. 37. Применение по п.36, в котором полисульфид гидроксисилана отвечает общей формуле (I)37. The application of clause 36, in which the hydroxysilane polysulfide meets the General formula (I)
Figure 00000005
Figure 00000005
 в которой радикалы R, одинаковые или разные, означают углеводородные группы, содержащие преимущественно от 1 до 15 атомов углерода;in which the radicals R, identical or different, mean hydrocarbon groups containing mainly from 1 to 15 carbon atoms; радикалы R’, одинаковые или разные, означают двухвалентные связывающие группы, содержащие преимущественно от 1 до 18 атомов углерода;R ’radicals, identical or different, mean divalent linking groups containing predominantly from 1 to 18 carbon atoms; а и b, одинаковые или разные, равны 1 или 2;a and b, the same or different, are equal to 1 or 2; x больше или равен 2.x is greater than or equal to 2. 38. Применение по п.37, в котором гидроксисиланом является моногидроксисилан (a=b=1).38. The use of claim 37, wherein the hydroxysilane is monohydroxysilane (a = b = 1). 39. Способ связывания неорганического и диенового эластомера в эластомерной композиции, отличающийся тем, что в по меньшей мере один диеновый эластомер вводят по меньшей мере один неорганический наполнитель в качестве усиливающего наполнителя и полифункциональный органосилан, имеющий по меньшей мере две функции, обозначаемые X и Y, который может быть привит, с одной стороны, к эластомеру с помощью функции Х и, с другой стороны, к неорганическому наполнителю с помощью функции Y, которая является гидроксисилильной функцией (≡Si-OH), и полученную смесь перемешивают термомеханически в одну или две стадии до достижения максимальной температуры от 110 до 190°С.39. A method of binding an inorganic and diene elastomer in an elastomeric composition, characterized in that at least one inorganic filler is introduced into at least one inorganic filler as a reinforcing filler and a multifunctional organosilane having at least two functions, designated X and Y, which can be grafted, on the one hand, to an elastomer using function X and, on the other hand, to an inorganic filler using function Y, which is a hydroxysilyl function (≡Si-OH), and obtained mixture was stirred thermomechanically in one or two stages, until a maximum temperature of 110 to 190 ° C. 40. Способ по п.39, в котором органосиланом является серусодержащий гидроксисилан, преимущественно полисульфид гидроксисилана.40. The method according to § 39, in which the organosilane is a sulfur-containing hydroxysilane, mainly polysulfide hydroxysilane. 41. Способ по п.40, в котором полисульфид гидроксисилана отвечает общей формуле (I)41. The method according to p, in which the hydroxysilane polysulfide meets the General formula (I)
Figure 00000006
Figure 00000006
 в которой радикалы R, одинаковые или разные, означают углеводородные группы, содержащие преимущественно от 1 до 15 атомов углерода;in which the radicals R, identical or different, mean hydrocarbon groups containing mainly from 1 to 15 carbon atoms; радикалы R’, одинаковые или разные, означают двухвалентные группы, содержащие преимущественно от 1 до 18 атомов углерода;R ’radicals, identical or different, mean divalent groups containing predominantly from 1 to 18 carbon atoms; а и b, одинаковые или разные, равны 1 или 2;a and b, the same or different, are equal to 1 or 2; x больше или равен 2.x is greater than or equal to 2. 42. Способ по п.41, в котором гидроксисиланом является моногидроксисилан (a=b=1).42. The method according to paragraph 41, in which the hydroxysilane is monohydroxysilane (a = b = 1).
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EP3996915A1 (en) 2019-07-09 2022-05-18 Compagnie Generale Des Etablissements Michelin A rubber composition
US20220251270A1 (en) 2019-07-26 2022-08-11 Exxonmobil Chemical Patents Inc. Hydrocarbon Polymer Modifiers Having Low Aromaticity and Uses Thereof
FR3099168B1 (en) 2019-07-26 2021-07-02 Michelin & Cie TIRE INCORPORATING A RUBBER COMPOSITION INCLUDING A SPECIFIC HYDROCARBON RESIN
FR3099169B1 (en) 2019-07-26 2021-07-02 Michelin & Cie TIRE INCORPORATING A RUBBER COMPOSITION INCLUDING A SPECIFIC HYDROCARBON RESIN
FR3099167B1 (en) 2019-07-26 2021-07-02 Michelin & Cie TIRE INCORPORATING A RUBBER COMPOSITION INCLUDING A SPECIFIC HYDROCARBON RESIN
FR3099166B1 (en) 2019-07-26 2022-02-11 Michelin & Cie TIRE INCORPORATING A RUBBER COMPOSITION COMPRISING A SPECIFIC HYDROCARBON RESIN
KR20220029695A (en) 2019-07-26 2022-03-08 엑손모빌 케미칼 패턴츠 인코포레이티드 Hydrocarbon polymer modifier with high aromaticity and use thereof
WO2021019709A1 (en) 2019-07-31 2021-02-04 Compagnie Generale Des Etablissements Michelin A laminate
WO2021019708A1 (en) 2019-07-31 2021-02-04 Compagnie Generale Des Etablissements Michelin A laminate
FR3100811B1 (en) 2019-09-18 2021-09-03 Michelin & Cie Functional ethylene and 1,3-diene copolymers
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FR3101878B1 (en) 2019-10-10 2021-10-01 Michelin & Cie Rubber compositions comprising an epoxidized diene elastomer and a crosslinking system
FR3103775B1 (en) 2019-11-28 2021-11-05 Michelin & Cie RUBBER TRACK INCLUDING POLYVINYL ALCOHOL FIBERS
FR3103819B1 (en) 2019-11-28 2023-07-21 Michelin & Cie OFF-ROAD TREAD INCLUDING POLYVINYL ALCOHOL FIBERS
EP4096935B1 (en) 2020-01-28 2024-03-13 Compagnie Generale Des Etablissements Michelin A rubber composition
WO2021166165A1 (en) 2020-02-20 2021-08-26 Compagnie Generale Des Etablissements Michelin A rubber composition
WO2021166166A1 (en) 2020-02-20 2021-08-26 Compagnie Generale Des Etablissements Michelin A rubber composition
EP4126563A1 (en) 2020-03-27 2023-02-08 Compagnie Generale Des Etablissements Michelin An article intended to come into contact with the ground, in particular a tire
FR3108910B1 (en) 2020-04-07 2023-06-02 Michelin & Cie RUBBER COMPOSITION COMPRISING POLYETHYLENE WITH A LOW MELTING TEMPERATURE
FR3109156B1 (en) 2020-04-09 2023-10-06 Michelin & Cie RUBBER COMPOSITION COMPRISING POLYAMIDE AT LOW MELTING TEMPERATURE
CN111823433A (en) * 2020-06-04 2020-10-27 江门市鑫辉密封科技有限公司 Mixing method for improving tensile strength of rubber
FR3111352B1 (en) 2020-06-11 2023-02-10 Michelin & Cie RUBBER COMPOSITION WITH IMPROVED RESISTANCE TO AGGRESSION
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FR3113906B1 (en) 2020-09-04 2022-08-05 Michelin & Cie RUBBER COMPOSITION BASED ON HIGHLY SATURATED DIENIQUE ELASTOMER
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FR3115542B1 (en) 2020-10-23 2023-12-15 Michelin & Cie Radio frequency communication module comprising an electronic device coated in an elastomeric material
FR3117123B1 (en) 2020-12-09 2023-12-15 Michelin & Cie RUBBER COMPOSITION WITH IMPROVED RESISTANCE TO MECHANICAL ASSEMBLY
FR3117122B1 (en) 2020-12-09 2023-12-15 Michelin & Cie TIRE FOR OFF-ROAD VEHICLES
FR3119169B1 (en) 2021-01-26 2022-12-30 Michelin & Cie TIRE INCORPORATING A RUBBER COMPOSITION COMPRISING A SPECIFIC HYDROCARBON RESIN
FR3119168B1 (en) 2021-01-26 2023-01-13 Michelin & Cie TIRE INCORPORATING A RUBBER COMPOSITION COMPRISING A SPECIFIC HYDROCARBON RESIN
WO2022164716A1 (en) 2021-01-26 2022-08-04 Exxonmobil Chemical Patents Inc. Hydrocarbon polymer modifiers having high aromaticity and low molecular weight and uses thereof
WO2022162823A1 (en) 2021-01-28 2022-08-04 Compagnie Generale Des Etablissements Michelin An article, in particular a tire
FR3121144B1 (en) 2021-03-29 2023-03-31 Michelin & Cie Composite comprising a metallic reinforcing element and an elastomeric composition comprising an adhesion promoter resin
FR3121143B1 (en) 2021-03-29 2023-03-03 Michelin & Cie Composite comprising a metallic reinforcing element and an elastomeric composition comprising an adhesion-promoting resin
FR3121145A1 (en) 2021-03-29 2022-09-30 Compagnie Generale Des Etablissements Michelin Composite comprising an elastomeric composition and a metallic reinforcing element
FR3124798A1 (en) 2021-06-30 2023-01-06 Compagnie Generale Des Etablissements Michelin RUBBER COMPOSITION
FR3127495B1 (en) 2021-09-30 2023-08-25 Michelin & Cie RUBBER ARTICLE RESISTANT TO MECHANICAL ASSEMBLY
FR3129396B1 (en) 2021-11-22 2023-11-10 Michelin & Cie Rubber composition
FR3129400B1 (en) 2021-11-22 2023-11-10 Michelin & Cie Rubber composition
FR3129397B1 (en) 2021-11-22 2023-11-10 Michelin & Cie Rubber composition
FR3133857B1 (en) 2022-03-23 2024-03-08 Michelin & Cie Elastomeric composition with improved properties
FR3135983A1 (en) 2022-05-31 2023-12-01 Compagnie Generale Des Etablissements Michelin Process for preparing a diene rubber composition.
FR3136768A1 (en) 2022-06-20 2023-12-22 Compagnie Generale Des Etablissements Michelin Diene rubber composition comprising a microsilica.
FR3138352A1 (en) 2022-07-29 2024-02-02 Compagnie Generale Des Etablissements Michelin Pneumatic with radial carcass reinforcement
FR3138350A1 (en) 2022-07-29 2024-02-02 Compagnie Generale Des Etablissements Michelin Pneumatic with radial carcass reinforcement
FR3138351A1 (en) 2022-07-29 2024-02-02 Compagnie Generale Des Etablissements Michelin Pneumatic with radial carcass reinforcement
FR3140373A1 (en) 2022-10-04 2024-04-05 Compagnie Generale Des Etablissements Michelin TIRE PROVIDED WITH AN EXTERNAL SIDEWALL BASED ON A COMPOSITION COMPRISING pyrolysis carbon black
FR3140374A1 (en) 2022-10-04 2024-04-05 Compagnie Generale Des Etablissements Michelin PNEUMATIC

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