KR20150006243A

KR20150006243A - Perfume Composition Containing Chamaecyparis Obtusa Phytoncide

Info

Publication number: KR20150006243A
Application number: KR20130079789A
Authority: KR
Inventors: 윤병덕
Original assignee: 윤병덕
Priority date: 2013-07-08
Filing date: 2013-07-08
Publication date: 2015-01-16

Abstract

In the present invention, provided is a natural scent composition including phytoncide to increase the antimicrobial activity, antimicrobial spectrum of phytoncide, and uniformity by improving mixture property of each component and to control the induction of skin stimulation. The present invention relates to a scent composition including a phytoncide, comprising 75-85 wt% of purified water and 15-25 wt% of mixture extracts including 75-85 wt% of phytincide extract; 14-24 wt% of herb extracts; 0.1-0.5 wt% of fruit extracts; 0.1-0.5 wt% of complex gold extract; and 0.05-0.15 wt% of polysorbate 80.

Description

(Perfume Composition Containing Chamaecyparis Obtusa Phytoncide)

The present invention relates to a perfume composition containing phytoncide, which is used in products such as cosmetics, detergents, and air fresheners that require fragrance ingredients.

Various types of fragrance products have been provided for the purpose of emitting fragrance from a specific object or space. Among them, there is a kind of sticking a direction component to the surface of the specific material in the form of sprinkling or roots to emit a fragrance from a specific product, and a kind of emitting a direction component into the air so as to feel the fragrance in a certain space.

The fragrance materials include natural fragrance and chemical synthetic fragrance, and most of the fragrance added to the fragrance produced in large quantities at present is chemically synthesized fragrance.

However, the fragrance produced by adding such an artificially synthesized chemically synthesized perfume is not natural, and is easily bored when it is used for a long period of time. In addition, it causes an allergy reaction to the skin due to the harmful chemical components contained in the body And since the pharmacological functions useful for the human body can not be expected, recently, interest in perfume using natural plant essential oils extracted from plants is increasing.

It is reasonable to make the main ingredient of the extract of Chungbuk incense extracted from the natural plants such as the whitish whites and spruce trees beneficial to the human body without using the synthetic fragrance so that there is no side effect to the human body and the pharmacological effect due to the useful ingredient of the essential oil It is considered. Chamaecyparis obtusa is an evergreen tree and is used for ornamental, industrial, medicinal purposes. It is made into tubular water and stewed water. It is widely used because it has excellent materials such as wood and wood. In the private sector, it is used as a medicinal ingredient in leaves, burns, epilepsy, frostbite, and fragrance. Essential oil, which is a volatile element present in trees, is a secondary metabolite of plants and has various physiological activities. Essential oil components extracted from coniferous trees such as white saplings provide various functions such as antibacterial, deodorization and insecticide. In particular, the essential oil extracted from the white cotton is a large amount of phytoncide.

Phytoncide is a term created in Russian by the combination of phyton (phyton), which means "plant", and cide, which means "kill." Every plant is attacked by bacteria and insects And emits a protective substance from the stimulus. In this case, the antimicrobial, insecticidal, and sterilizing substance emitted from the plant is phytoncide.

Phytoncide is a 100% natural substance made of terpenes, phenolic compounds, alkaloids and glycosides, which are difficult to artificially synthesize or combine. It is generally absorbed by humans through a forest bath so quickly that bacteria harmful to humans are selectively , It is a pure natural healing therapy which has various effects such as strong antimicrobial and antifungal action without stress, stress relieving, sedative action of the skin, induction of a sleeping face, improvement of allergic skin disease, and improvement of immune function.

As a result, phytoncide ingredients are added to various products that are accessible to everyday life such as fragrances, facial cleansers, cosmetics and medicines for busy modern people who can not often take a forest bath. Is actively promoted.

As a result of the study on phytoncide, the amount of phytoncide emitted from the plant as well as the efficacy of the phytoncide are different, and a large amount of phytoncide occurs in coniferous trees such as pine and pine trees. In particular, It is known that a lot of ingredient content and healing power cause strong phytoncide.

Therefore, the product containing the phytoncide component at present is mainly used essential oil extracted from cottonwood, and the steam distillation method is mainly used as a method of extracting oil from trees such as cottonwood, etc., Most of them are not soluble in water, so they are widely used in such a way that the aroma component is not changed by the heat of steam. Therefore, the study on the directionality and homogeneous diffusivity by the mixing of auxiliary components was poor.

There is a continuing demand for a technology capable of developing a multi-product using the fragrance ingredient of phytoncide.

The present invention provides a natural fragrance composition containing phytoncide, which can increase the antibacterial power of double phytoncide, broaden the antimicrobial spectrum, control the skin irritation, improve the mixing property of each component to increase the uniformity This is the purpose of the task.

Accordingly, the present invention provides, as a first preferred embodiment, 75 to 85% by weight of phytoncide extract; 14-24 wt.% Of herbal extract; From 0.1 to 0.5% by weight of fruit extract; 0.1 to 0.5% by weight of complex gold extract; And 0.05 to 0.15% by weight of polysorbate 80 as an active ingredient.

The herbal extract may be at least one selected from the group consisting of rosemary, lavender, peppermint and chamomile.

Wherein the fruit extract is at least one selected from the group consisting of grapefruit, orange and lemon.

The complex gold extract comprises gold, licorice, jujube and hwanggi.

Wherein the phytoncide extract is extracted by a low-temperature distillation method.

The phytoncide extract is characterized in that it is extracted from a tree selected from the group consisting of perennial, perennial, pine, conifer, cedar and pine.

15 to 25% by weight of the mixed extract; 0.001 to 2% by weight citric acid; 0.001 to 3% by weight of limonene; The purified water is characterized by being a liquid composition in which the residual amount is mixed.

The perfume composition containing the phytoncide of the present invention can be applied to cosmetic compositions, detergent compositions, air freshener compositions, and the like as natural preservatives, synthetic perfumes, and natural compositions without using synthetic colorants.

In addition, the antimicrobial activity and antimicrobial spectrum of phytoncide can be enhanced or widened, the skin irritation can be controlled, and the uniformity can be improved by improving the mixing of each component.

In addition, the perfume composition containing the phytoncide is effective for preventing air pollution such as air cleaning effect, airborne microorganism reduction effect, removal of pathogenic bacteria at the time of cleaning, relieving stress, strengthening intestine and cardiopulmonary function, And so on.

Hereinafter, the present invention will be described in more detail.

The present invention relates to a pharmaceutical composition comprising 75 to 85% by weight of phytoncide extract; 14-24 wt.% Of herbal extract; From 0.1 to 0.5% by weight of fruit extract; 0.1 to 0.5% by weight of complex gold extract; And 0.05 to 0.15% by weight of polysorbate 80 as an active ingredient. The present invention also relates to a perfume composition containing the phytonchide.

[Phytoncide extract]

In the present invention, phytoncide means an oil extract extracted from a tree.

At this time, it is revealed that the tree is any one of the following: woodwort, pine, conifer, cedar, cedar and pine. Particularly, pine trees are preferred to be harvested, and the amount extracted from conifer is higher than that of broad-leaved trees.

The phytoncide of the present invention may be one extracted by a low temperature distillation method.

In this case, the low temperature distillation method is a distillation method in which water vapor generated at the extraction at 40 to 90 ° C is cooled, minimizes the destruction of the distillation component, can heat downward for distillation extraction, and a U- Prepare a steam distillation apparatus consisting of two connected round flasks, and then add jigyeong water or minced water to a single round flask and then heat it to 120 ℃. At this time, the mixture is blended at a ratio of 80-120 parts by weight per 100 parts by weight of Nigiri or Mineral water.

After adding diethyl ether to the other round flask and maintaining the temperature at 40 to 90 ° C for 40 to 60 minutes, when the liquid distilled in the U-shaped glass tube is collected, the liquid is filtered through a filter paper And concentrated under reduced pressure at < RTI ID = 0.0 > 50 C < / RTI > for 30 minutes to remove the diethyl ether to give a white hen extract.

It has the merit of fragrance as raw material, clear color and transparent. When the phytonchid is extracted by the above-mentioned low-temperature distillation method, the phytoncide component is not damaged in its natural state, but the content is high, so that the user can feel the mood in the forest when used.

If the content of the phytoncide extract is less than 75% by weight, the phytoncide flavor may not be sufficient to feel the mood in the forest, and the content of the phytoncide extract may be more than 85% by weight, The content is excessive and the fragrance is not so good.

[Herb Extract]

In the present invention, herbal extracts can be used to increase the antibacterial activity of phytoncide and broaden the antimicrobial spectrum.

The herbal extract may be extracted from at least one herb selected from the group consisting of rosemary, lavender, peppermint and chamomile. The herb extract may be obtained using various extraction methods known in the art, Water, an anhydrous or hydrated lower alcohol having 1 to 4 carbon atoms (methanol, ethanol, propanol, butanol, etc.), a mixed solvent of the lower alcohol and water, acetone, ethyl acetate, chloroform and 1,3-butylene glycol Can be obtained by using a solvent.

The content of the herb extract may be 14 to 24% by weight in the mixed extract. If the content of herbal extract is less than 14% by weight, the antibacterial activity of phytoncide is lowered. If the content of herbal extract is 24% by weight, there is no benefit.

[Fruit extract]

In the present invention, the fruit extract can be used as a natural antiseptic preservative.

The fruit extract is extracted from at least one fruit selected from the group consisting of grapefruit, orange and lemon. The fruit extract can be obtained using various extraction methods known in the art, An extraction solvent selected from the group consisting of anhydrous or lower alcohol having 1 to 4 carbon atoms (methanol, ethanol, propanol, butanol), a mixed solvent of the lower alcohol and water, acetone, ethyl acetate, chloroform and 1,3- . &Lt; / RTI >

In order to obtain the above-mentioned fruit extract, the raw material was washed, and the weight ratio of the raw material and the purified water was added to the extractor at a ratio of 1: 3, and the extract was extracted at 95 ° C for 4 hours. The extract was cooled to 40 ° C, After filtration using a filter (1 ㎛), the filtered extract was concentrated under reduced pressure and heated at 90 캜 for 20 minutes to sterilize the concentrate. The concentrate and maltodextrin were mixed and dissolved in 30% and 70% It is possible.

The content of the fruit extract may be 0.1 to 0.5 wt.% In the mixed extract. If the content of the herbal extract is less than 0.1 wt.%, The sterilization preservation effect is decreased. If the content is 0.5 wt.

[Composite Gold Extract]

In the present invention, the complex gold extract can be used as a natural antiseptic preservative.

Golden (黄芩, Scutellaria baicalensis) is a perennial herb that is a herbaceous perennial plant of the dicotyledonous plant. The roots of gold are said to have an efficacy of cheongryeohwa (淸热泻火) by treating the inflammatory disease with fever (fever) or fire (fever) in oriental medicine to explain the fever and to heat it with a medicinal function. Thus, it is mainly applied to diseases such as fever, seawater (cough), feverish diarrhea, jaundice, and hematemesis (hematemesis), which are caused by external scams invading the human body.

Currently, pharmacologically, baicalin, baicalein, and wogonin have been isolated, and there have been reports of antidiarrheal, antipyretic, anti-inflammatory and anti-cancer effects. These golden extracts have the effect of natural antimicrobial agents in the present invention. Therefore, when the fragrance composition of the present invention is used as a fragrance, it has a strong antibacterial effect against harmful bacteria in the room. In addition, the gold extract can replace synthetic preservatives that can cause skin irritation such as skin allergies and troubles.

To obtain the golden extract, the same distillation extraction method as that of the phytoncide extract can be used. It is needless to say that the extract of Phytoncide extract can be simultaneously extracted with flour, wood chips, and golden roots in the flask.

In the present invention, the complex gold extract means an extract containing gold, licorice, jujube, and hwanggi. The extract contains 20 to 30 parts by weight of licorice, 20 to 30 parts by weight of jujube, 10 to 20 parts by weight And the content of each of the above-mentioned golden, licorice, jujube, and radish is the content optimized to improve the function of the composite gold extract as a natural antiseptic preservative.

The complex gold extract may be obtained by using various extraction methods known in the art, and preferably water, anhydrous or lower alcohol having 1 to 4 carbon atoms (methanol, ethanol, propanol, butanol, etc.) A mixed solvent of alcohol and water, an extraction solvent selected from the group consisting of acetone, ethyl acetate, chloroform and 1,3-butylene glycol.

The content of the complex gold extract may be 0.1 to 0.5 wt% in the mixed extract, and if the content of the complex gold extract is less than 0.1 wt%, the sterilization preservation effect is deteriorated. If the content is 0.5 wt%, there is no benefit.

It is needless to say that when extracting phytoncide extract, it is possible to simultaneously extract the flour and the chrysanthemum, the chrysanthemum, and the golden root together.

[Polysorbate 80]

Polysorbate 80 is a nonionic surfactant, and can improve the mixing property of each component contained in the perfume composition to improve the uniformity.

The content of the polysorbate 80 may be 0.05 to 0.15% by weight in the mixed extract. If the content of polysorbate 80 is less than 0.05% by weight, the uniformity of the perfume composition is lowered. If the content of polysorbate 80 is more than 0.15% There is no profit.

The mixed extract of the perfume composition containing the phytoncide of the present invention contains 75 to 85% by weight of phytoncide; 14-24 wt.% Of herbal extract; From 0.1 to 0.5% by weight of fruit extract; 0.1 to 0.5% by weight of complex gold extract; And 0.05 to 0.15% by weight of polysorbate 80.

On the other hand, the perfume composition containing the phytoncide of the present invention comprises the phytoncide extract as described above; Herbal extracts; Fruit extract; Complex gold extract; And polysorbate 80, and may contain 75 to 85% by weight of purified water in 15 to 25% by weight of the mixed extract, and may be in the form of a transparent liquid having a scent peculiar to scabbins. If the content of the mixed extract is less than 15% by weight or the content of purified water is more than 85% by weight, flavor-specific odor is insignificant. If the content of the mixed extract is more than 25% by weight or the content of purified water is less than 75% The content of the excess may be rather excessive.

The mixing ratio of the other perfume composition is 15 to 25% by weight of the mixed extract; 0.001 to 2% by weight citric acid; 0.001 to 3% by weight of limonene; It is also possible for the purified water to form a liquid composition in which the residual amount is mixed.

Such a perfume composition containing phytoncide can be used for cosmetics, foods, detergents, air fresheners, and the like, and is effective for preventing air pollution such as air cleaning effect, airborne microorganism reduction effect, And so on.

Hereinafter, the present invention will be described in more detail with reference to Examples and Comparative Examples. However, the scope of the present invention is not limited to the following examples.

Example 1

1-1. Phytoncide extract

The phytoncide was subjected to low-temperature distillation by distillative extraction at 40 ° C to 60 ° C by mixing any one or more of woods, pine trees, pine trees, conifer trees, cedar trees and pine trees.

1-2. Herbal extract

The rosemary extract was extracted with methanol.

1-3. Fruit extract

The orange was extracted and extracted with methanol to obtain an orange extract.

1-4. Composite Golden Extract

25 parts by weight of licorice, 25 parts by weight of jujube and 15 parts by weight of sulfur were extracted together with 100 parts by weight of gold, and extracted with methanol to obtain a composite gold extract.

1-5. Polysorbate 80

Polysorbate 80 (Carbonell Korea) was prepared.

The components were mixed according to the composition shown in Table 1 to prepare a mixed extract.

20% by weight of the mixed extract and 80% by weight of purified water were mixed to prepare a liquid perfume composition.

Example 1 to Example 5, Comparative Example 1 to Comparative Example 2

A perfume composition was prepared in the same manner as in Example 1, except that the mixed extract was prepared according to the composition shown in Table 1.

unit
(weight%) Phytoncide
extract Herbal extract Fruit extract Composite Golden Extract Polysorbate 80 ingredient content ingredient content Example 1 80 Rosemary 19.5 grapefruit 0.2 0.2 0.1 Example 2 85 Lavender 14.5 grapefruit 0.2 0.2 0.1 Example 3 75 Peppermint 24 grapefruit 0.5 0.4 0.1 Example 4 80 Rosemary 19.5 Orange 0.2 0.2 0.1 Example 5 80 Rosemary 19.5 lemon 0.2 0.2 0.1 Comparative Example 1 87 Rosemary 12.2 grapefruit 0.2 0.2 0.1 Comparative Example 2 74 Rosemary 15.5 grapefruit 0.2 0.2 0.1

The liquid perfume compositions prepared in Examples and Comparative Examples were sprayed to examine the flavor sensibility against 100 adults of 20 to 30 years old to evaluate the flavor of phytoncide as follows and the results are shown in Table 2 .

Top: High comfort and feeling of phytoncide

Middle: Comfort and feeling of phytoncide smell are normal

B: I can not feel the comfort and the smell of phytoncide

Sensory evaluation of flavor Prize medium Ha Example 1 96 4 0 Example 2 98 2 0 Example 3 99 One 0 Example 4 97 3 0 Example 5 96 4 0 Comparative Example 1 0 41 59 Comparative Example 2 0 37 63

As shown in Table 2, when the content of phytoncide was excessive (Comparative Example 1) or when the content was small (Comparative Example 2), it was found that phytoncide could not feel comfort or smell.

The composition of the present invention may be formulated in the form of powders, capsules, creams, gels, patches, sprays, ointments, etc. by conventional methods known in the art.

The perfume oil to be added to the phytoncide extract is a variety of natural fragrance which is collected from plants having various fragrance (fragrance), such as a soap and pepper flavor, and diffused into the room like phytoncide. As a result, unlike the conventional synthetic fragrance, It works to clear.

Sensory evaluation of flavor preference and mental and physical stability of the phytoncide extract prepared by mixing various natural flavoring agents, such as sour, peppermint, and the like, were conducted. As a result, 10 men and women were selected from each panel. The sensory evaluation was carried out by spraying the citrus fragrance composition of Example 6 in a panel room of 3 m in length, 3 m in length and 2 m in height without pollution, and then evaluated by a 5-point scale method in which the evaluators were kept in the panel room for 10 minutes. As a comparative example, a typical spray-type aromatic agent containing a synthetic fragrance as a main component was used, and the results are shown in Table 3 below

division Flavor preference Stability effect Example 6 4.7 4.6 Comparative Example 2.5 2.5

1: Very bad, 2: Bad, 3: Normal, 4: Good, 5: Very good

As shown in Table 3 above, the flavor preference and the stabilizing effect were excellent in the examples. In the case of the comparative example, the odor preference and the stabilizing effect were significantly lower than those of Example 6. From the above results, it can be confirmed that the phytoncide composition of the present invention is excellent in flavor and mood stability and sedative effect.

Particularly, the present invention is expected to have full effect of forest bath without any side effects because natural phytoncide extracts extracted from white flakes use various natural fragrances which are commercialized such as sour flavor, pepper flavor and the like.

While the present invention has been described in connection with what is presently considered to be practical exemplary embodiments, it is to be understood that the invention is not limited to the disclosed embodiments, but, on the contrary, is intended to cover various modifications and equivalent arrangements included within the spirit and scope of the appended claims. .

Claims

75 to 85% by weight of phytoncide extract; 14-24 wt.% Of herbal extract; From 0.1 to 0.5% by weight of fruit extract; 0.1 to 0.5% by weight of complex gold extract; And 0.05 to 0.15% by weight of polysorbate 80 as an active ingredient.

The method according to claim 1,
Wherein the herbal extract is at least one selected from the group consisting of rosemary, lavender, peppermint and chamomile.

The method according to claim 1,
Wherein the fruit extract is at least one selected from the group consisting of grapefruit, orange and lemon.

The method according to claim 1,
Wherein the complex gold extract comprises gold, licorice, jujube, and sulfur.

The method according to claim 1 or 4,
Wherein the complex gold extract is extracted by adding 25 wt% of licorice, 25 wt% of jujube, and 15 wt% of sulfur per 100 wt% of gold.

The method according to claim 1,
Wherein the phytoncide extract is extracted by a low-temperature distillation method.

The method according to claim 1,
Wherein the phytoncide extract is extracted from a tree selected from the group consisting of cottonwood, bamboo, pine, conifer, cedar and pine.

The method according to claim 1,
Wherein the liquid composition comprises 15 to 25% by weight of the mixed extract and 75 to 85% by weight of purified water.

The method according to claim 1,
15 to 25% by weight of the mixed extract; 0.001 to 2% by weight citric acid; 0.001 to 3% by weight of limonene; Wherein the purified water is a liquid composition in which residual amounts are mixed.