JPS5939719B2 - 核燃料体とその製法 - Google Patents
核燃料体とその製法Info
- Publication number
- JPS5939719B2 JPS5939719B2 JP51107307A JP10730776A JPS5939719B2 JP S5939719 B2 JPS5939719 B2 JP S5939719B2 JP 51107307 A JP51107307 A JP 51107307A JP 10730776 A JP10730776 A JP 10730776A JP S5939719 B2 JPS5939719 B2 JP S5939719B2
- Authority
- JP
- Japan
- Prior art keywords
- binder
- nuclear fuel
- fuel material
- ammonium
- uranium dioxide
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Expired
Links
- 239000003758 nuclear fuel Substances 0.000 title claims description 57
- 238000004519 manufacturing process Methods 0.000 title description 4
- 239000011230 binding agent Substances 0.000 claims description 74
- 238000005245 sintering Methods 0.000 claims description 53
- FCTBKIHDJGHPPO-UHFFFAOYSA-N uranium dioxide Inorganic materials O=[U]=O FCTBKIHDJGHPPO-UHFFFAOYSA-N 0.000 claims description 52
- 239000000463 material Substances 0.000 claims description 50
- ATRRKUHOCOJYRX-UHFFFAOYSA-N Ammonium bicarbonate Chemical compound [NH4+].OC([O-])=O ATRRKUHOCOJYRX-UHFFFAOYSA-N 0.000 claims description 47
- 239000001099 ammonium carbonate Substances 0.000 claims description 47
- OOAWCECZEHPMBX-UHFFFAOYSA-N oxygen(2-);uranium(4+) Chemical compound [O-2].[O-2].[U+4] OOAWCECZEHPMBX-UHFFFAOYSA-N 0.000 claims description 47
- 239000000203 mixture Substances 0.000 claims description 43
- 238000000034 method Methods 0.000 claims description 31
- 229910000013 Ammonium bicarbonate Inorganic materials 0.000 claims description 26
- 235000012538 ammonium bicarbonate Nutrition 0.000 claims description 26
- 239000007789 gas Substances 0.000 claims description 24
- 239000002245 particle Substances 0.000 claims description 19
- 238000010438 heat treatment Methods 0.000 claims description 12
- WZECUPJJEIXUKY-UHFFFAOYSA-N [O-2].[O-2].[O-2].[U+6] Chemical compound [O-2].[O-2].[O-2].[U+6] WZECUPJJEIXUKY-UHFFFAOYSA-N 0.000 claims description 7
- 229910000439 uranium oxide Inorganic materials 0.000 claims description 6
- 238000001816 cooling Methods 0.000 claims description 5
- 238000002156 mixing Methods 0.000 claims description 5
- BVCZEBOGSOYJJT-UHFFFAOYSA-N ammonium carbamate Chemical compound [NH4+].NC([O-])=O BVCZEBOGSOYJJT-UHFFFAOYSA-N 0.000 claims description 4
- YNSUIDWLZCFLML-UHFFFAOYSA-N azanium;azane;carbamic acid;hydrogen carbonate Chemical group [NH4+].[NH4+].NC([O-])=O.OC([O-])=O YNSUIDWLZCFLML-UHFFFAOYSA-N 0.000 claims description 4
- KXDHJXZQYSOELW-UHFFFAOYSA-N carbonic acid monoamide Natural products NC(O)=O KXDHJXZQYSOELW-UHFFFAOYSA-N 0.000 claims description 4
- 230000006835 compression Effects 0.000 claims description 4
- 238000007906 compression Methods 0.000 claims description 4
- RZKNJSIGVZOHKZ-UHFFFAOYSA-N diazanium carbonic acid carbonate Chemical compound [NH4+].[NH4+].OC(O)=O.OC(O)=O.[O-]C([O-])=O RZKNJSIGVZOHKZ-UHFFFAOYSA-N 0.000 claims description 4
- 229910001938 gadolinium oxide Inorganic materials 0.000 claims description 2
- 229940075613 gadolinium oxide Drugs 0.000 claims description 2
- CMIHHWBVHJVIGI-UHFFFAOYSA-N gadolinium(iii) oxide Chemical compound [O-2].[O-2].[O-2].[Gd+3].[Gd+3] CMIHHWBVHJVIGI-UHFFFAOYSA-N 0.000 claims description 2
- UTDLAEPMVCFGRJ-UHFFFAOYSA-N plutonium dihydrate Chemical compound O.O.[Pu] UTDLAEPMVCFGRJ-UHFFFAOYSA-N 0.000 claims 2
- FLDALJIYKQCYHH-UHFFFAOYSA-N plutonium(IV) oxide Inorganic materials [O-2].[O-2].[Pu+4] FLDALJIYKQCYHH-UHFFFAOYSA-N 0.000 claims 2
- 239000000843 powder Substances 0.000 description 45
- 239000008188 pellet Substances 0.000 description 35
- QGZKDVFQNNGYKY-UHFFFAOYSA-N Ammonia Chemical compound N QGZKDVFQNNGYKY-UHFFFAOYSA-N 0.000 description 23
- -1 Ammonium cations Chemical class 0.000 description 23
- 235000012501 ammonium carbonate Nutrition 0.000 description 21
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Chemical compound O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 17
- 150000001875 compounds Chemical class 0.000 description 15
- CURLTUGMZLYLDI-UHFFFAOYSA-N Carbon dioxide Chemical compound O=C=O CURLTUGMZLYLDI-UHFFFAOYSA-N 0.000 description 14
- 239000000446 fuel Substances 0.000 description 14
- 239000011148 porous material Substances 0.000 description 14
- 150000001450 anions Chemical class 0.000 description 13
- 229910001868 water Inorganic materials 0.000 description 12
- 230000008569 process Effects 0.000 description 9
- 239000000047 product Substances 0.000 description 9
- 229910052770 Uranium Inorganic materials 0.000 description 8
- 238000000465 moulding Methods 0.000 description 8
- JFALSRSLKYAFGM-UHFFFAOYSA-N uranium(0) Chemical compound [U] JFALSRSLKYAFGM-UHFFFAOYSA-N 0.000 description 8
- 229910021529 ammonia Inorganic materials 0.000 description 7
- 239000001569 carbon dioxide Substances 0.000 description 7
- 229910002092 carbon dioxide Inorganic materials 0.000 description 7
- 239000012535 impurity Substances 0.000 description 7
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 description 6
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 description 6
- 230000015572 biosynthetic process Effects 0.000 description 6
- 238000000354 decomposition reaction Methods 0.000 description 6
- 239000001301 oxygen Substances 0.000 description 6
- 229910052760 oxygen Inorganic materials 0.000 description 6
- 239000000919 ceramic Substances 0.000 description 5
- 239000001257 hydrogen Substances 0.000 description 5
- 229910052739 hydrogen Inorganic materials 0.000 description 5
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical group [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 4
- 229910052778 Plutonium Inorganic materials 0.000 description 4
- 229910052799 carbon Inorganic materials 0.000 description 4
- PPQREHKVAOVYBT-UHFFFAOYSA-H dialuminum;tricarbonate Chemical compound [Al+3].[Al+3].[O-]C([O-])=O.[O-]C([O-])=O.[O-]C([O-])=O PPQREHKVAOVYBT-UHFFFAOYSA-H 0.000 description 4
- 239000004033 plastic Substances 0.000 description 4
- OYEHPCDNVJXUIW-UHFFFAOYSA-N plutonium atom Chemical compound [Pu] OYEHPCDNVJXUIW-UHFFFAOYSA-N 0.000 description 4
- 238000003825 pressing Methods 0.000 description 4
- 239000003795 chemical substances by application Substances 0.000 description 3
- 238000005056 compaction Methods 0.000 description 3
- 238000004320 controlled atmosphere Methods 0.000 description 3
- 238000007723 die pressing method Methods 0.000 description 3
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 description 2
- BVKZGUZCCUSVTD-UHFFFAOYSA-L Carbonate Chemical compound [O-]C([O-])=O BVKZGUZCCUSVTD-UHFFFAOYSA-L 0.000 description 2
- 229940118662 aluminum carbonate Drugs 0.000 description 2
- 239000006227 byproduct Substances 0.000 description 2
- 238000012669 compression test Methods 0.000 description 2
- 230000000694 effects Effects 0.000 description 2
- 238000003801 milling Methods 0.000 description 2
- 229910000069 nitrogen hydride Inorganic materials 0.000 description 2
- 239000011860 particles by size Substances 0.000 description 2
- 238000002411 thermogravimetry Methods 0.000 description 2
- ZCUFMDLYAMJYST-UHFFFAOYSA-N thorium dioxide Chemical compound O=[Th]=O ZCUFMDLYAMJYST-UHFFFAOYSA-N 0.000 description 2
- 229910003452 thorium oxide Inorganic materials 0.000 description 2
- ZSLUVFAKFWKJRC-IGMARMGPSA-N 232Th Chemical compound [232Th] ZSLUVFAKFWKJRC-IGMARMGPSA-N 0.000 description 1
- 239000004215 Carbon black (E152) Substances 0.000 description 1
- ZOKXTWBITQBERF-UHFFFAOYSA-N Molybdenum Chemical compound [Mo] ZOKXTWBITQBERF-UHFFFAOYSA-N 0.000 description 1
- 229910052776 Thorium Inorganic materials 0.000 description 1
- 239000000654 additive Substances 0.000 description 1
- 230000002411 adverse Effects 0.000 description 1
- 238000005054 agglomeration Methods 0.000 description 1
- 230000002776 aggregation Effects 0.000 description 1
- 150000003868 ammonium compounds Chemical class 0.000 description 1
- VBIXEXWLHSRNKB-UHFFFAOYSA-N ammonium oxalate Chemical compound [NH4+].[NH4+].[O-]C(=O)C([O-])=O VBIXEXWLHSRNKB-UHFFFAOYSA-N 0.000 description 1
- 150000003863 ammonium salts Chemical class 0.000 description 1
- 238000004458 analytical method Methods 0.000 description 1
- SHZGCJCMOBCMKK-KGJVWPDLSA-N beta-L-fucose Chemical compound C[C@@H]1O[C@H](O)[C@@H](O)[C@H](O)[C@@H]1O SHZGCJCMOBCMKK-KGJVWPDLSA-N 0.000 description 1
- 230000008859 change Effects 0.000 description 1
- 239000003153 chemical reaction reagent Substances 0.000 description 1
- 238000005253 cladding Methods 0.000 description 1
- 239000000356 contaminant Substances 0.000 description 1
- 238000005260 corrosion Methods 0.000 description 1
- 230000007797 corrosion Effects 0.000 description 1
- 230000007423 decrease Effects 0.000 description 1
- 230000001419 dependent effect Effects 0.000 description 1
- 238000009792 diffusion process Methods 0.000 description 1
- 238000009826 distribution Methods 0.000 description 1
- 238000005516 engineering process Methods 0.000 description 1
- 238000003621 hammer milling Methods 0.000 description 1
- 150000004678 hydrides Chemical class 0.000 description 1
- 229930195733 hydrocarbon Natural products 0.000 description 1
- 238000010902 jet-milling Methods 0.000 description 1
- 239000011159 matrix material Substances 0.000 description 1
- VUZPPFZMUPKLLV-UHFFFAOYSA-N methane;hydrate Chemical compound C.O VUZPPFZMUPKLLV-UHFFFAOYSA-N 0.000 description 1
- 238000001000 micrograph Methods 0.000 description 1
- 229910052750 molybdenum Inorganic materials 0.000 description 1
- 239000011733 molybdenum Substances 0.000 description 1
- 229910052757 nitrogen Inorganic materials 0.000 description 1
- 239000011368 organic material Substances 0.000 description 1
- 239000002243 precursor Substances 0.000 description 1
- 238000010298 pulverizing process Methods 0.000 description 1
- 229910001220 stainless steel Inorganic materials 0.000 description 1
- 239000010935 stainless steel Substances 0.000 description 1
- 238000003860 storage Methods 0.000 description 1
- 150000003586 thorium compounds Chemical class 0.000 description 1
Classifications
-
- G—PHYSICS
- G21—NUCLEAR PHYSICS; NUCLEAR ENGINEERING
- G21C—NUCLEAR REACTORS
- G21C3/00—Reactor fuel elements and their assemblies; Selection of substances for use as reactor fuel elements
- G21C3/42—Selection of substances for use as reactor fuel
- G21C3/58—Solid reactor fuel Pellets made of fissile material
- G21C3/62—Ceramic fuel
- G21C3/623—Oxide fuels
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E30/00—Energy generation of nuclear origin
- Y02E30/30—Nuclear fission reactors
Landscapes
- Engineering & Computer Science (AREA)
- Physics & Mathematics (AREA)
- Chemical & Material Sciences (AREA)
- Ceramic Engineering (AREA)
- Plasma & Fusion (AREA)
- General Engineering & Computer Science (AREA)
- High Energy & Nuclear Physics (AREA)
- Inorganic Compounds Of Heavy Metals (AREA)
- Compositions Of Oxide Ceramics (AREA)
- Powder Metallurgy (AREA)
Applications Claiming Priority (1)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| US05/612,084 US4061700A (en) | 1975-09-10 | 1975-09-10 | Fugitive binder for nuclear fuel materials |
Publications (2)
| Publication Number | Publication Date |
|---|---|
| JPS5246299A JPS5246299A (en) | 1977-04-12 |
| JPS5939719B2 true JPS5939719B2 (ja) | 1984-09-26 |
Family
ID=24451655
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| JP51107307A Expired JPS5939719B2 (ja) | 1975-09-10 | 1976-09-09 | 核燃料体とその製法 |
Country Status (10)
Families Citing this family (33)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US4202849A (en) * | 1975-04-07 | 1980-05-13 | General Atomic Company | Method for making nuclear fuel element |
| US4284593A (en) * | 1978-05-26 | 1981-08-18 | United Kingdom Atomic Energy Authority | Preparation of shaped bodies |
| US4383953A (en) * | 1980-01-21 | 1983-05-17 | General Electric Company | Method of improving the green strength of nuclear fuel pellets |
| GB2067536B (en) * | 1980-01-21 | 1983-12-14 | Gen Electric | Nuclear fuel pellets |
| BR8101595A (pt) * | 1980-03-19 | 1981-09-22 | Alkem Gmbh | Processo para a preparacao de tabletes de combustiveis nucleares de oxido misto, soluveis em acido nitrico |
| DE3011227A1 (de) * | 1980-03-22 | 1981-10-01 | Haendler & Natermann GmbH, 3510 Hann Münden | Verfahren und vorrichtung zum etikettieren von behaeltern |
| US4389341A (en) * | 1981-06-15 | 1983-06-21 | General Electric Company | Fugitive binder-containing nuclear fuel material and method of production |
| US4453552A (en) * | 1981-06-22 | 1984-06-12 | Ensign John D | Electronic body temperature indicator |
| US4401608A (en) * | 1981-10-13 | 1983-08-30 | General Electric Company | Method for enlarging grain size of uranium oxide |
| US4427579A (en) | 1981-12-17 | 1984-01-24 | General Electric Company | Method of producing fugitive binder-containing nuclear fuel material |
| US4432915A (en) * | 1982-03-22 | 1984-02-21 | General Electric Company | Method for producing nuclear fuel pellets, and product thereof |
| FR2525208B1 (fr) * | 1982-04-19 | 1986-01-31 | Commissariat Energie Atomique | Procede de traitement d'une poudre d'oxyde metallique et utilisation de la poudre traitee pour la fabrication de pastilles de combustible nucleaire |
| DE3230698A1 (de) * | 1982-08-18 | 1984-02-23 | The Babcock & Wilcox Co., 70160 New Orleans, La. | Kern-brennstoff-herstellung und -abfall-aufbereitung |
| US4575436A (en) * | 1982-08-24 | 1986-03-11 | General Electric Company | Production of nuclear fuel products |
| DE3327640A1 (de) * | 1982-08-24 | 1984-03-01 | General Electric Co., Schenectady, N.Y. | Verbessertes verfahren zur herstellung von kernbrennstoffprodukten |
| DE3326848A1 (de) * | 1982-08-24 | 1984-03-01 | General Electric Co., Schenectady, N.Y. | Verfahren zur herstellung von kernbrennstoffprodukten |
| US4522769A (en) * | 1982-08-24 | 1985-06-11 | General Electric Company | Method for the manufacture of nuclear fuel products |
| US4696769A (en) * | 1983-07-27 | 1987-09-29 | General Electric Company | Method and binder for the manufacture of nuclear fuel pellets, and the product |
| JPS6070393A (ja) * | 1983-07-27 | 1985-04-22 | ゼネラル・エレクトリツク・カンパニイ | 核燃料ペレツト製造用の改良された方法および結合剤並びにそれによつて得られる製品 |
| US4637900A (en) * | 1984-01-13 | 1987-01-20 | The United States Of America As Represented By The United States Department Of Energy | Fabrication of high exposure nuclear fuel pellets |
| US4687605A (en) * | 1985-02-19 | 1987-08-18 | Westinghouse Electric Corp. | Manufacturing automation system for nuclear fuel rod production |
| US4816187A (en) * | 1985-06-17 | 1989-03-28 | General Electric Company | Binder system for the manufacture of nuclear pellets, and the method and product thereof |
| US4670198A (en) * | 1985-06-17 | 1987-06-02 | General Electric Company | Binder system for the manufacture of nuclear fuel pellets, and the method and product thereof |
| DE3802048A1 (de) * | 1988-01-25 | 1989-08-03 | Alkem Gmbh | Verfahren zum herstellen von kernbrennstoffsinterkoerpern |
| JP2689557B2 (ja) * | 1988-12-27 | 1997-12-10 | 三菱マテリアル株式会社 | Ｕｏ▲下２▼ペレットの製造方法 |
| JPH09127290A (ja) * | 1995-11-06 | 1997-05-16 | Mitsubishi Nuclear Fuel Co Ltd | 核燃料ペレットの焼結方法 |
| US6929236B1 (en) | 2002-04-19 | 2005-08-16 | Massachusetts Institute Of Technology | Apparatus for flow rate control |
| US6929235B1 (en) | 2002-04-19 | 2005-08-16 | Massachusetts Institute Of Technology | Apparatus for flow rate control |
| FR2861494B1 (fr) * | 2003-10-28 | 2005-12-23 | Commissariat Energie Atomique | Utilisation de carbonates mixtes frittes pour le confinement de carbone radioactif. |
| US9409825B2 (en) | 2013-08-20 | 2016-08-09 | Los Alamos National Security, Llc | Granulation of fine powder |
| US9437335B2 (en) * | 2013-09-03 | 2016-09-06 | Uchicago Argonne, Llc | Designed porosity materials in nuclear reactor components |
| RU2690155C1 (ru) * | 2018-05-31 | 2019-05-31 | Федеральное государственное унитарное предприятие "Научно-исследовательский институт "Научно-производственное объединение "ЛУЧ" (ФГУП "НИИ НПО "ЛУЧ") | Способ получения таблетированного пористого диоксида урана |
| RU2690492C1 (ru) * | 2018-05-31 | 2019-06-04 | Федеральное государственное унитарное предприятие "Научно-исследовательский институт Научно-производственное объединение "ЛУЧ" (ФГУП "НИИ НПО "ЛУЧ") | Способ получения таблетированного пористого диоксида урана |
Family Cites Families (9)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US3330889A (en) * | 1964-06-12 | 1967-07-11 | Samos George | Preparation of heat sources for radioisotope heated thermoelectric generators |
| US3312631A (en) * | 1965-04-15 | 1967-04-04 | Grace W R & Co | Method for making metal oxide microspheres |
| US3345437A (en) * | 1965-11-03 | 1967-10-03 | Grace W R & Co | Sol-gel microsphere forming process using dissolved ammonia in the dehydrating solvent |
| NL167606C (nl) * | 1969-12-09 | 1982-01-18 | Kema Nv | Werkwijze voor het bereiden van korrels. |
| US3872022A (en) * | 1970-08-10 | 1975-03-18 | Gen Electric | Sintering uranium oxide in the reaction products of hydrogen-carbon dioxide mixtures |
| BE793980A (fr) * | 1972-01-13 | 1973-07-12 | Atomic Energy Authority Uk | Combustible nucleaire ceramique ameliore |
| US3883623A (en) * | 1972-10-17 | 1975-05-13 | Gen Electric | Process for controlling end-point density of sintered uranium dioxide nuclear fuel bodies and product |
| GB1461263A (en) * | 1973-01-12 | 1977-01-13 | British Nuclear Fuels Ltd | Ceramic nuclear fuel pellets |
| US3963828A (en) * | 1973-09-06 | 1976-06-15 | Siemens Aktiengesellschaft | Manufacture of uranium dioxide powder |
-
1975
- 1975-09-10 US US05/612,084 patent/US4061700A/en not_active Expired - Lifetime
-
1976
- 1976-06-07 ZA ZA763383A patent/ZA763383B/xx unknown
- 1976-06-11 IL IL49773A patent/IL49773A0/xx unknown
- 1976-08-19 ES ES450826A patent/ES450826A1/es not_active Expired
- 1976-09-07 DE DE19762640102 patent/DE2640102A1/de active Granted
- 1976-09-09 JP JP51107307A patent/JPS5939719B2/ja not_active Expired
- 1976-09-09 IT IT27020/76A patent/IT1068271B/it active
- 1976-09-10 MX MX764905U patent/MX4857E/es unknown
- 1976-09-10 SE SE7610072A patent/SE422855B/xx not_active IP Right Cessation
-
1977
- 1977-01-31 US US05/764,378 patent/US4138360A/en not_active Expired - Lifetime
-
1981
- 1981-04-03 BE BE0/204369A patent/BE888276Q/fr not_active IP Right Cessation
Also Published As
| Publication number | Publication date |
|---|---|
| DE2640102C2 (GUID-C5D7CC26-194C-43D0-91A1-9AE8C70A9BFF.html) | 1988-08-11 |
| ZA763383B (en) | 1977-05-25 |
| IL49773A0 (en) | 1976-09-30 |
| MX4857E (es) | 1982-11-10 |
| IT1068271B (it) | 1985-03-21 |
| SE422855B (sv) | 1982-03-29 |
| JPS5246299A (en) | 1977-04-12 |
| US4061700A (en) | 1977-12-06 |
| US4138360A (en) | 1979-02-06 |
| ES450826A1 (es) | 1978-02-16 |
| SE7610072L (sv) | 1977-03-11 |
| DE2640102A1 (de) | 1977-03-24 |
| BE888276Q (fr) | 1981-10-05 |
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