JPH01501396A - 粘度調節のために遷移金属を含有する潤滑剤組成物 - Google Patents

粘度調節のために遷移金属を含有する潤滑剤組成物

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Publication number
JPH01501396A
JPH01501396A JP62500865A JP50086587A JPH01501396A JP H01501396 A JPH01501396 A JP H01501396A JP 62500865 A JP62500865 A JP 62500865A JP 50086587 A JP50086587 A JP 50086587A JP H01501396 A JPH01501396 A JP H01501396A
Authority
JP
Japan
Prior art keywords
lubricant
metal compound
composition
metal
lubricant composition
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
JP62500865A
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English (en)
Japanese (ja)
Inventor
リップル,デビッド ユ−ジ−ン
Original Assignee
ザ ルブリゾル コ−ポレ−ション
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by ザ ルブリゾル コ−ポレ−ション filed Critical ザ ルブリゾル コ−ポレ−ション
Publication of JPH01501396A publication Critical patent/JPH01501396A/ja
Pending legal-status Critical Current

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    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M141/00Lubricating compositions characterised by the additive being a mixture of two or more compounds covered by more than one of the main groups C10M125/00 - C10M139/00, each of these compounds being essential
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M129/00Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing oxygen
    • C10M129/02Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing oxygen having a carbon chain of less than 30 atoms
    • C10M129/04Hydroxy compounds
    • C10M129/10Hydroxy compounds having hydroxy groups bound to a carbon atom of a six-membered aromatic ring
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M129/00Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing oxygen
    • C10M129/02Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing oxygen having a carbon chain of less than 30 atoms
    • C10M129/26Carboxylic acids; Salts thereof
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M135/00Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing sulfur, selenium or tellurium
    • C10M135/08Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing sulfur, selenium or tellurium containing a sulfur-to-oxygen bond
    • C10M135/10Sulfonic acids or derivatives thereof
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M137/00Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing phosphorus
    • C10M137/12Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing phosphorus having a phosphorus-to-carbon bond
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M163/00Lubricating compositions characterised by the additive being a mixture of a compound of unknown or incompletely defined constitution and a non-macromolecular compound, each of these compounds being essential
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2207/00Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
    • C10M2207/02Hydroxy compounds
    • C10M2207/023Hydroxy compounds having hydroxy groups bound to carbon atoms of six-membered aromatic rings
    • C10M2207/027Neutral salts thereof
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2207/00Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
    • C10M2207/10Carboxylix acids; Neutral salts thereof
    • C10M2207/12Carboxylix acids; Neutral salts thereof having carboxyl groups bound to acyclic or cycloaliphatic carbon atoms
    • C10M2207/125Carboxylix acids; Neutral salts thereof having carboxyl groups bound to acyclic or cycloaliphatic carbon atoms having hydrocarbon chains of eight up to twenty-nine carbon atoms, i.e. fatty acids
    • CCHEMISTRY; METALLURGY
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    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2207/00Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
    • C10M2207/10Carboxylix acids; Neutral salts thereof
    • C10M2207/14Carboxylix acids; Neutral salts thereof having carboxyl groups bound to carbon atoms of six-membered aromatic rings
    • C10M2207/144Carboxylix acids; Neutral salts thereof having carboxyl groups bound to carbon atoms of six-membered aromatic rings containing hydroxy groups
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    • C10M2207/00Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
    • C10M2207/10Carboxylix acids; Neutral salts thereof
    • C10M2207/14Carboxylix acids; Neutral salts thereof having carboxyl groups bound to carbon atoms of six-membered aromatic rings
    • C10M2207/146Carboxylix acids; Neutral salts thereof having carboxyl groups bound to carbon atoms of six-membered aromatic rings having carboxyl groups bound to carbon atoms of six-membeered aromatic rings having a hydrocarbon substituent of thirty or more carbon atoms
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    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2207/00Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
    • C10M2207/10Carboxylix acids; Neutral salts thereof
    • C10M2207/16Naphthenic acids
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    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2215/00Organic non-macromolecular compounds containing nitrogen as ingredients in lubricant compositions
    • C10M2215/02Amines, e.g. polyalkylene polyamines; Quaternary amines
    • C10M2215/04Amines, e.g. polyalkylene polyamines; Quaternary amines having amino groups bound to acyclic or cycloaliphatic carbon atoms
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    • C10M2215/00Organic non-macromolecular compounds containing nitrogen as ingredients in lubricant compositions
    • C10M2215/26Amines
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    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2217/00Organic macromolecular compounds containing nitrogen as ingredients in lubricant compositions
    • C10M2217/04Macromolecular compounds from nitrogen-containing monomers obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds
    • C10M2217/046Polyamines, i.e. macromoleculars obtained by condensation of more than eleven amine monomers
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    • C10M2217/00Organic macromolecular compounds containing nitrogen as ingredients in lubricant compositions
    • C10M2217/06Macromolecular compounds obtained by functionalisation op polymers with a nitrogen containing compound
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    • C10M2219/00Organic non-macromolecular compounds containing sulfur, selenium or tellurium as ingredients in lubricant compositions
    • C10M2219/04Organic non-macromolecular compounds containing sulfur, selenium or tellurium as ingredients in lubricant compositions containing sulfur-to-oxygen bonds, i.e. sulfones, sulfoxides
    • C10M2219/044Sulfonic acids, Derivatives thereof, e.g. neutral salts
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    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2219/00Organic non-macromolecular compounds containing sulfur, selenium or tellurium as ingredients in lubricant compositions
    • C10M2219/04Organic non-macromolecular compounds containing sulfur, selenium or tellurium as ingredients in lubricant compositions containing sulfur-to-oxygen bonds, i.e. sulfones, sulfoxides
    • C10M2219/046Overbasedsulfonic acid salts
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    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2223/00Organic non-macromolecular compounds containing phosphorus as ingredients in lubricant compositions
    • C10M2223/02Organic non-macromolecular compounds containing phosphorus as ingredients in lubricant compositions having no phosphorus-to-carbon bonds
    • C10M2223/04Phosphate esters
    • C10M2223/045Metal containing thio derivatives
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    • C10M2223/00Organic non-macromolecular compounds containing phosphorus as ingredients in lubricant compositions
    • C10M2223/06Organic non-macromolecular compounds containing phosphorus as ingredients in lubricant compositions having phosphorus-to-carbon bonds
    • C10M2223/065Organic non-macromolecular compounds containing phosphorus as ingredients in lubricant compositions having phosphorus-to-carbon bonds containing sulfur
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    • C10N2010/00Metal present as such or in compounds
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    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2010/00Metal present as such or in compounds
    • C10N2010/02Groups 1 or 11
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    • C10N2010/00Metal present as such or in compounds
    • C10N2010/04Groups 2 or 12
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    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2010/00Metal present as such or in compounds
    • C10N2010/08Groups 4 or 14
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    • C10N2010/00Metal present as such or in compounds
    • C10N2010/10Groups 5 or 15
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    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2010/00Metal present as such or in compounds
    • C10N2010/12Groups 6 or 16
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    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2010/00Metal present as such or in compounds
    • C10N2010/14Group 7
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    • C10N2010/00Metal present as such or in compounds
    • C10N2010/16Groups 8, 9, or 10
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    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2040/00Specified use or application for which the lubricating composition is intended
    • C10N2040/25Internal-combustion engines
    • C10N2040/252Diesel engines
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    • C10N2040/00Specified use or application for which the lubricating composition is intended
    • C10N2040/25Internal-combustion engines
    • C10N2040/252Diesel engines
    • C10N2040/253Small diesel engines
    • FMECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F02COMBUSTION ENGINES; HOT-GAS OR COMBUSTION-PRODUCT ENGINE PLANTS
    • F02BINTERNAL-COMBUSTION PISTON ENGINES; COMBUSTION ENGINES IN GENERAL
    • F02B3/00Engines characterised by air compression and subsequent fuel addition
    • F02B3/06Engines characterised by air compression and subsequent fuel addition with compression ignition

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Organic Chemistry (AREA)
  • Lubricants (AREA)
  • Lubrication Of Internal Combustion Engines (AREA)
JP62500865A 1986-01-21 1987-01-12 粘度調節のために遷移金属を含有する潤滑剤組成物 Pending JPH01501396A (ja)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US82086086A 1986-01-21 1986-01-21
US820,860 1986-01-21

Publications (1)

Publication Number Publication Date
JPH01501396A true JPH01501396A (ja) 1989-05-18

Family

ID=25231911

Family Applications (1)

Application Number Title Priority Date Filing Date
JP62500865A Pending JPH01501396A (ja) 1986-01-21 1987-01-12 粘度調節のために遷移金属を含有する潤滑剤組成物

Country Status (16)

Country Link
EP (1) EP0290457B1 (fr)
JP (1) JPH01501396A (fr)
CN (1) CN1013685B (fr)
AU (1) AU604678B2 (fr)
BR (1) BR8707574A (fr)
CA (1) CA1290314C (fr)
DE (1) DE3788345T2 (fr)
DK (1) DK489487A (fr)
ES (1) ES2003209A6 (fr)
FI (1) FI883438A0 (fr)
HK (1) HK96694A (fr)
IN (1) IN167977B (fr)
MX (1) MX169569B (fr)
NO (1) NO174347C (fr)
WO (1) WO1987004454A2 (fr)
ZA (1) ZA87280B (fr)

Cited By (10)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2002537481A (ja) * 1999-02-25 2002-11-05 プラティナム、リサーチ、オーガナイズェイシャン、エル、エル、シー 触媒含有表面被覆組成物および方法
JP2006257406A (ja) * 2005-03-14 2006-09-28 Afton Chemical Corp 改良された抗酸化特性を得るための添加剤および潤滑組成物
JP2007138169A (ja) * 2005-11-16 2007-06-07 Afton Chemical Corp 摩擦調整をもたらす添加剤および潤滑剤調合物
JP2007162021A (ja) * 2005-12-09 2007-06-28 Afton Chemical Corp チタンを含有する潤滑油組成物
JP2007169635A (ja) * 2005-12-22 2007-07-05 Afton Chemical Corp 向上した耐摩耗特性を有する添加剤および潤滑剤配合物
WO2007102429A1 (fr) * 2006-03-07 2007-09-13 Nippon Oil Corporation Composition antioxydante, composition lubrifiante et procede de suppression de l'augmentation de viscosite d'un lubrifiant
JP2008534744A (ja) * 2005-03-28 2008-08-28 ザ ルブリゾル コーポレイション 潤滑剤中の添加剤としてのチタン化合物およびチタン錯体
JP2008223010A (ja) * 2007-03-15 2008-09-25 Afton Chemical Corp 磨耗特性を改善する添加剤および潤滑剤調合物
JP2008280515A (ja) * 2007-05-08 2008-11-20 Afton Chemical Corp リンの保持性を改善するための添加剤および潤滑剤の調合物
JP2021525302A (ja) * 2018-05-25 2021-09-24 シェブロン ユー.エス.エー. インコーポレイテッド マンガン含有潤滑剤を用いて直噴火花点火式エンジンにおける低速早期点火を防止又は低減する方法

Families Citing this family (24)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4849123A (en) * 1986-05-29 1989-07-18 The Lubrizol Corporation Drive train fluids comprising oil-soluble transition metal compounds
US5242608A (en) * 1986-12-17 1993-09-07 The Lubrizol Corporation Process for overbasing via metal borate formation
US5064545A (en) * 1986-12-17 1991-11-12 The Lubrizol Corporation Process for overbasing via metal borate formation
JP2582424B2 (ja) * 1986-12-17 1997-02-19 ザ ルブリゾル コーポレーション ホウ酸金属塩の形成によって,オーバーベース化する方法
US4952328A (en) * 1988-05-27 1990-08-28 The Lubrizol Corporation Lubricating oil compositions
US4981602A (en) * 1988-06-13 1991-01-01 The Lubrizol Corporation Lubricating oil compositions and concentrates
JPH0676588B2 (ja) * 1988-07-20 1994-09-28 株式会社ヴァイオレット 潤滑油用添加剤
US4957649A (en) * 1988-08-01 1990-09-18 The Lubrizol Corporation Lubricating oil compositions and concentrates
US4938881A (en) * 1988-08-01 1990-07-03 The Lubrizol Corporation Lubricating oil compositions and concentrates
AU636354B2 (en) * 1989-06-01 1993-04-29 Lubrizol Corporation, The Lubricating oil compositions and concentrates
US4941984A (en) * 1989-07-31 1990-07-17 The Lubrizol Corporation Lubricating oil compositions and methods for lubricating gasoline-fueled and/or alcohol-fueled, spark-ignited engines
FR2653780A1 (fr) * 1989-10-26 1991-05-03 Elf Aquitaine Additif surbase pour huiles lubrifiantes renfermant un derive du cuivre ou un derive du cuivre et du bore, son procede de preparation et compositions renfermant ledit additif .
ES2129495T3 (es) * 1993-05-18 1999-06-16 Indian Oil Corp Ltd Aceite lubrificante.
JP2000087067A (ja) 1998-07-17 2000-03-28 Tonen Corp 内燃機関用潤滑油組成物
CN1297729C (zh) * 2004-03-26 2007-01-31 田小红 围点打圆挖洞法
US7615519B2 (en) * 2004-07-19 2009-11-10 Afton Chemical Corporation Additives and lubricant formulations for improved antiwear properties
US7543445B2 (en) * 2004-10-19 2009-06-09 The Lubrizol Corporation Methods for regeneration and performance of a particulate filter of an internal combustion engine
US7648949B2 (en) * 2005-01-27 2010-01-19 The Lubrizol Corporation Low phosphorus cobalt complex-containing engine oil lubricant
EP2195404B2 (fr) * 2007-09-26 2016-03-02 The Lubrizol Corporation Composés et complexes de titane utilisés comme additifs dans des lubrifiants
EP2195403B1 (fr) 2007-09-26 2013-02-13 The Lubrizol Corporation Composés titane et complexes en tant qu'additifs dans des lubrifiants
CN101886014B (zh) * 2010-07-08 2013-02-27 湖南省华京粉体材料有限公司 一种含羧酸钨盐机油添加剂的制备方法
US20160186087A1 (en) * 2013-08-09 2016-06-30 The Lubrizol Corporation Reduced engine deposits from dispersant treated with cobalt
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JP2006257406A (ja) * 2005-03-14 2006-09-28 Afton Chemical Corp 改良された抗酸化特性を得るための添加剤および潤滑組成物
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JP2008534744A (ja) * 2005-03-28 2008-08-28 ザ ルブリゾル コーポレイション 潤滑剤中の添加剤としてのチタン化合物およびチタン錯体
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JP2007138169A (ja) * 2005-11-16 2007-06-07 Afton Chemical Corp 摩擦調整をもたらす添加剤および潤滑剤調合物
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JP2007162021A (ja) * 2005-12-09 2007-06-28 Afton Chemical Corp チタンを含有する潤滑油組成物
JP2011042801A (ja) * 2005-12-09 2011-03-03 Afton Chemical Corp チタンを含有する潤滑油組成物
JP2007169635A (ja) * 2005-12-22 2007-07-05 Afton Chemical Corp 向上した耐摩耗特性を有する添加剤および潤滑剤配合物
WO2007102429A1 (fr) * 2006-03-07 2007-09-13 Nippon Oil Corporation Composition antioxydante, composition lubrifiante et procede de suppression de l'augmentation de viscosite d'un lubrifiant
JP2008223010A (ja) * 2007-03-15 2008-09-25 Afton Chemical Corp 磨耗特性を改善する添加剤および潤滑剤調合物
JP2008280515A (ja) * 2007-05-08 2008-11-20 Afton Chemical Corp リンの保持性を改善するための添加剤および潤滑剤の調合物
JP2021525302A (ja) * 2018-05-25 2021-09-24 シェブロン ユー.エス.エー. インコーポレイテッド マンガン含有潤滑剤を用いて直噴火花点火式エンジンにおける低速早期点火を防止又は低減する方法

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MX169569B (es) 1993-07-13
ES2003209A6 (es) 1988-10-16
AU6941087A (en) 1987-08-14
NO873690D0 (no) 1987-09-03
NO174347B (no) 1994-01-10
WO1987004454A3 (fr) 1987-09-11
IN167977B (fr) 1991-01-19
BR8707574A (pt) 1989-03-14
CN87100331A (zh) 1987-09-16
DK489487D0 (da) 1987-09-18
FI883438A (fi) 1988-07-20
NO873690L (no) 1987-09-03
EP0290457A1 (fr) 1988-11-17
CN1013685B (zh) 1991-08-28
ZA87280B (en) 1987-09-30
DK489487A (da) 1987-09-18
CA1290314C (fr) 1991-10-08
NO174347C (no) 1994-04-20
HK96694A (en) 1994-09-23
EP0290457B1 (fr) 1993-12-01
DE3788345D1 (de) 1994-01-13
WO1987004454A2 (fr) 1987-07-30
DE3788345T2 (de) 1994-03-17
FI883438A0 (fi) 1988-07-20
AU604678B2 (en) 1991-01-03

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