JP5542992B2 - ガラスセラミックの接合材料およびその使用 - Google Patents
ガラスセラミックの接合材料およびその使用 Download PDFInfo
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- 239000000463 material Substances 0.000 title claims description 150
- 239000002241 glass-ceramic Substances 0.000 title claims description 54
- 239000011521 glass Substances 0.000 claims description 39
- 239000000446 fuel Substances 0.000 claims description 25
- 229910004298 SiO 2 Inorganic materials 0.000 claims description 20
- 238000004519 manufacturing process Methods 0.000 claims description 20
- 229910052751 metal Inorganic materials 0.000 claims description 17
- 239000002184 metal Substances 0.000 claims description 17
- 239000000919 ceramic Substances 0.000 claims description 15
- 239000012535 impurity Substances 0.000 claims description 12
- 238000005868 electrolysis reaction Methods 0.000 claims description 8
- 229910015999 BaAl Inorganic materials 0.000 claims description 6
- 239000000654 additive Substances 0.000 claims description 6
- 229910052783 alkali metal Inorganic materials 0.000 claims description 6
- 150000001340 alkali metals Chemical class 0.000 claims description 6
- 239000013078 crystal Substances 0.000 claims description 6
- 239000000945 filler Substances 0.000 claims description 6
- 229910018072 Al 2 O 3 Inorganic materials 0.000 claims description 5
- 229910015902 Bi 2 O 3 Inorganic materials 0.000 claims description 4
- 229910010413 TiO 2 Inorganic materials 0.000 claims description 4
- 229910000272 alkali metal oxide Inorganic materials 0.000 claims description 3
- 230000008025 crystallization Effects 0.000 description 21
- 238000002425 crystallisation Methods 0.000 description 20
- 238000010438 heat treatment Methods 0.000 description 13
- 239000006121 base glass Substances 0.000 description 12
- 238000002844 melting Methods 0.000 description 10
- 230000008018 melting Effects 0.000 description 10
- 238000000034 method Methods 0.000 description 9
- 239000000843 powder Substances 0.000 description 9
- 230000008569 process Effects 0.000 description 9
- 239000000126 substance Substances 0.000 description 8
- 229910000831 Steel Inorganic materials 0.000 description 7
- 238000005304 joining Methods 0.000 description 7
- 238000012545 processing Methods 0.000 description 7
- 239000010959 steel Substances 0.000 description 7
- 230000008901 benefit Effects 0.000 description 5
- 239000011230 binding agent Substances 0.000 description 5
- 238000005219 brazing Methods 0.000 description 5
- 239000000203 mixture Substances 0.000 description 5
- 239000007858 starting material Substances 0.000 description 5
- VYPSYNLAJGMNEJ-UHFFFAOYSA-N Silicium dioxide Chemical compound O=[Si]=O VYPSYNLAJGMNEJ-UHFFFAOYSA-N 0.000 description 4
- 229910045601 alloy Inorganic materials 0.000 description 4
- 239000000956 alloy Substances 0.000 description 4
- 229910052804 chromium Inorganic materials 0.000 description 4
- 239000011651 chromium Substances 0.000 description 4
- 230000009477 glass transition Effects 0.000 description 4
- RVTZCBVAJQQJTK-UHFFFAOYSA-N oxygen(2-);zirconium(4+) Chemical compound [O-2].[O-2].[Zr+4] RVTZCBVAJQQJTK-UHFFFAOYSA-N 0.000 description 4
- 238000007789 sealing Methods 0.000 description 4
- 238000005245 sintering Methods 0.000 description 4
- 229910000679 solder Inorganic materials 0.000 description 4
- 229910001928 zirconium oxide Inorganic materials 0.000 description 4
- ZOXJGFHDIHLPTG-UHFFFAOYSA-N Boron Chemical compound [B] ZOXJGFHDIHLPTG-UHFFFAOYSA-N 0.000 description 3
- VYZAMTAEIAYCRO-UHFFFAOYSA-N Chromium Chemical compound [Cr] VYZAMTAEIAYCRO-UHFFFAOYSA-N 0.000 description 3
- 229910052788 barium Inorganic materials 0.000 description 3
- DSAJWYNOEDNPEQ-UHFFFAOYSA-N barium atom Chemical compound [Ba] DSAJWYNOEDNPEQ-UHFFFAOYSA-N 0.000 description 3
- 229910052796 boron Inorganic materials 0.000 description 3
- 230000008859 change Effects 0.000 description 3
- 238000002485 combustion reaction Methods 0.000 description 3
- 230000008878 coupling Effects 0.000 description 3
- 238000010168 coupling process Methods 0.000 description 3
- 238000005859 coupling reaction Methods 0.000 description 3
- 229910052906 cristobalite Inorganic materials 0.000 description 3
- 230000007423 decrease Effects 0.000 description 3
- 239000000156 glass melt Substances 0.000 description 3
- 230000014759 maintenance of location Effects 0.000 description 3
- 239000007787 solid Substances 0.000 description 3
- 230000035882 stress Effects 0.000 description 3
- 238000009834 vaporization Methods 0.000 description 3
- 230000008016 vaporization Effects 0.000 description 3
- 229910017639 MgSi Inorganic materials 0.000 description 2
- 229910004283 SiO 4 Inorganic materials 0.000 description 2
- 230000002411 adverse Effects 0.000 description 2
- 238000003483 aging Methods 0.000 description 2
- 230000015572 biosynthetic process Effects 0.000 description 2
- 230000015556 catabolic process Effects 0.000 description 2
- 238000006243 chemical reaction Methods 0.000 description 2
- 230000000052 comparative effect Effects 0.000 description 2
- 238000001816 cooling Methods 0.000 description 2
- 230000007797 corrosion Effects 0.000 description 2
- 238000005260 corrosion Methods 0.000 description 2
- 238000006731 degradation reaction Methods 0.000 description 2
- 238000009826 distribution Methods 0.000 description 2
- 230000000694 effects Effects 0.000 description 2
- 239000003792 electrolyte Substances 0.000 description 2
- 239000000835 fiber Substances 0.000 description 2
- 239000007789 gas Substances 0.000 description 2
- 238000000227 grinding Methods 0.000 description 2
- 239000002667 nucleating agent Substances 0.000 description 2
- 238000007254 oxidation reaction Methods 0.000 description 2
- 230000000704 physical effect Effects 0.000 description 2
- 239000002994 raw material Substances 0.000 description 2
- 229910052706 scandium Inorganic materials 0.000 description 2
- SIXSYDAISGFNSX-UHFFFAOYSA-N scandium atom Chemical compound [Sc] SIXSYDAISGFNSX-UHFFFAOYSA-N 0.000 description 2
- 239000003566 sealing material Substances 0.000 description 2
- 229910001220 stainless steel Inorganic materials 0.000 description 2
- 239000010456 wollastonite Substances 0.000 description 2
- 229910052882 wollastonite Inorganic materials 0.000 description 2
- 229910052727 yttrium Inorganic materials 0.000 description 2
- VWQVUPCCIRVNHF-UHFFFAOYSA-N yttrium atom Chemical compound [Y] VWQVUPCCIRVNHF-UHFFFAOYSA-N 0.000 description 2
- 229910000599 Cr alloy Inorganic materials 0.000 description 1
- 229910017625 MgSiO Inorganic materials 0.000 description 1
- 101100496858 Mus musculus Colec12 gene Proteins 0.000 description 1
- 229910004122 SrSi Inorganic materials 0.000 description 1
- RTAQQCXQSZGOHL-UHFFFAOYSA-N Titanium Chemical compound [Ti] RTAQQCXQSZGOHL-UHFFFAOYSA-N 0.000 description 1
- 230000009471 action Effects 0.000 description 1
- 239000002318 adhesion promoter Substances 0.000 description 1
- 238000004458 analytical method Methods 0.000 description 1
- 229910052916 barium silicate Inorganic materials 0.000 description 1
- HMOQPOVBDRFNIU-UHFFFAOYSA-N barium(2+);dioxido(oxo)silane Chemical compound [Ba+2].[O-][Si]([O-])=O HMOQPOVBDRFNIU-UHFFFAOYSA-N 0.000 description 1
- 239000002585 base Substances 0.000 description 1
- 238000005452 bending Methods 0.000 description 1
- 230000011712 cell development Effects 0.000 description 1
- 239000000788 chromium alloy Substances 0.000 description 1
- 239000002131 composite material Substances 0.000 description 1
- 238000013329 compounding Methods 0.000 description 1
- 238000011109 contamination Methods 0.000 description 1
- 229910052878 cordierite Inorganic materials 0.000 description 1
- 238000000354 decomposition reaction Methods 0.000 description 1
- 238000004925 denaturation Methods 0.000 description 1
- 230000036425 denaturation Effects 0.000 description 1
- 230000001419 dependent effect Effects 0.000 description 1
- 238000011161 development Methods 0.000 description 1
- 230000018109 developmental process Effects 0.000 description 1
- JSKIRARMQDRGJZ-UHFFFAOYSA-N dimagnesium dioxido-bis[(1-oxido-3-oxo-2,4,6,8,9-pentaoxa-1,3-disila-5,7-dialuminabicyclo[3.3.1]nonan-7-yl)oxy]silane Chemical compound [Mg++].[Mg++].[O-][Si]([O-])(O[Al]1O[Al]2O[Si](=O)O[Si]([O-])(O1)O2)O[Al]1O[Al]2O[Si](=O)O[Si]([O-])(O1)O2 JSKIRARMQDRGJZ-UHFFFAOYSA-N 0.000 description 1
- 238000010292 electrical insulation Methods 0.000 description 1
- 238000005516 engineering process Methods 0.000 description 1
- 229910052634 enstatite Inorganic materials 0.000 description 1
- 239000006025 fining agent Substances 0.000 description 1
- 239000012530 fluid Substances 0.000 description 1
- 230000004927 fusion Effects 0.000 description 1
- 238000001483 high-temperature X-ray diffraction Methods 0.000 description 1
- 238000010406 interfacial reaction Methods 0.000 description 1
- BBCCCLINBSELLX-UHFFFAOYSA-N magnesium;dihydroxy(oxo)silane Chemical compound [Mg+2].O[Si](O)=O BBCCCLINBSELLX-UHFFFAOYSA-N 0.000 description 1
- 230000013011 mating Effects 0.000 description 1
- 238000005259 measurement Methods 0.000 description 1
- 230000007246 mechanism Effects 0.000 description 1
- 239000000155 melt Substances 0.000 description 1
- 150000002739 metals Chemical class 0.000 description 1
- 239000010445 mica Substances 0.000 description 1
- 229910052618 mica group Inorganic materials 0.000 description 1
- 238000002156 mixing Methods 0.000 description 1
- 230000003647 oxidation Effects 0.000 description 1
- 239000001301 oxygen Substances 0.000 description 1
- 229910052760 oxygen Inorganic materials 0.000 description 1
- -1 oxygen ion Chemical class 0.000 description 1
- 239000002245 particle Substances 0.000 description 1
- 239000004033 plastic Substances 0.000 description 1
- 238000003825 pressing Methods 0.000 description 1
- 230000001737 promoting effect Effects 0.000 description 1
- 230000009467 reduction Effects 0.000 description 1
- 238000006722 reduction reaction Methods 0.000 description 1
- 239000005394 sealing glass Substances 0.000 description 1
- 239000005368 silicate glass Substances 0.000 description 1
- 229910052566 spinel group Inorganic materials 0.000 description 1
- 230000006641 stabilisation Effects 0.000 description 1
- 238000011105 stabilization Methods 0.000 description 1
- 238000007655 standard test method Methods 0.000 description 1
- NVKTUNLPFJHLCG-UHFFFAOYSA-N strontium chromate Chemical compound [Sr+2].[O-][Cr]([O-])(=O)=O NVKTUNLPFJHLCG-UHFFFAOYSA-N 0.000 description 1
- 230000001629 suppression Effects 0.000 description 1
- 238000005382 thermal cycling Methods 0.000 description 1
- 230000008646 thermal stress Effects 0.000 description 1
- 229910052719 titanium Inorganic materials 0.000 description 1
- 239000010936 titanium Substances 0.000 description 1
- 238000011282 treatment Methods 0.000 description 1
- 229910052905 tridymite Inorganic materials 0.000 description 1
- 238000010626 work up procedure Methods 0.000 description 1
Classifications
-
- G—PHYSICS
- G03—PHOTOGRAPHY; CINEMATOGRAPHY; ANALOGOUS TECHNIQUES USING WAVES OTHER THAN OPTICAL WAVES; ELECTROGRAPHY; HOLOGRAPHY
- G03C—PHOTOSENSITIVE MATERIALS FOR PHOTOGRAPHIC PURPOSES; PHOTOGRAPHIC PROCESSES, e.g. CINE, X-RAY, COLOUR, STEREO-PHOTOGRAPHIC PROCESSES; AUXILIARY PROCESSES IN PHOTOGRAPHY
- G03C8/00—Diffusion transfer processes or agents therefor; Photosensitive materials for such processes
- G03C8/24—Photosensitive materials characterised by the image-receiving section
-
- C—CHEMISTRY; METALLURGY
- C03—GLASS; MINERAL OR SLAG WOOL
- C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
- C03C10/00—Devitrified glass ceramics, i.e. glass ceramics having a crystalline phase dispersed in a glassy phase and constituting at least 50% by weight of the total composition
- C03C10/0036—Devitrified glass ceramics, i.e. glass ceramics having a crystalline phase dispersed in a glassy phase and constituting at least 50% by weight of the total composition containing SiO2, Al2O3 and a divalent metal oxide as main constituents
-
- C—CHEMISTRY; METALLURGY
- C03—GLASS; MINERAL OR SLAG WOOL
- C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
- C03C3/00—Glass compositions
- C03C3/04—Glass compositions containing silica
- C03C3/062—Glass compositions containing silica with less than 40% silica by weight
- C03C3/064—Glass compositions containing silica with less than 40% silica by weight containing boron
-
- C—CHEMISTRY; METALLURGY
- C03—GLASS; MINERAL OR SLAG WOOL
- C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
- C03C3/00—Glass compositions
- C03C3/04—Glass compositions containing silica
- C03C3/062—Glass compositions containing silica with less than 40% silica by weight
- C03C3/064—Glass compositions containing silica with less than 40% silica by weight containing boron
- C03C3/068—Glass compositions containing silica with less than 40% silica by weight containing boron containing rare earths
-
- C—CHEMISTRY; METALLURGY
- C03—GLASS; MINERAL OR SLAG WOOL
- C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
- C03C8/00—Enamels; Glazes; Fusion seal compositions being frit compositions having non-frit additions
- C03C8/24—Fusion seal compositions being frit compositions having non-frit additions, i.e. for use as seals between dissimilar materials, e.g. glass and metal; Glass solders
-
- C—CHEMISTRY; METALLURGY
- C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
- C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
- C25B9/00—Cells or assemblies of cells; Constructional parts of cells; Assemblies of constructional parts, e.g. electrode-diaphragm assemblies; Process-related cell features
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H01M8/0271—Sealing or supporting means around electrodes, matrices or membranes
- H01M8/028—Sealing means characterised by their material
- H01M8/0282—Inorganic material
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
- Y10T403/00—Joints and connections
- Y10T403/47—Molded joint
- Y10T403/477—Fusion bond, e.g., weld, etc.
Landscapes
- Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Chemical Kinetics & Catalysis (AREA)
- General Chemical & Material Sciences (AREA)
- Life Sciences & Earth Sciences (AREA)
- Organic Chemistry (AREA)
- Materials Engineering (AREA)
- Geochemistry & Mineralogy (AREA)
- Electrochemistry (AREA)
- Sustainable Development (AREA)
- Sustainable Energy (AREA)
- Metallurgy (AREA)
- Manufacturing & Machinery (AREA)
- Ceramic Engineering (AREA)
- Crystallography & Structural Chemistry (AREA)
- Dispersion Chemistry (AREA)
- Inorganic Chemistry (AREA)
- Physics & Mathematics (AREA)
- General Physics & Mathematics (AREA)
- Glass Compositions (AREA)
- Fuel Cell (AREA)
- Compositions Of Oxide Ceramics (AREA)
Description
α(20-300) 20℃から300℃までの線熱膨張率
Tg ガラス転移温度
PR プロセス温度、log ηは4に相当する。ηは[dPas]である。
T焼結 焼結温度
T球体 球体温度
T半球体 半球体温度(semisphere temperature)
T流動 流動温度
1. 熱膨張率α(20-300)≧9.5×10-6K-1を有するガラスセラミックの接合材料であって、(酸化物に対するモル%で)
SiO2 3以上10未満
B2O3 16〜34
Al2O3 7〜15
CaO 8〜40
BaO 25〜38
MgO 0〜10
ZrO2 0〜5
Y2O3 0〜10
を含む、前記接合材料。
2. せいぜい不純物を除き、ZnOおよび/またはPbOおよび/またはBi2O3および/またはTiO2および/またはTeO2を含まない、1に記載のガラスセラミックの接合材料。
3. せいぜい不純物を除き、アルカリ金属および/またはアルカリ金属酸化物および/またはSrOを含まない、1または2に記載のガラスセラミックの接合材料。
4. 主結晶相として、BaAl2Si2O8を含む、1から3までのいずれかに記載のガラスセラミックの接合材料。
5. SiO2含有率(酸化物に対するモル%で)が、3%〜7%である、1から4までのいずれかに記載のガラスセラミックの接合材料。
6. CaO含有率(酸化物に対するモル%で)が、8%〜12%である、1から5までのいずれかに記載のガラスセラミックの接合材料。
7. 1から6までのいずれかに記載のガラスセラミックの接合材料と、(酸化物に対する質量%で)30質量%以下の充填剤、好ましくはMgOおよび/またはYSZおよび/またはウォラストナイト粉末および/または酸化ジルコニウム繊維の群から選択される充填剤とを含む接合材料。
8. 1から7までのいずれかに記載の接合材料の、
− 少なくとも2つの金属製部材の間の、特にフェライト鋼から構成される部材間の結合部であって、前記の少なくとも2つの金属製部材が、1から7までのいずれかに記載の接合材料によって結合される結合部、および/または
− 少なくとも2つのセラミック製部材の間の、特にイットリウムおよび/またはスカンジウム安定化酸化ジルコニウムから構成される部材間の結合部であって、前記の少なくとも2つのセラミック製部材が、1から7までのいずれかに記載の接合材料によって結合される結合部、および/または
− 少なくとも1つの金属製部材と少なくとも1つのセラミック製部材との間の、特にそれぞれの場合について上述した材料から構成される部材間の結合部であって、前記の少なくとも1つの金属製部材および前記少なくとも1つのセラミック製部材が、1から7までのいずれかに記載の接合材料によって結合される結合部
における使用。
9. 1から7までのいずれかに記載の接合材料の、燃料電池または電解ユニットにおける使用。
10. 燃料電池または電解セルまたはセンサおよび/またはアクチュエータにおける結合部の作製のための、または焼結体および/または焼結シートの製造のための、または他のガラスおよび/またはガラスセラミックスにおける添加材としての、1から4までのいずれかに記載の接合材料の使用。
Claims (10)
- 熱膨張率α(20-300)≧9.5×10-6K-1を有するガラスセラミックの接合材料であって、酸化物に対するモル%で、
SiO2 3以上10未満
B2O3 16〜34
Al2O3 7〜15
CaO 8〜40
BaO 25〜38
MgO 0〜10
ZrO2 0〜5
Y2O3 0〜10
を含む、前記接合材料。 - せいぜい不純物を除き、ZnOおよび/またはPbOおよび/またはBi2O3および/またはTiO2および/またはTeO2を含まない、請求項1に記載のガラスセラミックの接合材料。
- せいぜい不純物を除き、アルカリ金属および/またはアルカリ金属酸化物および/またはSrOを含まない、請求項1または2に記載のガラスセラミックの接合材料。
- 主結晶相として、BaAl2Si2O8を含む、請求項1から3までのいずれか1項に記載のガラスセラミックの接合材料。
- SiO2含有率が、酸化物に対するモル%で、3%〜7%である、請求項1から4までのいずれか1項に記載のガラスセラミックの接合材料。
- CaO含有率が、酸化物に対するモル%で、8%〜12%である、請求項1から5までのいずれか1項に記載のガラスセラミックの接合材料。
- 請求項1から6までのいずれか1項に記載のガラスセラミックの接合材料と、酸化物に対する質量%で30質量%以下の充填剤とを含む接合材料。
- 請求項1から7までのいずれか1項に記載の接合材料の、
− 少なくとも2つの金属製部材の間の結合部であって、前記の少なくとも2つの金属製部材が、請求項1から7までのいずれか1項に記載の接合材料によって結合される結合部、および/または
− 少なくとも2つのセラミック製部材の間の結合部であって、前記の少なくとも2つのセラミック製部材が、請求項1から7までのいずれか1項に記載の接合材料によって結合される結合部、および/または
− 少なくとも1つの金属製部材と少なくとも1つのセラミック製部材との間の結合部であって、前記の少なくとも1つの金属製部材および前記少なくとも1つのセラミック製部材が、請求項1から7までのいずれか1項に記載の接合材料によって結合される結合部
における使用。 - 請求項1から7までのいずれか1項に記載の接合材料の、燃料電池または電解ユニットにおける使用。
- 燃料電池または電解セルまたはセンサおよび/またはアクチュエータにおける結合部の作製のための、または焼結体および/または焼結シートの製造のための、または他のガラスおよび/またはガラスセラミックスにおける添加材としての、請求項1から4までのいずれか1項に記載の接合材料の使用。
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DE201210207405 DE102012207405B3 (de) | 2012-05-04 | 2012-05-04 | Glaskeramisches Fügematerial und dessen Verwendung |
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CN105060716A (zh) * | 2015-07-28 | 2015-11-18 | 张家港保税区佰昂特种玻璃有限公司 | 一种掺稀土的磷酸盐微晶玻璃及其制备方法 |
JP6636814B2 (ja) * | 2016-02-09 | 2020-01-29 | 株式会社ノリタケカンパニーリミテド | ガラス組成物およびその利用 |
US11225433B2 (en) * | 2016-02-19 | 2022-01-18 | Ferro Corporation | Sintering aid for glasses for machinable phyllosilicate based structures |
CN107235628B (zh) * | 2016-03-29 | 2020-03-10 | 中国科学院过程工程研究所 | 一种玻璃组合物及其制备方法和应用 |
WO2017181191A1 (en) * | 2016-04-15 | 2017-10-19 | The Penn State Research Foundation | Advanced ceramics to glass joints |
JP6414566B2 (ja) * | 2016-05-26 | 2018-10-31 | 株式会社村田製作所 | ガラス−セラミック−フェライト組成物および電子部品 |
CN107021774B (zh) * | 2017-04-14 | 2020-06-30 | 常州联德电子有限公司 | 平板式氧传感器使用的玻璃基复合密封材料及其密封方法 |
GB201721319D0 (en) | 2017-12-19 | 2018-01-31 | Coorstek Membrane Sciences As | Sealing Compositions |
GB201721341D0 (en) * | 2017-12-19 | 2018-01-31 | Coorstek Membrane Sciences As | Sealing compositions |
JP7016028B2 (ja) * | 2018-04-03 | 2022-02-04 | パナソニックIpマネジメント株式会社 | 燃料電池 |
EP3650415B1 (de) * | 2018-11-07 | 2024-02-07 | Schott Ag | Fügeverbindung umfassend ein kristalliesiertes glas, deren verwendung sowie kristallisierbares sowie zumindest teilweise kristallissiertes glas und dessen verwendung |
TWI703109B (zh) * | 2019-03-20 | 2020-09-01 | 法藍瓷股份有限公司 | 陶瓷件之接合方法 |
WO2021242714A1 (en) * | 2020-05-26 | 2021-12-02 | Heraeus Conamic North America Llc | Plasma resistant ceramic body formed from multiple pieces |
KR102308652B1 (ko) | 2020-05-27 | 2021-10-05 | 코닝 인코포레이티드 | 높은 탄성 계수 및 경도를 가지는 유리-세라믹 |
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US5112777A (en) * | 1991-01-09 | 1992-05-12 | Corning Incorporated | Glass-ceramic-bonded ceramic composites |
US6124224A (en) * | 1998-09-02 | 2000-09-26 | Ferro Corporation | High temperature sealing glass |
DE19857057C1 (de) * | 1998-12-10 | 2000-04-13 | Fraunhofer Ges Forschung | Verwendung von alkalifreien Glaskeramiken als Fügematerial für den Hochtemperatureinsatz |
US6362119B1 (en) * | 1999-06-09 | 2002-03-26 | Asahi Glass Company, Limited | Barium borosilicate glass and glass ceramic composition |
US6430966B1 (en) * | 1999-07-30 | 2002-08-13 | Battelle Memorial Institute | Glass-ceramic material and method of making |
DE10122327A1 (de) * | 2001-05-08 | 2002-11-28 | Forschungszentrum Juelich Gmbh | Glaslot als Fügematerial für den Hochtemperatureinsatz sowie Herstellung und Verwendung |
CN101682069B (zh) * | 2007-04-12 | 2013-11-20 | 康宁股份有限公司 | 密封材料、使用该材料的装置以及装置的制造方法 |
JP5171569B2 (ja) * | 2008-11-19 | 2013-03-27 | 浜松ホトニクス株式会社 | ファイバオプティックプレート及びその製造方法 |
DK2403812T3 (en) * | 2009-03-04 | 2019-03-18 | Schott Ag | CRYSTALLIZING GLASS SOLUTION AND USE THEREOF |
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