DE69911043D1 - Verfahren zum beschichten einer trägerplatte und diese trägerplatte enthaltende brennstoffzelle - Google Patents

Verfahren zum beschichten einer trägerplatte und diese trägerplatte enthaltende brennstoffzelle

Info

Publication number
DE69911043D1
DE69911043D1 DE69911043T DE69911043T DE69911043D1 DE 69911043 D1 DE69911043 D1 DE 69911043D1 DE 69911043 T DE69911043 T DE 69911043T DE 69911043 T DE69911043 T DE 69911043T DE 69911043 D1 DE69911043 D1 DE 69911043D1
Authority
DE
Germany
Prior art keywords
carrier plate
coating
fuel cell
support plate
cell containing
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
DE69911043T
Other languages
English (en)
Other versions
DE69911043T2 (de
Inventor
Christiaan Makkus
Edward Bullock
Hermannus Janssen
Michel Cassir
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
GEMEENSCHAPPELIJK CT VOOR ONDE
Energieonderzoek Centrum Nederland ECN
Original Assignee
GEMEENSCHAPPELIJK CT VOOR ONDE
Energieonderzoek Centrum Nederland ECN
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by GEMEENSCHAPPELIJK CT VOOR ONDE, Energieonderzoek Centrum Nederland ECN filed Critical GEMEENSCHAPPELIJK CT VOOR ONDE
Application granted granted Critical
Publication of DE69911043D1 publication Critical patent/DE69911043D1/de
Publication of DE69911043T2 publication Critical patent/DE69911043T2/de
Anticipated expiration legal-status Critical
Expired - Fee Related legal-status Critical Current

Links

Classifications

    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204Non-porous and characterised by the material
    • H01M8/0206Metals or alloys
    • H01M8/0208Alloys
    • H01M8/021Alloys based on iron
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C28/00Coating for obtaining at least two superposed coatings either by methods not provided for in a single one of groups C23C2/00 - C23C26/00 or by combinations of methods provided for in subclasses C23C and C25C or C25D
    • C23C28/30Coatings combining at least one metallic layer and at least one inorganic non-metallic layer
    • C23C28/32Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer
    • C23C28/321Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer with at least one metal alloy layer
    • C23C28/3215Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer with at least one metal alloy layer at least one MCrAlX layer
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C28/00Coating for obtaining at least two superposed coatings either by methods not provided for in a single one of groups C23C2/00 - C23C26/00 or by combinations of methods provided for in subclasses C23C and C25C or C25D
    • C23C28/30Coatings combining at least one metallic layer and at least one inorganic non-metallic layer
    • C23C28/32Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer
    • C23C28/322Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer only coatings of metal elements only
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C28/00Coating for obtaining at least two superposed coatings either by methods not provided for in a single one of groups C23C2/00 - C23C26/00 or by combinations of methods provided for in subclasses C23C and C25C or C25D
    • C23C28/30Coatings combining at least one metallic layer and at least one inorganic non-metallic layer
    • C23C28/34Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates
    • C23C28/345Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates with at least one oxide layer
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C28/00Coating for obtaining at least two superposed coatings either by methods not provided for in a single one of groups C23C2/00 - C23C26/00 or by combinations of methods provided for in subclasses C23C and C25C or C25D
    • C23C28/30Coatings combining at least one metallic layer and at least one inorganic non-metallic layer
    • C23C28/34Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates
    • C23C28/345Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates with at least one oxide layer
    • C23C28/3455Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates with at least one oxide layer with a refractory ceramic layer, e.g. refractory metal oxide, ZrO2, rare earth oxides or a thermal barrier system comprising at least one refractory oxide layer
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C4/00Coating by spraying the coating material in the molten state, e.g. by flame, plasma or electric discharge
    • C23C4/02Pretreatment of the material to be coated, e.g. for coating on selected surface areas
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204Non-porous and characterised by the material
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204Non-porous and characterised by the material
    • H01M8/0215Glass; Ceramic materials
    • H01M8/0217Complex oxides, optionally doped, of the type AMO3, A being an alkaline earth metal or rare earth metal and M being a metal, e.g. perovskites
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204Non-porous and characterised by the material
    • H01M8/0223Composites
    • H01M8/0228Composites in the form of layered or coated products
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/023Porous and characterised by the material
    • H01M8/0232Metals or alloys
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/14Fuel cells with fused electrolytes
    • H01M2008/147Fuel cells with molten carbonates
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00Electrolytes
    • H01M2300/0017Non-aqueous electrolytes
    • H01M2300/0048Molten electrolytes used at high temperature
    • H01M2300/0051Carbonates
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Inorganic Chemistry (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Sustainable Development (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Metallurgy (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Manufacturing & Machinery (AREA)
  • Sustainable Energy (AREA)
  • Organic Chemistry (AREA)
  • Ceramic Engineering (AREA)
  • Physics & Mathematics (AREA)
  • Plasma & Fusion (AREA)
  • Composite Materials (AREA)
  • Fuel Cell (AREA)
  • Other Surface Treatments For Metallic Materials (AREA)
  • Inert Electrodes (AREA)
DE69911043T 1998-10-08 1999-10-08 Verfahren zum beschichten einer trägerplatte und diese trägerplatte enthaltende brennstoffzelle Expired - Fee Related DE69911043T2 (de)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
NL1010269 1998-10-08
NL1010269A NL1010269C2 (nl) 1998-10-08 1998-10-08 Werkwijze voor het bekleden van een dragerplaat en MCFC-cel voorzien van een dergelijke dragerplaat.
PCT/NL1999/000624 WO2000021152A1 (en) 1998-10-08 1999-10-08 Method for coating a support plate and fuel cell provided with such a support plate

Publications (2)

Publication Number Publication Date
DE69911043D1 true DE69911043D1 (de) 2003-10-09
DE69911043T2 DE69911043T2 (de) 2004-06-03

Family

ID=19767936

Family Applications (1)

Application Number Title Priority Date Filing Date
DE69911043T Expired - Fee Related DE69911043T2 (de) 1998-10-08 1999-10-08 Verfahren zum beschichten einer trägerplatte und diese trägerplatte enthaltende brennstoffzelle

Country Status (10)

Country Link
US (1) US6761927B1 (de)
EP (1) EP1119881B1 (de)
JP (1) JP2002527612A (de)
AT (1) ATE249102T1 (de)
CA (1) CA2346486A1 (de)
DE (1) DE69911043T2 (de)
DK (1) DK1119881T3 (de)
ES (1) ES2211180T3 (de)
NL (1) NL1010269C2 (de)
WO (1) WO2000021152A1 (de)

Families Citing this family (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP1035608A3 (de) * 1999-02-09 2003-02-05 Nisshinbo Industries, Inc. Separator für Brennstoffzellen und Festelektrolytbrennstoffzellen mit diesem Separator
US6649031B1 (en) 1999-10-08 2003-11-18 Hybrid Power Generation Systems, Llc Corrosion resistant coated fuel cell bipolar plate with filled-in fine scale porosities and method of making the same
US7144648B2 (en) * 2002-11-22 2006-12-05 The Research Foundation Of State University Of New York Bipolar plate
EP1494300A1 (de) * 2003-07-04 2005-01-05 Nisshinbo Industries, Inc. Brennstoffzellenseparator aus porösem Material und seine Herstellung, Feststoff Polymer-Brennstoffzelle
KR101195180B1 (ko) * 2005-02-01 2012-10-29 가부시키가이샤 네오맥스 마테리아르 연료 전지용 세퍼레이터 및 그 제조 방법
US20070003813A1 (en) * 2005-06-30 2007-01-04 General Motors Corporation Stable conductive and hydrophilic fuel cell contact element
US8377607B2 (en) * 2005-06-30 2013-02-19 GM Global Technology Operations LLC Fuel cell contact element including a TiO2 layer and a conductive layer
US20070287057A1 (en) * 2006-06-09 2007-12-13 Elhamid Mahmoud H Abd Method for making a hydrophilic corrosion resistant coating on low grade stainless steel/alloys for bipolar plates
US8603703B2 (en) * 2006-07-26 2013-12-10 GM Global Technology Operations LLC Method for making super-hydrophilic and electrically conducting surfaces for fuel cell bipolar plates
US20080044716A1 (en) * 2006-08-16 2008-02-21 Gm Global Technology Operations, Inc. Durable layer structure and method for making same
JP5312855B2 (ja) * 2008-06-20 2013-10-09 東邦瓦斯株式会社 インターコネクタおよびその製造方法
GB201910455D0 (en) * 2019-07-22 2019-09-04 Teer Coatings Ltd Coating for the surface of an article and process for forming the coating

Family Cites Families (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2619417A1 (de) * 1976-05-03 1977-11-24 Walter H R Ott Verfahren zur herstellung von festhaftenden auftragungen im thermischen spritzverfahren mit dem spritzzusatzwerkstoff titan ausgefuehrt
US4226897A (en) * 1977-12-05 1980-10-07 Plasma Physics Corporation Method of forming semiconducting materials and barriers
JPH0192350A (ja) * 1987-10-01 1989-04-11 Osaka Gas Co Ltd 伝熱面の処理方法
US5805973A (en) * 1991-03-25 1998-09-08 General Electric Company Coated articles and method for the prevention of fuel thermal degradation deposits
JPH05339748A (ja) * 1992-06-10 1993-12-21 Mitsubishi Heavy Ind Ltd 複合皮膜の製造方法
US5287730A (en) * 1992-06-18 1994-02-22 Securus, Inc. Plumbing leakage test apparatus and method of use
KR100316305B1 (ko) * 1993-12-28 2002-04-06 하루타 히로시 백색장식부품및그제조방법
DE19523637C2 (de) * 1994-12-27 1997-08-14 Mtu Friedrichshafen Gmbh Verfahren zur Herstellung einer Korrosionsschutzbeschichtung, Substrat mit einer Korrosionsschutzbeschichtung sowie Verwendung eines solchen Substrats
WO1996035825A1 (de) * 1995-05-08 1996-11-14 Helmut Tannenberger Werkstück für anwendungen bei hohen temperaturen und verfahren zu seiner herstellung
DE19628823C2 (de) * 1996-07-17 1998-08-20 Mtu Friedrichshafen Gmbh Stromführendes Bauteil für eine Schmelzkarbonatbrennstoffzelle mit Korrosionsschutzbeschichtung
US6335105B1 (en) * 1999-06-21 2002-01-01 General Electric Company Ceramic superalloy articles

Also Published As

Publication number Publication date
DE69911043T2 (de) 2004-06-03
JP2002527612A (ja) 2002-08-27
WO2000021152A1 (en) 2000-04-13
DK1119881T3 (da) 2003-12-08
NL1010269C2 (nl) 2000-04-11
CA2346486A1 (en) 2000-04-13
EP1119881B1 (de) 2003-09-03
ATE249102T1 (de) 2003-09-15
ES2211180T3 (es) 2004-07-01
EP1119881A1 (de) 2001-08-01
US6761927B1 (en) 2004-07-13

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8339 Ceased/non-payment of the annual fee