CN107024760A - A kind of transmission-type light splitting focusing system for VUV LASER - Google Patents
A kind of transmission-type light splitting focusing system for VUV LASER Download PDFInfo
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Abstract
本发明提出的一种用于真空紫外激光的透射式分光聚焦系统,属于光束分光聚焦技术领域,该系统由三块或四块凸透镜和一个光阑组成,各凸透镜和光阑均垂直于光路且共光轴设置;其中,第一凸透镜、第二凸透镜前后排列于光阑同一侧,其余凸透镜位于光阑另一侧。本系统对四波混频产生的真空紫外激光(VUV)光源进行分光和聚焦,对基频光的分光率达到99.99%以上,VUV光(125nm‑150nm)的总透过率可达到10%以上。在聚焦时,还可采用高精度非球面凸透镜抵消球差,使本系统达到衍射极限,从而实现亚微米光斑聚焦。
A transmissive spectroscopic focusing system for vacuum ultraviolet laser proposed by the present invention belongs to the technical field of beam splitting and focusing. The system is composed of three or four convex lenses and a diaphragm. The optical axis is set; wherein, the first convex lens and the second convex lens are arranged on the same side of the diaphragm, and the remaining convex lenses are located on the other side of the diaphragm. This system splits and focuses the vacuum ultraviolet laser (VUV) light source generated by four-wave mixing. The splitting ratio of the fundamental frequency light reaches more than 99.99%, and the total transmittance of VUV light (125nm‑150nm) can reach more than 10%. . When focusing, a high-precision aspheric convex lens can also be used to offset spherical aberration, so that the system reaches the diffraction limit, thereby achieving submicron spot focusing.
Description
技术领域technical field
本发明属于光束分光聚焦技术领域,特别涉及一种用于真空紫外激光的透射式分光聚焦系统。The invention belongs to the technical field of beam splitting and focusing, and in particular relates to a transmissive splitting focusing system for vacuum ultraviolet lasers.
背景技术Background technique
运用四波混频技术可产生高强度真空紫外激光(VUV,波长范围120-150nm)。该激光光源具有单光子能量高、激光线宽窄、能量密度高以及发散角小等特点,广泛应用于原子分子激发态能级结构测量、分子反应动力学、以及质谱成像等领域。由于真空紫外激光波长短,可提供亚微米级别的空间分辨——理论上VUV光可聚焦至直径为100nm的光斑。因此,VUV光对亚微米级的生物细胞成像,纳米材料的微观结构分析等具有深远的意义。High-intensity vacuum ultraviolet laser (VUV, wavelength range 120-150nm) can be generated by using four-wave mixing technology. The laser light source has the characteristics of high single-photon energy, narrow laser linewidth, high energy density, and small divergence angle. It is widely used in the fields of atomic and molecular excited state energy level structure measurement, molecular reaction dynamics, and mass spectrometry imaging. Due to the short wavelength of vacuum ultraviolet laser, it can provide sub-micron spatial resolution-in theory, VUV light can be focused to a spot with a diameter of 100nm. Therefore, VUV light has far-reaching significance for submicron biological cell imaging and microstructure analysis of nanomaterials.
四波混频技术基于非线性光学原理,将输入光(即基频光,包括紫外光、可见光)中的一部分在混频介质中转换为VUV光后,剩下的基频光会与VUV光共同输出。VUV波长较基频光短,单光子能量较基频光高,但由此产生的VUV光强度只有基频光的百分之一或更小。由于输出光中还混有高强度的基频光,若不将VUV光与该高强度的基频光分离,将会损伤被测样本,或掩盖VUV光的效果。因此,需要将VUV光和基频光分离。The four-wave mixing technology is based on the principle of nonlinear optics. After a part of the input light (that is, the fundamental frequency light, including ultraviolet light and visible light) is converted into VUV light in the mixing medium, the remaining fundamental frequency light will be combined with the VUV light. common output. The VUV wavelength is shorter than the fundamental frequency light, and the single photon energy is higher than the fundamental frequency light, but the resulting VUV light intensity is only one percent or less of the fundamental frequency light. Since the output light is also mixed with high-intensity fundamental-frequency light, if the VUV light is not separated from the high-intensity fundamental-frequency light, the sample to be tested will be damaged, or the effect of the VUV light will be masked. Therefore, it is necessary to separate the VUV light from the fundamental frequency light.
将VUV光和基频光分离一般使用两个独立光学系统分别进行分光和聚焦。分光的常规技术是先使用棱镜或光栅将输出光中的VUV光和基频光进行分开。这种方法利用了棱镜或光栅对不同波长的光有不同的折射或衍射角度的性质,但出射的VUV光路改变了方向,大大增加了实验装置的难度和稳定使用。The separation of VUV light and fundamental frequency light generally uses two independent optical systems for splitting and focusing respectively. The conventional technology of light splitting is to use a prism or a grating to separate the VUV light and the fundamental frequency light in the output light. This method takes advantage of the fact that prisms or gratings have different refraction or diffraction angles for different wavelengths of light, but the outgoing VUV light path changes direction, which greatly increases the difficulty and stable use of the experimental device.
文献报道的棱镜分光系统之一(D.Riedel,Appl.Phys.A 69,375–380,1999)分光后再通过单透镜实现聚焦。输出光通过棱镜后传播方向发生改变。不同波长的光线偏移角度不同,从而实现分光。可见光路不在一条轴线上,使用起来会非常不便。One of the prism splitting systems reported in the literature (D. Riedel, Appl. Phys. A 69, 375-380, 1999) splits light and then achieves focusing through a single lens. The direction of propagation of the output light changes after passing through the prism. Different wavelengths of light are shifted at different angles to achieve light splitting. The visible light path is not on one axis, which is very inconvenient to use.
目前用于VUV光的聚焦系统可采用反射聚焦方式。反射式聚焦镜具有无色差的优点;但成本高,体积大,反射镀膜损伤阈值低。另外,表面光解化学反应会在光学表面生成污染层,反射率会随工作时间降低,造成VUV光强的损失;且反射镀膜清洗困难。特别是用于高强度VUV光时,反射式聚焦系统存在的上述问题会更加突出。The current focusing system for VUV light can adopt reflective focusing. Reflective focusing mirrors have the advantage of no chromatic aberration; however, they are expensive, bulky, and have a low damage threshold for reflective coatings. In addition, the surface photolysis chemical reaction will generate a pollution layer on the optical surface, and the reflectivity will decrease with the working time, resulting in the loss of VUV light intensity; and it is difficult to clean the reflective coating. Especially when used for high-intensity VUV light, the above-mentioned problems existing in the reflective focusing system will be more prominent.
综上,目前还未见用于高强度真空紫外激光的透射式分光聚焦系统。To sum up, there is no transmissive spectroscopic focusing system for high-intensity vacuum ultraviolet laser.
发明内容Contents of the invention
本发明的目的是为了克服已有技术的不足之处,提供一种用于真空紫外激光的透射式分光聚焦系统。本系统可用少至三片透镜达到同时分光和亚微米近衍射极限聚焦的目的。The object of the present invention is to provide a transmission type spectroscopic focusing system for vacuum ultraviolet laser in order to overcome the shortcomings of the prior art. The system can use as few as three lenses to achieve simultaneous light splitting and submicron near-diffraction-limit focusing.
本发明提出的一种用于真空紫外激光的透射式分光聚焦系统,包括三块凸透镜和一个光阑,各凸透镜和光阑均垂直于光路且共光轴设置;其中,第一凸透镜、第二凸透镜前后排列于光阑同一侧,第三凸透镜位于光阑另一侧;A transmissive spectroscopic focusing system for vacuum ultraviolet laser proposed by the present invention includes three convex lenses and a diaphragm, each convex lens and diaphragm are arranged perpendicular to the optical path and have a common optical axis; wherein, the first convex lens and the second convex lens The front and back are arranged on the same side of the diaphragm, and the third convex lens is located on the other side of the diaphragm;
令第一和第二凸透镜之间的距离、第二凸透镜和光阑之间的距离、光阑和第三凸透镜之间的距离分别为L1、L2、L3,令第一、第二、第三凸透镜在真空紫外激光波段的的焦距分别为f1、f2、f3,则各元件的参数满足以下公式:Let the distance between the first and second convex lenses, the distance between the second convex lens and the diaphragm, and the distance between the diaphragm and the third convex lens be L 1 , L 2 , and L 3 respectively, and let the first, second, and The focal lengths of the third convex lens in the vacuum ultraviolet laser band are f 1 , f 2 , and f 3 respectively, and the parameters of each element satisfy the following formula:
1.5×(f1+f2)>L1>f1+f2 (1)1.5×(f 1 +f 2 )>L 1 >f 1 +f 2 (1)
L1>2f1 (2)L 1 >2f 1 (2)
f2≥f1 (3)f 2 ≥ f 1 (3)
L3>f3 (5-1)L 3 >f 3 (5-1)
所述第三凸透镜的工作距离WD按照公式(6)计算:The working distance WD of the third convex lens is calculated according to formula (6):
本发明提出的另一种用于真空紫外激光的透射式分光聚焦系统,包括四块凸透镜和一个光阑,各凸透镜和光阑均垂直于光路且共光轴设置;其中,第一凸透镜、第二凸透镜前后排列于光阑同一侧,第三凸透镜、第四凸透镜前后排列于光阑另一侧;Another transmissive spectroscopic focusing system for vacuum ultraviolet laser proposed by the present invention includes four convex lenses and an aperture, each convex lens and aperture are arranged perpendicular to the optical path and have a common optical axis; wherein, the first convex lens, the second The convex lenses are arranged on the same side of the diaphragm, the third convex lens and the fourth convex lens are arranged on the other side of the diaphragm;
令第一和第二凸透镜之间的距离、第二凸透镜和光阑之间的距离、光阑和第三凸透镜之间的距离分别为L1、L2、L3,令第一、第二、第三及第四凸透镜在真空紫外激光波段的的焦距分别为f1、f2、f3、f4,则各元件的参数满足以下公式:Let the distance between the first and second convex lenses, the distance between the second convex lens and the diaphragm, and the distance between the diaphragm and the third convex lens be L 1 , L 2 , and L 3 respectively, and let the first, second, and The focal lengths of the third and fourth convex lenses in the vacuum ultraviolet laser band are f 1 , f 2 , f 3 , and f 4 respectively, and the parameters of each element satisfy the following formula:
1.5×(f1+f2)>L1>f1+f2 (1)1.5×(f 1 +f 2 )>L 1 >f 1 +f 2 (1)
L1>2f1 (2)L 1 >2f 1 (2)
f2≥f1 (3)f 2 ≥ f 1 (3)
L3=f3 (5-2);L 3 =f 3 (5-2);
所述第四凸透镜设置在第三透镜后方任意处,第四凸透镜的工作距离等于该透镜的焦距f4。The fourth convex lens is arranged anywhere behind the third lens, and the working distance of the fourth convex lens is equal to the focal length f 4 of the lens.
所述光阑的中心孔直径为1-50μm。The diameter of the central hole of the aperture is 1-50 μm.
本发明的特点及有益效果是:系统结构简单,成本低,体积小,光路同轴,光学表面损伤阈值高,污染清洗方便。本发明采用氟化镁和氟化锂等制成用于VUV光波段的光学元件,用最少三块球面或非球面凸透镜对四波混频产生的VUV光源进行分光和聚焦。对基频光的分光率达到99.99%以上,VUV光(125nm-150nm)的总透过率可达到10%以上。在聚焦时,配合非球面透镜抵消球差,使本系统达到衍射极限,从而实现亚微米衍射极限光斑聚焦。The characteristics and beneficial effects of the present invention are: simple system structure, low cost, small volume, coaxial optical path, high damage threshold of optical surface, and convenient pollution cleaning. The invention uses magnesium fluoride and lithium fluoride to make optical elements for VUV light band, and uses at least three spherical or aspheric convex lenses to split and focus the VUV light source generated by four-wave mixing. The light splitting rate of fundamental frequency light can reach more than 99.99%, and the total transmittance of VUV light (125nm-150nm) can reach more than 10%. When focusing, cooperate with the aspheric lens to offset the spherical aberration, so that the system reaches the diffraction limit, so as to realize the submicron diffraction limit spot focusing.
附图说明Description of drawings
图1是本发明提出的一种透射式分光聚焦系统的光路结构示意图。FIG. 1 is a schematic diagram of the optical path structure of a transmissive spectroscopic focusing system proposed by the present invention.
图2是本发明提出的另一种透射式分光聚焦系统的光路结构示意图。Fig. 2 is a schematic diagram of the optical path structure of another transmissive spectroscopic focusing system proposed by the present invention.
具体实施方式detailed description
以下结合附图和具体实施例对本发明作进一步详细说明:Below in conjunction with accompanying drawing and specific embodiment the present invention is described in further detail:
本发明提出一种用于真空紫外激光的透射式分光聚焦系统,由三块凸透镜及一个光阑构成,整体结构如图1所示,各凸透镜采用氟化镁或氟化锂制成,各凸透镜和光阑均垂直于光路且共光轴设置;其中,第一凸透镜1、第二凸透镜2前后排列于光阑5同一侧,第三凸透镜3位于光阑5另一侧。将经四波混频得到的输出光作为本分光聚焦系统的入射光,入射光经过第一、第二凸透镜后该入射光中的真空紫外激光汇聚并穿过光阑5的中心孔,基频光由于凸透镜色散被光阑5遮挡;通过该第三凸透镜对真空紫外激光进行聚焦。The present invention proposes a transmissive spectroscopic focusing system for vacuum ultraviolet laser, which consists of three convex lenses and a diaphragm. The overall structure is shown in Figure 1. Each convex lens is made of magnesium fluoride or lithium fluoride. Each convex lens The first convex lens 1 and the second convex lens 2 are arranged on the same side of the diaphragm 5, and the third convex lens 3 is located on the other side of the diaphragm 5. The output light obtained by four-wave mixing is used as the incident light of this spectroscopic focusing system. After the incident light passes through the first and second convex lenses, the vacuum ultraviolet laser in the incident light converges and passes through the central hole of the diaphragm 5. The fundamental frequency The light is blocked by the diaphragm 5 due to the dispersion of the convex lens; the vacuum ultraviolet laser is focused through the third convex lens.
各元件的设置的距离如下:The setting distance of each component is as follows:
令第一和第二凸透镜之间的距离、第二凸透镜和光阑之间的距离、光阑和第三凸透镜之间的距离分别为L1、L2、L3,令第一、第二、第三凸透镜在真空紫外激光波段的的焦距分别为f1、f2、f3,则L1、L2满足以下公式可达到设计分光效果的同时确保光阑和第一、第二凸透镜不会受到损坏:Let the distance between the first and second convex lenses, the distance between the second convex lens and the diaphragm, and the distance between the diaphragm and the third convex lens be L 1 , L 2 , and L 3 respectively, and let the first, second, and The focal lengths of the third convex lens in the vacuum ultraviolet laser band are f 1 , f 2 , and f 3 , then L 1 , L 2 satisfy the following formulas, which can achieve the designed light splitting effect while ensuring that the diaphragm and the first and second convex lenses will not damaged by:
1.5×(f1+f2)>L1>f1+f2 (1)1.5×(f 1 +f 2 )>L 1 >f 1 +f 2 (1)
L1>2f1 (2)L 1 >2f 1 (2)
f2≥f1 (3)f 2 ≥ f 1 (3)
第二凸透镜和光阑之间的距离L2可通过公式(4)确定:The distance L between the second convex lens and the diaphragm can be determined by formula (4):
此时基频光在第二凸透镜位置的光斑大小大于1/3W,且基频光光密度小于入射基频光的9倍,其中,W为入射光光束直径。当使用焦距f2更长的第二透镜二时,可以使第二透镜处基频光的这个光密度数值变小。At this time, the spot size of the fundamental frequency light at the position of the second convex lens is larger than 1/3W, and the optical density of the fundamental frequency light is less than 9 times of the incident fundamental frequency light, wherein W is the beam diameter of the incident light. When the second lens 2 with a longer focal length f 2 is used, the optical density value of the fundamental frequency light at the second lens can be made smaller.
所述光阑的中心孔直径D可取1-50微米,大小可根据被测样本的热损伤阈值来选择。光阑可同时起到分光和提高VUV光束质量的作用。该光阑对基频光的衰减率Q(通过光阑中心孔的光能量与入射光总能量之比,衰减率越大分光效果越好),可用下式来计算:Q=1-(D/W)2。当入射光光束直径为5毫米时,衰减率在99.99%到99.99999%之间。虽然光阑中心孔直径越小分光效果越好,但对光阑位置的调试精度要求会相应增加。The diameter D of the central hole of the aperture can be 1-50 microns, and the size can be selected according to the thermal damage threshold of the sample to be tested. The aperture can simultaneously split the light and improve the quality of the VUV beam. The attenuation rate Q of the diaphragm to the fundamental frequency light (the ratio of the light energy through the central hole of the diaphragm to the total energy of the incident light, the greater the attenuation rate, the better the spectral effect), can be calculated by the following formula: Q=1-(D /w) 2 . When the diameter of the incident light beam is 5 mm, the attenuation rate is between 99.99% and 99.99999%. Although the smaller the diameter of the central hole of the diaphragm, the better the light splitting effect, but the adjustment accuracy requirements for the position of the diaphragm will increase accordingly.
为了保证光束在第三凸透镜3后面汇聚,第三凸透镜至光阑的距离L3及第三凸透镜的焦距f3应满足:In order to ensure that the light beam converges behind the third convex lens 3 , the distance L3 from the third convex lens to the diaphragm and the focal length f3 of the third convex lens should satisfy:
L3>f3 (5-1)L 3 >f 3 (5-1)
第三凸透镜的工作距离WD应按照公式(6)计算:The working distance WD of the third convex lens should be calculated according to formula (6):
本发明提出的另一种用于真空紫外激光的透射式分光聚焦系统,由四块凸透镜及一个光阑构成,整体结构如图2所示,该系统是在上述三块凸透镜的分光聚焦系统的基础上,保持第一凸透镜1、第二凸透镜2和光阑5的参数和位置不变的情况下,将第三凸透镜至光阑的距离L3调整为第三凸透镜的焦距f3,使光束经过第三凸透镜后形成准直光,同时在第三凸透镜后方的任意位置处同轴设置第四凸透镜4以实现最终的聚焦,第四凸透镜的工作距离与第四凸透镜的焦距相等。该四块凸透镜构成分光聚焦系统的基频光衰减率与上述三块凸透镜的分光聚焦系统一致。四块凸透镜分光聚焦系统相较于三块凸透镜分光聚焦系统的优点是最终的VUV焦点位置可调,即图2中L4长度可取任意正值,光路总长度更为灵活。Another transmission-type spectroscopic focusing system for vacuum ultraviolet laser proposed by the present invention is composed of four convex lenses and a diaphragm. The overall structure is shown in Figure 2. Basically, while keeping the parameters and positions of the first convex lens 1, the second convex lens 2 and the diaphragm 5 unchanged, the distance L 3 from the third convex lens to the diaphragm is adjusted to the focal length f 3 of the third convex lens, so that the light beam passes through Collimated light is formed behind the third convex lens, and a fourth convex lens 4 is coaxially arranged at any position behind the third convex lens to achieve final focusing. The working distance of the fourth convex lens is equal to the focal length of the fourth convex lens. The attenuation rate of the fundamental frequency light of the spectral focusing system constituted by the four convex lenses is consistent with that of the spectral focusing system of the above three convex lenses. The advantage of the four-convex lens splitting and focusing system compared to the three-convex lens splitting and focusing system is that the final VUV focus position is adjustable, that is, the length of L4 in Figure 2 can take any positive value, and the total length of the optical path is more flexible.
下面通过两个具体实施例对本发明的技术方案做进一步说明。这两个实施例均可以达到分光、聚焦一体化并且光路同轴的效果。并且结构简单,维护方便,成本低。The technical solution of the present invention will be further described below through two specific examples. Both of these two embodiments can achieve the effect of integrating light splitting and focusing and coaxial optical paths. Moreover, the structure is simple, the maintenance is convenient, and the cost is low.
实施例1为三块凸透镜的分光聚焦系统,具体组成如下:Embodiment 1 is the spectroscopic focusing system of three convex lenses, and the specific composition is as follows:
本实施例中入射光的光斑直径为4mm,光阑的中心孔直径D为10μm,VUV光的波长为125nm、基频光的波长为255-640nm;第一凸透镜、第二凸透镜、第三凸透镜的焦距分别为f1=50mm、f2=80mm、f3=40mm,第一凸透镜与第二凸透镜之间的距离L1=140mm、第二凸透镜与光阑之间的距离L2=183mm、第三凸透镜与光阑之间的距离L3=450mm,可得到工作距离为52mm,衍射极限光斑大小为500nm的参数。In the present embodiment, the spot diameter of the incident light is 4 mm, the central hole diameter D of the diaphragm is 10 μm, the wavelength of the VUV light is 125 nm, and the wavelength of the fundamental frequency light is 255-640 nm; the first convex lens, the second convex lens, and the third convex lens The focal lengths are respectively f 1 =50mm, f 2 =80mm, f 3 =40mm, the distance between the first convex lens and the second convex lens L 1 =140mm, the distance between the second convex lens and the diaphragm L 2 =183mm, The distance between the third convex lens and the diaphragm is L 3 =450mm, and the parameters of the working distance of 52mm and the diffraction-limited spot size of 500nm can be obtained.
本实施例中的凸透镜全部使用氟化镁制成,对125nmVUV光的透过率为13%,对255-640nm基频光的衰减率为99.93%。此时波长为255nm的UV光(紫外光)在光阑处的光斑大小为12mm。第一凸透镜、第二凸透镜、第三凸透镜可采用球面镜。由于球面镜会产生球差,也可采用非球面透镜替代球面镜减小球差,达到近衍射极限性能。The convex lenses in this embodiment are all made of magnesium fluoride, the transmittance to 125nm VUV light is 13%, and the attenuation rate to 255-640nm fundamental frequency light is 99.93%. At this time, the spot size of UV light (ultraviolet light) with a wavelength of 255 nm at the diaphragm is 12 mm. The first convex lens, the second convex lens and the third convex lens can adopt spherical mirrors. Since spherical mirrors will produce spherical aberration, aspheric lenses can also be used instead of spherical mirrors to reduce spherical aberration and achieve near-diffraction-limit performance.
实施例2为四块凸透镜的分光聚焦系统,具体组成如下:Embodiment 2 is the spectroscopic focusing system of four convex lenses, and concrete composition is as follows:
在实施例1的基础上将第三凸透镜更换为焦距为450mm的凸透镜,第一、第二凸透镜和光阑的参数和位置保持不变。第三凸透镜的作用是将发散的VUV光准直为直径为20mm的准直光束。然后将焦距为52mm的第四凸透镜4放置在第三凸透镜3后面50mm处,即可得工作距离为52mm、衍射极限光斑大小为500nm的参数。本实施例凸透镜全部使用氟化镁制成,对125nmVUV光的透过率为10%、对255-640nm基频光的衰减率为99.93%。第一、第二、第三、第四凸透镜可采用球面镜。由于球面镜会产生球差,也可采用非球面透镜替代球面镜减小球差,达到近衍射极限性能。On the basis of Embodiment 1, the third convex lens is replaced by a convex lens with a focal length of 450mm, and the parameters and positions of the first and second convex lenses and the diaphragm remain unchanged. The function of the third convex lens is to collimate the divergent VUV light into a collimated beam with a diameter of 20 mm. Then place the fourth convex lens 4 with a focal length of 52 mm at a position 50 mm behind the third convex lens 3 to obtain the parameters of a working distance of 52 mm and a diffraction-limited spot size of 500 nm. The convex lens in this embodiment is all made of magnesium fluoride, the transmittance to 125nm VUV light is 10%, and the attenuation rate to 255-640nm fundamental frequency light is 99.93%. The first, second, third and fourth convex lenses can be spherical mirrors. Since spherical mirrors will produce spherical aberration, aspheric lenses can also be used instead of spherical mirrors to reduce spherical aberration and achieve near-diffraction-limit performance.
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