CN106784213B - A kind of ring cavity nano wire electrical pumping single-photon source device - Google Patents

A kind of ring cavity nano wire electrical pumping single-photon source device Download PDF

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Publication number
CN106784213B
CN106784213B CN201710028757.5A CN201710028757A CN106784213B CN 106784213 B CN106784213 B CN 106784213B CN 201710028757 A CN201710028757 A CN 201710028757A CN 106784213 B CN106784213 B CN 106784213B
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nano wire
ring cavity
pin
photon source
type electrode
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CN106784213A (en
Inventor
陈飞良
李沫
黄锋
张晖
李倩
王旺平
康健彬
李俊泽
张健
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Institute of Electronic Engineering of CAEP
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    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01LSEMICONDUCTOR DEVICES NOT COVERED BY CLASS H10
    • H01L33/00Semiconductor devices having potential barriers specially adapted for light emission; Processes or apparatus specially adapted for the manufacture or treatment thereof or of parts thereof; Details thereof
    • H01L33/02Semiconductor devices having potential barriers specially adapted for light emission; Processes or apparatus specially adapted for the manufacture or treatment thereof or of parts thereof; Details thereof characterised by the semiconductor bodies
    • H01L33/04Semiconductor devices having potential barriers specially adapted for light emission; Processes or apparatus specially adapted for the manufacture or treatment thereof or of parts thereof; Details thereof characterised by the semiconductor bodies with a quantum effect structure or superlattice, e.g. tunnel junction
    • H01L33/06Semiconductor devices having potential barriers specially adapted for light emission; Processes or apparatus specially adapted for the manufacture or treatment thereof or of parts thereof; Details thereof characterised by the semiconductor bodies with a quantum effect structure or superlattice, e.g. tunnel junction within the light emitting region, e.g. quantum confinement structure or tunnel barrier
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01LSEMICONDUCTOR DEVICES NOT COVERED BY CLASS H10
    • H01L33/00Semiconductor devices having potential barriers specially adapted for light emission; Processes or apparatus specially adapted for the manufacture or treatment thereof or of parts thereof; Details thereof
    • H01L33/02Semiconductor devices having potential barriers specially adapted for light emission; Processes or apparatus specially adapted for the manufacture or treatment thereof or of parts thereof; Details thereof characterised by the semiconductor bodies
    • H01L33/10Semiconductor devices having potential barriers specially adapted for light emission; Processes or apparatus specially adapted for the manufacture or treatment thereof or of parts thereof; Details thereof characterised by the semiconductor bodies with a light reflecting structure, e.g. semiconductor Bragg reflector

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  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Computer Hardware Design (AREA)
  • Microelectronics & Electronic Packaging (AREA)
  • Power Engineering (AREA)
  • Led Devices (AREA)
  • Optical Modulation, Optical Deflection, Nonlinear Optics, Optical Demodulation, Optical Logic Elements (AREA)
  • Light Receiving Elements (AREA)

Abstract

The invention discloses a kind of ring cavity nano wire electrical pumping single-photon source devices, it is characterised in that: including p-type electrode, pin nano wire, the quantum dot being embedded into nano wire, multilayer concentric ring cavity, n-type electrode, n-type material and substrate.The advantages of this device, is: while realizing electrical pumping work, the circular ring shape Bragg microcavity constituted using multilayer concentric annulus, in the center of circle, quantum dot sites generate the enhancing of electromagnetic field local, the radiation efficiency of Purcell effect enhancing quantum dot single-photon source can be utilized, it again can be in the diverging of the two spaces dimension limitation photon perpendicular to nano wire, it is emitted single photon only along nano wire direction, is easy to and fiber coupling, greatly improve light Collection utilization efficiency.Ring cavity nano wire electrical pumping single-photon source device of the invention can be widely applied to quantum information, quantum calculation, quantum authentication, quantum accurate measurement related fields.

Description

A kind of ring cavity nano wire electrical pumping single-photon source device
Technical field
The present invention relates to single-photon source, semiconductor micro-nano photonic device, quantum information field, in particular to a kind of ring cavities to receive Rice noodles electrical pumping single-photon source device.
Technical background
Single-photon source is not only quantum information processing, quantum cryptography, the linear optical computing of quantum and quantum cryptology Important component, the fields such as microabsorption measurement, ultra-high sensitive magnetic-field measurement, biological fluorescent labelling and imaging also have weight Want application value.In the generation scheme of numerous single photon emissions, the single-photon source based on quantum dot compares other single-photon sources Suffer from very big superiority in all respects, such as have breadth of spectrum line is narrow, oscillator strength is high, photofading will not occur or flashing, Time jitter is small, repetition rate is high, emission band can cover each wave band from ultraviolet to infrared, is suitable for electric pump etc..In general, Quantum dot emission single photon is all not have directive, and its spontaneous radiation low efficiency in free space, causes to be difficult It is really practical.
In order to improve the emission effciency of single-photon source, quantum dot can be placed in microcavity by acquisition high-quality single-photon source, Using purcell effect, i.e., the spontaneous radiation of atom can be by greatly compared with the spontaneous radiation in free space in microcavity Reinforce, so that the quantum efficiency of single photon emission can be improved using microcavity.For electric pump device, the presence of microcavity can To greatly reduce the operating voltage of electrical pumping, to improve the stability of device.Usually use photon crystal micro cavity or DBR Microcavity obtains high-quality single-photon source.However, photon crystal micro cavity and electrical pumping device architecture compatibility are bad, and to short Its structure size of wave wave band is small, preparation is very big;DBR microcavity then can only limit light, Er Qieqi in one dimension of vertical direction It is required that quantum dot emission wavelength is precisely aligned with DBR chamber resonant wavelength, cause the high quality DBR microcavity suitable for electric pump to extension Equipment requirement is high, preparation difficulty is big.
Summary of the invention
It is an object of the invention to overcome the deficiencies in the prior art described above, it is simple to provide a kind of suitable electrical pumping, preparation And the ring cavity nano wire electrical pumping single-photon source device of light can be limited on two dimensions.
To achieve the above object, the present invention is as follows using technical solution:
A kind of ring cavity nano wire electrical pumping single-photon source device, from top to bottom successively include: p-type electrode, pin nano wire, Quantum dot, multilayer concentric ring cavity, n-type electrode, lower layer's n-type material and substrate;Wherein:
The substrate is located at the bottom, and the upper surface of substrate is lower layer's n-type material, and the upper surface of lower layer's n-type material is pin nanometers Line, quantum dot, multilayer concentric ring cavity, n-type electrode, p-type electrode are located at the upper surface of pin nano wire;
The multilayer concentric ring cavity is located at the outer layer of pin nano wire using pin nano wire as the center of circle;
The n-type electrode is located at the outer layer of multilayer concentric ring cavity using pin nano wire as the center of circle in a ring, and close to lower layer n The edge of profile material (6);
The pin nano wire is located on the center of lower layer's n-type material, and quantum dot embedding is in the intrinsic layer of pin nano wire (2) In.
The material of the p-type electrode includes one of graphene, ITO, AZO, Au, Ti, Ni, Pt or a variety of mixing.It is right The material transparent to emergent light is used in the device for going out light upwards from substrate face, for going out the device of light downwards from substrate back Using the material to emergent light high reflection.
The pin nano wire is by p-type material, Intrinsical, three layers of the n-type material pin structure constituted.Wherein, p-type layer material Material position forms Ohmic contact in top layer, with p-type electrode.
The quantum dot is located in the intrinsic layer of pin nano wire, is the material that forbidden bandwidth is less than pin nano wire, with pin Nano wire constitutes single quantum together.
The multilayer concentric ring cavity replaces structure using pin nano wire as the center of circle, by the different material of two or more refractive index At material includes air, dielectric insulation materials, metal material.The multilayer concentric ring cavity is that multilayer concentric annulus is constituted Circular ring shape Bragg microcavity can generate the enhancing of electromagnetic field local, can utilize amber in center location, i.e. pin nanometers of line position Sai Er effect enhances the radiation efficiency of quantum dot single-photon source, and can limit light in the two spaces dimension perpendicular to nano wire The diverging of son makes single photon only be emitted along nano wire direction, greatly improve light Collection utilization efficiency.
The n-type electrode and lower layer's n-type material form N-shaped Ohmic contact, the material of n-type electrode be graphene, ITO, Any one or more mixing in AZO, Au, Ti, Ni, Pt;
Lower layer's n-type material is consistent with the material of n-type material in pin nano wire.
The substrate uses the material transparent to emergent light for going out the device of light downwards from substrate back.
Ring cavity nano wire electrical pumping single-photon source device proposed by the present invention can be as being emitted upwards from substrate face Single-photon source device, and can be as the single-photon source device being emitted downwards from substrate back.As normal emergence single-photon source device When part, p-type electrode uses the material transparent to emergent light, such as graphene, ITO, AZO;Single-photon source device is being emitted as back When, p-type electrode uses the material to emergent light high reflection, such as metal Au, Pt, Ti/Au, at this moment can limit photon only along nanometer The outgoing of line N-shaped one end, further improves the directionality of single-photon source.
Beneficial effects of the present invention are as follows:
1, it while realizing electrical pumping work, can be imitated using the radiation of Purcell effect enhancing quantum dot single-photon source Rate, and single photon can be made only to be emitted along nano wire direction in the diverging of the two spaces dimension limitation photon perpendicular to nano wire, It is easy to integrated with fiber coupling, greatlys improve light Collection utilization efficiency;
It 2, can be as the single-photon source device being emitted upwards from substrate face and as being emitted downwards from substrate back Single-photon source device, and as back be emitted single-photon source device when can limit photon only along nano wire one end be emitted, into The directionality of one step improvement single-photon source.
Detailed description of the invention
Fig. 1 is three dimensional structure diagram of the invention.
Fig. 2 is structural schematic diagram of the structure shown in Fig. 1 along circle ring center section.
Fig. 3 is the AlGaN/GaN ring cavity nano wire electrical pumping single-photon source device based on graphene transparent p-type electrode Purcell enhancement factor calculated value.
Wherein, appended drawing reference are as follows: 1 is p-type electrode;2 be pin nano wire;3 be quantum dot;4 be multilayer concentric ring cavity;5 are N-type electrode;6 be lower layer's n-type material;7 be substrate.
Specific embodiment
Embodiment 1
A kind of AlGaN/GaN ring cavity nano wire electrical pumping single-photon source device based on graphene transparent p-type electrode.As Fig. 1, Shown in 2, in which: 1 is graphene transparent p-type electrode;2 receive for p-AlGaN/i-AlGaN/GaN-Qdot/i-AlGaN/n-AlGaN Rice noodles;3 be the GaN quantum dot being embedded into pin AlGaN nano wire;4 be AlGaN and spin on glass (SOG) is constituted The thickness of multilayer concentric ring cavity, concentric ring cavity is a quarter of effective wavelength;5 n-type electrodes constituted for Pt/Au;6 be N-shaped AlGaN epitaxial material;7 be AlN substrate.The Bragg grating that this structure is made of multilayer concentric ring cavity limits vertical nano-wire The photon of two spaces dimension diverging emits single photon only along nano wire both ends, has good directionality, and concentric ring Localized modes photon density increase in microcavity greatly increases the rate of quantum dot radiation single photon.Fig. 3 is for launch wavelength The Purcell enhancement factor that the AlGaN/GaN quantum dot of 325nm/nano wire single-photon source device calculates, has reached 80 times.
The device the preparation method is as follows:
The list of p-AlGaN/i-AlGaN/GaN-Qdot/i-AlGaN/n-AlGaN multilayered structure is first grown on AlN substrate Quantum Well epitaxial wafer;Then the nanometer figure of annular concentric and center circle is generated on it by electron beam lithography or nano impression Shape;Thereafter ring cavity nanowire structure is generated using dry etching combination wet etching;Utilize spin on glass (SOG) will later The gap of ring cavity is filled, and in nano wire apical growth graphene transparent p-type electrode;Finally annular is etched in ring cavity structure peripheral Table top simultaneously deposits Pt/Au n-type electrode.
Embodiment 2
A kind of InGaAs/InAs ring cavity nano wire electrical pumping single-photon source device based on Ti/Au high reflection p-type electrode.Such as Fig. 1, shown in 2, in which: 1 is Ti/Au high reflection p-type electrode;2 be p-InGaAs/i-InGaAs/InAs/i-InGaAs/n- InGaAs nano wire;3 be the InAs quantum dot being embedded into pin InGaAs nano wire;4 be Al2O3The multilayer constituted with air The thickness of concentric ring cavity, concentric ring cavity is a quarter of effective wavelength;5 n-type electrodes constituted for Ni/Au;6 be N-shaped InGaAs epitaxial material;7 be GaAs substrate.The Bragg grating that this structure is made of multilayer concentric ring cavity limits vertical nanowires The photon of line two spaces dimension diverging limits the photon dissipated along nano wire p-type end by Ti/Au high reflection p-type electrode, thus Emit single photon downwards only along the super substrate back in nano wire N-shaped one end, and the localized modes photon density in concentric ring microcavity Increasing greatly increases the rate of quantum dot radiation single photon.
The device the preparation method is as follows: first make circle SiO on gaas substrates2Nano graph mask, then on it Selective area growth p-InGaAs/i-InGaAs/InAs/i-InGaAs/n-InGaAs nanowire structure;ALD deposition skill is utilized later Art is by nano wire periphery Al2O3It fills and leads up, and in apical growth Ti/Au high reflection p-type electrode;It thereafter is the center of circle around nano wire Circular nano figure is generated, and ring cavity structure is generated using dry etching combination wet etching;Finally carved in ring cavity structure peripheral Erosion circular table simultaneously deposits Ni/Au n-type electrode.
The above embodiment is only preferred case of the invention, and the interest field that the present invention is advocated is not limited to these Embodiment, any modification for not departing from the spirit and scope of the present invention, deformation all should belong to protection scope of the present invention.

Claims (6)

1. a kind of ring cavity nano wire electrical pumping single-photon source device, it is characterised in that: including p-type electrode (1), pin nano wire (2), quantum dot (3), multilayer concentric ring cavity (4), n-type electrode (5), lower layer's n-type material (6) and substrate (7);
The substrate (7) is located at the bottom, and the upper surface of substrate (7) is lower layer's n-type material (6), the upper surface of lower layer's n-type material (6) For pin nano wire (2), quantum dot (3), multilayer concentric ring cavity (4), n-type electrode (5), p-type electrode (1) is located at pin nano wire The upper surface of (2);P-type electrode (1) material includes one of graphene, ITO, AZO, Au, Ti, Ni, Pt or a variety of mixing; Device for going out light upwards from substrate face uses the material transparent to emergent light, for going out the device of light downwards from substrate back Part uses the material to emergent light high reflection;The pin nano wire (2) is made of pin knot p-type material, Intrinsical, n-type material Structure;Wherein, p-type material is located at top layer, forms Ohmic contact with p-type electrode (1);
The multilayer concentric ring cavity (4) is with the outer layer that pin nano wire (2) are that the center of circle is located at pin nano wire (2);
The n-type electrode (5) is located at the outer layer of multilayer concentric ring cavity (4) in a ring with pin nano wire (2) for the center of circle, and close The edge of lower layer's n-type material (6);
The pin nano wire (2) is located on the center of lower layer's n-type material (6), and quantum dot (3) is embedded into pin nano wire (2) originally It levies in layer.
2. ring cavity nano wire electrical pumping single-photon source device according to claim 1, it is characterised in that: the quantum dot (3) in the intrinsic layer of pin nano wire (2), the material of pin nano wire (2) is less than using forbidden bandwidth, with pin nano wire (2) single quantum is constituted together.
3. ring cavity nano wire electrical pumping single-photon source device according to claim 1, it is characterised in that: the multilayer concentric Ring cavity (4) is alternately made of the different material of two or more refractive index, and the material includes air, dielectric insulation materials, gold Belong to material.
4. ring cavity nano wire electrical pumping single-photon source device according to claim 1, it is characterised in that: the n-type electrode (5) with lower layer's n-type material (6) formed N-shaped Ohmic contact, the material of n-type electrode (5) include graphene, ITO, AZO, Au, Ti, One of Ni, Pt or a variety of mixing.
5. ring cavity nano wire electrical pumping single-photon source device according to claim 1, it is characterised in that: lower layer's N-shaped Material (6) is consistent with the n-type material material in pin nano wire (2).
6. ring cavity nano wire electrical pumping single-photon source device according to claim 1, it is characterised in that: the substrate (7) Device for going out light downwards from substrate back uses the material transparent to emergent light.
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CN107359404B (en) * 2017-07-25 2023-06-16 中国工程物理研究院电子工程研究所 Ring cavity nano-antenna for regulating and controlling radiation of multiple random incoherent single photon emitters
CN108365517B (en) * 2018-01-03 2020-12-29 中山大学 Preparation method of bicolor single photon source structure and prepared structure
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WO2023215601A1 (en) * 2022-05-05 2023-11-09 The Regents Of The University Of Colorado, A Body Corporate Quantum light source with dual optical cavities

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