BR112016017431A8 - poliol poliéster (p1), processo para a produção de espumas rígidas de poliuretano ou de espumas rígidas de poliisocianurato, componente de poliol (pk), espuma rígida e uso de um poliol poliéster (p1) - Google Patents

poliol poliéster (p1), processo para a produção de espumas rígidas de poliuretano ou de espumas rígidas de poliisocianurato, componente de poliol (pk), espuma rígida e uso de um poliol poliéster (p1) Download PDF

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Publication number
BR112016017431A8
BR112016017431A8 BR112016017431A BR112016017431A BR112016017431A8 BR 112016017431 A8 BR112016017431 A8 BR 112016017431A8 BR 112016017431 A BR112016017431 A BR 112016017431A BR 112016017431 A BR112016017431 A BR 112016017431A BR 112016017431 A8 BR112016017431 A8 BR 112016017431A8
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Brazil
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rigid
polyol
mol
polyester polyol
foams
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BR112016017431A
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English (en)
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Kampf Gunnar
Kaluschke Tobias
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Basf Se
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Publication of BR112016017431A8 publication Critical patent/BR112016017431A8/pt

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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/4009—Two or more macromolecular compounds not provided for in one single group of groups C08G18/42 - C08G18/64
    • C08G18/4018—Mixtures of compounds of group C08G18/42 with compounds of group C08G18/48
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G63/00—Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
    • C08G63/66—Polyesters containing oxygen in the form of ether groups
    • C08G63/668—Polyesters containing oxygen in the form of ether groups derived from polycarboxylic acids and polyhydroxy compounds
    • C08G63/672—Dicarboxylic acids and dihydroxy compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/08—Processes
    • C08G18/14—Manufacture of cellular products
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/08—Processes
    • C08G18/16—Catalysts
    • C08G18/18—Catalysts containing secondary or tertiary amines or salts thereof
    • C08G18/1833—Catalysts containing secondary or tertiary amines or salts thereof having ether, acetal, or orthoester groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/42—Polycondensates having carboxylic or carbonic ester groups in the main chain
    • C08G18/4205—Polycondensates having carboxylic or carbonic ester groups in the main chain containing cyclic groups
    • C08G18/4208—Polycondensates having carboxylic or carbonic ester groups in the main chain containing cyclic groups containing aromatic groups
    • C08G18/4211—Polycondensates having carboxylic or carbonic ester groups in the main chain containing cyclic groups containing aromatic groups derived from aromatic dicarboxylic acids and dialcohols
    • C08G18/4219—Polycondensates having carboxylic or carbonic ester groups in the main chain containing cyclic groups containing aromatic groups derived from aromatic dicarboxylic acids and dialcohols from aromatic dicarboxylic acids and dialcohols in combination with polycarboxylic acids and/or polyhydroxy compounds which are at least trifunctional
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/42—Polycondensates having carboxylic or carbonic ester groups in the main chain
    • C08G18/4288—Polycondensates having carboxylic or carbonic ester groups in the main chain modified by higher fatty oils or their acids or by resin acids
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/48—Polyethers
    • C08G18/4825—Polyethers containing two hydroxy groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/48—Polyethers
    • C08G18/487—Polyethers containing cyclic groups
    • C08G18/4879—Polyethers containing cyclic groups containing aromatic groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
    • C08G18/72—Polyisocyanates or polyisothiocyanates
    • C08G18/74—Polyisocyanates or polyisothiocyanates cyclic
    • C08G18/76—Polyisocyanates or polyisothiocyanates cyclic aromatic
    • C08G18/7657—Polyisocyanates or polyisothiocyanates cyclic aromatic containing two or more aromatic rings
    • C08G18/7664—Polyisocyanates or polyisothiocyanates cyclic aromatic containing two or more aromatic rings containing alkylene polyphenyl groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
    • C08G18/72—Polyisocyanates or polyisothiocyanates
    • C08G18/74—Polyisocyanates or polyisothiocyanates cyclic
    • C08G18/76—Polyisocyanates or polyisothiocyanates cyclic aromatic
    • C08G18/7657—Polyisocyanates or polyisothiocyanates cyclic aromatic containing two or more aromatic rings
    • C08G18/7664—Polyisocyanates or polyisothiocyanates cyclic aromatic containing two or more aromatic rings containing alkylene polyphenyl groups
    • C08G18/7671—Polyisocyanates or polyisothiocyanates cyclic aromatic containing two or more aromatic rings containing alkylene polyphenyl groups containing only one alkylene bisphenyl group
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G63/00—Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
    • C08G63/66—Polyesters containing oxygen in the form of ether groups
    • C08G63/668—Polyesters containing oxygen in the form of ether groups derived from polycarboxylic acids and polyhydroxy compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J9/00—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof
    • C08J9/0014—Use of organic additives
    • C08J9/0038—Use of organic additives containing phosphorus
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J9/00—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof
    • C08J9/04—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof using blowing gases generated by a previously added blowing agent
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J9/00—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof
    • C08J9/04—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof using blowing gases generated by a previously added blowing agent
    • C08J9/12—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof using blowing gases generated by a previously added blowing agent by a physical blowing agent
    • C08J9/14—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof using blowing gases generated by a previously added blowing agent by a physical blowing agent organic
    • C08J9/141—Hydrocarbons
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L75/00—Compositions of polyureas or polyurethanes; Compositions of derivatives of such polymers
    • C08L75/04—Polyurethanes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G2110/00—Foam properties
    • C08G2110/0025—Foam properties rigid
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2203/00—Foams characterized by the expanding agent
    • C08J2203/14—Saturated hydrocarbons, e.g. butane; Unspecified hydrocarbons
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2375/00—Characterised by the use of polyureas or polyurethanes; Derivatives of such polymers
    • C08J2375/04—Polyurethanes
    • C08J2375/08—Polyurethanes from polyethers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L2666/00—Composition of polymers characterized by a further compound in the blend, being organic macromolecular compounds, natural resins, waxes or and bituminous materials, non-macromolecular organic substances, inorganic substances or characterized by their function in the composition
    • C08L2666/66—Substances characterised by their function in the composition
    • C08L2666/84—Flame-proofing or flame-retarding additives

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  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Manufacturing & Machinery (AREA)
  • Polyurethanes Or Polyureas (AREA)
  • Polyesters Or Polycarbonates (AREA)

Abstract

a presente invenção se refere aos polióis poliéster que são obtidos ou obteníveis por meio de esterificação de a partir de 10 até 70%-mol de pelo menos um composto selecionado do grupo consistindo em ácido tereftálico (tpa), dimetil tereftalato (dmt), polietileno tereftalato (pet), anidrido de ácido ftálico (psa), ácido ftálico e ácido isoftálico, de a partir de 0,1 até 30% mol de um ou mais ácidos graxos e/ou derivados de ácidos graxos, de a partir de 10 até 70 mol-% de um ou mais dióis alifáticos ou cicloalifáticos tendo de 2 a 18 átomos de c ou alcoxilatos dos mesmos, de a partir de a partir 5 até 70%-mol de um poliol poliéter, produzido pela alcoxilação de uma molécula aromática de acionador de partida tendo uma funcionalidade que é maior que ou igual a 2 e de a partir de 0 até 70%-mol de um tri- poliol ou que seja diferente de poliol poliéter, em cada caso em relação à quantidade total dos componentes empregados, com a soma das quantidades dos componentes empregados sendo 100 mol-%. a presente invenção ainda se refere a um método para a produção de espumas rígidas de poliuretano ou espumas rígidas poli-isocianurato, compreendendo a reação de um componente de isocianato com um componente poliol (pk) contendo um poliol poliéster de acordo com a invenção e outros componentes, em que o componente poliol como tal, bem como a espuma rígida de poliuretano ou espuma rígida de poli-isocianurato são obtidas ou obteníveis pelo método de acordo com a invenção. a presente invenção se refere também à utilização de um poliol poliéster (p1), de acordo com a invenção para geração de espumas rígidas de poliuretano ou espuma rígida de poli-isocianurato.
BR112016017431A 2014-02-11 2015-01-27 poliol poliéster (p1), processo para a produção de espumas rígidas de poliuretano ou de espumas rígidas de poliisocianurato, componente de poliol (pk), espuma rígida e uso de um poliol poliéster (p1) BR112016017431A8 (pt)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
EP14154645 2014-02-11
PCT/EP2015/051569 WO2015121057A1 (de) 2014-02-11 2015-01-27 Verfahren zur herstellung von polyurethan-hartschäumen und polyisocyanurat-hartschäumen

Publications (1)

Publication Number Publication Date
BR112016017431A8 true BR112016017431A8 (pt) 2020-06-16

Family

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Family Applications (1)

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BR112016017431A BR112016017431A8 (pt) 2014-02-11 2015-01-27 poliol poliéster (p1), processo para a produção de espumas rígidas de poliuretano ou de espumas rígidas de poliisocianurato, componente de poliol (pk), espuma rígida e uso de um poliol poliéster (p1)

Country Status (12)

Country Link
US (1) US10259906B2 (pt)
EP (1) EP3105274B1 (pt)
JP (1) JP2017509738A (pt)
KR (1) KR102338624B1 (pt)
CN (1) CN105980438A (pt)
BR (1) BR112016017431A8 (pt)
CA (1) CA2938060A1 (pt)
ES (1) ES2673860T3 (pt)
MX (1) MX367477B (pt)
PL (1) PL3105274T3 (pt)
RU (1) RU2016136382A (pt)
WO (1) WO2015121057A1 (pt)

Families Citing this family (9)

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HRP20231045T1 (hr) 2018-02-16 2023-12-22 H. B. Fuller Company Metoda za proizvodnju električnih ćelija sa zalivnom masom
CA3096666A1 (en) * 2018-04-10 2019-10-17 Stepan Company Polyol blends and rigid foams with improved low-temperature r-values
US20210198412A1 (en) * 2018-08-16 2021-07-01 Basf Se Environmentally friendly driven polyurethane spray foam systems
WO2020089439A1 (en) * 2018-11-02 2020-05-07 Covestro Deutschland Ag A rigid polyurethane precast panel
CN111138618A (zh) * 2018-11-02 2020-05-12 科思创德国股份有限公司 聚氨酯硬质预制板
CN114213797A (zh) * 2022-01-11 2022-03-22 陈小云 一种耐磨防刮smc模塑料及其制备方法
WO2023194140A1 (en) 2022-04-04 2023-10-12 Basf Se Value chain return process for the recovery of phosphorous ester-based flame retardants from polyurethane rigid foams
WO2024094788A1 (en) 2022-11-03 2024-05-10 Basf Se Value chain return process for the recovery of not bonded additives by extraction from polyurethane or polyisocyanurate rigid foams and depolymerization of the polyurethane rigid foams
WO2024094787A1 (en) 2022-11-03 2024-05-10 Basf Se Value chain return process for the recovery and of polymeric methylene phenylene amine (pmda) as its hci salt from the depolymerization of spend polyurethane and polyisocyanurate rigid foams

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DE1003714B (de) 1956-01-25 1957-03-07 Glanzstoff Ag Verfahren zum Abbau von Polyaethylenterephthalat zu Terephthalsaeuredimethylester
US4529744A (en) * 1982-10-25 1985-07-16 Stepan Company Compatibilized aromatic polyester polyols
US5051528A (en) 1990-04-24 1991-09-24 Eastman Kodak Company Recovery process for ethylene glycol and dimethylterephthalate
US6461536B2 (en) * 1998-02-09 2002-10-08 Basf Corporation Stable polyester polyol composition
WO2006100756A1 (ja) 2005-03-22 2006-09-28 Kawasaki Kasei Chemicals Ltd. ポリエステルポリオールの製造方法
JP2009516022A (ja) * 2005-11-14 2009-04-16 ダウ グローバル テクノロジーズ インコーポレイティド 向上した熱伝導率を有する硬質ポリウレタン発泡体の成形方法
PT2340269E (pt) 2008-10-15 2012-12-05 Basf Se Poliéster-polióis à base do ácido tereftálico
MX342673B (es) * 2010-12-02 2016-10-07 Basf Se Polioles de poliester basados en acidos dicarboxilicos aromaticos.
US20120214891A1 (en) * 2011-02-23 2012-08-23 Basf Se Polyester polyols based on aromatic dicarboxylic acids
EP2688933B1 (de) * 2011-03-22 2015-05-13 Basf Se Pu hartschaum mit niedriger wärmeleitfähigkeit und guter thermischer stabilität
CN104039856B (zh) * 2012-01-02 2017-03-01 巴斯夫欧洲公司 制备聚氨酯硬质泡沫和聚异氰脲酸酯硬质泡沫的方法
US20130251975A1 (en) * 2012-03-23 2013-09-26 Basf Se Producing rigid polyurethane foams and rigid polyisocyanurate foams

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Publication number Publication date
CN105980438A (zh) 2016-09-28
MX2016009946A (es) 2016-11-11
CA2938060A1 (en) 2015-08-20
RU2016136382A3 (pt) 2018-07-25
EP3105274B1 (de) 2018-03-14
PL3105274T3 (pl) 2018-08-31
RU2016136382A (ru) 2018-03-15
US10259906B2 (en) 2019-04-16
ES2673860T3 (es) 2018-06-26
KR102338624B1 (ko) 2021-12-14
WO2015121057A1 (de) 2015-08-20
MX367477B (es) 2019-08-23
EP3105274A1 (de) 2016-12-21
KR20160119838A (ko) 2016-10-14
JP2017509738A (ja) 2017-04-06
US20160347904A1 (en) 2016-12-01

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