RU2015148344A - Производство углеводородов из каталического реактора фишера-тропша - Google Patents

Производство углеводородов из каталического реактора фишера-тропша Download PDF

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RU2015148344A
RU2015148344A RU2015148344A RU2015148344A RU2015148344A RU 2015148344 A RU2015148344 A RU 2015148344A RU 2015148344 A RU2015148344 A RU 2015148344A RU 2015148344 A RU2015148344 A RU 2015148344A RU 2015148344 A RU2015148344 A RU 2015148344A
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Родни Дж. АЛЛАМ
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ДжиТиЭлПЕТРОЛ ЭлЭлСи
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    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2/00—Production of liquid hydrocarbon mixtures of undefined composition from oxides of carbon
    • C10G2/30—Production of liquid hydrocarbon mixtures of undefined composition from oxides of carbon from carbon monoxide with hydrogen
    • C10G2/32—Production of liquid hydrocarbon mixtures of undefined composition from oxides of carbon from carbon monoxide with hydrogen with the use of catalysts
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    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
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    • C10K—PURIFYING OR MODIFYING THE CHEMICAL COMPOSITION OF COMBUSTIBLE GASES CONTAINING CARBON MONOXIDE
    • C10K3/00—Modifying the chemical composition of combustible gases containing carbon monoxide to produce an improved fuel, e.g. one of different calorific value, which may be free from carbon monoxide
    • C10K3/06—Modifying the chemical composition of combustible gases containing carbon monoxide to produce an improved fuel, e.g. one of different calorific value, which may be free from carbon monoxide by mixing with gases
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    • B01D53/14—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols by absorption
    • B01D53/1456—Removing acid components
    • B01D53/1475—Removing carbon dioxide
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    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
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    • C01B2203/0227—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step
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    • C01B2203/0205—Processes for making hydrogen or synthesis gas containing a reforming step
    • C01B2203/0227—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step
    • C01B2203/0244—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step the reforming step being an autothermal reforming step, e.g. secondary reforming processes
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    • C01B2203/04—Integrated processes for the production of hydrogen or synthesis gas containing a purification step for the hydrogen or the synthesis gas
    • C01B2203/042—Purification by adsorption on solids
    • C01B2203/043—Regenerative adsorption process in two or more beds, one for adsorption, the other for regeneration
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    • C01B2203/04—Integrated processes for the production of hydrogen or synthesis gas containing a purification step for the hydrogen or the synthesis gas
    • C01B2203/0465—Composition of the impurity
    • C01B2203/047—Composition of the impurity the impurity being carbon monoxide
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    • C01B2203/0465—Composition of the impurity
    • C01B2203/0475—Composition of the impurity the impurity being carbon dioxide
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    • C01B2203/08—Methods of heating or cooling
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    • C01B2203/0888—Methods of cooling by evaporation of a fluid
    • C01B2203/0894—Generation of steam
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    • C01B2203/12—Feeding the process for making hydrogen or synthesis gas
    • C01B2203/1205—Composition of the feed
    • C01B2203/1211—Organic compounds or organic mixtures used in the process for making hydrogen or synthesis gas
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    • C01B2203/1288—Evaporation of one or more of the different feed components
    • C01B2203/1294—Evaporation by heat exchange with hot process stream
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    • C01B2203/14—Details of the flowsheet
    • C01B2203/142—At least two reforming, decomposition or partial oxidation steps in series
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    • C01B2203/80—Aspect of integrated processes for the production of hydrogen or synthesis gas not covered by groups C01B2203/02 - C01B2203/1695
    • C01B2203/84—Energy production
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/40—Characteristics of the process deviating from typical ways of processing
    • C10G2300/4043—Limiting CO2 emissions
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/32—Hydrogen storage
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
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    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00—Technologies relating to chemical industry
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Claims (21)

1. Объединенная система для производства углеводородов, содержащая:
РОХ, в котором углеводородный топливный газ частично окисляют в присутствии газообразного кислорода, чтобы производить первый промежуточный продукт синтез-газ;
GHR в сочетании с РОХ, в котором углеводородный топливный газ подвергают риформингу с паром, чтобы производить второй промежуточный продукт синтез-газ, который объединяют с первым промежуточным продуктом синтез-газом, чтобы образовать поток продукта синтез-газа;
газовую турбину, в которой газообразный окислитель сжимают, чтобы производить сжатый газообразный окислитель, горючий топливный газ сжигают в присутствии по меньшей мере части указанного сжатого газообразного окислителя, чтобы производить газообразные продукты сгорания, и указанные газообразные продукты сгорания расширяют, чтобы производить энергию и расширенные газообразные продукты сгорания;
теплообменник для нагрева первого потока пара за счет потока расширенных газообразных продуктов сгорания, чтобы производить нагретый первый поток пара;
первую трубу для подачи потока расширенных газообразных продуктов сгорания от расширительного средства в первое теплообменное средство;
вторую трубу для подачи по меньшей мере части нагретого первого потока пара из первого теплообменного средства в систему для выработки синтез-газа;
воздухоразделительную установку (“ASU”);
элемент для передачи по меньшей мере части электроэнергии, производимой посредством газовой турбины, к ASU и
реакционный каталитический процесс Фишера-Тропша с более чем одной ступенью реакции и отделение продукта - жидкого углеводорода, включающий удаление по меньшей мере части СО2, присутствующего в отделенном отходящем газе, из первой ступени или второй ступени, используя процесс отделения СО2.
2. Система по п. 1, в которой использованный реакционный каталитический процесс Фишера-Тропша представляет собой абсорбционный процесс, использующий химический или физический растворитель для удаления СО2 из потока газа и его производства как, по существу, чистого продукта СО2.
3. Система по п.п. 1 и 2, в которой по меньшей мере часть отделенного СО2 рециркулируют в систему для производства Н2+СО и используют, как часть подаваемых потоков, превращенных в Н2+СО.
4. Система по п.п. 1 и 2, в котором по меньшей мере часть отделенного СО2 отводят из установки как, по существу, чистый продукт.
5. Система по п.п. 1 и 2, в котором количество удаленного СО2 оставляет остаточное количество СО2 в потоке газа, что приводит в результате к отношению СО2 к (Н2+СО+СО2) в подаваемом газе на окончательной ступени реакции ФТ менее чем 18% молярных.
6. Система по п.п. 1-2, в котором отделенный отходящий газ из ступени ФТ сжимают, чтобы поддержать парциальное давление Н2+СО от 20 до 40 бар и также, чтобы достичь, по существу, высокого давления, чтобы возвратить часть отделенного отходящего газа из окончательной ступени ФТ на вход в систему для выработки Н2+СО без необходимости в любом дополнительном сжатии.
7. Система по п.п. 1-2, в котором часть чистого водорода, присутствующего в подаваемом газе, отделяют от подаваемого газа Н2+СО перед первой ступенью реактора Фишера-Тропша.
8. Система по п. 7, в котором суммарные потоки подаваемого газа на все ступени системы реактора Фишера-Тропша имеют общее отношение Н2 к СО от 2,0 до 2,3.
9. Система по п.п. 7, в котором отношение Н2 к СО на каждой ступени реактора в системе Фишера-Тропша имеет отношение Н2 к СО от 1,5 до 2,0.
10. Система по п.п. 7, в котором отделенный водород используют, чтобы добавить водород к отделенному газу, покидающему сепаратор продукта реактора Фишера-Тропша для того, чтобы установить отношение Н2 к СО от 1,5 до 2,0 в подаваемом газе Н2+СО, входящем в следующий реактор Фишера-Тропша после нагрева.
11. Система по п. 7, в котором водород отделяют от подаваемого газа Н2+СО в систему Фишера-Тропша, используя многослойную установку адсорбции с перепадом давления.
12. Система по п. 11, в котором отработанный газ из адсорбера с перепадом давления сжимают до давления подачи Н2+СО и смешивают с подачей Н2+СО на первую ступень реактора Фишера-Тропша.
RU2015148344A 2013-04-12 2014-04-11 Производство углеводородов из каталического реактора фишера-тропша RU2015148344A (ru)

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US11795402B2 (en) * 2021-10-06 2023-10-24 Kepler GTL LLC Systems, methods and apparatus for producing sustainable aviation fuel

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JPH09208974A (ja) * 1996-01-29 1997-08-12 Sekiyu Shigen Kaihatsu Kk 二酸化炭素含有天然ガスを原料とする液体燃料油の製造方法
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JP5301318B2 (ja) * 2009-02-27 2013-09-25 独立行政法人石油天然ガス・金属鉱物資源機構 Ｆｔガス成分からの炭化水素回収方法及び炭化水素回収装置
US8769961B2 (en) * 2009-04-17 2014-07-08 Gtlpetrol Llc Generating power from natural gas with carbon dioxide capture
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