PL751B1 - Method for producing oxyphenylquinoline bicarbonate acid and its derivatives. - Google Patents

Method for producing oxyphenylquinoline bicarbonate acid and its derivatives. Download PDF

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Publication number
PL751B1
PL751B1 PL751A PL75120A PL751B1 PL 751 B1 PL751 B1 PL 751B1 PL 751 A PL751 A PL 751A PL 75120 A PL75120 A PL 75120A PL 751 B1 PL751 B1 PL 751B1
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Poland
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acid
derivatives
producing
oxyphenylquinoline
parts
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PL751A
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Polish (pl)
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Publication of PL751B1 publication Critical patent/PL751B1/en

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Znaleziono, ze przez kondensacje 'kwasu wy, zwiazek cenny przy leczeniu chorób ar- acetosalicylowego (GOCH3 — OH —COOH= tretyczmo reumatycznych. Przemiana tych = f: 2 :1) z kwasem izatynowym otrzymuje zwiazków odbywa sie wedle wzoru nastepu- sie kwas oksyfenylochinolino-dwukarbono- jacego: CO — COOH A/ V\ + NHa CH3 CO COH / - oh C —COOH A/ \H i COOH / "- OH + '2H20 Nowy zwiazek nie rozpuszcza sie w wo¬ dzie i w ligroinie wcale, slabo w alkoholu i w alkoholu metylowym. Otrzymuje sie go, jako zóltawy proszek, który topi sie przy 283—284°, rozkladajac sie przytem. Tworzy on sól dwusodowa, której rozczym ma smak slodki i zabarwiony zostaje na zólto przez dodanie lugu sodowego.Znaleziono nadto, ze mozna otrzymac ten sam kwas oksyfenylochinolinodwukarbono- wy przez nagrzewanie kwasu p-aldehydo-sa- • licylowego z anilina i kwasem pyrogrono- wym w rozczynie alkoholowym.Mozna równiez wytwarzac pochodne kwa¬ su oksyfenilochinolinodwukarbonowego, bar¬ dzo do tego ostatniego podobne, przez uzyciezamiast aniliny jej homologów albo pochod¬ nych, a zamiast kwasu acetosalicylowego, jego homologów w rodzaju np. kwasu aceto- o-kresotyinowego, albo aceto-rni-kresotynowe- go, albo toz zamiast kwasu iz-atynowego, je¬ go pochodnych, jak np. kwasu metyleno dwuoksyiziatynowego.Przyklady. 1. Do rozczyinu kwasu izatynowego, któ¬ ry powstal z rozpuszczenia 147 czesci iza- tyny w 600 czesciach 33% lugu potasowego, dodaje sie 180 czesci kwasu acetoisalicylo- wego i ogrzewa sie ten rozczyn na; lazni wodnej. Z rozczynu stracony kwasem solnym wypada kwas oksyfenylochinolLnodwukarbo- nowy, który sie nastepnie odfiltrowuje i przemywa cieplym alkoholem; ewentualnie moze on byc oczyszczony przez krystalizacje jego soli dwusodowej lub eteru dwuetylo- wego o punkcie topliwosci 103°, które moz¬ na otrzymac w sposób znany. 2. 166 czesci p-aldehydokwasu salicylo¬ wego rozpuszcza sie z 93 'Czesciami aniliny w 1000 czesciach alkoholu. Do rozczynu po¬ wstajacego zwiazku dodaje sie 88 czesci kwasu pyrogronowego i nagrzewa w ciagu 3—4 godzin az do wrzenia; po oddestylowa¬ niu alkoholu, rozpuszczamy osad w rozczy- nie wody, i z rozczynu alkalicznego zostaje kwas fenylochinolinokairbonowy stracony przez dodanie kwasu solnego. Dla otrzyma¬ nia zwiazku chemicznie czystego nalezy po¬ stapic, jak podane w przykladzie 1. PL PLIt has been found that through condensation of acid, a compound valuable in the treatment of aracetalicylic diseases (GOCH3 - OH —COOH = tretic rheumatic diseases. -dicarbonate: CO - COOH A / V \ + NHa CH3 CO COH / - oh C —COOH A / \ H and COOH / "- OH + '2H 2 O The new compound does not dissolve in water and ligroin at all, poorly in alcohol and methyl alcohol, it is obtained as a yellowish powder which melts at 283 ° -284 ° and decomposes in this case. It forms a disodium salt, the diluent of which has a sweet taste and is colored yellow by adding sodium liquor. that the same oxyphenylquinoline dicarboxylic acid can be obtained by heating p-aldehyde salicylic acid with aniline and pyrogronic acid in an alcoholic solution. It is also possible to produce oxyphenylquinoline dicarboxylic acid derivatives, very similar to the latter, by using Instead of aniline, its homologues or derivatives, and instead of acetalicylic acid, its homologues such as aceto-cotinic acid or aceto-cotinic acid, or tois instead of isatinic acid, its derivatives, such as e.g. methylene dioxyisiatinic acid. 1. 180 parts of acetoisalicylic acid are added to the isatinic acid solution, which is formed by dissolving 147 parts of isatin in 600 parts of 33% potassium liquor, and heating this solution; water bath. Oxyphenylquinol-dicarboic acid is lost from the solution, lost with hydrochloric acid, which is then filtered off and washed with warm alcohol; it may optionally be purified by crystallization of its disodium salt or diethyl ether having a melting point of 103 °, which can be obtained in a known manner. 2. 166 parts of p-aldehyde salicylic acid is dissolved with 93 'parts of aniline in 1000 parts of alcohol. 88 parts of pyrogronic acid are added to the resulting solution and heated for 3 or 4 hours until boiling; after distilling off the alcohol, we dissolve the precipitate in a dilution of water, and the alkaline solution is left with phenylquinoline carboxic acid lost by adding hydrochloric acid. To obtain a chemically pure compound, follow the steps given in example 1. PL PL

Claims (1)

1. Zastrzezenie patentowe. Metoda wytwarzania kwasu oksyfenylo- chinolinokarbonowego, tern znamienna, ze sie kandensuje badz p-aldehydokwas salicy¬ lowy, badz jego homologi z kwasem pyro- gronowym i anilina, a równiez poichodine albo homologi tej; ostatniej, albo kwas p-a- cetosalicylowy, jako tez jego homologi z kwasem izatynoiwym lub jego pochodnemi. Farbwerke vorm. Meister Lucius & Bruning. Zastepca1: M. S k r z y p k o w s k i, rzecznik patentowy. ZAKL.GRAF.K0ZIANSK1CH W KRAKIWE PL PL1. Patent claim. A method of producing oxyphenylquinolinecarbonic acid, characterized by the fact that either p-aldehyde salicylic acid is candied or its homologues with pyruvic acid and aniline, and also with poichodine or a homologue thereof; the last, or p-α-cetosalicylic acid, as also its homologues with isatinic acid or its derivative. Farbwerke vorm. Meister Lucius & Bruning. Zastepca1: M. S k r z y p o w s k i, patent attorney. ZAKL.GRAF.K0ZIANSK1CH IN KRAKIWE PL PL
PL751A 1920-07-12 Method for producing oxyphenylquinoline bicarbonate acid and its derivatives. PL751B1 (en)

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PL751B1 true PL751B1 (en) 1924-10-31

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