PL400412A1 - 1-methylpiperidinium ionic liquids with the theophylline anion and a method for their preparation - Google Patents

1-methylpiperidinium ionic liquids with the theophylline anion and a method for their preparation

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Publication number
PL400412A1
PL400412A1 PL400412A PL40041212A PL400412A1 PL 400412 A1 PL400412 A1 PL 400412A1 PL 400412 A PL400412 A PL 400412A PL 40041212 A PL40041212 A PL 40041212A PL 400412 A1 PL400412 A1 PL 400412A1
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PL
Poland
Prior art keywords
theophylline
methylpiperidinium
anion
ionic liquids
residue
Prior art date
Application number
PL400412A
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Polish (pl)
Other versions
PL223215B1 (en
Inventor
Juliusz Pernak
Bartosz Markiewicz
Roksana Kordala
Katarzyna Materna
Original Assignee
Politechnika Poznanska
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Application filed by Politechnika Poznanska filed Critical Politechnika Poznanska
Priority to PL400412A priority Critical patent/PL223215B1/en
Publication of PL400412A1 publication Critical patent/PL400412A1/en
Publication of PL223215B1 publication Critical patent/PL223215B1/en

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  • Medicinal Preparation (AREA)

Abstract

Przedmiotem wynalazku sa 1-metylopiperydyniowe ciecze jonowe z anionem teofiliniowym o wzorze ogólnym 1, w którym R oznacza prosto lancuchowa grupe alkilowa zawierajaca od 1 do 20 atomów wegla, lub proton, lub grupe arylowa, lub allilowa, lub winylowa, lub chloroetylowa, lub hydroksyetylowa, lub benzylowa, majace zastosowanie jako zwiazki powierzchniowo czynne. W odmianie sposób ich wytwarzania polega na tym, ze sól teofiliny o wzorze ogólnym 2, w której M oznacza atom litu, lub sodu, lub potasu, lub srebra, lub grupe NH4, poddaje sie reakcji z czwartorzedowym halogenkiem 1-metylopipe-rydyniowym o wzorze ogólnym 3, w którym X oznacza chlor, lub brom, lub jod w stosunku molowym 1:0,8-1,5 w rozpuszczalniku organicznym. Calosc miesza sie w temperaturze od 273 do 363K, w czasie co najmniej 15 minut, po czym oddziela roztwór od powstajacego osadu, który stanowi sól nieorganiczna. Nastepnie odparowuje sie rozpuszczalnik organiczny. Pozostalosc przemywa bezwodnym acetonem do usuniecia pozostalosci soli oraz nadmiaru nieprzereagowanej teofiliny, dalej pozostalosc suszy sie pod obnizonym cisnieniem w temperaturze 303 do 343 K, w czasie co najmniej 15 minut.The subject of the invention are 1-methylpiperidinium ionic liquids with theophylline anion of general formula 1, wherein R is a straight chain alkyl group containing from 1 to 20 carbon atoms, or a proton, or an aryl, or allyl, or vinyl, or chloroethyl or hydroxyethyl group or benzyl, which may be used as surfactants. In a variation, the method of their preparation consists in reacting theophylline salt of general formula II, in which M is lithium, or sodium, or potassium, or silver, or NH4, with a 1-methyl piperidinium quaternary halide of formula general 3, wherein X is chlorine, or bromine, or iodine in a molar ratio of 1: 0.8-1.5 in an organic solvent. The whole is stirred at a temperature of 273 to 363K for at least 15 minutes, then separates the solution from the resulting precipitate, which is the inorganic salt. The organic solvent is then evaporated. The residue is washed with anhydrous acetone to remove salt residues and excess unreacted theophylline, then the residue is dried under reduced pressure at 303 to 343 K for at least 15 minutes.

PL400412A 2012-08-16 2012-08-16 1-methylpiperidinium ionic liquids with the theophylline anion and a method for their preparation PL223215B1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
PL400412A PL223215B1 (en) 2012-08-16 2012-08-16 1-methylpiperidinium ionic liquids with the theophylline anion and a method for their preparation

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
PL400412A PL223215B1 (en) 2012-08-16 2012-08-16 1-methylpiperidinium ionic liquids with the theophylline anion and a method for their preparation

Publications (2)

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PL400412A1 true PL400412A1 (en) 2014-02-17
PL223215B1 PL223215B1 (en) 2016-10-31

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PL400412A PL223215B1 (en) 2012-08-16 2012-08-16 1-methylpiperidinium ionic liquids with the theophylline anion and a method for their preparation

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PL223215B1 (en) 2016-10-31

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