PL10168B3 - Method for the preparation of disodium salts of 4-imino-methylene-sulfuric-2-metallocapto-benzole-i-sulfonic acids. - Google Patents

Method for the preparation of disodium salts of 4-imino-methylene-sulfuric-2-metallocapto-benzole-i-sulfonic acids. Download PDF

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Publication number
PL10168B3
PL10168B3 PL10168A PL1016826A PL10168B3 PL 10168 B3 PL10168 B3 PL 10168B3 PL 10168 A PL10168 A PL 10168A PL 1016826 A PL1016826 A PL 1016826A PL 10168 B3 PL10168 B3 PL 10168B3
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Poland
Prior art keywords
imino
sulfonic acids
methylene
metallocapto
benzole
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Application number
PL10168A
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Polish (pl)
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Publication of PL10168B3 publication Critical patent/PL10168B3/en

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Description

Najdluzszy czas trwania patentu do 24 stycznia 1944 r.The longest patent term is January 24, 1944.

Opisana w patencie Nr 9910 sól dwuso- dowa kwasu 4-imino-metyleno-siarkawo-2- zloto-merkapto-benzeno-7-sulfonowego (po¬ równaj przyklad III) moze byc tez otrzy¬ mana, jak to zostalo znalezione, na drodze dzialania siarczynem-formaldehydo-sodo- wym na sól sodowa kwasu 4-amino-2-zloto- merkapto-benzeno-7-sulfonowego (porów¬ naj przyklad II patentu glównego).The disodium salt of 4-imino-methylene-sulfurous-2-gold-mercapto-benzene-7-sulfonic acid described in Patent No. 9910 (e.g., Example III) can also be obtained, as has been found, by action of sodium sulfite-formaldehyde on the sodium salt of 4-amino-2-gold-mercapto-benzene-7-sulfonic acid (see Example 2 of the main patent).

W podobny sposób dochodzi sie do ana: logicznych zwiazków, podstawionych ciez- kiemi metalami.The ana is reached in a similar way: logical relations, substituted with heavy metals.

Przyklad I. Rozpuszcza sie 42,3 czesci i-amino-2-zloto-merkapto-benzeno-/-sulfo- nianu sodu w 200-stu czesciach wody, doda¬ je sie 13 czesci siarczynu-formaidehydo- sodowego i powstaly roztwór ogrzewa do wrzenia przy jednoczesnem sklócaniu. Po¬ tem z cieczy po ochlodzeniu jej wytraca sie alkoholem powstaly zwiazek kwasno- siarczyno-formaldehydowy. Zwiazek ten jest jasno-zólty, latwo rozpuszcza sie w wodzie i zawiera 36% zlota.EXAMPLE 1 42.3 parts of sodium i-amino-2-gold-mercapto-benzene-n-sulphonate are dissolved in 200 parts of water, 13 parts of sodium formidehydrate sulphite are added and the resulting solution is heated to boiling while confusing After cooling the liquid, the acid-sulfite-formaldehyde compound formed is precipitated with alcohol. This compound is light yellow, easily dissolves in water and contains 36% gold.

Przyklad II. 33,4 czesci 4-amino-2-sre- bro-merkapto-benzeno-/-sulfonianu sodu rozpuszcza sie w 150-ciu czesciach wody, dodaje 14 czesci siarczynu-formaldehydo- sodowego i roztwór ogrzewa do wrzenia przy jednoczesnem sklócaniu. Po ochlodze* niu, wytraca sie zapomoca alkoholu po-wstaly zwiazek kwasno-siarczyno-formal- dehydowy.Example II. 33.4 parts of sodium 4-amino-2-silver-mercapto-benzene sulphonate are dissolved in 150 parts of water, 14 parts of sodium formaldehyde sulphite are added and the solution is heated to the boil while quenching. After cooling, the resulting acid-sulfite-formaldehyde compound is destroyed with alcohol.

Spl dwusodowa- k^jasu 4-imino-metyle- no-siarkawo-2-srebro-merkapto-benzeno-7- sulfonowego jest proszkiem zlekka zabar¬ wionym na zólto, w wodzie latwo rozpu¬ szczalnym, o zawartosci srebra w wysoko¬ sci 24%, Przyklad III, Rozpuszcza sie 29,5 czesci 4-amino-2-bizmuto-merkapto - benzeno - 7- sulfonianu sodu w 150 czesciach wody, do¬ daje 14 czesci siarczynu-formaldehydo-so- dowego i ciecz ogrzewa do wrzenia. Z prze¬ zroczystego, czerwonawo-brunatnego roz¬ tworu wytraca sie alkoholem, po ochlodze¬ niu, produkt kondensacji, pod postacia la¬ two rozpuszczalnego w wodzie proszku, po¬ siadajacego zawartosc bizmutu w wysoko¬ sci 16,5% i zabarwionego na kolor poma- ranczowo-zólty.Spl disodium salt of 4-imino-methyl-sulfur-2-silver-mercapto-benzene-7-sulfonic acid is a slightly yellow colored powder, easily soluble in water, with a silver content of 24%, Example III, Dissolve 29.5 parts of sodium 4-amino-2-bismuth-mercapto-benzene-7- sulfonate in 150 parts of water, add 14 parts of sodium formaldehyde sulfite and heat the liquid to boiling . The clear, reddish-brown solution is triturated with alcohol after cooling, the condensation product in the form of a water-soluble powder with a bismuth content of 16.5% and a color tint. orange-yellow.

Claims (1)

1. Zastrzezenie patentowe, Odmiana sposobu, zastrzezonego paten¬ tem Nr 9910, znamienna tern, ze w celu o- trzymania dwusodowych soli kwasów 4- imino-metyleno-siarkawo-2-metalo-merkap- to-benzeno-./-sulfonowych dziala sie siar- czynem-formaldehydo-sodowym na sole so¬ dowe kwasów 4-amino-2-metalo-merkapto- bsnzeno-/-sulfonowych. Schering-Kahlbaum A, G, Zastepca: M. Skrzypkowski, rzecznik patentowy. Druk L. Boguslawskiego, Warszawa.1. Patent claim, A variation of the method claimed in patent No. 9910, characterized by the fact that in order to obtain disodium salts of 4-imino-methylene-sulfur-2-metallo-mercap-to-benzene / sulfonic acids it works with sodium formaldehyde sulfite into the sodium salts of 4-amino-2-metal-mercapto-bsnzene-/ -sulfonic acids. Schering-Kahlbaum A, G, Zastepca: M. Skrzypkowski, patent attorney. Print by L. Boguslawski, Warsaw.
PL10168A 1926-11-17 Method for the preparation of disodium salts of 4-imino-methylene-sulfuric-2-metallocapto-benzole-i-sulfonic acids. PL10168B3 (en)

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PL10168B3 true PL10168B3 (en) 1929-04-30

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